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Author  |
n_TOF Collaboration (Mingrone, F. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
Neutron capture cross section measurement of U-238 at the CERN n_TOF facility in the energy region from 1 eV to 700 keV |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
95 |
Issue |
3 |
Pages |
034604 - 14pp |
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Abstract |
The aim of this work is to provide a precise and accurate measurement of the U-238(n,gamma) reaction cross section in the energy region from 1 eV to 700 keV. This reaction is of fundamental importance for the design calculations of nuclear reactors, governing the behavior of the reactor core. In particular, fast reactors, which are experiencing a growing interest for their ability to burn radioactive waste, operate in the high energy region of the neutron spectrum. In this energy region most recent evaluations disagree due to inconsistencies in the existing measurements of up to 15%. In addition, the assessment of nuclear data uncertainty performed for innovative reactor systems shows that the uncertainty in the radiative capture cross section of U-238 should be further reduced to 1-3% in the energy region from 20 eV to 25 keV. To this purpose, addressed by the Nuclear Energy Agency as a priority nuclear data need, complementary experiments, one at the GELINA and two at the nTOF facility, were proposed and carried out within the 7th Framework Project ANDES of the European Commission. The results of one of these U-238(n, gamma) measurements performed at the nTOF CERN facility are presented in this work. The gamma-ray cascade following the radiative neutron capture has been detected exploiting a setup of two C6D6 liquid scintillators. Resonance parameters obtained from this work are on average in excellent agreement with the ones reported in evaluated libraries. In the unresolved resonance region, this work yields a cross section in agreement with evaluated libraries up to 80 keV, while for higher energies our results are significantly higher. |
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Address |
[Mingrone, F.; Berthoumieux, E.; Brugger, M.; Calviani, M.; Cerutti, F.; Chiaveri, E.; Chin, M.; Guerrero, C.; Hernandez-Prieto, A.; Kadi, Y.; Losito, R.; Rubbia, C.; Tsinganis, A.; Vlachoudis, V.] CERN, European Org Nucl Res, Geneva, Switzerland, Email: federica.mingrone@cern.ch |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Conference |
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Notes |
WOS:000396022500002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3030 |
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Author |
n_TOF Collaboration (Michalopoulou, V. et al); Babiano-Suarez, V.; Caballero, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L. |
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Title |
Measurement of the neutron-induced fission cross section of Th-230 at the CERN n_TOF facility |
Type |
Journal Article |
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Year |
2023 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
108 |
Issue |
1 |
Pages |
014616 - 15pp |
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Abstract |
The neutron-induced fission cross section of Th-230 has been measured at the neutron time-of-flight facility n_TOF located at CERN. The experiment was performed at the experimental area EAR-1 with a neutron flight path of 185 m, using Micromegas detectors for the detection of the fission fragments. The Th-230(n, f ) cross section was determined relative to the U-235(n, f ) one, covering the energy range from the fission threshold up to 400 MeV. The results from the present work are compared with existing cross-section datasets and the observed discrepancies are discussed and analyzed. Finally, using the code EMPIRE 3.2.3 a theoretical study, based on the statistical model, was performed leading to a satisfactory reproduction of the experimental results with the proper tuning of the respective parameters, while for incident neutron energy beyond 200 MeV the fission of( 230)Th was described by Monte Carlo simulations. |
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Address |
[Michalopoulou, V; Stamatopoulos, A.; Diakaki, M.; Vlastou, R.; Kokkoris, M.; Tassan-Got, L.] Natl Tech Univ Athens, Dept Phys, Zografou Campus, Athens, Greece, Email: veatriki.michalopoulou@cern.ch |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Conference |
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Notes |
WOS:001063908000001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5700 |
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Author |
n_TOF Collaboration (Mendoza, E. et al); Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement and analysis of the Am-241 neutron capture cross section at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
5 |
Pages |
054616 - 21pp |
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Keywords |
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Abstract |
