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Author  |
n_TOF Collaboration (Mastromarco, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Cross section measurements of Gd-155,Gd-157(n,) induced by thermal and epithermal neutrons |
Type |
Journal Article |
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Year |
2019 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
55 |
Issue |
1 |
Pages |
9 - 20pp |
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Abstract |
Neutron capture cross section measurements on Gd-155 and Gd-157 were performed using the time-of-flight technique at the nTOF facility at CERN on isotopically enriched samples. The measurements were carried out in the nTOF experimental area EAR1, at 185 m from the neutron source, with an array of 4 C6D6 liquid scintillation detectors. At a neutron kinetic energy of 0.0253 eV, capture cross sections of 62.2(2.2) and 239.8(8.4) kilobarn have been derived for Gd-155 and Gd-157, respectively, with up to 6% deviation relative to values presently reported in nuclear data libraries, but consistent with those values within 1.6 standard deviations. A resonance shape analysis has been performed in the resolved resonance region up to 181 eV and 307 eV, respectively for Gd-155 and Gd-157, where on average, resonance parameters have been found in good agreement with evaluations. Above these energies and up to 1 keV, the observed resonance-like structure of the cross section has been analysed and characterised. From a statistical analysis of the observed neutron resonances we deduced: neutron strength function of 2.01(28)x10-4 and 2.17(41)x10-4; average total radiative width of 106.8(14) meV and 101.1(20) meV and s-wave resonance spacing 1.6(2) eV and 4.8(5) eV for n + Gd-155 and n + Gd-157 systems, respectively. |
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Address |
[Mastromarco, M.; Barbagallo, M.; Colonna, N.; Damone, L. A.; Mazzone, A.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: massimi@bo.infn.it |
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Springer |
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English |
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ISSN |
1434-6001 |
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Conference |
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Notes |
WOS:000456675600003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3892 |
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Author |
n_TOF Collaboration (Mastromarco, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
High accuracy, high resolution U-235(n,f) cross section from n_TOF (CERN) from 18 meV to 10 keV |
Type |
Journal Article |
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Year |
2022 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
58 |
Issue |
8 |
Pages |
147 - 13pp |
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Abstract |
The U-235(n,f) cross section was measured in a wide energy range (18 meV-170 keV) at the nTOF facility at CERN, relative to Li-6(n,t) and B-10(n,alpha) standard reactions, with high resolution and accuracy, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. In this paper we report on the results in the region between 18 meV and 10 keV neutron energy. A resonance analysis has been performed up to 200 eV, with the code SAMMY. The resulting fission kernels are compared with the ones extracted on the basis of the resonance parameters of the most recent major evaluated data libraries. A comparison of the nTOF data with the evaluated cross sections is also performed from thermal to 10 keV neutron energy for the energy-averaged cross section in energy groups of suitably chosen width. A good agreement, within 0.5%, is found on average between the new results and the latest evaluated data files ENDF/B-VIII.0 and JEFF-3.3, as well as with respect to the broad group average fission cross section established in the framework of the standard working group of IAEA (the so-called reference file). However, some discrepancies, of up to 4%, are still present in some specific energy regions. The new dataset here presented, characterized by a unique combination of high resolution and accuracy, low background and wide energy range, can help to improve the evaluations from the Resolved Resonance Region up to 10 keV, also reducing the uncertainties that affect this region. |
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Address |
[Mastromarco, M.; Colonna, N.; Diacono, D.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: amaducci@lns.infn.it |
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Springer |
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English |
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ISSN |
1434-6001 |
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Expedition |
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Conference |
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Notes |
WOS:000840312100002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5328 |
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Author |
n_TOF Collaboration (Massimi, C. et al.); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
Neutron spectroscopy of Mg-26 states: Constraining the stellar neutron source Ne-22(alpha, n)Mg-25 |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physics Letters B |
Abbreviated Journal |
Phys. Lett. B |
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Volume |
768 |
Issue |
