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Author |
n_TOF Collaboration (Lerendegui-Marco, J. et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
2 |
Pages |
024605 - 21pp |
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Keywords |
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Abstract |
The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA. |
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Address |
[Lerendegui-Marco, J.; Guerrero, C.; Quesada, J. M.; Cortes-Giraldo, M. A.; Praena, J.; Sabate-Gilarte, M.] Univ Seville, Dept Fis Atom Mol & Nucl, E-41012 Seville, Spain, Email: cguerrero4@us.es |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Notes |
WOS:000424190700001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration  |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3474 |
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Author |
AGATA Collaboration (Lalovic, N. et al); Gadea, A.; Domingo-Pardo, C. |
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Title |
Study of isomeric states in Pb-198, Pb-200, Pb-202, Pb-206 and Hg-206 populated in fragmentation reactions |
Type |
Journal Article |
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Year |
2018 |
Publication |
Journal of Physics G |
Abbreviated Journal |
J. Phys. G |
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Volume |
45 |
Issue |
3 |
Pages |
035105 - 27pp |
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Keywords |
gamma-ray spectroscopy; relativistic projectile fragmentation; direct reactions; isomeric decays; electromagnetic transitions; nuclear shell model |
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Abstract |
Isomeric states in isotopes in the vicinity of doubly-magic Pb-208 were populated following reactions of a relativistic Pb-208 primary beam impinging on a Be-9 fragmentation target. Secondary beams of Pb-198,Pb-200,Pb-202,Pb-206 and Hg-206 were isotopically separated and implanted in a passive stopper positioned in the focal plane of the GSI Fragment Separator. Delayed gamma rays were detected with the Advanced Gamma Tracking Array (AGATA). Decay schemes were reevaluated and interpreted with shell-model calculations. The momentum-dependent population of isomeric states in the two-nucleon hole nuclei Pb-206/Hg-206 was found to differ from the population of multi neutron-hole isomeric states in Pb-198,Pb-200,Pb-202. |
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Address |
[Lalovic, N.; Rudolph, D.; Sarmiento, L. G.; Golubev, P.; Fahlander, C.; Gellanki, J.] Lund Univ, Dept Phys, SE-22100 Lund, Sweden, Email: Natasa.Lalovic@nuclear.lu.se |
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Iop Publishing Ltd |
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English |
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ISSN |
0954-3899 |
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Notes |
WOS:000424906600001 |
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no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3488 |
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Author |
n_TOF Collaboration (Barbagallo, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Experimental setup and procedure for the measurement of the Be-7(n,p)Li-7 reaction at n_TOF |
Type |
Journal Article |
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Year |
2018 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
887 |
Issue |
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Pages |
27-33 |
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Keywords |
Cosmological Lithium problem; Big bang nucleosynthesis; Be-7(n,p)Li-7 reaction; n_TOF spallation neutron source |
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Abstract |
Following the completion of the second neutron beam line and the related experimental area (EAR2) at the n_TOF spallation neutron source at CERN, several experiments were planned and performed. The high instantaneous neutron flux available in EAR2 allows to investigate neutron induced reactions with charged particles in the exit channel even employing targets made out of small amounts of short-lived radioactive isotopes. After the successful measurement of the Be-7(n,alpha)alpha cross section, the Be-7(n,p)Li-7 reaction was studied in order to provide still missing cross section data of relevance for Big Bang Nucleosynthesis (BBN), in an attempt to find a solution to the cosmological Lithium abundance problem. This paper describes the experimental setup employed in such a measurement and its characterization. |
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Address |
[Barbagallo, M.; Mastromarco, M.; Damone, L. A.; Mazzone, A.; Colonna, N.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: finocchiaro@lns.infn.ir |
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Publisher |
Elsevier Science Bv |
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English |
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Edition |
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ISSN |
0168-9002 |
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Notes |
WOS:000427814400005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3528 |
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Author |
