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Clement, E. et al, Domingo-Pardo, C., & Gadea, A. (2023). Spectroscopic quadrupole moments in 124Xe. Phys. Rev. C, 107(1), 014324–8pp.
Abstract: Background: The Xe isotopic chain with four valence protons above the Z = 50 shell closure is an ideal laboratory for the study of the evolution of nuclear deformation. At the N = 82 shell closure, 136Xe presents all characteristics of a doubly closed shell nucleus with a spherical shape. In the very neutron-deficient isotopes close to N = 50, the alpha-decay chain of Xe was investigated to probe the radioactive decay properties near the drip-line and the magicity of 100Sn. Additionally, the Xe isotopes present higher order symmetries in the nuclear deformation such as the octupole degree of freedom near N = 60 and N = 90 or O(6) symmetry in stable isotopes.Purpose: The relevance of the O(6) symmetry has been investigated by measuring the spectroscopic quadrupole moment of the first excited states in 124Xe. In the O(6) symmetry limit, the spectroscopic quadrupole moment of collective states is expected to be null.Method: A stable 124Xe beam with energies of 4.03A MeV and 4.11A MeV was used to bombard a natW target at the GANIL facility. Excited states were populated via the safe Coulomb excitation reaction. The collision of the heavy ions with a large Z at low energy make this reaction sensitive to the diagonal E2 matrix element of the excited states. The recoils were detected in the VAMOS++ magnetic spectrometer and the gamma rays in the AGATA tracking array. The least squares fitting code GOSIA was used for the analysis to extract both E2 and M1 transitional and E2 diagonal matrix elements.Results: The rotational ground state band was populated up to the 8+1 state as well as the 2+2 and 4+2 states. Using high precision spectroscopic data to constrain the GOSIA fit, the spectroscopic quadrupole moments of the 2+1 , 4+1 , and 6+1 states were determined for the first time. Conclusions: The spectroscopic quadrupole moments were found to be negative, large, and constant in the ground state band underlining the prolate axially deformed ground state band of 124Xe. The present experimental data confirm that the is broken in 124Xe.
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Colonna, N., Belloni, F., Berthoumieux, E., Calviani, M., Domingo-Pardo, C., Guerrero, C., et al. (2010). Advanced nuclear energy systems and the need of accurate nuclear data: the n_TOF project at CERN. Energy Environ. Sci., 3(12), 1910–1917.
Abstract: To satisfy the world's constantly increasing demand for energy, a suitable mix of different energy sources has to be devised. In this scenario, an important role could be played by nuclear energy, provided that major safety, waste and proliferation issues affecting current nuclear reactors are satisfactorily addressed. To this purpose, a large effort has been under way for a few years towards the development of advanced nuclear systems with the aim of closing the fuel cycle. Generation IV reactors, with full or partial waste recycling capability, accelerator driven systems, as well as new fuel cycles are the main options being investigated. The design of advanced systems requires improvements in basic nuclear data, such as cross-sections for neutron-induced reactions on actinides. In this paper, the main concepts of advanced reactor systems are described, together with the related needs of new and accurate nuclear data. The present activity in this field at the neutron facility n_TOF at CERN is discussed.
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Delafosse, C. et al, Gadea, A., Perez-Vidal, R. M., & Domingo-Pardo, C. (2018). Pseudospin Symmetry and Microscopic Origin of Shape Coexistence in the Ni-78 Region: A Hint from Lifetime Measurements. Phys. Rev. Lett., 121(19), 192502–7pp.