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Pages |
1-6 |
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Keywords |
s Process; alpha+Ne-22; Neutron spectroscopy |
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Abstract |
This work reports on accurate, high-resolution measurements of the Mg-25(n, gamma)Mg-26 and Mg-25(n, tot) cross sections in the neutron energy range from thermal to about 300 keV, leading to a significantly improved Mg-25(n, gamma)Mg-26 parametrization. The relevant resonances for n+Mg-25 were characterized from a combined R-matrix analysis of the experimental data. This resulted in an unambiguous spin/parity assignment of the corresponding excited states in Mg-26. With this information experimental upper limits of the reaction rates for Ne-22(alpha, n)Mg-25 and Ne-22(alpha, gamma)Mg-26 were established, potentially leading to a significantly higher (alpha, n)/(alpha, gamma) ratio than previously evaluated. The impact of these results has been studied for stellar models in the mass range 2 to 25 M-circle dot. (C) 2017 The Author(s). Published by Elsevier B.V. |
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Address |
[Massimi, C.; Barbagallo, M.; Becvar, F.; Bisterzok, S.; Castelluccio, D. M.; Eleftheriadis, C.; Finocchiaro, P.; Kokkoris, M.; Marganiec, J.; Plompen, A.; Praena, J.; Rubbia, C.; Weiss, C.] Ist Nazl Fis Nucl, Bologna, Italy, Email: cristian.massimi@bo.infn.it |
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Publisher |
Elsevier Science Bv |
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English |
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ISSN |
0370-2693 |
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Conference |
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Notes |
WOS:000400677700001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3112 |
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Author |
n_TOF Collaboration (Lerendegui-Marco, J. et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
2 |
Pages |
024605 - 21pp |
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Keywords |
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Abstract |
The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA. |
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Address |
[Lerendegui-Marco, J.; Guerrero, C.; Quesada, J. M.; Cortes-Giraldo, M. A.; Praena, J.; Sabate-Gilarte, M.] Univ Seville, Dept Fis Atom Mol & Nucl, E-41012 Seville, Spain, Email: cguerrero4@us.es |
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Publisher |
Amer Physical Soc |
Place of Publication |
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English |
Summary Language |
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Abbreviated Series Title |
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Edition |
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ISSN |
2469-9985 |
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Notes |
WOS:000424190700001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3474 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Lederer-Woods, C. et al.); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Destruction of the cosmic gamma-ray emitter Al-26 in massive stars: Study of the key Al-26(n, p) reaction |
Type |
Journal Article |
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Year |
2021 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
104 |
Issue |
2 |
Pages |
L022803 - 7pp |
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Keywords |
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Abstract |
The Al-26(n, p) Mg-26 reaction is the key reaction impacting on the abundances of the cosmic gamma-ray emitter Al-26 produced in massive stars and impacts on the potential pollution of the early solar system with Al-26 by asymptotic giant branch stars. We performed a measurement of the Al-26(n, p) Mg-26 cross section at the high-flux beam line EAR-2 at the n_TOF facility (CERN). We report resonance strengths for eleven resonances, nine being measured for the first time, while there is only one previous measurement for the other two. Our resonance strengths are significantly lower than the only previous values available. Our cross-section data range to 150 keV neutron energy, which is sufficient for a reliable determination of astrophysical reactivities up to 0.5 GK stellar temperature. |
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Address |
[Lederer-Woods, C.; Woods, P. J.; Davinson, T.; Kahl, D.; Lonsdale, S. J.] Univ Edinburgh, Sch Phys & Astron, Peter Guthrie Tait Rd, Edinburgh EH9 3FD, Midlothian, Scotland, Email: claudia.lederer-woods@ed.ac.uk |
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Publisher |
Amer Physical Soc |
Place of Publication |
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English |
Summary Language |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Expedition |
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Conference |
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Notes |
WOS:000691442700005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4949 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Lederer-Woods, C. et al.); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Destruction of the cosmic gamma-ray emitter Al-26 in massive stars: Study of the key Al-26(n, alpha) reaction |
Type |
Journal Article |
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Year |
2021 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
104 |
Issue |
3 |
