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NEXT Collaboration(Renner, J. et al), Alvarez, V., Carcel, S., Cervera-Villanueva, A., Diaz, J., Ferrario, P., et al. (2015). Ionization and scintillation of nuclear recoils in gaseous xenon. Nucl. Instrum. Methods Phys. Res. A, 793, 62–74.
Abstract: Ionization and scintillation produced by nuclear recoils in gaseous xenon at approximately 14 bar have been simultaneously observed in an electroluminescent time projection chamber. Neutrons from radioisotope a-Be neutron sources were used to induce xenon nuclear recoils, and the observed recoil spectra were compared to a detailed Monte Carlo employing estimated ionization and scintillation yields for nuclear recoils. The ability to discriminate between electronic and nuclear recoils using the ratio of ionization to primary scintillation is demonstrated. These results encourage further investigation on the use of xenon in the gas phase as a detector medium in dark matter direct detection experiments.
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NEXT Collaboration(Cebrian, S. et al), Alvarez, V., Carcel, S., Cervera-Villanueva, A., Diaz, J., Ferrario, P., et al. (2015). Accurate gamma and MeV-electron track reconstruction with an ultra-low diffusion Xenon/TMA TPC at 10 atm. Nucl. Instrum. Methods Phys. Res. A, 804, 8–24.
Abstract: We report the performance of a 10 atm Xenon/trimethylamine time projection chamber (TPC) for the detection of X-rays (30 keV) and gamma-rays (0.511-1.275 MeV) in conjunction with the accurate tracking of the associated electrons. When operated at such a high pressure and in similar to 1%-admixtures, trimethylamine (TMA) endows Xenon with an extremely low electron diffusion (1.3 +/- 0.13 mm-sigma (longitudinal), 0.95 +/- 0.20 mm-sigma (transverse) along 1 m drift) besides forming a convenient Penning-Fluorescent' mixture. The TPC, that houses 1.1 kg of gas in its fiducial volume, operated continuously for 100 live-days in charge amplification mode. The readout was performed through the recently introduced microbulk Micromegas technology and the AFTER chip, providing a 3D voxelization of 8 mm x 8 mm x 1.2 mm for approximately 10 cm/MeV-long electron tracks. Resolution in energy (epsilon) at full width half maximum (R) inside the fiducial volume ranged from R = 14.6% (30 keV) to R = 4.6% (1.275 MeV). This work was developed as part of the R&D program of the NEXT collaboration for future detector upgrades in the search of the neutrino-less double beta decay (beta beta 0 nu) in Xe-136, specifically those based on novel gas mixtures. Therefore we ultimately focus on the calorimetric and topological properties of the reconstructed MeV-electron tracks. In particular, the obtained energy resolution has been decomposed in its various contributions and improvements towards achieving the R =1.4%root MeV/epsilon levels obtained in small sensors are discussed.
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NEXT Collaboration(Azevedo, C. D. R. et al), Gomez-Cadenas, J. J., Alvarez, V., Benlloch-Rodriguez, J. M., Botas, A., Carcel, S., et al. (2018). Microscopic simulation of xenon-based optical TPCs in the presence of molecular additives. Nucl. Instrum. Methods Phys. Res. A, 877, 157–172.
Abstract: We introduce a simulation framework for the transport of high and low energy electrons in xenon-based optical time projection chambers (OTPCs). The simulation relies on elementary cross sections (electron-atom and electron-molecule) and incorporates, in order to compute the gas scintillation, the reaction/quenching rates (atom-atom and atom-molecule) of the first 41 excited states of xenon and the relevant associated excimers, together with their radiative cascade. The results compare positively with observations made in pure xenon and its mixtures with CO2 and CF4 in a range of pressures from 0.1 to 10 bar. This work sheds some light on the elementary processes responsible for the primary and secondary xenon-scintillation mechanisms in the presence of additives, that are of interest to the OTPC technology.
