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Author |
Nichols, A.L.; Dimitriou, P.; Algora, A.; Fallot, M.; Giot, L.; Kondev, F.G.; Yoshida, T.; Karny, M.; Mukherjee, G.; Rasco, B.C.; Rykaczewski, K.P.; Sonzogni, A.A.; Tain, J.L. |
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Title |
Improving fission-product decay data for reactor applications: part I-decay heat |
Type |
Journal Article |
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Year |
2023 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
59 |
Issue |
4 |
Pages |
78 - 78pp |
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Abstract |
Effort has been expended to assess the relative merits of undertaking further decay-data measurements of the main fission-product contributors to the decay heat of neutron-irradiated fissionable fuel and related actinides by means of Total Absorption Gamma-ray Spectroscopy (TAGS – sometimes abbreviated to TAS) and Discrete Gamma-ray Spectroscopy (DGS). This review has been carried out following similar work performed under the auspices of OECD/WPEC-Subgroup 25 (2005-2007) and the International Atomic Energy Agency (2009, 2014), and various highly relevant TAGS measurements completed as a consequence of such assessments. We present our recommendations for new decay-data evaluations, along with possible requirements for total absorption and discrete high-resolution gamma-ray spectroscopy studies that cover approximately 120 fission products and various isomeric states. |
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Address |
[Nichols, A. L.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England, Email: P.Dimitriou@iaea.org |
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Springer |
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English |
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1434-6001 |
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Conference |
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Notes |
WOS:000984480400001 |
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no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5527 |
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Author |
n_TOF Collaboration (Torres-Sanchez, P. et al); Babiano-Suarez, V.; Caballero, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L. |
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Title |
Measurement of the 14N(n, p) 14C cross section at the CERN n_TOF facility from subthermal energy to 800 keV |
Type |
Journal Article |
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Year |
2023 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
107 |
Issue |
6 |
Pages |
064617 - 15pp |
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Abstract |
Background: The 14N(n, p) 14C reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where 14N acts as a neutron poison in the s process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region, and resonance region. Purpose: We aim to measure the 14N(n, p) 14C cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and provide calculations of Maxwellian averaged cross sections (MACS). Method: We apply the time-of-flight technique at Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. 10B(n, & alpha;) 7Li and 235U(n, f ) reactions are used as references. Two detection systems are run simultaneously, one on beam and another off beam. Resonances are described with the R-matrix code SAMMY. Results: The cross section was measured from subthermal energy to 800 keV, resolving the first two resonances (at 492.7 and 644 keV). A thermal cross section was obtained (1.809 & PLUSMN; 0.045 b) that is lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations. A 1/v energy dependence of the cross section was confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed determination of the 14N(n, p) cross section over a wide energy range for the first time. We have obtained cross sections with high accuracy (2.5%) from subthermal energy to 800 keV and used these data to calculate the MACS for kT = 5 to kT = 100 keV. |
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Address |
[Torres-Sanchez, Pablo; Praena, Javier; Porras, Ignacio; Ogallar, Francisco] Univ Granada, Granada, Spain, Email: pablotorres@ugr.es |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Conference |
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Notes |
WOS:001063209900001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5701 |
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Author |
n_TOF Collaboration (Domingo-Pardo, C. et al); Babiano-Suarez, V.; Balibrea-Correa, J.; Caballero, L.; Ladarescu, I.; Lerendegui-Marco, J.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Advances and new ideas for neutron-capture astrophysics experiments at CERN n_TOF |
Type |
Journal Article |
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Year |
2023 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
59 |
Issue |
1 |
Pages |
8 - 11pp |
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Keywords |
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Abstract |
This article presents a few selected developments and future ideas related to the measurement of (n, gamma ) data of astrophysical interest at CERN n_TOF. The MC-aided analysis methodology for the use of low-efficiency radiation detectors in time-of-flight neutron-capture measurements is discussed, with particular emphasis on the systematic accuracy. Several recent instrumental advances are also presented, such as the development of total-energy detectors with gamma- ray imaging capability for background suppression, and the development of an array of small-volume organic scintilla tors aimed at exploiting the high instantaneous neutron-flux of EAR2. Finally, astrophysics prospects related to the intermediate i neutron-capture process of nucleosynthesis are discussed in the context of the new NEAR activation area. |
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Address |
[Domingo-Pardo, C.; Babiano-Suarez, V.; Balibrea-Correa, J.; Caballero, L.; Ladarescu, I.; Lerendegui-Marco, J.; Tain, J. L.; Tarifeno-Saldivia, A.] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia, Spain, Email: domingo@ific.uv.es |
