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Author Perkowski, J. et al; Babiano-Suarez, V.; Balibrea Correa, J.; Domingo-Pardo, C.; Ladarescu, I.; Lerendegui-Marco, J.
Title Multi-section fission ionization chamber for measurement of 239Pu(n, γ) reaction in fission tagging method Type Journal Article
Year 2024 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume 1067 Issue Pages (down) 169649 - 8pp
Keywords Radiative neutron capture cross section; Fission; Ionization chamber; Pu-239; n_TOF facility; CERN
Abstract The Pu-239(n, gamma) reaction cross section is very important for operation of both thermal and fast reactors, when loaded with MOX fuels. According to the NEA/OECD High Priority Request List the precision of cross section data for this reaction should be improved. The cross section of (n, f) reaction is much higher compared to (n, gamma) for this isotope. In such conditions the fission tagging technique could be applied to identify the fission background. In the past, this technique was successfully used for capture measurements at the nTOF facility at CERN. The multi-section fission ionization chamber was constructed and used in the combination with Total Absorption Calorimeter (TAC) for detecting gamma rays for the precise measurement of Pu-239(n, gamma) reaction cross section at the nTOF facility.
Address [Perkowski, J.; Andrzejewski, J.; Gawlik-Ramiega, A.] Univ Lodz, Lodz, Poland, Email: jaroslaw.perkowski@uni.lodz.pl
Corporate Author Thesis
Publisher Elsevier Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:001373452600001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 6385
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Author Lerendegui-Marco, J.; Babiano-Suarez, V.; Domingo-Pardo, C.; Ladarescu, I.; Tarifeno-Saldivia, A.; de la Fuente-Rosales, G.
Title Pushing the high count rate limits of scintillation detectors for challenging neutron-capture experiments Type Journal Article
Year 2024 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume 1064 Issue Pages (down) 169385 - 13pp
Keywords Dead-time; Pile-up; Time-of-flight; Radiative capture; Total energy detector; Pulse-height weighting technique
Abstract One of the critical aspects for the accurate determination of neutron capture cross sections when combining time-of-flight and total energy detector techniques is the characterization and control of systematic uncertainties associated to the measuring devices. In this work we explore the most conspicuous effects associated to harsh count rate conditions: dead-time and pile-up effects. Both effects, when not properly treated, can lead to large systematic uncertainties and bias in the determination of neutron cross sections. In the majority of neutron capture measurements carried out at the CERN nTOF facility, the detectors of choice are the C6D6 liquid-based either in form of large-volume cells or recently commissioned sTED detector array, consisting of much smaller-volume modules. To account for the aforementioned effects, we introduce a Monte Carlo model for these detectors mimicking harsh count rate conditions similar to those happening at the CERN nTOF 20 m flight path vertical measuring station. The model parameters are extracted by comparison with the experimental data taken at the same facility during 2022 experimental campaign. We propose a novel methodology to consider both, dead-time and pile-up effects simultaneously for these fast detectors and check the applicability to experimental data from Au-197(n, gamma), including the saturated 4.9 eV resonance which is an important component of normalization for neutron cross section measurements.
Address [Balibrea-Correa, J.; Lerendegui-Marco, J.; Babiano-Suarez, V.; Domingo-Pardo, C.; Ladarescu, I.; Tarifeno-Saldivia, A.; de la Fuente-Rosales, G.] Univ Valencia, Inst Fis Corpuscular, CSIC, Valencia, Spain, Email: javier.balibrea@ific.uv.es
Corporate Author Thesis
Publisher Elsevier Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:001270371600001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 6270
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Author Balibrea-Correa, J.; Lerendegui-Marco, J.; Babiano-Suarez, V.; Caballero, L.; Calvo, D.; Ladarescu, I.; Olleros-Rodriguez, P.; Domingo-Pardo, C.
Title Machine Learning aided 3D-position reconstruction in large LaCl3 crystals Type Journal Article
Year 2021 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume 1001 Issue Pages (down) 165249 - 17pp
Keywords Gamma-ray; Position sensitive detectors; Monolithic crystals; Compton imaging; Machine Learning; Convolutional Neural Networks; Total Energy Detector; Neutron capture cross-section
Abstract We investigate five different models to reconstruct the 3D gamma-ray hit coordinates in five large LaCl3(Ce) monolithic crystals optically coupled to pixelated silicon photomultipliers. These scintillators have a base surface of 50 x 50 mm(2) and five different thicknesses, from 10 mm to 30 mm. Four of these models are analytical prescriptions and one is based on a Convolutional Neural Network. Average resolutions close to 1-2 mm fwhm are obtained in the transverse crystal plane for crystal thicknesses between 10 mm and 20 mm using analytical models. For thicker crystals average resolutions of about 3-5 mm fwhm are obtained. Depth of interaction resolutions between 1 mm and 4 mm are achieved depending on the distance of the interaction point to the photosensor surface. We propose a Machine Learning algorithm to correct for linearity distortions and pin-cushion effects. The latter allows one to keep a large field of view of about 70%-80% of the crystal surface, regardless of crystal thickness. This work is aimed at optimizing the performance of the so-called Total Energy Detector with Compton imaging capability (i-TED) for time-of-flight neutron capture cross-section measurements.
