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Guadilla, V. et al; Algora, A.; Tain, J.L.; Agramunt, J.; Jordan, M.D.; Montaner-Piza, A.; Orrigo, S.E.A.; Rubio, B.; Valencia, E.; Gelletly, W.; Monserrate, M. |
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Title |
Experimental study of Tc-100 beta decay with total absorption gamma-ray spectroscopy |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
96 |
Issue |
1 |
Pages |
014319 - 10pp |
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Keywords |
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Abstract |
The beta decay of Tc-100 has been studied by using the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. In this work the new Decay Total Absorption gamma-ray Spectrometer in coincidence with a cylindrical plastic beta detector has been employed. The beta intensity to the ground state obtained from the analysis is in good agreement with previous high-resolution measurements. However, differences in the feeding to the first-excited state as well as weak feeding to a new level at high excitation energy have been deduced from this experiment. Theoretical calculations performed in the quasiparticle random-phase approximation framework are also reported. Comparison of these calculations with our measurement serves as a benchmark for calculations of the double beta decay of Mo-100. |
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Address |
[Guadilla, V.; Algora, A.; Tain, J. L.; Agramunt, J.; Jordan, D.; Montaner-Piza, A.; Orrigo, S. E. A.; Rubio, B.; Valencia, E.; Gelletly, W.; Monserrate, M.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46071 Valencia, Spain, Email: guadilla@ific.uv.es; |
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Publisher |
Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Conference |
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Notes |
WOS:000406526600002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3225 |
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Permanent link to this record |
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Author |
Rice, S. et al; Algora, A.; Tain, J.L.; Valencia, E.; Agramunt, J.; Rubio, B.; Estevez, E.; Jordan, M.D. |
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Title |
Total absorption spectroscopy study of the beta decay of Br-86 and Rb-91 |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
96 |
Issue |
1 |
Pages |
014320 - 10pp |
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Keywords |
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Abstract |
The beta decays of Br-86 and Rb-91 have been studied using the total absorption spectroscopy technique. The radioactive nuclei were produced at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla and further purified using the JYFLTRAP. Br-86 and Rb-91 are considered to be major contributors to the decay heat in reactors. In addition, Rb-91 was used as a normalization point in direct measurements of mean gamma energies released in the beta decay of fission products by Rudstam et al. assuming that this decaywas well known from high-resolution measurements. Our results show that both decays were suffering from the Pandemonium effect and that the results of Rudstam et al. should be renormalized. The relative impact of the studied decays in the prediction of the decay heat and antineutrino spectrum from reactors has been evaluated. |
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Address |
[Rice, S.; Gelletly, W.; Regan, P. H.; Bowry, M.; Farrelly, G. F.; Mason, P.; Podolyak, Zs.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England, Email: algora@ific.uv.es |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Conference |
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Notes |
WOS:000406526600003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3226 |
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Permanent link to this record |
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Author |
Guadilla, V.; Algora, A.; Tain, J.L.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Orrigo, S.E.A.; Rubio, B.; Valencia, E. |
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Title |
Total absorption gamma-ray spectroscopy of niobium isomers |
Type |
Journal Article |
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Year |
2019 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
100 |
Issue |
2 |
Pages |
024311 - 15pp |
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Keywords |
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Abstract |
The beta-intensity distributions of the decays of Nb-100gs,Nb-100m and Nb-102gs,Nb-102m have been determined using the total absorption gamma-ray spectroscopy technique. The JYFLTRAP double Penning trap system was employed in a campaign of challenging measurements performed with the decay total absorption gamma-ray spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. Different strategies were applied to disentangle the isomeric states involved, lying very close in energy. The low-spin component of each niobium case was populated through the decay of the zirconium parent, which was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained beta-intensity distributions for these zirconium decays. The beta-strength distributions evaluated with these results were compared with calculations in a quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of Zr-100,Zr-102. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The beta-intensities of the decay of Nb-102m, for which there were no previous data, were obtained. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported, and here we detail the significant impact on decay heat calculations. |
