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Author |
n_TOF Collaboration (Lerendegui-Marco, J. et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
2 |
Pages |
024605 - 21pp |
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Keywords |
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Abstract  |
The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA. |
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Address |
[Lerendegui-Marco, J.; Guerrero, C.; Quesada, J. M.; Cortes-Giraldo, M. A.; Praena, J.; Sabate-Gilarte, M.] Univ Seville, Dept Fis Atom Mol & Nucl, E-41012 Seville, Spain, Email: cguerrero4@us.es |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Notes |
WOS:000424190700001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3474 |
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Author |
Guadilla, V. et al; Algora, A.; Tain, J.L.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Nacher, E.; Orrigo, S.E.A.; Rubio, B.; Valencia, E. |
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Title |
Total absorption gamma-ray spectroscopy of the ss decays of Y-96gs,Y-m |
Type |
Journal Article |
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Year |
2022 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
106 |
Issue |
1 |
Pages |
014306 - 14pp |
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Abstract |
The ss decays of the ground state (gs) and isomeric state (m) of Y-96 have been studied with the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8(+) isomeric state from the 0(-) ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The ss-intensity distributions of both decays have been independently determined. In the analyses the deexcitation of the 1581.6 keV level in Zr-96, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the ss-detector efficiency, influencing the ss-intensity distribution obtained. Our results for Y-96gs (0(-)) confirm the large ground state to ground state ss-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to 96.6(-2.1)(+0.3) % of the total ss intensity. Given that the decay of Y-96gs is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of Y-96m (8(+)), previously undetected ss intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption gamma-ray spectroscopy measurements of ss decays with highly fragmented deexcitation patterns. Y-96m (8(+)) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average ss and gamma energies differ significantly from the previous values in evaluated databases. The discrepancy is far above the previously quoted uncertainties. Finally, we also report on the successful implementation of an innovative total absorption gamma-ray spectroscopy analysis of the module-multiplicity gated spectra, as a first proof of principle to distinguish between decaying states with very different spin-parity values. |
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Address |
[Guadilla, V; Le Meur, L.; Fallot, M.; Briz, J. A.; Estienne, M.; Giot, L.; Porta, A.; Cucoanes, A.; Shiba, T.; Zakari-Issoufou, A-A] Univ Nantes, Subatech, IMT Atlantique, CNRS IN2P3, F-44307 Nantes, France, Email: vguadilla@fuw.edu.pl |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Notes |
WOS:000832364800001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5313 |
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Author |
n_TOF Collaboration (Cano-Ott, D. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron Capture Measuremetns on Minor Actinides at the n_TOF Facility at CERN: Past, Present and Future |
Type |
Journal Article |
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Year |
2011 |
Publication |
Journal of the Korean Physical Society |
Abbreviated Journal |
J. Korean Phys. Soc. |
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Volume |
59 |
Issue |
2 |
Pages |
1809-1812 |
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Keywords |
n_TOF; Total Absorption Calorimeter; TAC; Neutron capture; Cross section; Nuclear waste; Transmutation; Generation IV; Accelerator driven system; ADS; Nuclear reactor; Nuclear energy; Nuclear data; Barium fluoride; Actinides; Plutonium; Americium; Uranium |
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Abstract |
The successful development of advanced nuclear systems for sustainable energy production and nuclear waste management depends on high quality nuclear data libraries. Recent sensitivity studies and reports [1-3] have identified the need for substantially improving the accuracy of neutron cross-section data for minor actinides. The n_TOF collaboration has initiated an ambitious experimental program for the measurement of neutron capture cross sections of minor actinides. Two experimental setups have been constructed for this purpose: a Total Absorption Calorimeter (TAC) [4] for measuring neutron capture cross-sections of low-mass and/or radioactive samples and a set of two low neutron sensitivity C(6)D(6) detectors for the less radioactive materials. |
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Address |
[Cano-Ott, D; Alvarez-Velarde, F; Gonzalez-Romero, E; Guerrero, C; Martinez, T; Mendoza, E; Villamarin, D; Vicente, MC] Ctr Invest Energet Medioambientales & Technol CIE, Madrid, Spain, Email: daniel.cano@ciemat.es |
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Korean Physical Soc |
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English |
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ISSN |
0374-4884 |
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Conference |
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Notes |
WOS:000294080700085 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
737 |
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Author |
n_TOF Collaboration (Mastromarco, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
High accuracy, high resolution U-235(n,f) cross section from n_TOF (CERN) from 18 meV to 10 keV |
Type |
Journal Article |
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Year |
2022 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
58 |
Issue |
8 |
Pages |
147 - 13pp |
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Keywords |
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Abstract |