The Am-241(n, gamma) cross section has been measured at the nTOF facility at CERN with the nTOF BaF2 Total Absorption Calorimeter in the energy range between 0.2 eV and 10 keV. Our results are analyzed as resolved resonances up to 700 eV, allowing a more detailed description of the cross section than in the current evaluations, which contain resolved resonances only up to 150-160 eV. The cross section in the unresolved resonance region is perfectly consistent with the predictions based on the average resonance parameters deduced from the resolved resonances, thus obtaining a consistent description of the cross section in the full neutron energy range under study. Below 20 eV, our results are in reasonable agreement with JEFF-3.2 as well as with the most recent direct measurements of the resonance integral, and differ up to 20-30% with other experimental data. Between 20 eV and 1 keV, the disagreement with other experimental data and evaluations gradually decreases, in general, with the neutron energy. Above 1 keV, we find compatible results with previously existing values. |
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Address |
[Mendoza, E.; Cano-Ott, D.; Balibrea, J.; Becares, V; Garcia, A. R.; Gonzalez, E.; Lopez, D.; Martinez, T.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain, Email: emilio.mendoza@ciemat.es |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Conference |
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Notes |
WOS:000433032300001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3584 |
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Author |
n_TOF Collaboration (Mazzone, A. et al); Babiano-Suarez, V; Caballero, L.; Domingo-Pardo, C.; Ladarescu, I; Tain, J.L. |
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Title |
Measurement of the Gd-154(n, gamma) cross section and its astrophysical implications |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physics Letters B |
Abbreviated Journal |
Phys. Lett. B |
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Volume |
804 |
Issue |
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Pages |
135405 - 6pp |
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Keywords |
s process; Gd-154; Neutron time of flight; n_TOF |
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Abstract |
The neutron capture cross section of Gd-154 was measured from 1 eV to 300 keV in the experimental area located 185 m from the CERN n_TOF neutron spallation source, using a metallic sample of gadolinium, enriched to 67% in Gd-154. The capture measurement, performed with four C6D6 scintillation detectors, has been complemented by a transmission measurement performed at the GELINA time-of-flight facility (JRC-Geel), thus minimising the uncertainty related to sample composition. An accurate Maxwellian averaged capture cross section (MACS) was deduced over the temperature range of interest for s process nucleosynthesis modelling. We report a value of 880(50) mb for the MACS at kT = 30 keV, significantly lower compared to values available in literature. The new adopted Gd-154(n, gamma) cross section reduces the discrepancy between observed and calculated solar s-only isotopic abundances predicted by s-process nucleosynthesis models. |
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Address |
[Mazzone, A.; Barbagallo, M.; Colonna, N.; Damone, L. A.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Bari, Italy, Email: Cristian.Massimi@bo.infn.it |
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Publisher |
Elsevier |
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English |
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Abbreviated Series Title |
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Series Issue |
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Edition |
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ISSN |
0370-2693 |
ISBN |
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Conference |
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Notes |
WOS:000548740300022 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4464 |
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Author |
n_TOF Collaboration (Mastromarco, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Cross section measurements of Gd-155,Gd-157(n,) induced by thermal and epithermal neutrons |
Type |
Journal Article |
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Year |
2019 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
55 |
Issue |
1 |
Pages |
9 - 20pp |
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Keywords |
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Abstract |
Neutron capture cross section measurements on Gd-155 and Gd-157 were performed using the time-of-flight technique at the nTOF facility at CERN on isotopically enriched samples. The measurements were carried out in the nTOF experimental area EAR1, at 185 m from the neutron source, with an array of 4 C6D6 liquid scintillation detectors. At a neutron kinetic energy of 0.0253 eV, capture cross sections of 62.2(2.2) and 239.8(8.4) kilobarn have been derived for Gd-155 and Gd-157, respectively, with up to 6% deviation relative to values presently reported in nuclear data libraries, but consistent with those values within 1.6 standard deviations. A resonance shape analysis has been performed in the resolved resonance region up to 181 eV and 307 eV, respectively for Gd-155 and Gd-157, where on average, resonance parameters have been found in good agreement with evaluations. Above these energies and up to 1 keV, the observed resonance-like structure of the cross section has been analysed and characterised. From a statistical analysis of the observed neutron resonances we deduced: neutron strength function of 2.01(28)x10-4 and 2.17(41)x10-4; average total radiative width of 106.8(14) meV and 101.1(20) meV and s-wave resonance spacing 1.6(2) eV and 4.8(5) eV for n + Gd-155 and n + Gd-157 systems, respectively. |
