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Author n_TOF Collaboration (Mastromarco, M. et al); Domingo-Pardo, C.; Tain, J.L.
Title High accuracy, high resolution U-235(n,f) cross section from n_TOF (CERN) from 18 meV to 10 keV Type Journal Article
Year 2022 Publication European Physical Journal A Abbreviated Journal Eur. Phys. J. A
Volume 58 Issue 8 Pages 147 - 13pp
Keywords
Abstract (down) The U-235(n,f) cross section was measured in a wide energy range (18 meV-170 keV) at the nTOF facility at CERN, relative to Li-6(n,t) and B-10(n,alpha) standard reactions, with high resolution and accuracy, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. In this paper we report on the results in the region between 18 meV and 10 keV neutron energy. A resonance analysis has been performed up to 200 eV, with the code SAMMY. The resulting fission kernels are compared with the ones extracted on the basis of the resonance parameters of the most recent major evaluated data libraries. A comparison of the nTOF data with the evaluated cross sections is also performed from thermal to 10 keV neutron energy for the energy-averaged cross section in energy groups of suitably chosen width. A good agreement, within 0.5%, is found on average between the new results and the latest evaluated data files ENDF/B-VIII.0 and JEFF-3.3, as well as with respect to the broad group average fission cross section established in the framework of the standard working group of IAEA (the so-called reference file). However, some discrepancies, of up to 4%, are still present in some specific energy regions. The new dataset here presented, characterized by a unique combination of high resolution and accuracy, low background and wide energy range, can help to improve the evaluations from the Resolved Resonance Region up to 10 keV, also reducing the uncertainties that affect this region.
Address [Mastromarco, M.; Colonna, N.; Diacono, D.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: amaducci@lns.infn.it
Corporate Author Thesis
Publisher Springer Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1434-6001 ISBN Medium
Area Expedition Conference
Notes WOS:000840312100002 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5328
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Author n_TOF Collaboration (Cano-Ott, D. et al); Domingo-Pardo, C.; Tain, J.L.
Title Neutron Capture Measuremetns on Minor Actinides at the n_TOF Facility at CERN: Past, Present and Future Type Journal Article
Year 2011 Publication Journal of the Korean Physical Society Abbreviated Journal J. Korean Phys. Soc.
Volume 59 Issue 2 Pages 1809-1812
Keywords n_TOF; Total Absorption Calorimeter; TAC; Neutron capture; Cross section; Nuclear waste; Transmutation; Generation IV; Accelerator driven system; ADS; Nuclear reactor; Nuclear energy; Nuclear data; Barium fluoride; Actinides; Plutonium; Americium; Uranium
Abstract (down) The successful development of advanced nuclear systems for sustainable energy production and nuclear waste management depends on high quality nuclear data libraries. Recent sensitivity studies and reports [1-3] have identified the need for substantially improving the accuracy of neutron cross-section data for minor actinides. The n_TOF collaboration has initiated an ambitious experimental program for the measurement of neutron capture cross sections of minor actinides. Two experimental setups have been constructed for this purpose: a Total Absorption Calorimeter (TAC) [4] for measuring neutron capture cross-sections of low-mass and/or radioactive samples and a set of two low neutron sensitivity C(6)D(6) detectors for the less radioactive materials.
Address [Cano-Ott, D; Alvarez-Velarde, F; Gonzalez-Romero, E; Guerrero, C; Martinez, T; Mendoza, E; Villamarin, D; Vicente, MC] Ctr Invest Energet Medioambientales & Technol CIE, Madrid, Spain, Email: daniel.cano@ciemat.es
Corporate Author Thesis
Publisher Korean Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0374-4884 ISBN Medium
Area Expedition Conference
Notes WOS:000294080700085 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ elepoucu @ Serial 737
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Author Girard-Alcindor, V. et al; Domingo-Pardo, C.
