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Azevedo, C. D. R., Baeza, A., Chauveau, E., Corbacho, J. A., Diaz, J., Domange, J., et al. (2023). Design, setup and routine operation of a water treatment system for the monitoring of low activities of tritium in water. Nucl. Eng. Technol., 55(7), 2349–2355.
Abstract: In the TRITIUM project, an on-site monitoring system is being developed to measure tritium (3H) levels in water near nuclear power plants. The quite low-energy betas emitted by 3H have a very short average path in water (5 mm as shown by simulations for 18 keV electrons). This path would be further reduced by impurities present in the water, resulting in a significant reduction of the detection efficiency. Therefore, one of the essential requirements of the project is the elimination of these impurities through a filtration process and the removal of salts in solution. This paper describes a water treatment system developed for the project that meets the following requirements: the water produced should be of nearpure water quality according to ISO 3696 grade 3 standard (conductivity < 10 mS/cm); the system should operate autonomously and be remotely monitored.
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SuperNEMO Collaboration(Argyriades, J. et al), Carcel, S., Diaz, J., Monrabal, F., Serra, L., & Yahlali, N. (2010). Results of the BiPo-1 prototype for radiopurity measurements for the SuperNEMO double beta decay source foils. Nucl. Instrum. Methods Phys. Res. A, 622(1), 120–128.
Abstract: The development of BiPo detectors is dedicated to the measurement of extremely high radiopurity in (TI)-T-208 and Bi-214 for the SuperNEMO double beta decay source foils. A modular prototype, called BiPo-1, with 0.8 m(2) of sensitive surface area, has been running in the Modane Underground Laboratory since February, 2008. The goal of BiPo-1 is to measure the different components of the background and in particular the surface radiopurity of the plastic scintillators that make up the detector. The first phase of data collection has been dedicated to the measurement of the radiopurity in (TI)-T-208. After more than one year of background measurement, a surface activity of the scintillators of A((TI)-T-208) = 1.5 μBq/m(2) is reported here. Given this level of background, a larger BiPo detector having 12 m(2) of active surface area, is able to qualify the radiopurity of the SuperNEMO selenium double beta decay foils with the required sensitivity of A((TI)-T-208) <2 μBq/kg (90% CL.) with a six month measurement.
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NEMO-3 Collaboration(Argyriades, J. et al), Diaz, J., Martin-Albo, J., Monrabal, F., Novella, P., Serra, L., et al. (2011). Spectral modeling of scintillator for the NEMO-3 and SuperNEMO detectors. Nucl. Instrum. Methods Phys. Res. A, 625(1), 20–28.
Abstract: We have constructed a GEANT4-based detailed software model of photon transport in plastic sontillator blocks and have used it to study the NEMO-3 and SuperNEMO calorimeters employed in experiments designed to search for neutnnoless double beta decay We compare our simulations to measurements using conversion electrons from a calibration source of (BI)-B-207 and show that the agreement is improved if wavelength-dependent properties of the calorimeter are taken into account In this article we briefly describe our modeling approach and results of our studies.
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Gil, A., Diaz, J., Gomez-Cadenas, J. J., Herrero, V., Rodriguez, J., Serra, L., et al. (2012). Front-end electronics for accurate energy measurement of double beta decays. Nucl. Instrum. Methods Phys. Res. A, 695, 407–409.
Abstract: NEXT, a double beta decay experiment that will operate in Canfranc Underground Laboratory (Spain), aims at measuring the neutrinoless double-beta decay of the 136Xe isotope using a TPC filled with enriched Xenon gas at high pressure operated in electroluminescence mode. One technological challenge of the experiment is to achieve resolution better than 1% in the energy measurement using a plane of UV sensitive photomultipliers readout with appropriate custom-made front-end electronics. The front-end is designed to be sensitive to the single photo-electron to detect the weak primary scintillation light produced in the chamber, and also to be able to cope with the electroluminescence signal (several hundred times higher and with a duration of microseconds). For efficient primary scintillation detection and precise energy measurement of the electroluminescent signals the front-end electronics features low noise and adequate amplification. The signal shaping provided allows the digitization of the signals at a frequency as low as 40 MHz.