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Address |
[Mastromarco, M.; Barbagallo, M.; Colonna, N.; Damone, L. A.; Mazzone, A.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: massimi@bo.infn.it |
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Publisher |
Springer |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000456675600003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3892 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Mastromarco, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
High accuracy, high resolution U-235(n,f) cross section from n_TOF (CERN) from 18 meV to 10 keV |
Type |
Journal Article |
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Year |
2022 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
58 |
Issue |
8 |
Pages |
147 - 13pp |
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Keywords |
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Abstract |
The U-235(n,f) cross section was measured in a wide energy range (18 meV-170 keV) at the nTOF facility at CERN, relative to Li-6(n,t) and B-10(n,alpha) standard reactions, with high resolution and accuracy, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. In this paper we report on the results in the region between 18 meV and 10 keV neutron energy. A resonance analysis has been performed up to 200 eV, with the code SAMMY. The resulting fission kernels are compared with the ones extracted on the basis of the resonance parameters of the most recent major evaluated data libraries. A comparison of the nTOF data with the evaluated cross sections is also performed from thermal to 10 keV neutron energy for the energy-averaged cross section in energy groups of suitably chosen width. A good agreement, within 0.5%, is found on average between the new results and the latest evaluated data files ENDF/B-VIII.0 and JEFF-3.3, as well as with respect to the broad group average fission cross section established in the framework of the standard working group of IAEA (the so-called reference file). However, some discrepancies, of up to 4%, are still present in some specific energy regions. The new dataset here presented, characterized by a unique combination of high resolution and accuracy, low background and wide energy range, can help to improve the evaluations from the Resolved Resonance Region up to 10 keV, also reducing the uncertainties that affect this region. |
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Address |
[Mastromarco, M.; Colonna, N.; Diacono, D.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: amaducci@lns.infn.it |
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Publisher |
Springer |
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English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Expedition |
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Conference |
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Notes |
WOS:000840312100002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5328 |
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Author |
n_TOF Collaboration (Massimi, C. et al.); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
Neutron spectroscopy of Mg-26 states: Constraining the stellar neutron source Ne-22(alpha, n)Mg-25 |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physics Letters B |
Abbreviated Journal |
Phys. Lett. B |
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Volume |
768 |
Issue |
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Pages |
1-6 |
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Keywords |
s Process; alpha+Ne-22; Neutron spectroscopy |
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Abstract |
This work reports on accurate, high-resolution measurements of the Mg-25(n, gamma)Mg-26 and Mg-25(n, tot) cross sections in the neutron energy range from thermal to about 300 keV, leading to a significantly improved Mg-25(n, gamma)Mg-26 parametrization. The relevant resonances for n+Mg-25 were characterized from a combined R-matrix analysis of the experimental data. This resulted in an unambiguous spin/parity assignment of the corresponding excited states in Mg-26. With this information experimental upper limits of the reaction rates for Ne-22(alpha, n)Mg-25 and Ne-22(alpha, gamma)Mg-26 were established, potentially leading to a significantly higher (alpha, n)/(alpha, gamma) ratio than previously evaluated. The impact of these results has been studied for stellar models in the mass range 2 to 25 M-circle dot. (C) 2017 The Author(s). Published by Elsevier B.V. |
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Address |
[Massimi, C.; Barbagallo, M.; Becvar, F.; Bisterzok, S.; Castelluccio, D. M.; Eleftheriadis, C.; Finocchiaro, P.; Kokkoris, M.; Marganiec, J.; Plompen, A.; Praena, J.; Rubbia, C.; Weiss, C.] Ist Nazl Fis Nucl, Bologna, Italy, Email: cristian.massimi@bo.infn.it |
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Publisher |
Elsevier Science Bv |
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English |
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ISSN |