n_TOF Collaboration (Praena, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Preparation and characterization of S-33 samples for S-33(n,alpha)Si-30 cross-section measurements at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2018 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
890 |
Issue |
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Pages |
142-147 |
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Keywords |
Neutron induced alpha emission; Thermal evaporation; Rutherford backscattering |
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Abstract |
Thin S-33 samples for the study of the S-33(n,alpha)Si-30 cross-section at the n_TOF facility at CERN were made by thermal evaporation of S-33 powder onto a dedicated substrate made of kapton covered with thin layers of copper, chromium and titanium. This method has provided for the first time bare sulfur samples a few centimeters in diameter. The samples have shown an excellent adherence with no mass loss after few years and no sublimation in vacuum at room temperature. The determination of the mass thickness of S-33 has been performed by means of Rutherford backscattering spectrometry. The samples have been successfully tested under neutron irradiation. |
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Address |
[Praena, J.; Porras, I.] Univ Granada, Granada, Spain, Email: jpraena@ugr.es |
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Elsevier Science Bv |
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English |
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ISSN |
0168-9002 |
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Notes |
WOS:000427814900020 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3537 |
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Author |
n_TOF Collaboration (Praena, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement and resonance analysis of the S-33(n,alpha)Si-30 cross section at the CERN n_TOF facility in the energy region from 10 to 300 keV |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
6 |
Pages |
064603 - 10pp |
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Abstract |
The (33)(n , alpha)Si-30 cross section has been measured at the neutron time-of-flight (n_TOF) facility at CERN in the neutron energy range from 10 to 300 keV relative to the B-10(n, alpha)(7) Li cross-section standard. Both reactions were measured simultaneously with a set of micromegas detectors. The flight path of 185 m has allowed us to obtain the cross section with high-energy resolution. An accurate description of the resonances has been performed by means of the multilevel multichannel R-matrix code SAMMY. The results show a significantly higher area of the biggest resonance (13.45 keV) than the unique high-resolution (n , alpha) measurement. The new parametrization of the 13.45-keV resonance is similar to that of the unique transmission measurement. This resonance is a matter of research in neutron-capture therapy. The S-33(n, alpha)Si-30 cross section has been studied in previous works because of its role in the production of S-36 in stars, which is currently overproduced in stellar models compared to observations. |
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Address |
[Praena, J.; Porras, I] Univ Granada, Granada, Spain, Email: jpraena@ugr.es |
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Publisher |
Amer Physical Soc |
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English |
Summary Language |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Conference |
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Notes |
WOS:000434017300004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3597 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Damone, L. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Be-7 (n,p)Li-7 Reaction and the Cosmological Lithium Problem: Measurement of the Cross Section in a Wide Energy Range at n_TOF at CERN |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
121 |
Issue |
4 |
Pages |
042701 - 7pp |
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Keywords |
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Abstract |
We report on the measurement of the Be-7(n,p)Li-7 cross section from thermal to approximately 325 keV neutron energy, performed in the high-flux experimental area (EAR2) of the n_TOF facility at CERN. This reaction plays a key role in the lithium yield of the big bang nucleosynthesis (BBN) for standard cosmology. The only two previous time-of-flight measurements performed on this reaction did not cover the energy window of interest for BBN, and they showed a large discrepancy between each other. The measurement was performed with a Si telescope and a high-purity sample produced by implantation of a Be-7 ion beam at the ISOLDE facility at CERN. While a significantly higher cross section is found at low energy, relative to current evaluations, in the region of BBN interest, the present results are consistent with the values inferred from the time-reversal Li-7(p,n)Be-7 reaction, thus yielding only a relatively minor improvement on the so-called cosmological lithium problem. The relevance of these results on the near-threshold neutron production in the p + Li-7 reaction is also discussed. |
