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Briz, J. A., Nacher, E., Borge, M. J. G., Algora, A., Rubio, B., Dessagne, P., et al. (2015). Shape study of the N = Z nucleus Kr-72 via beta decay. Phys. Rev. C, 92(5), 054326–10pp.
Abstract: The beta decay of the N = Z nucleus Kr-72 has been studied with the total absorption spectroscopy technique at ISOLDE (CERN). A total B(GT) = 0.79(4)g(A)(2)/4 pi has been found up to an excitation energy of 2.7 MeV. The B(GT) distribution obtained is compared with predictions from state-of-the-art theoretical calculations to learn about the ground state deformation of Kr-72. Although a dominant oblate deformation is suggested by direct comparison with quasiparticle random phase approximation (QRPA) calculations, beyond-mean-field and shell-model calculations favor a large oblate-prolate mixing in the ground state.
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Nacher, E., Rubio, B., Algora, A., Cano-Ott, D., Tain, J. L., Gadea, A., et al. (2016). Observations of the Gamow-Teller resonance in the rare-earth nuclei above Gd-146 populated in beta decay. Phys. Rev. C, 93(1), 014308–13pp.
Abstract: The rare-earth region of the nuclear table around the quasi-doubly magic nucleus Gd-146 is one of the very few places in which the Gamow-Teller (GT) resonance can be populated in beta decay. The appropriate technique to study such a phenomenon is total absorption spectroscopy, thanks to which one can measure the B(GT) distribution in beta-decay experiments even when it is very fragmented and lies at high excitation energy in the daughter nucleus. Results on the GT resonance measured in the beta decay of the odd-Z, N = 83 nuclei Tb-148, Ho-150, and Tm-152 are presented in this work and compared with shell-model calculations. The tail of the resonance is clearly observed up to the limit imposed by the Q value. This observation is important in the context of the understanding of the “quenching” of the GT strength.
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n_TOF Collaboration(Diakaki, M. et al), Domingo-Pardo, C., & Tain, J. L. (2016). Neutron-induced fission cross section of Np-237 in the keV to MeV range at the CERN n_TOF facility. Phys. Rev. C, 93(3), 034614–12pp.
Abstract: The neutron-induced fission cross section of Np-237 was experimentally determined at the high-resolution and high-intensity facility n_TOF, at CERN, in the energy range 100 keV to 9 MeV, using the U-235(n, f) and U-238(n, f) cross section standards below and above 2 MeV, respectively. A fast ionization chamber was used in order to detect the fission fragments from the reactions and the targets were characterized as far as their mass and homogeneity are concerned by means of a spectroscopy and Rutherford backscattering spectroscopy respectively. Theoretical calculations within the Hauser-Feshbach formalism have been performed, employing the EMPIRE code, and the model parameters were tuned in order to successfully reproduce the experimental fission cross-sectional data and simultaneously all the competing reaction channels.
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Valencia, E. et al, Tain, J. L., Algora, A., Agramunt, J., Estevez, E., Jordan, M. D., et al. (2017). Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters Br-87, Br-88, and Rb-94. Phys. Rev. C, 95(2), 024320–18pp.
Abstract: We investigate the decay of Br-87,Br-88 and Rb-94 using total absorption gamma-ray spectroscopy. These important fission products are beta-delayed neutron emitters. Our data show considerable beta gamma intensity, so far unobserved in high-resolution gamma-ray spectroscopy, from states at high excitation energy. We also find significant differences with the beta intensity that can be deduced from existing measurements of the beta spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for U-235 fission at cooling times in the range 1-100 s. We also use summation calculations to evaluate the impact of present data on reactor antineutrino spectra. We find a significant effect at antineutrino energies in the range of 5 to 9 MeV. In addition, we observe an unexpected strong probability for. emission from neutron unbound states populated in the daughter nucleus. The. branching is compared to Hauser-Feshbach calculations, which allow one to explain the large value for bromine isotopes as due to nuclear structure. However the branching for Rb-94, although much smaller, hints of the need to increase the radiative width gamma by one order of magnitude. This increase in gamma would lead to a similar increase in the calculated (n, gamma) cross section for this very neutron-rich nucleus with a potential impact on r process abundance calculations.
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n_TOF Collaboration(Mingrone, F. et al), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2017). Neutron capture cross section measurement of U-238 at the CERN n_TOF facility in the energy region from 1 eV to 700 keV. Phys. Rev. C, 95(3), 034604–14pp.
Abstract: The aim of this work is to provide a precise and accurate measurement of the U-238(n,gamma) reaction cross section in the energy region from 1 eV to 700 keV. This reaction is of fundamental importance for the design calculations of nuclear reactors, governing the behavior of the reactor core. In particular, fast reactors, which are experiencing a growing interest for their ability to burn radioactive waste, operate in the high energy region of the neutron spectrum. In this energy region most recent evaluations disagree due to inconsistencies in the existing measurements of up to 15%. In addition, the assessment of nuclear data uncertainty performed for innovative reactor systems shows that the uncertainty in the radiative capture cross section of U-238 should be further reduced to 1-3% in the energy region from 20 eV to 25 keV. To this purpose, addressed by the Nuclear Energy Agency as a priority nuclear data need, complementary experiments, one at the GELINA and two at the nTOF facility, were proposed and carried out within the 7th Framework Project ANDES of the European Commission. The results of one of these U-238(n, gamma) measurements performed at the nTOF CERN facility are presented in this work. The gamma-ray cascade following the radiative neutron capture has been detected exploiting a setup of two C6D6 liquid scintillators. Resonance parameters obtained from this work are on average in excellent agreement with the ones reported in evaluated libraries. In the unresolved resonance region, this work yields a cross section in agreement with evaluated libraries up to 80 keV, while for higher energies our results are significantly higher.