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NEXT Collaboration(Alvarez, V. et al), Carcel, S., Cervera-Villanueva, A., Diaz, J., Ferrario, P., Gil, A., et al. (2013). Near-intrinsic energy resolution for 30-662 keV gamma rays in a high pressure xenon electroluminescent TPC. Nucl. Instrum. Methods Phys. Res. A, 708, 101–114.
Abstract: We present the design, data and results from the NEXT prototype for Double Beta and Dark Matter (NEXT-DBDM) detector, a high-pressure gaseous natural xenon electroluminescent time projection chamber (TPC) that was built at the Lawrence Berkeley National Laboratory. It is a prototype of the planned NEXT-100 Xe-136 neutrino-less double beta decay (0 nu beta beta) experiment with the main objectives of demonstrating near-intrinsic energy resolution at energies up to 662 keV and of optimizing the NEXT-100 detector design and operating parameters. Energy resolutions of similar to 1% FWHM for 662 keV gamma rays were obtained at 10 and 15 atm and similar to 5% FWHM for 30 keV fluorescence xenon X-rays. These results demonstrate that 0.5% FWHM resolutions for the 2459 keV hypothetical neutrino-less double beta decay peak are realizable. This energy resolution is a factor 7-20 better than that of the current leading 0 nu beta beta experiments using liquid xenon and thus represents a significant advancement. We present also first results from a track imaging system consisting of 64 silicon photo-multipliers recently installed in NEXT-DBDM that, along with the excellent energy resolution, demonstrates the key functionalities required for the NEXT-100 0 nu beta beta search.
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NEXT Collaboration(Renner, J. et al), Alvarez, V., Carcel, S., Cervera-Villanueva, A., Diaz, J., Ferrario, P., et al. (2015). Ionization and scintillation of nuclear recoils in gaseous xenon. Nucl. Instrum. Methods Phys. Res. A, 793, 62–74.
Abstract: Ionization and scintillation produced by nuclear recoils in gaseous xenon at approximately 14 bar have been simultaneously observed in an electroluminescent time projection chamber. Neutrons from radioisotope a-Be neutron sources were used to induce xenon nuclear recoils, and the observed recoil spectra were compared to a detailed Monte Carlo employing estimated ionization and scintillation yields for nuclear recoils. The ability to discriminate between electronic and nuclear recoils using the ratio of ionization to primary scintillation is demonstrated. These results encourage further investigation on the use of xenon in the gas phase as a detector medium in dark matter direct detection experiments.
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NEXT Collaboration(Cebrian, S. et al), Alvarez, V., Carcel, S., Cervera-Villanueva, A., Diaz, J., Ferrario, P., et al. (2015). Accurate gamma and MeV-electron track reconstruction with an ultra-low diffusion Xenon/TMA TPC at 10 atm. Nucl. Instrum. Methods Phys. Res. A, 804, 8–24.
Abstract: We report the performance of a 10 atm Xenon/trimethylamine time projection chamber (TPC) for the detection of X-rays (30 keV) and gamma-rays (0.511-1.275 MeV) in conjunction with the accurate tracking of the associated electrons. When operated at such a high pressure and in similar to 1%-admixtures, trimethylamine (TMA) endows Xenon with an extremely low electron diffusion (1.3 +/- 0.13 mm-sigma (longitudinal), 0.95 +/- 0.20 mm-sigma (transverse) along 1 m drift) besides forming a convenient Penning-Fluorescent' mixture. The TPC, that houses 1.1 kg of gas in its fiducial volume, operated continuously for 100 live-days in charge amplification mode. The readout was performed through the recently introduced microbulk Micromegas technology and the AFTER chip, providing a 3D voxelization of 8 mm x 8 mm x 1.2 mm for approximately 10 cm/MeV-long electron tracks. Resolution in energy (epsilon) at full width half maximum (R) inside the fiducial volume ranged from R = 14.6% (30 keV) to R = 4.6% (1.275 MeV). This work was developed as part of the R&D program of the NEXT collaboration for future detector upgrades in the search of the neutrino-less double beta decay (beta beta 0 nu) in Xe-136, specifically those based on novel gas mixtures. Therefore we ultimately focus on the calorimetric and topological properties of the reconstructed MeV-electron tracks. In particular, the obtained energy resolution has been decomposed in its various contributions and improvements towards achieving the R =1.4%root MeV/epsilon levels obtained in small sensors are discussed.