Title New narrow resonances observed in the unbound nucleus F-15 Type Journal Article
Year 2022 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 105 Issue 5 Pages L051301 - 7pp
Keywords
Abstract (down) The structure of the unbound F-15 nucleus is investigated using the inverse kinematics resonant scattering of a radioactive O-14 beam impinging on a CH2 target. The analysis of H-1(O-14, p) O-14 and H-1(O-14, 2p) N-13 reactions allowed the confirmation of the previously observed narrow 1/2(-) resonance, near the two-proton decay threshold, and the identification of two new narrow 5/2(-) and 3/2(-) resonances. The newly observed levels decay by 1p emission to the ground of O-14, and by sequential 2p emission to the ground state of N-13 via the 1(-) resonance of O-14. Gamow shell model (GSM) analysis of the experimental data suggests that the wave functions of the 5/2(-) and 3/2(-) resonances may be collectivized by the continuum coupling to nearby 2p- and 1p-decay channels. The observed excitation function H-1(O-14, p) O-14 and resonance spectrum in F-15 are well reproduced in the unified framework of the GSM.
Address [Girard-Alcindor, V.; Santos, F. de Oliveira; Ploszajczak, M.; Lemasson, A.; Clement, E.; Ramos, D.; Rejmund, M.; Ackermann, D.; Bastin, B.; Caceres, L.; De France, G.; Giraud, S.; Goupil, J.; Grevy, S.; Kamalou, O.; Kamenyero, A.; Leblond, S.; Lefevre, A.; Li, H.; Morfouace, P.; Stodel, C.; Thomas, J. C.] Grand Accelerateur Natl Ions Lourds GANIL, CEA, DRF CNRS, IN2P3, Bvd Henri Becquerel, F-14076 Caen, France, Email: stefan@ipno.in2p3.fr
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000811520800003 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5268
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Author n_TOF Collaboration (Lerendegui-Marco, J. et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility Type Journal Article
Year 2018 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 97 Issue 2 Pages 024605 - 21pp
Keywords
Abstract (down) The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA.
Address [Lerendegui-Marco, J.; Guerrero, C.; Quesada, J. M.; Cortes-Giraldo, M. A.; Praena, J.; Sabate-Gilarte, M.] Univ Seville, Dept Fis Atom Mol & Nucl, E-41012 Seville, Spain, Email: cguerrero4@us.es
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000424190700001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3474
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Author Hinke, C.B. et al; Domingo-Pardo, C.
Title Superallowed Gamow-Teller decay of the doubly magic nucleus Sn-100 Type Journal Article
Year 2012 Publication Nature Abbreviated Journal Nature
Volume 486 Issue 7403 Pages 341-345
Keywords
Abstract (down) The shell structure of atomic nuclei is associated with 'magic numbers' and originates in the nearly independent motion of neutrons and protons in a mean potential generated by all nucleons. During beta(+)-decay, a proton transforms into a neutron in a previously not fully occupied orbital, emitting a positron-neutrino pair with either parallel or antiparallel spins, in a Gamow-Teller or Fermi transition, respectively. The transition probability, or strength, of a Gamow-Teller transition depends sensitively on the underlying shell structure and is usually distributed among many states in the neighbouring nucleus. Here we report measurements of the half-life and decay energy for the decay of Sn-100, the heaviest doubly magic nucleus with equal numbers of protons and neutrons. In the beta-decay of Sn-100, a large fraction of the strength is observable because of the large decay energy. We determine the largest Gamow-Teller strength so far measured in allowed nuclear beta-decay, establishing the 'superallowed' nature of this Gamow-Teller transition. The large strength and the low-energy states in the daughter nucleus, In-100, are well reproduced by modern, large-scale shell model calculations.
Address [Hinke, C. B.; Boehmer, M.; Faestermann, T.; Gernhaeuser, R.; Kruecken, R.; Maier, L.; Steiger, K.; Straub, K.; Nebel, F.; Schwertel, S.] Tech Univ Munich, Phys Dept E12, D-85748 Garching, Germany, Email: thomas.faestermann@ph.tum.de
Corporate Author Thesis
Publisher Nature Publishing Group Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0028-0836 ISBN Medium
Area Expedition Conference
Notes WOS:000305466800032 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 1055
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Author Perez-Vidal, R.M. et al; Gadea, A.; Jurado, M.; Domingo-Pardo, C.; Huyuk, T.