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NEXT Collaboration(Trindade, A. M. F. et al), Alvarez, V., Benlloch-Rodriguez, J. M., Botas, A., Carcel, S., Carrion, J. V., et al. (2018). Study of the loss of xenon scintillation in xenon-trimethylamine mixtures. Nucl. Instrum. Methods Phys. Res. A, 905, 22–28.
Abstract: This work investigates the capability of TMA ((CH3)(3)N) molecules to shift the wavelength of Xe VUV emission (160-188 nm) to a longer, more manageable, wavelength (260-350 nm). Light emitted from a Xe lamp was passed through a gas chamber filled with Xe-TMA mixtures at 800 Torr and detected with a photomultiplier tube. Using bandpass filters in the proper transmission ranges, no reemitted light was observed experimentally. Considering the detection limit of the experimental system, if reemission by TMA molecules occurs, it is below 0.3% of the scintillation absorbed in the 160-188 nm range. An absorption coefficient value for xenon VUV light by TMA of 0.43 +/- 0.03 cm(-1) Torr(-1) was also obtained. These results can be especially important for experiments considering TMA as a molecular additive to Xe in large volume optical time projection chambers.
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NEXT Collaboration(Felkai, R. et al), Sorel, M., Lopez-March, N., Gomez-Cadenas, J. J., Alvarez, V., Benlloch-Rodriguez, J. M., et al. (2018). Helium-Xenon mixtures to improve the topological signature in high pressure gas xenon TPCs. Nucl. Instrum. Methods Phys. Res. A, 905, 82–90.
Abstract: Within the framework of xenon-based double beta decay experiments, we propose the possibility to improve the background rejection of an electroluminescent Time Projection Chamber (EL TPC) by reducing the diffusion of the drifting electrons while keeping nearly intact the energy resolution of a pure xenon EL TPC. Based on state-of-the-art microscopic simulations, a substantial addition of helium, around 10 or 15 %, may reduce drastically the transverse diffusion down to 2.5 mm/root m from the 10.5 mm/root m of pure xenon. The longitudinal diffusion remains around 4 mm/root m. Light production studies have been performed as well. They show that the relative variation in energy resolution introduced by such a change does not exceed a few percent, which leaves the energy resolution practically unchanged. The technical caveats of using photomultipliers close to an helium atmosphere are also discussed in detail.
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Azevedo, C. D. R., Baeza, A., Chauveau, E., Corbacho, J. A., Diaz, J., Domange, J., et al. (2020). Simulation results of a real-time in water tritium monitor. Nucl. Instrum. Methods Phys. Res. A, 982, 164555–7pp.
Abstract: In this work we present simulation results for a modular tritium in-water real-time monitor. The system allows for scalability in order to achieve the required sensitivity. The modules are composed by 340 uncladed scintillating fibers immersed in water and 2 photosensors in coincidence for light readout. Light yield and Birks' coefficient uncertainties for low energy beta particles is discussed. A study of the detection efficiency according to the fiber length is presented. Discussion on the system requirements and background mitigation for a device with sensitivity of 100 Bq/L, required to comply with the European directive 2013/51/Euratom, is presented. Due to the low energetic beta emission from tritium a detection efficiency close to 3.3% was calculated for a single 2 mm round fiber.
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NEXT Collaboration(Jones, B. J. P. et al), Carcel, S., Carrion, J. V., Diaz, J., Martin-Albo, J., Martinez, A., et al. (2022). The dynamics of ions on phased radio-frequency carpets in high pressure gases and application for barium tagging in xenon gas time projection chambers. Nucl. Instrum. Methods Phys. Res. A, 1039, 167000–19pp.