The U-235(n,f) cross section was measured in a wide energy range (18 meV-170 keV) at the nTOF facility at CERN, relative to Li-6(n,t) and B-10(n,alpha) standard reactions, with high resolution and accuracy, with a setup based on a stack of six samples and six silicon detectors placed in the neutron beam. In this paper we report on the results in the region between 18 meV and 10 keV neutron energy. A resonance analysis has been performed up to 200 eV, with the code SAMMY. The resulting fission kernels are compared with the ones extracted on the basis of the resonance parameters of the most recent major evaluated data libraries. A comparison of the nTOF data with the evaluated cross sections is also performed from thermal to 10 keV neutron energy for the energy-averaged cross section in energy groups of suitably chosen width. A good agreement, within 0.5%, is found on average between the new results and the latest evaluated data files ENDF/B-VIII.0 and JEFF-3.3, as well as with respect to the broad group average fission cross section established in the framework of the standard working group of IAEA (the so-called reference file). However, some discrepancies, of up to 4%, are still present in some specific energy regions. The new dataset here presented, characterized by a unique combination of high resolution and accuracy, low background and wide energy range, can help to improve the evaluations from the Resolved Resonance Region up to 10 keV, also reducing the uncertainties that affect this region. |
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Address |
[Mastromarco, M.; Colonna, N.; Diacono, D.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: amaducci@lns.infn.it |
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Publisher |
Springer |
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English |
Summary Language |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Expedition |
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Conference |
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Notes |
WOS:000840312100002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5328 |
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Author |
n_TOF Collaboration (Paradela, C. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
High-accuracy determination of the U-238/U-235 fission cross section ratio up to approximate to 1 GeV at n_TOF at CERN |
Type |
Journal Article |
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Year |
2015 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
91 |
Issue |
2 |
Pages |
024602 - 11pp |
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Keywords |
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Abstract |
The U-238 to U-235 fission cross section ratio has been determined at nTOF up to approximate to 1 GeV, with two different detection systems, in different geometrical configurations. A total of four datasets has been collected and compared. They are all consistent to each other within the relative systematic uncertainty of 3-4%. The data collected at nTOF have been suitably combined to yield a unique fission cross section ratio as a function of neutron energy. The result confirms current evaluations up to 200 MeV. Good agreement is also observed with theoretical calculations based on the INCL++ /Gemini++ combination up to the highest measured energy. The n_TOF results may help solve a long-standing discrepancy between the two most important experimental datasets available so far above 20 MeV, while extending the neutron energy range for the first time up to approximate to 1 GeV. |
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Address |
[Paradela, C.; Tarrio, D.; Leal-Cidoncha, E.; Duran, I.; Alvarez, H.] Univ Santiago de Compostela, Santiago De Compostela, Spain, Email: nicola.colonna@ba.infn.it |
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Corporate Author |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000350174000004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2139 |
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Author |
n_TOF Collaboration (Gunsing, F. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Measurement of resolved resonances of Th-232(n, gamma) at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2012 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
85 |
Issue |
6 |
Pages |
064601 - 17pp |
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Keywords |
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Abstract |
The yield of the neutron capture reaction Th-232(n, gamma) has been measured at the neutron time-of-flight facility n_TOF at CERN in the energy range from 1 eV to 1 MeV. The reduction of the acquired data to the capture yield for resolved resonances from 1 eV to 4 keV is described and compared to a recent evaluated data set. The resonance parameters were used to assign an orbital momentum to each resonance. A missing level estimator was used to extract the s-wave level spacing of D-0 = 17.2 +/- 0.9 eV. |
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Address |
[Gunsing, F.; Berthoumieux, E.; Aerts, G.; Andriamonje, S.; Dridi, W.; Pancin, J.; Perrot, L.; Plukis, A.] CEA Saclay, DSM, Irfu, SPhN, F-91191 Gif Sur Yvette, France, Email: gunsing@cea.fr |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000304693700002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1048 |
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Author |
Hall, O. et al; Agramunt, J.; Algora, A.; Domingo-Pardo, C.; Morales, A.I.; Rubio, B.; Tain, J.L.; Tolosa-Delgado, A. |
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Title |
beta-delayed neutron emission of r-process nuclei at the N=82 shell closure |
Type |
Journal Article |
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Year |
2021 |
Publication |
Physics Letters B |
Abbreviated Journal |
Phys. Lett. B |
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Volume |
816 |
Issue |
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Pages |
136266 - 7pp |
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Keywords |
beta-delayed neutron emission; r-processimportant |
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Abstract |