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Springer |
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English |
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Abbreviated Series Title |
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ISSN |
1434-6001 |
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Conference |
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Notes |
WOS:000926364900001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5479 |
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Author |
Orrigo, S.E.A.; Tain, J.L.; Mont-Geli, N.; Tarifeño-Saldivia, A.; Fraile, L.M.; Grieger, M.; Agramunt, J.; Algora, A.; Bemmerer, D.; Calvino, F.; Cortes, G.; De Blas, A.; Dillmann, I.; Dominguez Bugarin, A.; Garcia, R.; Nacher, E.; Tolosa-Delgado, A. |
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Title |
Long-term evolution of the neutron rate at the Canfranc Underground Laboratory |
Type |
Journal Article |
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Year |
2022 |
Publication |
European Physical Journal C |
Abbreviated Journal |
Eur. Phys. J. C |
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Volume |
82 |
Issue |
9 |
Pages |
814 - 11pp |
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Abstract |
We report results on the long-term variation of the neutron counting rate at the Canfranc Underground Laboratory, of importance for several low-background experiments installed there, including rare-event searches. The measurement campaign was performed employing the High Efficiency Neutron Spectrometry Array (HENSA) mounted in Hall A and lasted 412 live days. The present study is the first long-term measurement of the neutron rate with sensitivity over a wide range of neutron energies (from thermal up to 0.1 GeV and beyond) performed in any underground laboratory so far. Data on the environmental variables inside the experimental hall (radon concentration, air temperature, air pressure and humidity) were also acquired during all the measurement campaign. We have investigated for the first time the evolution of the neutron rate for different energies of the neutrons and its correlation with the ambient variables. |
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Address |
[Orrigo, S. E. A.; Tain, J. L.; Agramunt, J.; Algora, A.; Nacher, E.; Tolosa-Delgado, A.] Univ Valencia, Inst Fis Corpuscular, CSIC, Valencia 46071, Spain, Email: Sonja.Orrigo@ific.uv.es |
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Springer |
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English |
Summary Language |
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Abbreviated Series Title |
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ISSN |
1434-6044 |
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Conference |
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Notes |
WOS:000853333800003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5358 |
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Author |
Guadilla, V. et al; Algora, A.; Tain, J.L.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Nacher, E.; Orrigo, S.E.A.; Rubio, B.; Valencia, E. |
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Title |
Total absorption gamma-ray spectroscopy of the ss decays of Y-96gs,Y-m |
Type |
Journal Article |
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Year |
2022 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
106 |
Issue |
1 |
Pages |
014306 - 14pp |
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Abstract |
The ss decays of the ground state (gs) and isomeric state (m) of Y-96 have been studied with the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8(+) isomeric state from the 0(-) ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The ss-intensity distributions of both decays have been independently determined. In the analyses the deexcitation of the 1581.6 keV level in Zr-96, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the ss-detector efficiency, influencing the ss-intensity distribution obtained. Our results for Y-96gs (0(-)) confirm the large ground state to ground state ss-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to 96.6(-2.1)(+0.3) % of the total ss intensity. Given that the decay of Y-96gs is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of Y-96m (8(+)), previously undetected ss intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption gamma-ray spectroscopy measurements of ss decays with highly fragmented deexcitation patterns. Y-96m (8(+)) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average ss and gamma energies differ significantly from the previous values in evaluated databases. The discrepancy is far above the previously quoted uncertainties. Finally, we also report on the successful implementation of an innovative total absorption gamma-ray spectroscopy analysis of the module-multiplicity gated spectra, as a first proof of principle to distinguish between decaying states with very different spin-parity values. |
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Address |
[Guadilla, V; Le Meur, L.; Fallot, M.; Briz, J. A.; Estienne, M.; Giot, L.; Porta, A.; Cucoanes, A.; Shiba, T.; Zakari-Issoufou, A-A] Univ Nantes, Subatech, IMT Atlantique, CNRS IN2P3, F-44307 Nantes, France, Email: vguadilla@fuw.edu.pl |
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Publisher |
Amer Physical Soc |
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English |
Summary Language |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000832364800001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5313 |
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Author |
n_TOF Collaboration (Mastromarco, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
High accuracy, high resolution U-235(n,f) cross section from n_TOF (CERN) from 18 meV to 10 keV |
Type |
Journal Article |
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Year |
2022 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
58 |
Issue |
8 |
Pages |
147 - 13pp |
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Keywords |