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Address |
[Guadilla, V; Algora, A.; Tain, J. L.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Orrigo, S. E. A.; Rubio, B.; Valencia, E.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46071 Valencia, Spain, Email: guadilla@ific.uv.es; |
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Publisher |
Amer Physical Soc |
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English |
Summary Language |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
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Expedition |
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Conference |
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Notes |
WOS:000480237600001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4105 |
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Permanent link to this record |
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Author |
Guadilla, V. et al; Tain, J.L.; Algora, A.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Nacher, E.; Orrigo, S.E.A.; Rubio, B.; Valencia, E. |
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Title |
Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters I-137 and Rb-95 |
Type |
Journal Article |
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Year |
2019 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
100 |
Issue |
4 |
Pages |
044305 - 17pp |
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Keywords |
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Abstract |
The decays of the beta-delayed neutron emitters( 137)I and Rb-95 have been studied with the total absorption gamma-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyvaskyla allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption gamma-ray spectrometer, a segmented detector composed of 18 NaI(T1) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt gamma rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of beta intensity to states above the neutron separation energy that deexcite by gamma rays, comparable to the neutron emission probability. The competition between gamma deexcitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the beta-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers. |
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Address |
[Guadilla, V; Tain, J. L.; Algora, A.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Nacher, E.; Orrigo, S. E. A.; Rubio, B.; Valencia, E.] Univ Valencia, Inst Fis Corpuscular, CSIC, E-46071 Valencia, Spain, Email: guadilla@ific.uv.es |
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Corporate Author |
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Publisher |
Amer Physical Soc |
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English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000489250100001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4169 |
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Permanent link to this record |
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Author |
Algora, A.; Ganioglu, E.; Sarriguren, P.; Guadilla, V.; Fraile, L.M.; Nacher, E.; Rubio, B.; Tain, J.L.; Agramunt, J.; Gelletly, W.; Briz, J.A.; Cakirli, R.B.; Fallot, M.; Jordan, D.; Halasz, Z.; Kuti, I.; Montaner, A.; Onillon, A.; Orrigo, S.E.A.; Cerdan, A.P.; Rice, S.; Vedia, V.; Valencia, E. |
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Title |
Total absorption gamma-ray spectroscopy study of the beta-decay of Hg-186 |
Type |
Journal Article |
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Year |
2021 |
Publication |
Physics Letters B |
Abbreviated Journal |
Phys. Lett. B |
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Volume |
819 |
Issue |
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Pages |
136438 - 7pp |
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Keywords |
Betadecay; Totalabsorption spectroscopy; Shape coexistence |
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Abstract |
The Gamow-Teller strength distribution of the decay of Hg-186 into Au-186 has been determined for the first time using the total absorption gamma spectroscopy technique and has been compared with theoretical QRPA calculations using the SLy4 Skyrme force. The measured Gamow-Teller strength distribution and the half-life are described by mixing oblate and prolate configurations independently in the parent and daughter nuclei. In this theoretical framework the best description of the experimental beta strength is obtained with dominantly prolate components for both parent Hg-186 and daughter Au-186. The approach also allowed us to determine an upper limit of the oblate component in the parent state. The complexity of the analysis required the development of a new approach in the analysis of the X-ray gated total absorption spectrum. |
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Address |
[Algora, A.; Guadilla, V; Nacher, E.; Rubio, B.; Tain, J. L.; Agramunt, J.; Jordan, D.; Montaner, A.; Orrigo, S. E. A.; Cerdan, A. Perez; Valencia, E.] Univ Valencia, Inst Fis Corpuscular, CSIC, E-46071 Valencia, Spain, Email: algora@ific.uv.es; |
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Publisher |
Elsevier |
Place of Publication |
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English |
Summary Language |