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Address |
[Damone, L.; Barbagallo, M.; Mastromarco, M.; Colonna, N.; Mazzone, A.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: alberto.mengoni@enea.it |
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Corporate Author |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0031-9007 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000439547100004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3674 |
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Author |
Caballero-Folch, R. et al; Agramunt, J.; Tain, J.L.; Algora, A.; Domingo-Pardo, C.; Guadilla, V.; Montaner-Piza, A.; Orrigo, S.E.A.; Rubio, B.; Tarifeño-Saldivia, A.; Tolosa-Delgado, A. |
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Title |
First determination of beta-delayed multiple neutron emission beyond A=100 through direct neutron measurement: The P-2n value of Sb-136 |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
98 |
Issue |
3 |
Pages |
034310 - 10pp |
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Keywords |
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Abstract |
Background: beta-delayed multiple neutron emission has been observed for some nuclei with A <= 100 being the Rb-100 the heaviest beta 2n emitter measured to date. So far only 25 P-2n values have been determined for the approximate to 300 nuclei that may decay in this way. Accordingly it is of interest to measure P-2n values for the other possible multiple neutron emitters throughout the chart of the nuclides. It is of particular interest to make such a measurement for nuclei with A > 100 to test the predictions of theoretical models and simulation tools for the decays of heavy nuclei in the region of very neutron-rich nuclei. In addition the decay properties of these nuclei are fundamental for the understanding of astrophysical nucleosynthesis processes such as the r-process and safety inputs for nuclear reactors. Purpose: To determine for the first time the two-neutron branching ratio the P-2n value for Sb-136 through a direct neutron measurement and to provide precise P-1n values for Sb-136 and Te-136. Method: A pure beam of each isotope of interest was provided by the JYFLTRAP Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility of the University of Jyvaskyla Finland. The purified ions were implanted into a moving tape at the end of the beam line. The detection setup consisted of a plastic scintillator placed right behind the implantation point after the tape to register the beta decays and the BELEN detector based on neutron counters embedded in a polyethylene matrix. The analysis was based on the study of the beta- and neutron-growth-and-decay curves and the beta-one-neutron and beta-two-neutron time correlations which allowed us the determination of the neutron branching ratios. Results: The P-2n value of Sb-136 was found to be 0.14(3)% and the measured P-1n values for Sb-136 and Te-136 were found to be 32.2(15)% and 1.47(6)% respectively. Conclusions: The measured P-2n value is a factor 44 smaller than predicted by the finite-range droplet model plus the quasiparticle random-phase approximation (FRDM+QRPA) model used for r-process calculations. |
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Address |
[Caballero-Folch, R.; Dillmann, I] TRIUMF, Vancouver, BC V6T 2A3, Canada, Email: rcaballero-folch@triumf.ca |
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Publisher |
Amer Physical Soc |
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English |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Expedition |
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Conference |
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Notes |
WOS:000444207600003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3728 |
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Author |
Delafosse, C. et al; Gadea, A.; Perez-Vidal, R.M.; Domingo-Pardo, C. |
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Title |
Pseudospin Symmetry and Microscopic Origin of Shape Coexistence in the Ni-78 Region: A Hint from Lifetime Measurements |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
121 |
Issue |
19 |
Pages |
192502 - 7pp |
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Keywords |
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Abstract |
Lifetime measurements of excited states of the light N = 52 isotones Kr-88, Se-86, and Ge-84 have been performed, using the recoil distance Doppler shift method and VAMOS and AGATA spectrometers for particle identification and gamma spectroscopy, respectively. The reduced electric quadrupole transition probabilities B(E2; 2(+)-> 0(+)) and B(E2; 4(+)-> 2(+)) were obtained for the first time for the hard-to-reach 84Ge. While the B(E2; 2(+)-> 0(+) ) values of Kr-88, Se-86 saturate the maximum quadrupole collectivity offered by the natural valence (3s, 2d, 1g(7/2), 1h(11/2)) space of an inert Ni-78 core, the value obtained for Ge-84 largely exceeds it, suggesting that shape coexistence phenomena, previously reported at N less than or similar to 49, extend beyond N = 50. The onset of collectivity at Z = 32 is understood as due to a pseudo-SU(3) organization of the proton single-particle sequence reflecting a clear manifestation of pseudospin symmetry. It is realized that the latter provides actually reliable guidance for understanding the observed proton and neutron single particle structure in the whole medium-mass region, from Ni to Sn, pointing towards the important role of the isovector-vector rho field in shell-structure evolution. |