Title Evidence of Partial Seniority Conservation in the pi g9/2 Shell for the N=50 Isotones Type Journal Article
Year 2022 Publication Physical Review Letters Abbreviated Journal Phys. Rev. Lett.
Volume 129 Issue 11 Pages 112501 - 7pp
Keywords
Abstract (down) The reduced transition probabilities for the 4+1 -2+1 and 2+1 -0+1 transitions in 92Mo and 94Ru and for the 4+1 -2+1 and 6+1 -4+1 transitions in 90Zr have been determined in this experiment making use of a multinucleon transfer reaction. These results have been interpreted on the basis of realistic shell-model calculations in the f5=2, p3=2, p1=2, and g9=2 proton valence space. Only the combination of extensive lifetime information and large scale shell-model calculations allowed the extent of the seniority conservation in the N = 50 g9=2 orbital to be understood. The conclusion is that seniority is largely conserved in the first 71g9=2 orbital.
Address [Perez-Vidal, R. M.; Gadea, A.; Domingo-Pardo, C.; Huyuk, T.] Univ Valencia, Inst Fis Corpuscular, CSIC, E-46980 Valencia, Spain, Email: perezvidal@lnl.infn.it
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0031-9007 ISBN Medium
Area Expedition Conference
Notes WOS:000861160200004 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5374
Permanent link to this record
 

 
Author n_TOF Collaboration (Belloni, F. et al); Domingo-Pardo, C.; Tain, J.L.
Title Measurement of the neutron-induced fission cross-section of Am-243 relative to U-235 from 0.5 to 20 MeV Type Journal Article
Year 2011 Publication European Physical Journal A Abbreviated Journal Eur. Phys. J. A
Volume 47 Issue 12 Pages 160 - 8pp
Keywords
Abstract (down) The ratio of the neutron-induced fission cross-sections of Am-243 and U-235 was measured in the energy range from 0.5 to 20 MeV with uncertainties of approximate to 4%. The experiment was performed at the CERN n_TOF facility using a fast ionization chamber. With the good counting statistics that could be achieved thanks to the high instantaneous flux and the low backgrounds, the present results are useful for resolving discrepancies in previous data sets and are important for future reactors with improved fuel burn-up.
Address [Belloni, F.; Calviani, M.; Mastinu, P.; Milazzo, P. M.; Abbondanno, U.; Fujii, K.; Gramegna, F.; Moreau, C.] Ist Nazl Fis Nucl INFN, Lab Nazl Legnaro, Trieste, Italy, Email: paolo.milazzo@ts.infn.it
Corporate Author Thesis
Publisher Springer Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1434-6001 ISBN Medium
Area Expedition Conference
Notes WOS:000300285100005 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 904
Permanent link to this record
 

 
Author n_TOF Collaboration (Wright, T. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Measurement of the U-238(n,gamma) cross section up to 80 keV with the Total Absorption Calorimeter at the CERN n_TOF facility Type Journal Article
Year 2017 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 96 Issue 6 Pages 064601 - 11pp
Keywords
Abstract (down) The radiative capture cross section of a highly pure (99.999%), 6.125(2) grams and 9.56(5) x 10(-4) atoms/barn areal density U-238 sample has been measured with the Total Absorption Calorimeter (TAC) in the 185 m flight path at the CERN neutron time-of-flight facility n_TOF. This measurement is in response to the NEA High Priority Request list, which demands an accuracy in this cross section of less than 3% below 25 keV. These data have undergone careful background subtraction, with special care being given to the background originating from neutrons scattered by the 238U sample. Pileup and dead-time effects have been corrected for. The measured cross section covers an energy range between 0.2 eV and 80 keV, with an accuracy that varies with neutron energy, being better than 4% below 25 keV and reaching at most 6% at higher energies.
Address [Wright, T.; Billowes, J.; Ryan, J. A.; Ware, T.] Univ Manchester, Manchester, Lancs, England, Email: tobias.wright@manchester.ac.uk
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000416848700005 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3392
Permanent link to this record
 

 
Author n_TOF Collaboration (Mosconi, M. et al); Domingo-Pardo, C.; Tain, J.L.