Abstract: Lifetime measurements of excited states of the light N = 52 isotones Kr-88, Se-86, and Ge-84 have been performed, using the recoil distance Doppler shift method and VAMOS and AGATA spectrometers for particle identification and gamma spectroscopy, respectively. The reduced electric quadrupole transition probabilities B(E2; 2(+)-> 0(+)) and B(E2; 4(+)-> 2(+)) were obtained for the first time for the hard-to-reach 84Ge. While the B(E2; 2(+)-> 0(+) ) values of Kr-88, Se-86 saturate the maximum quadrupole collectivity offered by the natural valence (3s, 2d, 1g(7/2), 1h(11/2)) space of an inert Ni-78 core, the value obtained for Ge-84 largely exceeds it, suggesting that shape coexistence phenomena, previously reported at N less than or similar to 49, extend beyond N = 50. The onset of collectivity at Z = 32 is understood as due to a pseudo-SU(3) organization of the proton single-particle sequence reflecting a clear manifestation of pseudospin symmetry. It is realized that the latter provides actually reliable guidance for understanding the observed proton and neutron single particle structure in the whole medium-mass region, from Ni to Sn, pointing towards the important role of the isovector-vector rho field in shell-structure evolution.
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Dillmann, I., Coquard, L., Domingo-Pardo, C., Kappeler, F., Marganiec, J., Uberseder, E., et al. (2011). Cross sections for proton-induced reactions on Pd isotopes at energies relevant for the gamma process. Phys. Rev. C, 84(1), 015802–11pp.
Abstract: Proton-activation reactions on natural and enriched palladium samples were investigated via the activation technique in the energy range of E(p) = 2.75-9 MeV, close to the upper end of the respective Gamow window of the. process. We have determined cross sections for (102)Pd(p,gamma)(103)Ag, (104)Pd(p,gamma)(105)Ag, and (105)Pd(p,n)(105)Ag, as well as partial cross sections of (104)Pd(p,n)(104)Ag(g), (105)Pd(p,gamma)(106)Ag(m), (106)Pd(p,n)(106)Ag(m), and (110)Pd(p,n)(110)Ag(m) with uncertainties between 3% and 15% for constraining theoretical Hauser-Feshbach rates and for direct use in gamma-process calculations.
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Domingo-Pardo, C. (2016). Beta-delayed neutron emission: first measurements in the heavy mass region and future prospects. Acta Phys. Pol. B, 47(3), 729–737.
Abstract: Beta-delayed neutrons play a key role in the formation of heavy elements in explosive stellar environments. The final r-process abundance distribution, including the rare-earth peak, is tailored to a large extent by the neutrons released after the beta decay of very exotic neutron-rich nuclei encountered along the r-process path and during the freeze-out phase. Such scenarios involve a vast amount of – yet undiscovered – nuclei, and most of them are expected to be neutron emitters. In this respect, existing beta-delayed neutron emission data is rather scarce, spanning from the lightest isotopes up to the region of the fission-fragments with masses up to A similar to 150. This contribution gives an overview on the latest measurements of neutron branching ratios in the heavy mass region around N = 126, which was practically unexplored in the past. Present plans to access very exotic nuclei at the RIB-facility of RIKEN in the framework of the BRIKEN project, are presented, together with the expected impact in r-process nucleosynthesis studies.
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Domingo-Pardo, C. (2016). i-TED: A novel concept for high-sensitivity (n,gamma) cross-section measurements. Nucl. Instrum. Methods Phys. Res. A, 825, 78–86.
Abstract: A new method for measuring (n, gamma) cross-sections aiming at enhanced signal-to-background ratio is presented. This new approach is based on the combination of the pulse-height weighting technique with a total energy detection system that features gamma-ray imaging capability (i-TED). The latter allows one to exploit Compton imaging techniques to discriminate between true capture gamma-rays arising from the sample under study and background gamma-rays coming from contaminant neutron (prompt or delayed) captures in the surrounding environment. A general proof-of-concept detection system for this application is presented in this paper together with a description of the imaging method and a conceptual demonstration based on Monte Carlo simulations.
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Domingo-Pardo, C. (2012). A new technique for 3D gamma-ray imaging: Conceptual study of a 3D camera. Nucl. Instrum. Methods Phys. Res. A, 675, 123–132.
Abstract: A novel technique for 3D gamma-ray imaging is presented. This method combines the positron annihilation Compton scattering imaging technique with a supplementary position sensitive detector, which registers gamma-rays scattered in the object at angles of about 90 degrees. The 3D coordinates of the scattering location can be determined rather accurately by applying the Compton principle. This method requires access to the object from two orthogonal sides and allows one to achieve a position resolution of few mm in all three space coordinates. A feasibility study for a 3D camera is presented based on Monte Carlo calculations.