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NEXT Collaboration(Azevedo, C. D. R. et al), Gomez-Cadenas, J. J., Alvarez, V., Benlloch-Rodriguez, J. M., Botas, A., Carcel, S., et al. (2018). Microscopic simulation of xenon-based optical TPCs in the presence of molecular additives. Nucl. Instrum. Methods Phys. Res. A, 877, 157–172.
Abstract: We introduce a simulation framework for the transport of high and low energy electrons in xenon-based optical time projection chambers (OTPCs). The simulation relies on elementary cross sections (electron-atom and electron-molecule) and incorporates, in order to compute the gas scintillation, the reaction/quenching rates (atom-atom and atom-molecule) of the first 41 excited states of xenon and the relevant associated excimers, together with their radiative cascade. The results compare positively with observations made in pure xenon and its mixtures with CO2 and CF4 in a range of pressures from 0.1 to 10 bar. This work sheds some light on the elementary processes responsible for the primary and secondary xenon-scintillation mechanisms in the presence of additives, that are of interest to the OTPC technology.
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NEXT Collaboration(Trindade, A. M. F. et al), Alvarez, V., Benlloch-Rodriguez, J. M., Botas, A., Carcel, S., Carrion, J. V., et al. (2018). Study of the loss of xenon scintillation in xenon-trimethylamine mixtures. Nucl. Instrum. Methods Phys. Res. A, 905, 22–28.
Abstract: This work investigates the capability of TMA ((CH3)(3)N) molecules to shift the wavelength of Xe VUV emission (160-188 nm) to a longer, more manageable, wavelength (260-350 nm). Light emitted from a Xe lamp was passed through a gas chamber filled with Xe-TMA mixtures at 800 Torr and detected with a photomultiplier tube. Using bandpass filters in the proper transmission ranges, no reemitted light was observed experimentally. Considering the detection limit of the experimental system, if reemission by TMA molecules occurs, it is below 0.3% of the scintillation absorbed in the 160-188 nm range. An absorption coefficient value for xenon VUV light by TMA of 0.43 +/- 0.03 cm(-1) Torr(-1) was also obtained. These results can be especially important for experiments considering TMA as a molecular additive to Xe in large volume optical time projection chambers.
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NEXT Collaboration(Felkai, R. et al), Sorel, M., Lopez-March, N., Gomez-Cadenas, J. J., Alvarez, V., Benlloch-Rodriguez, J. M., et al. (2018). Helium-Xenon mixtures to improve the topological signature in high pressure gas xenon TPCs. Nucl. Instrum. Methods Phys. Res. A, 905, 82–90.
Abstract: Within the framework of xenon-based double beta decay experiments, we propose the possibility to improve the background rejection of an electroluminescent Time Projection Chamber (EL TPC) by reducing the diffusion of the drifting electrons while keeping nearly intact the energy resolution of a pure xenon EL TPC. Based on state-of-the-art microscopic simulations, a substantial addition of helium, around 10 or 15 %, may reduce drastically the transverse diffusion down to 2.5 mm/root m from the 10.5 mm/root m of pure xenon. The longitudinal diffusion remains around 4 mm/root m. Light production studies have been performed as well. They show that the relative variation in energy resolution introduced by such a change does not exceed a few percent, which leaves the energy resolution practically unchanged. The technical caveats of using photomultipliers close to an helium atmosphere are also discussed in detail.
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