Pages |
L032803 - 6pp |
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Keywords |
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Abstract |
Neutron destruction reactions of the cosmic gamma-ray emitter Al-26 are of importance to determine the amount of Al-26 ejected into our galaxy by supernova explosions and for Al-26 production in asymptotic giant branch stars. We performed a new measurement of the Al-26(n, alpha) reaction up to 160-keV neutron energy at the neutron time-of-flight facilities n_TOF at CERN and GELINA at EC-JRC. We provide strengths for ten resonances, six of them for the first time. We use our data to calculate astrophysical reactivities for stellar temperatures up to 0.7 GK. Our results resolve a discrepancy between the two previous direct measurements of this reaction, and indicate higher stellar destruction rates than the most recently recommended reactivity. |
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Address |
[Lederer-Woods, C.; Woods, P. J.; Davinson, T.; Estrade, A.; Kahl, D.; Lonsdale, S. J.] Univ Edinburgh, Sch Phys & Astron, Peter Guthrie Tait Rd, Edinburgh EH9 3FD, Midlothian, Scotland, Email: claudia.lederer-woods@ed.ac.uk |
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Publisher |
Amer Physical Soc |
Place of Publication |
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English |
Summary Language |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000704560300002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4988 |
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Author |
n_TOF Collaboration (Lederer-Woods, C. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement of Ge-73(n, gamma) cross sections and implications for stellar nucleosynthesis |
Type |
Journal Article |
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Year |
2019 |
Publication |
Physics Letters B |
Abbreviated Journal |
Phys. Lett. B |
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Volume |
790 |
Issue |
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Pages |
458-465 |
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Keywords |
Nucleosynthesis; Neutron capture; s process; Germanium; n_TOF |
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Abstract |
Ge-73(n, gamma) cross sections were measured at the neutron time-of-flight facility n_TOF at CERN up to neutron energies of 300 keV, providing for the first time experimental data above 8 keV. Results indicate that the stellar cross section at kT = 30 keV is 1.5 to 1.7 times higher than most theoretical predictions. The new cross sections result in a substantial decrease of Ge-73 produced in stars, which would explain the low isotopic abundance of Ge-73 in the solar system. |
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Address |
[Lederer-Woods, C.; Battino, U.; Tattersalla, A.; Dietz, M.] Univ Edinburgh, Sch Phys & Astron, Edinburgh, Midlothian, Scotland, Email: claudia.lederer-woods@ed.ac.uk |
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Publisher |
Elsevier Science Bv |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0370-2693 |
ISBN |
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Expedition |
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Conference |
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Notes |
WOS:000460118200058 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3936 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Lederer-Woods, C. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Ge-74(n, gamma) cross section below 70 keV measured at n_TOF CERN |
Type |
Journal Article |
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Year |
2022 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
58 |
Issue |
12 |
Pages |
239 - 9pp |
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Keywords |
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Abstract |
Neutron capture reaction cross sections on Ge-74 are of importance to determine Ge-74 production during the astrophysical slow neutron capture process. We present new resonance data on Ge-74(n, gamma ) reactions below 70 keV neutron energy. We calculate Maxwellian averaged cross sections, combining our data below 70 keV with evaluated cross sections at higher neutron energies. Our stellar cross sections are in agreement with a previous activation measurement performed at Forschungszentrum Karlsruhe by Marganiec et al., once their data has been re-normalised to account for an update in the reference cross section used in that experiment. |
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Address |
[Lederer-Woods, C.; Lonsdale, S. J.; Woods, P. J.] Univ Edinburgh, Sch Phys & Astron, Edinburgh, Midlothian, Scotland, Email: claudia.lederer-woods@ed.ac.uk |
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Publisher |
Springer |
Place of Publication |
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English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000913761400001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5472 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Gunsing, F. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Nuclear data activities at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2016 |
Publication |
European Physical Journal Plus |
Abbreviated Journal |
Eur. Phys. J. Plus |
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Volume |
131 |
Issue |
10 |
Pages |
371 - 13pp |
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Keywords |