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Caballero-Folch, R. et al, Domingo-Pardo, C., Agramunt, J., Algora, A., Rubio, B., & Tain, J. L. (2017). beta-decay half-lives and beta-delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb, and Bi, beyond N=126. Phys. Rev. C, 95(6), 064322–16pp.
Abstract: Background: There have been measurements on roughly 230 nuclei that are beta-delayed neutron emitters. They range from He-8 up to La-150. Apart from 210Tl, with a branching ratio of only 0.007%, no other neutron emitter has been measured beyond A = 150. Therefore, new data are needed, particularly in the region of heavy nuclei around N = 126, in order to guide theoretical models and help understand the formation of the third r-process peak at A similar to 195. Purpose: To measure both beta-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb, and Bi isotopes beyond N = 126. Method: Ions of interest were produced by fragmentation of a U-238 beam, selected and identified via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) was used to measure ion implants and beta decays. An array of 30 He-3 tubes embedded in a polyethylene matrix (BELEN) was used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time correlations. The latter were analyzed with an analytical model and results for the half-lives and neutron-branching ratios were derived by using the binned maximum-likelihood method. Results: Twenty new beta-decay half-lives are reported for Au204-206, Hg208-211, Tl211-216, Pb215-218, and Bi218-220, nine of them for the first time. Neutron emission probabilities are reported for Hg-210,Hg-211 and Tl211-216. Conclusions: The new beta-decay half-lives are in good agreement with previous measurements on nuclei in this region. The measured neutron emission probabilities are comparable to or smaller than values predicted by global models such as relativistic Hartree Bogoliubov plus the relativistic quasi-particle random phase approximation (RHB + RQRPA).
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Jordan, M. D., Montaner-Piza, A., et al. (2017). Experimental study of Tc-100 beta decay with total absorption gamma-ray spectroscopy. Phys. Rev. C, 96(1), 014319–10pp.
Abstract: The beta decay of Tc-100 has been studied by using the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. In this work the new Decay Total Absorption gamma-ray Spectrometer in coincidence with a cylindrical plastic beta detector has been employed. The beta intensity to the ground state obtained from the analysis is in good agreement with previous high-resolution measurements. However, differences in the feeding to the first-excited state as well as weak feeding to a new level at high excitation energy have been deduced from this experiment. Theoretical calculations performed in the quasiparticle random-phase approximation framework are also reported. Comparison of these calculations with our measurement serves as a benchmark for calculations of the double beta decay of Mo-100.
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Rice, S. et al, Algora, A., Tain, J. L., Valencia, E., Agramunt, J., Rubio, B., et al. (2017). Total absorption spectroscopy study of the beta decay of Br-86 and Rb-91. Phys. Rev. C, 96(1), 014320–10pp.
Abstract: The beta decays of Br-86 and Rb-91 have been studied using the total absorption spectroscopy technique. The radioactive nuclei were produced at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla and further purified using the JYFLTRAP. Br-86 and Rb-91 are considered to be major contributors to the decay heat in reactors. In addition, Rb-91 was used as a normalization point in direct measurements of mean gamma energies released in the beta decay of fission products by Rudstam et al. assuming that this decaywas well known from high-resolution measurements. Our results show that both decays were suffering from the Pandemonium effect and that the results of Rudstam et al. should be renormalized. The relative impact of the studied decays in the prediction of the decay heat and antineutrino spectrum from reactors has been evaluated.
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n_TOF Collaboration(Wright, T. et al), Domingo-Pardo, C., Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2017). Measurement of the U-238(n,gamma) cross section up to 80 keV with the Total Absorption Calorimeter at the CERN n_TOF facility. Phys. Rev. C, 96(6), 064601–11pp.
Abstract: The radiative capture cross section of a highly pure (99.999%), 6.125(2) grams and 9.56(5) x 10(-4) atoms/barn areal density U-238 sample has been measured with the Total Absorption Calorimeter (TAC) in the 185 m flight path at the CERN neutron time-of-flight facility n_TOF. This measurement is in response to the NEA High Priority Request list, which demands an accuracy in this cross section of less than 3% below 25 keV. These data have undergone careful background subtraction, with special care being given to the background originating from neutrons scattered by the 238U sample. Pileup and dead-time effects have been corrected for. The measured cross section covers an energy range between 0.2 eV and 80 keV, with an accuracy that varies with neutron energy, being better than 4% below 25 keV and reaching at most 6% at higher energies.
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n_TOF Collaboration(Lerendegui-Marco, J. et al.), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2018). Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility. Phys. Rev. C, 97(2), 024605–21pp.
Abstract: The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA.
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