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Abstract |
The U-235(n,f) cross section was measured in a wide energy range (18 meV-170 keV) at the nTOF facility at CERN, relative to Li-6(n,t) and B-10(n,alpha) standard reactions, with high resolution and accuracy, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. In this paper we report on the results in the region between 18 meV and 10 keV neutron energy. A resonance analysis has been performed up to 200 eV, with the code SAMMY. The resulting fission kernels are compared with the ones extracted on the basis of the resonance parameters of the most recent major evaluated data libraries. A comparison of the nTOF data with the evaluated cross sections is also performed from thermal to 10 keV neutron energy for the energy-averaged cross section in energy groups of suitably chosen width. A good agreement, within 0.5%, is found on average between the new results and the latest evaluated data files ENDF/B-VIII.0 and JEFF-3.3, as well as with respect to the broad group average fission cross section established in the framework of the standard working group of IAEA (the so-called reference file). However, some discrepancies, of up to 4%, are still present in some specific energy regions. The new dataset here presented, characterized by a unique combination of high resolution and accuracy, low background and wide energy range, can help to improve the evaluations from the Resolved Resonance Region up to 10 keV, also reducing the uncertainties that affect this region. |
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Address |
[Mastromarco, M.; Colonna, N.; Diacono, D.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: amaducci@lns.infn.it |
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Publisher |
Springer |
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Language |
English |
Summary Language |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000840312100002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5328 |
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Author |
Dimitriou, P. et al; Tain, J.L.; Algora, A. |
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Title |
Development of a Reference Database for Beta-Delayed Neutron Emission |
Type |
Journal Article |
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Year |
2021 |
Publication |
Nuclear Data Sheets |
Abbreviated Journal |
Nucl. Data Sheets |
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Volume |
173 |
Issue |
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Pages |
144-238 |
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Keywords |
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Abstract |
Beta-delayed neutron emission is important for nuclear structure and astrophysics as well as for reactor applications. Significant advances in nuclear experimental techniques in the past two decades have led to a wealth of new measurements that remain to be incorporated in the databases. We report on a coordinated effort to compile and evaluate all the available beta-delayed neutron emission data. The different measurement techniques have been assessed and the data have been compared with semi-microscopic and microscopic-macroscopic models. The new microscopic database has been tested against aggregate total delayed neutron yields, time-dependent group parameters in 6-and 8-group re-presentation, and aggregate delayed neutron spectra. New recommendations of macroscopic delayed-neutron data for fissile materials of interest to applications are also presented. |
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Address |
[Dimitriou, P.; Verpelli, M.] IAEA, NAPC Nucl Data Sect, A-1400 Vienna, Austria, Email: p.dimitriou@iaea.org |
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Publisher |
Academic Press Inc Elsevier Science |
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English |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0090-3752 |
ISBN |
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Expedition |
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Conference |
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Notes |
WOS:000647012500006 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4828 |
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Author |
Algora, A.; Ganioglu, E.; Sarriguren, P.; Guadilla, V.; Fraile, L.M.; Nacher, E.; Rubio, B.; Tain, J.L.; Agramunt, J.; Gelletly, W.; Briz, J.A.; Cakirli, R.B.; Fallot, M.; Jordan, D.; Halasz, Z.; Kuti, I.; Montaner, A.; Onillon, A.; Orrigo, S.E.A.; Cerdan, A.P.; Rice, S.; Vedia, V.; Valencia, E. |
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Title |
Total absorption gamma-ray spectroscopy study of the beta-decay of Hg-186 |
Type |
Journal Article |
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Year |
2021 |
Publication |
Physics Letters B |
Abbreviated Journal |
Phys. Lett. B |
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Volume |
819 |
Issue |
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Pages |
136438 - 7pp |
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Keywords |
Betadecay; Totalabsorption spectroscopy; Shape coexistence |
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Abstract |
The Gamow-Teller strength distribution of the decay of Hg-186 into Au-186 has been determined for the first time using the total absorption gamma spectroscopy technique and has been compared with theoretical QRPA calculations using the SLy4 Skyrme force. The measured Gamow-Teller strength distribution and the half-life are described by mixing oblate and prolate configurations independently in the parent and daughter nuclei. In this theoretical framework the best description of the experimental beta strength is obtained with dominantly prolate components for both parent Hg-186 and daughter Au-186. The approach also allowed us to determine an upper limit of the oblate component in the parent state. The complexity of the analysis required the development of a new approach in the analysis of the X-ray gated total absorption spectrum. |
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Address |