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Original Title |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0370-2693 |
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Expedition |
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Conference |
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Notes |
WOS:000679259200010 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4923 |
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Permanent link to this record |
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Author |
Guadilla, V. et al; Algora, A.; Tain, J.L.; Agramunt, J.; Jordan, D.; Monserrate, M.; Montaner-Piza, A.; Nacher, E.; Orrigo, S.E.A.; Rubio, B.; Valencia, E. |
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Title |
Total absorption gamma-ray spectroscopy of the ss decays of Y-96gs,Y-m |
Type |
Journal Article |
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Year |
2022 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
106 |
Issue |
1 |
Pages |
014306 - 14pp |
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Keywords |
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Abstract |
The ss decays of the ground state (gs) and isomeric state (m) of Y-96 have been studied with the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8(+) isomeric state from the 0(-) ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The ss-intensity distributions of both decays have been independently determined. In the analyses the deexcitation of the 1581.6 keV level in Zr-96, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the ss-detector efficiency, influencing the ss-intensity distribution obtained. Our results for Y-96gs (0(-)) confirm the large ground state to ground state ss-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to 96.6(-2.1)(+0.3) % of the total ss intensity. Given that the decay of Y-96gs is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of Y-96m (8(+)), previously undetected ss intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption gamma-ray spectroscopy measurements of ss decays with highly fragmented deexcitation patterns. Y-96m (8(+)) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average ss and gamma energies differ significantly from the previous values in evaluated databases. The discrepancy is far above the previously quoted uncertainties. Finally, we also report on the successful implementation of an innovative total absorption gamma-ray spectroscopy analysis of the module-multiplicity gated spectra, as a first proof of principle to distinguish between decaying states with very different spin-parity values. |
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Address |
[Guadilla, V; Le Meur, L.; Fallot, M.; Briz, J. A.; Estienne, M.; Giot, L.; Porta, A.; Cucoanes, A.; Shiba, T.; Zakari-Issoufou, A-A] Univ Nantes, Subatech, IMT Atlantique, CNRS IN2P3, F-44307 Nantes, France, Email: vguadilla@fuw.edu.pl |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000832364800001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5313 |
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Permanent link to this record |
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Author |
Tain, J.L.; Algora, A.; Agramunt, J.; Guadilla, V.; Jordan, M.D.; Montaner-Piza, A.; Rubio, B.; Valencia, E.; Cano-Ott, D.; Gelletly, W.; Martinez, T.; Mendoza, E.; Podolyak, Z.; Regan, P.; Simpson, J.; Smith, A.J.; Strachan, J. |
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Title |
A decay total absorption spectrometer for DESPEC at FAIR |
Type |
Journal Article |
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Year |
2015 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
803 |
Issue |
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Pages |
36-46 |
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Keywords |
Total absorption gamma-ray spectrometer; Scintillation detectors; Beta decay; High-energy beam fragmentation facilities |
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Abstract |
This paper presents the design of a total absorption gamma-ray spectrometer for the determination of beta-decay intensity distributions of exotic nuclear species at the focal plane of the FAIR-NUSTAR Super Fragment Separator. The spectrometer is a key instrument in the DESPEC experiment and the proposed implementation follows extensive design studies and prototype tests. Two options were contemplated, based on Nal(TI) and LaBr3:Ce inorganic scintillation crystals respectively. Monte Carlo simulations and technical considerations determined the optimal configurations consisting of sixteen 15 x 15 x 25 cm(3) crystals for the Nal(Tl) option and one hundred and twenty-eight 5.5 x 5.5 x 11 cm(3) crystals for the LaBr3:Ce option. Minimization of dead material was crucial for maximizing the spectrometer full-energy peak efficiency. Module prototypes were build to verify constructional details and characterize their performance. The measured energy and timing resolution was found to agree rather well with estimates based on simulations of scintillation light transport and collection. The neutron sensitivity of the spectrometer, important when measuring beta-delayed neutron emitters, was investigated by means of Monte Carlo simulations. |
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Address |
[Tain, J. L.; Algora, A.; Agramunt, J.; Guadilla, V.; Jordan, M. D.; Montaner-Piza, A.; Rubio, B.; Valencia, E.] Univ Valencia, Inst Fis Corpuscular, CSIC, E-46071 Valencia, Spain, Email: tain@ific.uv.es |