Address [Balibrea-Correa, J.; Lerendegui-Marco, J.; Babiano-Suarez, V.; Caballero, L.; Calvo, D.; Ladarescu, I.; Olleros-Rodriguez, P.; Domingo-Pardo, C.] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia, Spain, Email: javier.balibrea@ific.uv.es
Corporate Author Thesis
Publisher Elsevier Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:000641308300007 Approved no
Is ISI yes International Collaboration no
Call Number IFIC @ pastor @ Serial 4803
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Author n_TOF Collaboration (Manna, A. et al); Babiano-Suarez, V.; Caballero-Ontanaya, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L.
Title New insights on fission of 235U induced by high energy neutrons from a new measurement at n_TOF Type Journal Article
Year 2025 Publication Physics Letters B Abbreviated Journal Phys. Lett. B
Volume 860 Issue Pages (down) 139213 - 8pp
Keywords Nuclear reaction; Neutron-induced reaction; n_TOF; High energy; Fission process; Cross section measurement; Uranium-235
Abstract The U-235(n, f) reaction cross section was measured relative to neutron-proton elastic scattering for the first time in the energy region from 10 MeV to 440 MeV at the CERN n_TOF facility, extending the upper limit of the only previous measurement in the literature by more than 200 MeV. For neutron energies below 200 MeV, our results agree within one standard deviation with data in literature. Above 200 MeV, the comparison of model calculations to our data indicates the need to introduce a transient time in neutron-induced fission to allow the simultaneous description of (n, f) and (p, f) reactions.
Address [Manna, A.; Camprini, P. Console; Massimi, C.; Mengoni, A.; Vannini, G.; Ventura, A.; Castelluccio, D. M.; Junghans, A.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy, Email: alice.manna@bo.infn.it;
Corporate Author Thesis
Publisher Elsevier Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0370-2693 ISBN Medium
Area Expedition Conference
Notes WOS:001399996800001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 6468
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Author n_TOF Collaboration (Amaducci, S. et al); Babiano-Suarez, V.; Caballero-Ontanaya, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Measurement of the 140Ce(n,γ) Cross Section at n_TOF and Its Astrophysical Implications for the Chemical Evolution of the Universe Type Journal Article
Year 2024 Publication Physical Review Letters Abbreviated Journal Phys. Rev. Lett.
Volume 132 Issue 12 Pages (down) 122701 - 8pp
Keywords
Abstract 140Ce(n, gamma) is a key reaction for slow neutron -capture (s -process) nucleosynthesis due to being a bottleneck in the reaction flow. For this reason, it was measured with high accuracy (uncertainty approximate to 5%) at the n_TOF facility, with an unprecedented combination of a high purity sample and low neutron -sensitivity detectors. The measured Maxwellian averaged cross section is up to 40% higher than previously accepted values. Stellar model calculations indicate a reduction around 20% of the s -process contribution to the Galactic cerium abundance and smaller sizeable differences for most of the heavier elements. No variations are found in the nucleosynthesis from massive stars.
Address [Amaducci, S.; Cosentino, L.; Finocchiaro, P.; Brown, A.] INFN, Lab Nazl Sud, Catania, Italy
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0031-9007 ISBN Medium
Area Expedition Conference
Notes WOS:001202102900011 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 6074
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Author Torres-Sanchez, P.; Lerendegui-Marco, J.; Balibrea-Correa, J.; Babiano-Suarez, V.; Gameiro, B.; Ladarescu, I.; Alvarez-Rodriguez, P.; Daugas, J.M.; Koester, U.; Michelagnoli, C.; Pedrosa-Rivera, M.; Porras, I.; Ruiz-Magaña, M.J.; Ruiz-Ruiz, C.; Domingo-Pardo, C.
Title The potential of the i-TED Compton camera array for real-time boron imaging and determination during treatments in Boron Neutron Capture Therapy Type Journal Article
Year 2025 Publication Applied Radiation and Isotopes Abbreviated Journal Appl. Radiat. Isot.