[Algora, A.; Guadilla, V; Nacher, E.; Rubio, B.; Tain, J. L.; Agramunt, J.; Jordan, D.; Montaner, A.; Orrigo, S. E. A.; Cerdan, A. Perez; Valencia, E.] Univ Valencia, Inst Fis Corpuscular, CSIC, E-46071 Valencia, Spain, Email: algora@ific.uv.es; |
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Publisher |
Elsevier |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0370-2693 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000679259200010 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4923 |
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| Permanent link to this record |
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Author |
Algora, A.; Tain, J.L.; Rubio, B.; Fallot, M.; Gelletly, W. |
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Title |
Beta-decay studies for applied and basic nuclear physics |
Type |
Journal Article |
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Year |
2021 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
57 |
Issue |
3 |
Pages |
85 - 28pp |
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Keywords |
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Abstract |
In this reviewwe will present the results of recent beta-decay studies using the total absorption technique that cover topics of interest for applications, nuclear structure and astrophysics. The decays studied were selected primarily because they have a large impact on the prediction of (a) the decay heat in reactors, important for the safety of present and future reactors and (b) the reactor electron anti-neutrino spectrum, of interest for particle/nuclear physics and reactor monitoring. For these studies the total absorption technique was chosen, since it is the only method that allows one to obtain beta-decay probabilities free from a systematic error called the Pandemonium effect. The total absorption technique is based on the detection of the. cascades that follow the initial beta decay. For this reason the technique requires the use of calorimeters with very high. detection efficiency. The measurements presented and discussed here were performed mainly at the IGISOL facility of the University of Jyvaskyla (Finland) using isotopically pure beams provided by the JYFLTRAP Penning trap. Examples are presented to show that the results of our measurements on selected nuclei have had a large impact on predictions of both the decay heat and the anti-neutrino spectrum from reactors. Some of the cases involve beta-delayed neutron emission thus one can study the competition between gamma – and neutron-emission from states above the neutron separation energy. The gamma-to-neutron emission ratios can be used to constrain neutron capture (n, gamma) cross sections for unstable nuclei of interest in astrophysics. The information obtained from the measurements can also be used to test nuclear model predictions of half-lives and Pn values for decays of interest in astrophysical network calculations. These comparisons also provide insights into aspects of nuclear structure in particular regions of the nuclear chart. |
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Address |
[Algora, A.; Tain, J. L.; Rubio, B.] Univ Valencia, CSIC, IFIC, Paterna, Spain, Email: algora@ific.uv.es |
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Publisher |
Springer |
Place of Publication |
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English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000625127600001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4754 |
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Author |
Grieger, M.; Hensel, T.; Agramunt, J.; Bemmerer, D.; Degering, D.; Dillmann, I.; Fraile, L.M.; Jordan, D.; Koster, U.; Marta, M.; Muller, S.E.; Szucs, T.; Tain, J.L.; Zuber, K. |
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Title |
Neutron flux and spectrum in the Dresden Felsenkeller underground facility studied by moderated He-3 counters |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review D |
Abbreviated Journal |
Phys. Rev. D |
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Volume |
101 |
Issue |
12 |
Pages |
123027 - 15pp |
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Keywords |
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Abstract |
Ambient neutrons may cause significant background for underground experiments. Therefore, it is necessary to investigate their flux and energy spectrum in order to devise a proper shielding. Here, two sets of altogether ten moderated He-3 neutron counters are used for a detailed study of the ambient neutron background in tunnel IV of the Felsenkeller facility, underground below 45 m of rock in Dresden/Germany. One of the moderators is lined with lead and thus sensitive to neutrons of energies higher than 10 MeV. For each He-3 counter moderator assembly, the energy-dependent neutron sensitivity was calculated with the FLUKA code. The count rates of the ten detectors were then fitted with the MAXED and GRAVEL packages. As a result, both the neutron energy spectrum from 10(-9) to 300 MeV and the flux integrated over the same energy range were determined experimentally. The data show that at a given depth, both the flux and the spectrum vary significantly depending on local conditions. Energy-integrated fluxes of (0.61 +/- 0.05), (1.96 +/- 0.15), and (4.6 +/- 0.4) x 10(-4) cm(-2) s(-1), respectively, are measured for three sites within Felsenkeller tunnel IV which have similar muon flux but different shielding wall configurations. The integrated neutron flux data and the obtained spectra for the three sites are matched reasonably well by FLUKA Monte Carlo calculations that are based on the known muon flux and composition of the measurement room walls. |
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Address |
[Grieger, M.; Hensel, T.; Bemmerer, D.; Mueller, S. E.; Szuecs, T.] Helmholtz Zentrum Dresden Rossendorf HZDR, D-01328 Dresden, Germany, Email: d.bemmerer@hzdr.de |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1550-7998 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000542517900002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4442 |
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