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Corporate Author |
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Thesis |
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Publisher |
Elsevier Science Bv |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0168-9002 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000363464600007 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2431 |
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Permanent link to this record |
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Author |
Tain, J.L. et al; Valencia, E.; Algora, A.; Agramunt, J.; Rubio, B.; Estevez, E.; Jordan, M.D. |
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Title |
Enhanced gamma-Ray Emission from Neutron Unbound States Populated in beta Decay |
Type |
Journal Article |
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Year |
2015 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
115 |
Issue |
6 |
Pages |
062502 - 5pp |
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Keywords |
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Abstract |
Total absorption spectroscopy is used to investigate the beta-decay intensity to states above the neutron separation energy followed by gamma-ray emission in Br-87,Br-88 and Rb-94. Accurate results are obtained thanks to a careful control of systematic errors. An unexpectedly large. intensity is observed in all three cases extending well beyond the excitation energy region where neutron penetration is hindered by low neutron energy. The gamma branching as a function of excitation energy is compared to Hauser-Feshbach model calculations. For Br-87 and Br-88 the gamma branching reaches 57% and 20%, respectively, and could be explained as a nuclear structure effect. Some of the states populated in the daughter can only decay through the emission of a large orbital angular momentum neutron with a strongly reduced barrier penetrability. In the case of neutron-rich Rb-94 the observed 4.5% branching is much larger than the calculations performed with standard nuclear statistical model parameters, even after proper correction for fluctuation effects on individual transition widths. The difference can be reconciled by introducing an enhancement of 1 order of magnitude in the photon strength to neutron strength ratio. An increase in the photon strength function of such magnitude for very neutron-rich nuclei, if it proves to be correct, leads to a similar increase in the (n, gamma) cross section that would have an impact on r process abundance calculations. |
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Address |
[Tain, J. L.; Valencia, E.; Algora, A.; Agramunt, J.; Rubio, B.; Estevez, E.; Jordan, M. D.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46071 Valencia, Spain, Email: tain@ific.uv.es |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0031-9007 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000359059100002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2319 |
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Permanent link to this record |
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Author |
Valencia, E. et al; Tain, J.L.; Algora, A.; Agramunt, J.; Estevez, E.; Jordan, M.D.; Rubio, B. |
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Title |
Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters Br-87, Br-88, and Rb-94 |
Type |
Journal Article |
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Year |
2017 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
95 |
Issue |
2 |
Pages |
024320 - 18pp |
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Keywords |
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Abstract |
We investigate the decay of Br-87,Br-88 and Rb-94 using total absorption gamma-ray spectroscopy. These important fission products are beta-delayed neutron emitters. Our data show considerable beta gamma intensity, so far unobserved in high-resolution gamma-ray spectroscopy, from states at high excitation energy. We also find significant differences with the beta intensity that can be deduced from existing measurements of the beta spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for U-235 fission at cooling times in the range 1-100 s. We also use summation calculations to evaluate the impact of present data on reactor antineutrino spectra. We find a significant effect at antineutrino energies in the range of 5 to 9 MeV. In addition, we observe an unexpected strong probability for. emission from neutron unbound states populated in the daughter nucleus. The. branching is compared to Hauser-Feshbach calculations, which allow one to explain the large value for bromine isotopes as due to nuclear structure. However the branching for Rb-94, although much smaller, hints of the need to increase the radiative width gamma by one order of magnitude. This increase in gamma would lead to a similar increase in the calculated (n, gamma) cross section for this very neutron-rich nucleus with a potential impact on r process abundance calculations. |
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Address |
[Valencia, E.; Tain, J. L.; Algora, A.; Agramunt, J.; Estevez, E.; Jordan, M. D.; Rubio, B.] Univ Valencia, CSIC, Inst Fis Corpuscular, Apartado Correos 22085, E-46071 Valencia, Spain, Email: tain@ific.uv.es |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000394662200002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3015 |
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Permanent link to this record |