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Address |
[Delafosse, C.; Verney, D.; Marevic, P.; Gottardo, A.; Babo, M.; Franchoo, S.; Ibrahim, F.; Matea, I; Olivier, L.; Portail, C.; Stefan, I] Univ Paris Saclay, Univ Paris Sud, CNRS IN2P3, Inst Phys Nucl, F-91406 Orsay, France, Email: verney@ipno.in2p3.fr |
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Publisher |
Amer Physical Soc |
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English |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0031-9007 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000449791600008 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3800 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Mastromarco, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Cross section measurements of Gd-155,Gd-157(n,) induced by thermal and epithermal neutrons |
Type |
Journal Article |
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Year |
2019 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
55 |
Issue |
1 |
Pages |
9 - 20pp |
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Keywords |
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Abstract |
Neutron capture cross section measurements on Gd-155 and Gd-157 were performed using the time-of-flight technique at the nTOF facility at CERN on isotopically enriched samples. The measurements were carried out in the nTOF experimental area EAR1, at 185 m from the neutron source, with an array of 4 C6D6 liquid scintillation detectors. At a neutron kinetic energy of 0.0253 eV, capture cross sections of 62.2(2.2) and 239.8(8.4) kilobarn have been derived for Gd-155 and Gd-157, respectively, with up to 6% deviation relative to values presently reported in nuclear data libraries, but consistent with those values within 1.6 standard deviations. A resonance shape analysis has been performed in the resolved resonance region up to 181 eV and 307 eV, respectively for Gd-155 and Gd-157, where on average, resonance parameters have been found in good agreement with evaluations. Above these energies and up to 1 keV, the observed resonance-like structure of the cross section has been analysed and characterised. From a statistical analysis of the observed neutron resonances we deduced: neutron strength function of 2.01(28)x10-4 and 2.17(41)x10-4; average total radiative width of 106.8(14) meV and 101.1(20) meV and s-wave resonance spacing 1.6(2) eV and 4.8(5) eV for n + Gd-155 and n + Gd-157 systems, respectively. |
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Address |
[Mastromarco, M.; Barbagallo, M.; Colonna, N.; Damone, L. A.; Mazzone, A.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: massimi@bo.infn.it |
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Publisher |
Springer |
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English |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Conference |
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Notes |
WOS:000456675600003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3892 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Lederer-Woods, C. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement of Ge-73(n, gamma) cross sections and implications for stellar nucleosynthesis |
Type |
Journal Article |
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Year |
2019 |
Publication |
Physics Letters B |
Abbreviated Journal |
Phys. Lett. B |
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Volume |
790 |
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Pages |
458-465 |
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Keywords |
Nucleosynthesis; Neutron capture; s process; Germanium; n_TOF |
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Abstract |
Ge-73(n, gamma) cross sections were measured at the neutron time-of-flight facility n_TOF at CERN up to neutron energies of 300 keV, providing for the first time experimental data above 8 keV. Results indicate that the stellar cross section at kT = 30 keV is 1.5 to 1.7 times higher than most theoretical predictions. The new cross sections result in a substantial decrease of Ge-73 produced in stars, which would explain the low isotopic abundance of Ge-73 in the solar system. |
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Address |
[Lederer-Woods, C.; Battino, U.; Tattersalla, A.; Dietz, M.] Univ Edinburgh, Sch Phys & Astron, Edinburgh, Midlothian, Scotland, Email: claudia.lederer-woods@ed.ac.uk |
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Publisher |
Elsevier Science Bv |
Place of Publication |
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Language |
English |
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Original Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0370-2693 |
ISBN |
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Notes |
WOS:000460118200058 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3936 |
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