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Abstract |
Nuclear data in general, and neutron-induced reaction cross sections in particular, are important for a wide variety of research fields. They play a key role in the safety and criticality assessment of nuclear technology, not only for existing power reactors but also for radiation dosimetry, medical applications, the transmutation of nuclear waste, accelerator-driven systems, fuel cycle investigations and future reactor systems as in Generation IV. Applications of nuclear data are also related to research fields as the study of nuclear level densities and stellar nucleosynthesis. Simulations and calculations of nuclear technology applications largely rely on evaluated nuclear data libraries. The evaluations in these libraries are based both on experimental data and theoretical models. Experimental nuclear reaction data are compiled on a worldwide basis by the international network of Nuclear Reaction Data Centres (NRDC) in the EXFOR database. The EXFOR database forms an important link between nuclear data measurements and the evaluated data libraries. CERN's neutron time-of-flight facility nTOF has produced a considerable amount of experimental data since it has become fully operational with the start of the scientific measurement programme in 2001. While for a long period a single measurement station (EAR1) located at 185 m from the neutron production target was available, the construction of a second beam line at 20 m (EAR2) in 2014 has substantially increased the measurement capabilities of the facility. An outline of the experimental nuclear data activities at CERN's neutron time-of-flight facility nTOF will be presented. |
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Address |
[Gunsing, F.; Belloni, F.; Berthoumieux, E.; Diakaki, M.; Dupont, E.] CEA Saclay, Irfu, Gif Sur Yvette, France, Email: gunsing@cea.fr |
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Publisher |
Springer Heidelberg |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2190-5444 |
ISBN |
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Area |
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Conference |
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Notes |
WOS:000386722000001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2850 |
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Author |
n_TOF Collaboration (Guerrero, C. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron Capture on the s-Process Branching Point Tm-171 via Time-of-Flight and Activation |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
125 |
Issue |
14 |
Pages |
142701 - 8pp |
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Keywords |
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Abstract |
The neutron capture cross sections of several unstable nuclides acting as branching points in the s process are crucial for stellar nucleosynthesis studies. The unstable Tm-171 (t(1/2) = 1.92 yr) is part of the branching around mass A similar to 170 but its neutron capture cross section as a function of the neutron energy is not known to date. In this work, following the production for the first time of more than 5 mg of Tm-171 at the high-flux reactor Institut Laue-Langevin in France, a sample was produced at the Paul Scherrer Institute in Switzerland. Two complementary experiments were carried out at the neutron time-of-flight facility (nTOF) at CERN in Switzerland and at the SARAF liquid lithium target facility at Soreq Nuclear Research Center in Israel by time of flight and activation, respectively. The result of the time -of-flight experiment consists of the first ever set of resonance parameters and the corresponding average resonance parameters, allowing us to make an estimation of the Maxwellian-averaged cross sections (MACS) by extrapolation. The activation measurement provides a direct and more precise measurement of the MACS at 30 keV: 384 (40) mb, with which the estimation from the nTOF data agree at the limit of 1 standard deviation. This value is 2.6 times lower than the JEFF-3.3 and ENDF/B-VIII evaluations, 25% lower than that of the Bao et al. compilation, and 1.6 times larger than the value recommended in the KAlloNiS (v1) database, based on the only previous experiment. Our result affects the nucleosynthesis at the A similar to 170 branching, namely, the Yb-171 abundance increases in the material lost by asymptotic giant branch stars, providing a better match to the available pre-solar SiC grain measurements compared to the calculations based on the current JEFF-3.3 model-based evaluation. |
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Address |
[Guerrero, C.; Lerendegui-Marco, J.; Quesada, J. M.; Cortes-Giraldo, M. A.; Millan-Callado, M. A.; Praena, J.; Rodriguez-Gonzalez, T.; Sabate-Gilarte, M.] Univ Seville, Seville, Spain, Email: cguerrero4@us.es |
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Amer Physical Soc |
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English |
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0031-9007 |
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WOS:000574781200004 |
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no |
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yes |
International Collaboration |
yes |
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IFIC @ pastor @ |
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4551 |
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