n_TOF Collaboration(Alcayne, V. et al), Babiano-Suarez, V., Caballero-Ontanaya, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2026). Measurement of the 244Cm neutron capture cross section at the n_TOF facility at CERN. Ann. Nucl. Energy, 227, 111977–14pp.
Abstract: Accurate neutron capture cross section data for minor actinides are essential for the safe and efficient management of high level radioactive waste produced during the operation of nuclear reactors. In particular, Cm-244, with a half-life of 18.11 years, dominates neutron emission in spent fuel and also contributes significantly to the decay heat and radiotoxicity. Furthermore, neutron capture on Cm-244 opens the pathway for the formation of heavier isotopes such as Bk, Cf, and other Cm isotopes. Sensitivity studies for present and future nuclear reactors have highlighted the need to reduce the uncertainties in the Cm-244 capture cross section. Experimental data on the capture cross section of this isotope are scarce due to the challenges associated with its measurements. Prior to the presented measurement and two recent measurements conducted at J-PARC, only one set of data for the Cm-244 capture cross section existed, obtained in 1969 during an underground nuclear explosion experiment. The capture cross section of Cm-244 has been measured at the nTOF facility at CERN with three different experimental setups: one at Experimental Area 1 (EAR1) using the Total Absorption Calorimeter and two measurements at Experimental Area 2 (EAR2) with C6D6 detectors, employing two different samples. The results from these three measurements were found to be compatible and then combined. In total, 17 resonances of Cm-244 were measured at nTOF below 300 eV. The radiative kernels obtained in this measurement are in good agreement with JENDL-4.0 for the majority of the resonances. Additionally, they are compatible with the recent JENDL-5 library below 50 eV, while at higher energies, the majority of radiative kernels from this evaluation based on the recent measurement by Kawase et al., are not compatible. Additionally, the Cm-244 samples also contained Pu-240. Resonances of this isotope were analyzed in the energy range between 20 and 180 eV, and the results were found to be consistent with previous measurements and evaluations, that enhances confidence in the Cm-244 results.
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n_TOF Collaboration(Alcayne, V. et al), Balibrea-Correa, J., Domingo-Pardo, C., Lerendegui-Marco, J., Babiano-Suarez, V., & Ladarescu, I. (2024). A Segmented Total Energy Detector (sTED) optimized for (n,γ) cross-section measurements at n_TOF EAR2. Radiat. Phys. Chem., 217, 111525–11pp.
Abstract: The neutron time-of-flight facility nTOF at CERN is a spallation source dedicated to measurements of neutroninduced reaction cross-sections of interest in nuclear technologies, astrophysics, and other applications. Since 2014, Experimental ARea 2 (EAR2) is operational and delivers a neutron fluence of similar to 4 center dot 10(7) neutrons per nominal proton pulse, which is similar to 50 times higher than the one of Experimental ARea 1 (EAR1) of similar to 8 center dot 10(5) neutrons per pulse. The high neutron flux at EAR2 results in high counting rates in the detectors that challenged the previously existing capture detection systems. For this reason, a Segmented Total Energy Detector (sTED) has been developed to overcome the limitations in the detector's response, by reducing the active volume per module and by using a photo-multiplier (PMT) optimized for high counting rates. This paper presents the main characteristics of the sTED, including energy and time resolution, response to gamma-rays, and provides as well details of the use of the Pulse Height Weighting Technique (PHWT) with this detector. The sTED has been validated to perform neutron-capture cross-section measurements in EAR2 in the neutron energy range from thermal up to at least 400 keV. The detector has already been successfully used in several measurements at nTOF EAR2.
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n_TOF Collaboration(Alcayne, V. et al), Caballero-Ontanaya, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2024). Measurement and analysis of the 246Cm and 248Cm neutron capture cross-sections at the EAR2 of the n_TOF facility at CERN. Eur. Phys. J. A, 60(12), 246–20pp.
Abstract: The 246Cm(n,γ) and 248Cm(n,γ) cross-sections have been measured at the Experimental Area 2 (EAR2) of the nTOF facility at CERN with three C6D6 detectors. This measurement is part of a collective effort to improve the capture cross-section data for Minor Actinides (MAs), which are required to estimate the production and transmutation rates of these isotopes in light water reactors and innovative reactor systems. In particular, the neutron capture in 246Cm and 248Cm open the path for the formation of other Cm isotopes and heavier elements such as Bk and Cf and the knowledge of (n,γ) cross-sections of these Cm isotopes plays an important role in the transport, transmutation and storage of the spent nuclear fuel. The reactions 246Cm(n,γ) and 248Cm(n,γ) have been the two first capture measurements analyzed at nTOF EAR2. Until this experiment and two recent measurements performed at J-PARC, there was only one set of data of the capture cross-sections of 246Cm and 248Cm, that was obtained in 1969 in an underground nuclear explosion experiment. In the measurement at n_TOF a total of 13 resonances of 246Cm between 4 and 400 eV and 5 of 248Cm between 7 and 100 eV have been identified and fitted. The radiative kernels obtained for 246Cm are compatible with JENDL-5, but some of them are not with JENDL-4, which has been adopted by JEFF-3.3 and ENDF/B-VIII.0. The radiative kernels obtained for the first three 248Cm resonances are compatible with JENDL-5, however, the other two are not compatible with any other evaluation and are 20% and 60% larger than JENDL-5.
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