Volume 217 Issue Pages (down) 111649 - 9pp
Keywords Boron neutron capture therapy; Compton imaging; Detector development; 3D reconstruction
Abstract This paper explores the adaptation and application of i-TED Compton imagers for real-time dosimetry in Boron Neutron Capture Therapy (BNCT). The i-TED array, previously utilized in nuclear astrophysics experiments at CERN, is being optimized for detecting and imaging 478 keV gamma-rays, critical for accurate BNCT dosimetry. Detailed Monte Carlo simulations were used to optimize the i-TED detector configuration and enhance its performance in the challenging radiation environment typical of BNCT. Additionally, advanced 3D image reconstruction algorithms, including a combination of back-projection and List-Mode Maximum Likelihood Expectation Maximization (LM-MLEM), are implemented and validated through simulations. Preliminary experimental tests at the Institut Laue-Langevin (ILL) demonstrate the potential of i-TED in simplified conditions, with ongoing experiments focusing on testing imaging capabilities in realistic BNCT conditions.
Address [Torres-Sanchez, Pablo; Lerendegui-Marco, Jorge; Balibrea-Correa, Javier; Babiano-Suarez, Victor; Gameiro, Bernardo; Ladarescu, Ion; Domingo-Pardo, Cesar] Univ Valencia, Inst Fis Corpuscular, CSIC, Valencia, Spain, Email: pablo.torres@ific.uv.es
Corporate Author Thesis
Publisher Pergamon-Elsevier Science Ltd Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0969-8043 ISBN Medium
Area Expedition Conference
Notes WOS:001420228100001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 6515
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Author n_TOF Collaboration (Alcayne, V. et al); Balibrea-Correa, J.; Domingo-Pardo, C.; Lerendegui-Marco, J.; Babiano-Suarez, V.; Ladarescu, I.
Title A Segmented Total Energy Detector (sTED) optimized for (n,γ) cross-section measurements at n_TOF EAR2 Type Journal Article
Year 2024 Publication Radiation Physics and Chemistry Abbreviated Journal Radiat. Phys. Chem.
Volume 217 Issue Pages (down) 111525 - 11pp
Keywords Neutron capture; PHWT; Scintillation detectors; Monte Carlo simulation
Abstract The neutron time-of-flight facility nTOF at CERN is a spallation source dedicated to measurements of neutroninduced reaction cross-sections of interest in nuclear technologies, astrophysics, and other applications. Since 2014, Experimental ARea 2 (EAR2) is operational and delivers a neutron fluence of similar to 4 center dot 10(7) neutrons per nominal proton pulse, which is similar to 50 times higher than the one of Experimental ARea 1 (EAR1) of similar to 8 center dot 10(5) neutrons per pulse. The high neutron flux at EAR2 results in high counting rates in the detectors that challenged the previously existing capture detection systems. For this reason, a Segmented Total Energy Detector (sTED) has been developed to overcome the limitations in the detector's response, by reducing the active volume per module and by using a photo-multiplier (PMT) optimized for high counting rates. This paper presents the main characteristics of the sTED, including energy and time resolution, response to gamma-rays, and provides as well details of the use of the Pulse Height Weighting Technique (PHWT) with this detector. The sTED has been validated to perform neutron-capture cross-section measurements in EAR2 in the neutron energy range from thermal up to at least 400 keV. The detector has already been successfully used in several measurements at nTOF EAR2.
Address [Alcayne, V.; Cano-Ott, D.; Garcia, J.; Gonzalez-Romero, E.; Martinez, T.; de Rada, A. Perez; Plaza, J.; Sanchez-Caballero, A.; Mendoza, E.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain, Email: victor.alcayne@ciemat.es
Corporate Author Thesis
Publisher Pergamon-Elsevier Science Ltd Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0969-806x ISBN Medium
Area Expedition Conference
Notes WOS:001185584800001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5999
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Author n_TOF Collaboration (Sosnin, N.V. et al.); Babiano-Suarez, V.; Caballero, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L.
Title Measurement of the 77Se(n,gamma) cross section up to 200 keV at the n_TOF facility at CERN Type Journal Article
Year 2023 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 107 Issue 6 Pages (down) 065805 - 9pp
Keywords
Abstract The 77Se(n,gamma) reaction is of importance for 77Se abundance during the slow neutron capture process in massive stars. We have performed a new measurement of the 77Se radiative neutron capture cross section at the Neutron Time-of-Flight facility at CERN. Resonance capture kernels were derived up to 51 keV and cross sections up to 200 keV. Maxwellian-averaged cross sections were calculated for stellar temperatures between kT = 5 keV and kT = 100 keV, with uncertainties between 4.2% and 5.7%. Our results lead to substantial decreases of 14% and 19% in 77Se abundances produced through the slow neutron capture process in selected stellar models of 15M0 and 2M0, respectively, compared to using previous recommendation of the cross section.