0370-2693 |
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Expedition |
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Conference |
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Notes |
WOS:000400677700001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3112 |
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Author |
n_TOF Collaboration (Lerendegui-Marco, J. et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
2 |
Pages |
024605 - 21pp |
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Keywords |
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Abstract |
The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA. |
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Address |
[Lerendegui-Marco, J.; Guerrero, C.; Quesada, J. M.; Cortes-Giraldo, M. A.; Praena, J.; Sabate-Gilarte, M.] Univ Seville, Dept Fis Atom Mol & Nucl, E-41012 Seville, Spain, Email: cguerrero4@us.es |
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Amer Physical Soc |
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English |
Summary Language |
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Abbreviated Series Title |
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Series Volume |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Expedition |
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Conference |
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Notes |
WOS:000424190700001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3474 |
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Author |
n_TOF Collaboration (Lederer-Woods, C. et al.); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Destruction of the cosmic gamma-ray emitter Al-26 in massive stars: Study of the key Al-26(n, p) reaction |
Type |
Journal Article |
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Year |
2021 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
104 |
Issue |
2 |
Pages |
L022803 - 7pp |
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Keywords |
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Abstract |
The Al-26(n, p) Mg-26 reaction is the key reaction impacting on the abundances of the cosmic gamma-ray emitter Al-26 produced in massive stars and impacts on the potential pollution of the early solar system with Al-26 by asymptotic giant branch stars. We performed a measurement of the Al-26(n, p) Mg-26 cross section at the high-flux beam line EAR-2 at the n_TOF facility (CERN). We report resonance strengths for eleven resonances, nine being measured for the first time, while there is only one previous measurement for the other two. Our resonance strengths are significantly lower than the only previous values available. Our cross-section data range to 150 keV neutron energy, which is sufficient for a reliable determination of astrophysical reactivities up to 0.5 GK stellar temperature. |
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Address |
[Lederer-Woods, C.; Woods, P. J.; Davinson, T.; Kahl, D.; Lonsdale, S. J.] Univ Edinburgh, Sch Phys & Astron, Peter Guthrie Tait Rd, Edinburgh EH9 3FD, Midlothian, Scotland, Email: claudia.lederer-woods@ed.ac.uk |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
ISBN |
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Expedition |
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Conference |
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Notes |
WOS:000691442700005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4949 |
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Author |
n_TOF Collaboration (Lederer-Woods, C. et al.); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Destruction of the cosmic gamma-ray emitter Al-26 in massive stars: Study of the key Al-26(n, alpha) reaction |
Type |
Journal Article |
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Year |
2021 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
104 |
Issue |
3 |
Pages |
L032803 - 6pp |
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Keywords |
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Abstract |
Neutron destruction reactions of the cosmic gamma-ray emitter Al-26 are of importance to determine the amount of Al-26 ejected into our galaxy by supernova explosions and for Al-26 production in asymptotic giant branch stars. We performed a new measurement of the Al-26(n, alpha) reaction up to 160-keV neutron energy at the neutron time-of-flight facilities n_TOF at CERN and GELINA at EC-JRC. We provide strengths for ten resonances, six of them for the first time. We use our data to calculate astrophysical reactivities for stellar temperatures up to 0.7 GK. Our results resolve a discrepancy between the two previous direct measurements of this reaction, and indicate higher stellar destruction rates than the most recently recommended reactivity. |
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Address |
[Lederer-Woods, C.; Woods, P. J.; Davinson, T.; Estrade, A.; Kahl, D.; Lonsdale, S. J.] Univ Edinburgh, Sch Phys & Astron, Peter Guthrie Tait Rd, Edinburgh EH9 3FD, Midlothian, Scotland, Email: claudia.lederer-woods@ed.ac.uk |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Notes |
WOS:000704560300002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
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4988 |
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