Title Neutron physics of the Re/Os clock. I. Measurement of the (n, gamma) cross sections of Os-186,Os-187,Os-188 at the CERN n_TOF facility Type Journal Article
Year 2010 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 82 Issue 1 Pages 015802 - 10pp
Keywords
Abstract (down) The precise determination of the neutron capture cross sections of Os-186 and Os-187 is important to define the s-process abundance of Os-187 at the formation of the solar system. This quantity can be used to evaluate the radiogenic component of the abundance of Os-187 due to the decay of the unstable Re-187 (t(1/2) = 41.2 Gyr) and from this to infer the time duration of the nucleosynthesis in our galaxy (Re/Os cosmochronometer). The neutron capture cross sections of Os-186, Os-187, and Os-188 have been measured at the CERN n_TOF facility from 1 eV to 1 MeV, covering the entire energy range of astrophysical interest. The measurement has been performed by time-of-flight technique using isotopically enriched samples and two C6D6 scintillation detectors for recording the prompt. rays emitted in the capture events. Maxwellian averaged capture cross sections have been determined for thermal energies between kT = 5 and 100 keV corresponding to all possible s-process scenarios. The estimated uncertainties for the values at 30 keV are 4.1, 3.3, and 4.7% for Os-186, Os-187, and Os-188, respectively.
Address [Mosconi, M.; Domingo-Pardo, C.; Kaeppeler, F.; Audouin, L.; Bisterzo, S.; Dillmann, I.; Heil, M.; Plag, R.; Voss, F.; Walter, S.; Wisshak, K.] KIT, Inst Kernphys, D-76021 Karlsruhe, Germany, Email: Marita.Mosconi@ptb.de
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0556-2813 ISBN Medium
Area Expedition Conference
Notes ISI:000279940200007 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ elepoucu @ Serial 409
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Author Guerrero, C.; Cano-Ott, D.; Mendoza, E.; Tain, J.L.; Algora, A.; Berthoumieux, E.; Colonna, N.; Domingo-Pardo, C.; Gonzalez-Romero, E.; Heil, M.; Jordan, D.; Kappeler, F.; Lampoudis, C.; Martinez, T.; Massimi, C.; Plag, R.
Title Monte Carlo simulation of the n_TOF Total Absorption Calorimeter Type Journal Article
Year 2012 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume 671 Issue Pages 108-117
Keywords Monte Carlo simulation; Geant4; Neutron cross-sections; Time-of-flight; Neutron capture
Abstract (down) The n_TOF Total Absorption Calorimeter (TAC) is a 4 pi BaF2 segmented detector used at CERN for measuring neutron capture cross-sections of importance for the design of advanced nuclear reactors. This work presents the simulation code that has been developed in GEANT4 for the accurate determination of the detection efficiency of the TAC for neutron capture events. The code allows to calculate the efficiency of the TAC for every neutron capture state, as a function of energy, crystal multiplicity, and counting rate. The code includes all instrumental effects such as the single crystal detection threshold and energy resolution, finite size of the coincidence time window, and signal pile-up. The results from the simulation have been validated with experimental data for a large set of electromagnetic de-excitation patterns: beta-decay of well known calibration sources, neutron capture reactions in light nuclei with well known level schemes like Ti-nat, reference samples used in (n,gamma) measurements like Au-197 and experimental data from an actinide sample like Pu-240. The systematic uncertainty in the determination of the detection efficiency has been estimated for all the cases. As a representative example, the accuracy reached for the case of Au-197(n,gamma) ranges between 0.5% and 2%, depending on the experimental and analysis conditions. Such a value matches the high accuracy required for the nuclear cross-section data needed in advanced reactor design.
Address [Guerrero, C.; Cano-Ott, D.; Mendoza, E.; Gonzalez-Romero, E.; Martinez, T.] CIEMAT, Ctr Invest Energet Medioambientales & Tecnol, E-28040 Madrid, Spain, Email: carlos.guerrero@cern.ch
Corporate Author Thesis
Publisher Elsevier Science Bv Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:000301474600013 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 973
Permanent link to this record