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Domingo-Pardo, C., Goel, N., Engert, T., Gerl, J., Kojouharov, I., Schaffner, H., et al. (2011). A novel gamma-ray imaging method for the pulse-shape characterization of position sensitive semiconductor radiation detectors. Nucl. Instrum. Methods Phys. Res. A, 643(1), 79–88.
Abstract: A new technique for the pulse-shape characterization of gamma-ray position sensitive germanium detectors is presented. This method combines the pulse shape comparison scan (PSCS) principle with a gamma-ray imaging technique. The latter is provided by a supplementary, high performance, position sensitive gamma-ray scintillator detector. We describe the basic aspects of the method and we show measurements made for the study of pulse-shapes in a non-segmented planar HPGe detector. A preliminary application of the PSCS is carried out, although a more detailed investigation is being performed with highly segmented position sensitive detectors.
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Dudouet, J. et al, Domingo-Pardo, C., Gadea, A., & Perez-Vidal, R. M. (2017). Kr-96(36)60-Low-Z Boundary of the Island of Deformation at N=60. Phys. Rev. Lett., 118(16), 162501–6pp.
Abstract: Prompt.-ray spectroscopy of the neutron-rich Kr-96, produced in transfer-and fusion-induced fission reactions, has been performed using the combination of the Advanced Gamma Tracking Array and the VAMOS + +spectrometer. A second excited state, assigned to J pi = 4(+), is observed for the first time, and a previously reported level energy of the first 2+ excited state is confirmed. The measured energy ratio R-4/2 = E(4(+))/E(2(+)) = 2.12(1) indicates that this nucleus does not show a well-developed collectivity contrary to that seen in heavier N = 60 isotones. This new measurement highlights an abrupt transition of the degree of collectivity as a function of the proton number at Z = 36, of similar amplitude to that observed at N = 60 at higher Z values. A possible reason for this abrupt transition could be related to the insufficient proton excitations in the g(9/2), d(5/2), and s(1/2) orbitals to generate strong quadrupole correlations or to the coexistence of competing different shapes. An unexpected continuous decrease of R-4/2 as a function of the neutron number up to N = 60 is also evidenced. This measurement establishes the Kr isotopic chain as the low-Z boundary of the island of deformation for N = 60 isotones. A comparison with available theoretical predictions using different beyond mean-field approaches shows that these models fail to reproduce the abrupt transitions at N = 60 and Z = 36.
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Esposito, R. et al, & Domingo-Pardo, C. (2021). Design of the third-generation lead-based neutron spallation target for the neutron time-of-flight facility at CERN. Phys. Rev. Accel. Beams, 24(9), 093001–17pp.
Abstract: The neutron time-of-flight (n_TOF) facility at the European Laboratory for Particle Physics (CERN) is a pulsed white-spectrum neutron spallation source producing neutrons for two experimental areas: the Experimental Area 1 (EAR1), located 185 m horizontally from the target, and the Experimental Area 2 (EAR2), located 20 m above the target. The target, based on pure lead, is impacted by a high-intensity 20-GeV/c pulsed proton beam. The facility was conceived to study neutron-nucleus interactions for neutron kinetic energies between a few meV to several GeV, with applications of interest for nuclear astrophysics, nuclear technology, and medical research. After the second-generation target reached the end of its lifetime, the facility underwent a major upgrade during CERN's Long Shutdown 2 (LS2, 2019-2021), which included the installation of the new third-generation neutron target. The first- and second-generation targets were based on water-cooled massive lead blocks and were designed focusing on EAR1, since EAR2 was built later. The new target is cooled by nitrogen gas to avoid erosion-corrosion and contamination of cooling water with radioactive lead spallation products. Moreover, the new design is optimized also for the vertical flight path and EAR2. This paper presents an overview of the target design focused on both physics and thermomechanical performance, and includes a description of the nitrogen cooling circuit and radiation protection studies.
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