Theoretical models of beta-delayed neutron emission are used as crucial inputs in r-process calculations. Benchmarking the predictions of these models is a challenge due to a lack of currently available experimental data. In this work the beta-delayed neutron emission probabilities of 33 nuclides in the important mass regions south and south-west of Sn-132 are presented, 16 for the first time. The measurements were performed at RIKEN using the Advanced Implantation Detector Array (AIDA) and the BRIKEN neutron detector array. The P-1n values presented constrain the predictions of theoretical models in the region, affecting the final abundance distribution of the second r-process peak at A approximate to 130. |
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Address |
[Hall, O.; Davinson, T.; Bruno, C. G.; Griffin, C. J.; Kahl, D.] Univ Edinburgh, Sch Phys & Astron, Edinburgh EH9 3FD, Midlothian, Scotland, Email: oscar.hall@ed.ac.uk |
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Publisher |
Elsevier |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0370-2693 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000647421500016 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4819 |
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Author |
n_TOF Collaboration (Praena, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Preparation and characterization of S-33 samples for S-33(n,alpha)Si-30 cross-section measurements at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2018 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
890 |
Issue |
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Pages |
142-147 |
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Keywords |
Neutron induced alpha emission; Thermal evaporation; Rutherford backscattering |
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Abstract |
Thin S-33 samples for the study of the S-33(n,alpha)Si-30 cross-section at the n_TOF facility at CERN were made by thermal evaporation of S-33 powder onto a dedicated substrate made of kapton covered with thin layers of copper, chromium and titanium. This method has provided for the first time bare sulfur samples a few centimeters in diameter. The samples have shown an excellent adherence with no mass loss after few years and no sublimation in vacuum at room temperature. The determination of the mass thickness of S-33 has been performed by means of Rutherford backscattering spectrometry. The samples have been successfully tested under neutron irradiation. |
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Address |
[Praena, J.; Porras, I.] Univ Granada, Granada, Spain, Email: jpraena@ugr.es |
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Publisher |
Elsevier Science Bv |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0168-9002 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000427814900020 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3537 |
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Author |
Jordan, D.; Algora, A.; Tain, J.L. |
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Title |
An event generator for simulations of complex beta-decay experiments |
Type |
Journal Article |
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Year |
2016 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
828 |
Issue |
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Pages |
52-57 |
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Keywords |
Monte Carlo event generator; Complex beta-decay experiments simulations |
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Abstract |
This article describes a Monte Carlo event generator for the design, optimization and performance characterization of beta decay spectroscopy experimental set-ups. The event generator has been developed within the Geant4 simulation architecture and provides new features and greater flexibility in comparison with the current available decay generator. |
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Address |
[Jordan, D.; Algora, A.; Tain, J. L.] Univ Valencia, CSIC, Ctr Mixto, Inst Fis Corpuscular, Valencia, Spain, Email: jordan@ific.uv.es |
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Elsevier Science Bv |
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English |
Summary Language |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0168-9002 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000377399700007 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2714 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Domingo-Pardo, C. et al); Babiano-Suarez, V.; Balibrea-Correa, J.; Caballero, L.; Ladarescu, I.; Lerendegui-Marco, J.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Advances and new ideas for neutron-capture astrophysics experiments at CERN n_TOF |
Type |
Journal Article |
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Year |
2023 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
59 |
Issue |
1 |
Pages |
8 - 11pp |
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Keywords |
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Abstract |
This article presents a few selected developments and future ideas related to the measurement of (n, gamma ) data of astrophysical interest at CERN n_TOF. The MC-aided analysis methodology for the use of low-efficiency radiation detectors in time-of-flight neutron-capture measurements is discussed, with particular emphasis on the systematic accuracy. Several recent instrumental advances are also presented, such as the development of total-energy detectors with gamma- ray imaging capability for background suppression, and the development of an array of small-volume organic scintilla tors aimed at exploiting the high instantaneous neutron-flux of EAR2. Finally, astrophysics prospects related to the intermediate i neutron-capture process of nucleosynthesis are discussed in the context of the new NEAR activation area. |
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Address |
[Domingo-Pardo, C.; Babiano-Suarez, V.; Balibrea-Correa, J.; Caballero, L.; Ladarescu, I.; Lerendegui-Marco, J.; Tain, J. L.; Tarifeno-Saldivia, A.] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia, Spain, Email: domingo@ific.uv.es |
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Publisher |
Springer |
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English |
Summary Language |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
|
Medium |
|
|
| |
Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
WOS:000926364900001 |
Approved |
no |
|
| |
Is ISI |
yes |
International Collaboration |
yes |
|
| |
Call Number |
IFIC @ pastor @ |
Serial |
5479 |
|
| Permanent link to this record |
