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n_TOF Collaboration(Belloni, F. et al), Domingo-Pardo, C., & Tain, J. L. (2013). Measurement of the neutron-induced fission cross-section of Am-241 at the time-of-flight facility n_TOF. Eur. Phys. J. A, 49(1), 2–6pp.
Abstract: The neutron-induced fission cross-section of Am-241 has been measured relative to the standard fission cross-section of U-235 between 0.5 and 20 MeV. The experiment was performed at the CERN nTOF facility. Fission fragments were detected by a fast ionization chamber by discriminating against the alpha-particles from the high radioactivity of the samples. The high instantaneous neutron flux and the low background of the nTOF facility enabled us to obtain uncertainties of approximate to 5%. With the present results it was possible to resolve discrepancies between previous data sets and to confirm current evaluations, thus providing important information for design studies of future reactors with improved fuel burn-up.
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n_TOF Collaboration(Amaducci, S. et al), Babiano-Suarez, V., Caballero-Ontanaya, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2021). First Results of the Ce-140(n,gamma)Ce-141 Cross-Section Measurement at n_TOF. Universe, 7(6), 200–11pp.
Abstract: An accurate measurement of the Ce-140(n,gamma) energy-dependent cross-section was performed at the n_TOF facility at CERN. This cross-section is of great importance because it represents a bottleneck for the s-process nucleosynthesis and determines to a large extent the cerium abundance in stars. The measurement was motivated by the significant difference between the cerium abundance measured in globular clusters and the value predicted by theoretical stellar models. This discrepancy can be ascribed to an overestimation of the Ce-140 capture cross-section due to a lack of accurate nuclear data. For this measurement, we used a sample of cerium oxide enriched in Ce-140 to 99.4%. The experimental apparatus consisted of four deuterated benzene liquid scintillator detectors, which allowed us to overcome the difficulties present in the previous measurements, thanks to their very low neutron sensitivity. The accurate analysis of the p-wave resonances and the calculation of their average parameters are fundamental to improve the evaluation of the Ce-140 Maxwellian-averaged cross-section.
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Mistry, A. K. et al, Tain, J. L., Agramunt, J., Algora, A., Guadilla, V., Morales, A. I., et al. (2022). The DESPEC setup for GSI and FAIR. Nucl. Instrum. Methods Phys. Res. A, 1033, 166662–18pp.
Abstract: The DEcay SPECtroscopy (DESPEC) setup for nuclear structure investigations was developed and commissioned at GSI, Germany in preparation for a full campaign of experiments at the FRS and Super-FRS. In this paper, we report on the first employment of the setup in the hybrid configuration with the AIDA implanter coupled to the FATIMA LaBr3(Ce) fast-timing array, and high-purity germanium detectors. Initial results are shown from the first experiments carried out with the setup. An overview of the setup and function is discussed, including technical advancements along the path.
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Jordan, D. et al, Algora, A., Tain, J. L., Rubio, B., Agramunt, J., Perez-Cerdan, A. B., et al. (2013). Total absorption study of the beta decay of Tc-102,Tc-104,Tc-105. Phys. Rev. C, 87(4), 044318–14pp.
Abstract: The beta-feeding probabilities for three important contributors to the decay heat in nuclear reactors, namely Tc-102,Tc-104,Tc-105, have been measured using the total absorption spectroscopy technique. For the measurements, sources of very high isobaric purity have been obtained using a Penning trap (JYFLTRAP). A detailed description of the data analysis is given and the results are compared with high-resolution measurements and theoretical calculations. DOI: 10.1103/PhysRevC.87.044318
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Agramunt, J. et al, Algora, A., Domingo-Pardo, C., Jordan, D., Rubio, B., Tain, J. L., et al. (2014). New Beta-delayed Neutron Measurements in the Light-mass Fission Group. Nucl. Data Sheets, 120, 74–77.
Abstract: A new accurate determination of beta-delayed neutron emission probabilities from nuclei in the low mass region of the light fission group has been performed. The measurements were carried out using the BELEN 4 pi neutron counter at the IGISOL-JYFL mass separator in combination with a Penning trap. The new results significantly improve the uncertainties of neutron emission probabilities for Br-91, As-86, As-85, and Ge-85 nuclei.
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Agramunt, J. et al, Tain, J. L., Albiol, F., Algora, A., Domingo-Pardo, C., Jordan, M. D., et al. (2016). Characterization of a neutron-beta counting system with beta-delayed neutron emitters. Nucl. Instrum. Methods Phys. Res. A, 807, 69–78.