Abstract: Radio-frequency (RF) carpets with ultra-fine pitches are examined for ion transport in gases at atmospheric pressures and above. We develop new analytic and computational methods for modeling RF ion transport at densities where dynamics are strongly influenced by buffer gas collisions. An analytic description of levitating and sweeping forces from phased arrays is obtained, then thermodynamic and kinetic principles are used to calculate ion loss rates in the presence of collisions. This methodology is validated against detailed microscopic SIMION simulations. We then explore a parameter space of special interest for neutrinoless double beta decay experiments: transport of barium ions in xenon at pressures from 1 to 10 bar. Our computations account for molecular ion formation and pressure dependent mobility as well as finite temperature effects. We discuss the challenges associated with achieving suitable operating conditions, which lie beyond the capabilities of existing devices, using presently available or near-future manufacturing techniques.
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Azevedo, C. D. R., Baeza, A., Chauveau, E., Corbacho, J. A., Diaz, J., Domange, J., et al. (2023). Design, setup and routine operation of a water treatment system for the monitoring of low activities of tritium in water. Nucl. Eng. Technol., 55(7), 2349–2355.
Abstract: In the TRITIUM project, an on-site monitoring system is being developed to measure tritium (3H) levels in water near nuclear power plants. The quite low-energy betas emitted by 3H have a very short average path in water (5 mm as shown by simulations for 18 keV electrons). This path would be further reduced by impurities present in the water, resulting in a significant reduction of the detection efficiency. Therefore, one of the essential requirements of the project is the elimination of these impurities through a filtration process and the removal of salts in solution. This paper describes a water treatment system developed for the project that meets the following requirements: the water produced should be of nearpure water quality according to ISO 3696 grade 3 standard (conductivity < 10 mS/cm); the system should operate autonomously and be remotely monitored.
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NEXT Collaboration, Carcel, S., Carrion, J. V., Felkai, R., Kekic, M., Lopez-March, N., et al. (2020). Mitigation of backgrounds from cosmogenic Xe-137 in xenon gas experiments using He-3 neutron capture. J. Phys. G, 47(7), 075001–17pp.
Abstract: Xe-136 is used as the target medium for many experiments searching for 0 nu beta beta. Despite underground operation, cosmic muons that reach the laboratory can produce spallation neutrons causing activation of detector materials. A potential background that is difficult to veto using muon tagging comes in the form of Xe-137 created by the capture of neutrons on Xe-136. This isotope decays via beta decay with a half-life of 3.8 min and a Q(beta) of similar to 4.16 MeV. This work proposes and explores the concept of adding a small percentage of He-3 to xenon as a means to capture thermal neutrons and reduce the number of activations in the detector volume. When using this technique we find the contamination from Xe-137 activation can be reduced to negligible levels in tonne and multi-tonne scale high pressure gas xenon neutrinoless double beta decay experiments running at any depth in an underground laboratory.
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Fernandes, L. M. P., Freitas, E. D. C., Ball, M., Gomez-Cadenas, J. J., Monteiro, C. M. B., Yahlali, N., et al. (2010). Primary and secondary scintillation measurements in a Xenon Gas Proportional Scintillation Counter. J. Instrum., 5, P09006–15pp.
Abstract: NEXT is a new experiment to search for neutrinoless double beta decay using a 100 kg radio-pure high-pressure gaseous xenon TPC. The detector requires excellent energy resolution, which can be achieved in a Xe TPC with electroluminescence readout. Hamamatsu R8520-06SEL photomultipliers are good candidates for the scintillation readout. The performance of this photomultiplier, used as VUV photosensor in a gas proportional scintillation counter, was investigated. Initial results for the detection of primary and secondary scintillation produced as a result of the interaction of 5.9 keV X-rays in gaseous xenon, at room temperature and at pressures up to 3 bar, are presented. An energy resolution of 8.0% was obtained for secondary scintillation produced by 5.9 keV X-rays. No significant variation of the primary scintillation was observed for different pressures (1, 2 and 3 bar) and for electric fields up to 0.8 V cm(-1) torr(-1) in the drift region, demonstrating negligible recombination luminescence. A primary scintillation yield of 81 +/- 7 photons was obtained for 5.9 keV X-rays, corresponding to a mean energy of 72 +/- 6 eV to produce a primary scintillation photon in xenon.
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