Address [V. Sosnin, N.; Lederer-Woods, C.; Garg, R.; Dietz, M.; Murphy, A. St. J.; Lonsdale, S.; Woods, P. J.] Univ Edinburgh, Sch Phys & Astron, Edinburgh, Scotland, Email: nsosnin@ed.ac.uk
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:001023903800002 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5599
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Author n_TOF Collaboration (Sosnin, N.V. et al); Babiano-Suarez, V.; Caballero-Ontanaya, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L.
Title Measurement of the 78Se(n, γ)79Se cross section up to 600 keV at the n_TOF facility at CERN Type Journal Article
Year 2024 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 110 Issue 6 Pages (down) 065805 - 12pp
Keywords
Abstract The Se-78(n, gamma)Se-79 cross section has a high impact on the abundances of Se-78 produced during the slow neutron capture process (s process) in massive stars. A measurement of the Se-78 radiative neutron capture cross section has been performed at the Neutron Time-of-Flight facility at CERN using a set of liquid scintillation detectors that have been optimized for a low sensitivity to neutrons. We present resonance capture kernels up to 70 keV and cross section from 70 to 600 keV. Maxwellian-averaged cross section (MACS) values were calculated for stellar temperatures between kT = 5 and 100 keV, with uncertainties between 4.6% and 5.8%. The new MACS values result in substantial decreases of 20-30% of Se-78 abundances produced in the s process in massive stars and AGB stars. Massive stars are now predicted to produce subsolar Se-78/Se-76 ratios, which is expected since Se-76 is an s-only isotope, while solar Se-78 abundances have also contributions from other nucleosynthesis processes.
Address [Sosnin, N. V.; Lederer-Woods, C.; Garg, R.; Dietz, M.; Lonsdale, S. J.; Murphy, A. St. J.; Woods, P. J.] Univ Edinburgh, Sch Phys & Astron, Edinburgh, Midlothian, Scotland, Email: nikolay.sosnin@manchester.ac.uk
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:001389541600005 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 6498
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Author n_TOF Collaboration (Garcia-Infantes, F. et al); Babiano-Suarez, V.; Balibrea-Correa, J.; Casanovas-Hoste, A.; Domingo-Pardo, C.; Ladarescu, I.; Lerendegui-Marco, J.
Title Measurement of the 176Yb(n,γ) cross section at the n_TOF facility at CERN Type Journal Article
Year 2024 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 110 Issue 6 Pages (down) 064619 - 16pp
Keywords
Abstract Background: The Yb-176(n, gamma)Yb-177 -> 177Lu reaction is of interest in nuclear medicine as it is the preferred production route for 177Lu. This radioisotope has seen a very fast growth of usage in nuclear medicine in recent years due to its outstanding properties. New data on this reaction could provide useful information for production at new facilities. Purpose: We aim to resolve resonances in the Yb-176(n, gamma)Yb-177 reaction for the first time. Previous capture measurement provided data at thermal point and encompassed integral measurements in the range from 3 keV to 1 MeV, where three time-of-flight measurements are available, but with low resolution to resolve the resonances. Transmission measurements from the 1970s resolved and analyzed some resonances. Method: We measure the neutron capture cross section of Yb-176(n, gamma)Yb-177 by means of the time-of-flight technique at the Experimental Area 1 of the n_TOF facility at CERN using an enriched (Yb2O3)-Yb-176 sample and an array of four C6D6 liquid scintillation detectors. Results: We have resolved 164 resonances up to 21 keV, including 96 new ones. We also provide new capture experimental data from 90 eV to 3 keV, and we extend the resolved resonance region up to 21 keV. In addition, resonance decay widths, Gamma(gamma) and Gamma(n), are provided for all resonances together with resonance energies. Conclusions: The Yb-176(n, gamma) Yb-177 reaction has been measured, providing resonance parameters for the first time from a few eV to 21 keV. The analysis of the resonances has been carried out and compared with previous works and existing libraries, revealing discrepancies due to the new information on Gamma(gamma) parameters. Our results are consistent with the Gamma(n) parameters obtained in transmission measurements.
Address [Garcia-Infantes, F.; Praena, J.; Es-Sghir, H. Amar; Martinez-Canada, M.; Porras, I.; Torres-Sanchez, P.] Univ Granada, Granada, Spain
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:001389562300002 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 6514
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