Abstract: A new detection system for the measurement of beta-delayed neutron emission probabilities has been characterized using fission products with well known beta-delayed neutron emission properties. The setup consists of BELEN-20, a 4 pi-neutron counter with twenty He-3 proportional tubes arranged inside a large polyethylene neutron moderator, a thin Si detector for beta counting and a self-triggering digital data acquisition system. The use of delayed-neutron precursors with different neutron emission windows allowed the study of the effect of energy dependency on neutron, beta and beta-neutron rates. The observed effect is well reproduced by Monte Carlo simulations. The impact of this dependency on the accuracy of neutron emission probabilities is discussed. A new accurate value of the neutron emission probability for the important delayed-neutron precursor I-137 was obtained, P-n = 7.76(14)%.
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Estevez, E. et al, Algora, A., Rubio, B., Bernabeu, J., Nacher, E., Tain, J. L., et al. (2011). beta-decay study of (150)Er, (152)Yb, and (156)Yb: Candidates for a monoenergetic neutrino beam facility. Phys. Rev. C, 84(3), 034304–6pp.
Abstract: The beta decays of (150)Er, (152)Yb, and (156)Yb nuclei are investigated using the total absorption spectroscopy technique. These nuclei can be considered possible candidates for forming the beam of a monoenergetic neutrino beam facility based on the electron capture (EC) decay of radioactive nuclei. Our measurements confirm that for the cases studied the EC decay proceeds mainly to a single state in the daughter nucleus.
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Algora, A., Ganioglu, E., Sarriguren, P., Guadilla, V., Fraile, L. M., Nacher, E., et al. (2021). Total absorption gamma-ray spectroscopy study of the beta-decay of Hg-186. Phys. Lett. B, 819, 136438–7pp.
Abstract: The Gamow-Teller strength distribution of the decay of Hg-186 into Au-186 has been determined for the first time using the total absorption gamma spectroscopy technique and has been compared with theoretical QRPA calculations using the SLy4 Skyrme force. The measured Gamow-Teller strength distribution and the half-life are described by mixing oblate and prolate configurations independently in the parent and daughter nuclei. In this theoretical framework the best description of the experimental beta strength is obtained with dominantly prolate components for both parent Hg-186 and daughter Au-186. The approach also allowed us to determine an upper limit of the oblate component in the parent state. The complexity of the analysis required the development of a new approach in the analysis of the X-ray gated total absorption spectrum.
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Algora, A. et al, Jordan, D., Tain, J. L., Rubio, B., Agramunt, J., Perez-Cerdan, A. B., et al. (2010). Reactor Decay Heat in Pu-239: Solving the gamma Discrepancy in the 4-3000-s Cooling Period. Phys. Rev. Lett., 105(20), 202501–4pp.
Abstract: The beta feeding probability of Tc-102,Tc- 104,Tc- 105,Tc- 106,Tc- 107, Mo-105, and Nb-101 nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the gamma component of the decay heat for Pu-239 in the 4-3000 s range.
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Algora, A., Tain, J. L., Rubio, B., Fallot, M., & Gelletly, W. (2021). Beta-decay studies for applied and basic nuclear physics. Eur. Phys. J. A, 57(3), 85–28pp.
Abstract: In this reviewwe will present the results of recent beta-decay studies using the total absorption technique that cover topics of interest for applications, nuclear structure and astrophysics. The decays studied were selected primarily because they have a large impact on the prediction of (a) the decay heat in reactors, important for the safety of present and future reactors and (b) the reactor electron anti-neutrino spectrum, of interest for particle/nuclear physics and reactor monitoring. For these studies the total absorption technique was chosen, since it is the only method that allows one to obtain beta-decay probabilities free from a systematic error called the Pandemonium effect. The total absorption technique is based on the detection of the. cascades that follow the initial beta decay. For this reason the technique requires the use of calorimeters with very high. detection efficiency. The measurements presented and discussed here were performed mainly at the IGISOL facility of the University of Jyvaskyla (Finland) using isotopically pure beams provided by the JYFLTRAP Penning trap. Examples are presented to show that the results of our measurements on selected nuclei have had a large impact on predictions of both the decay heat and the anti-neutrino spectrum from reactors. Some of the cases involve beta-delayed neutron emission thus one can study the competition between gamma – and neutron-emission from states above the neutron separation energy. The gamma-to-neutron emission ratios can be used to constrain neutron capture (n, gamma) cross sections for unstable nuclei of interest in astrophysics. The information obtained from the measurements can also be used to test nuclear model predictions of half-lives and Pn values for decays of interest in astrophysical network calculations. These comparisons also provide insights into aspects of nuclear structure in particular regions of the nuclear chart.
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