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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Gelletly, W., Jordan, D., et al. (2018). Characterization and performance of the DTAS detector. Nucl. Instrum. Methods Phys. Res. A, 910, 79–89.
Abstract: DTAS is a segmented total absorption y-ray spectrometer developed for the DESPEC experiment at FAIR. It is composed of up to eighteen NaI(Tl) crystals. In this work we study the performance of this detector with laboratory sources and also under real experimental conditions. We present a procedure to reconstruct offline the sum of the energy deposited in all the crystals of the spectrometer, which is complicated by the effect of NaI(Tl) light-yield non-proportionality. The use of a system to correct for time variations of the gain in individual detector modules, based on a light pulse generator, is demonstrated. We describe also an event-based method to evaluate the summing-pileup electronic distortion in segmented spectrometers. All of this allows a careful characterization of the detector with Monte Carlo simulations that is needed to calculate the response function for the analysis of total absorption gamma-ray spectroscopy data. Special attention was paid to the interaction of neutrons with the spectrometer, since they are a source of contamination in studies of beta-delayed neutron emitting nuclei.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters I-137 and Rb-95. Phys. Rev. C, 100(4), 044305–17pp.
Abstract: The decays of the beta-delayed neutron emitters( 137)I and Rb-95 have been studied with the total absorption gamma-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyvaskyla allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption gamma-ray spectrometer, a segmented detector composed of 18 NaI(T1) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt gamma rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of beta intensity to states above the neutron separation energy that deexcite by gamma rays, comparable to the neutron emission probability. The competition between gamma deexcitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the beta-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Jordan, D., Monserrate, M., et al. (2020). Determination of beta-decay ground state feeding of nuclei of importance for reactor applications. Phys. Rev. C, 102(6), 064304–12pp.
Abstract: In beta-decay studies the determination of the decay probability to the ground state (g.s.) of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed gamma-ray emission. In this work we revisit the 4 pi gamma – beta method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the beta-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large g.s. branches. The method is relevant for nuclear structure studies as well. Pertinent formulas are revised and extended to the special case of beta-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain g.s. feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method.
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Guadilla, V., Algora, A., Estienne, M., Fallot, M., Gelletly, W., Porta, A., et al. (2024). First measurements with a new fl-electron detector for spectral shape studies. J. Instrum., 19(2), P02027–21pp.
Abstract: The shape of the electron spectrum emitted in /3 decay carries a wealth of information about nuclear structure and fundamental physics. In spite of that, few dedicated measurements have been made of /3 -spectrum shapes. In this work we present a newly developed detector for /3 electrons based on a telescope concept. A thick plastic scintillator is employed in coincidence with a thin silicon detector. The first measurements employing this detector have been carried out with mono -energetic electrons from the high-energy resolution electron -beam spectrometer at Bordeaux. Here we report on the good reproduction of the experimental spectra of mono -energetic electrons using Monte Carlo simulations. This is a crucial step for future experiments, where a detailed Monte Carlo characterization of the detector is needed to determine the shape of the /3 -electron spectra by deconvolution of the measured spectra with the response function of the detector. A chamber to contain two telescope assemblies has been designed for future /3 -decay experiments at the Ion Guide Isotope Separator On -Line facility in Jyvaskyla, aimed at improving our understanding of reactor antineutrino spectra.
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Guadilla, V., Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of niobium isomers. Phys. Rev. C, 100(2), 024311–15pp.
Abstract: The beta-intensity distributions of the decays of Nb-100gs,Nb-100m and Nb-102gs,Nb-102m have been determined using the total absorption gamma-ray spectroscopy technique. The JYFLTRAP double Penning trap system was employed in a campaign of challenging measurements performed with the decay total absorption gamma-ray spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. Different strategies were applied to disentangle the isomeric states involved, lying very close in energy. The low-spin component of each niobium case was populated through the decay of the zirconium parent, which was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained beta-intensity distributions for these zirconium decays. The beta-strength distributions evaluated with these results were compared with calculations in a quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of Zr-100,Zr-102. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The beta-intensities of the decay of Nb-102m, for which there were no previous data, were obtained. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported, and here we detail the significant impact on decay heat calculations.
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Guastalla, G. et al, Algora, A., & Domingo-Pardo, C. (2013). Coulomb Excitation of Sn-104 and the Strength of the Sn-100 Shell Closure. Phys. Rev. Lett., 110(17), 172501–5pp.
Abstract: A measurement of the reduced transition probability for the excitation of the ground state to the first 2(+) state in Sn-104 has been performed using relativistic Coulomb excitation at GSI. Sn-104 is the lightest isotope in the Sn chain for which this quantity has been measured. The result is a key point in the discussion of the evolution of nuclear structure in the proximity of the doubly magic nucleus Sn-100. The value B(E2; 0(+) -> 2(+)) = 0.10(4) e(2)b(2) is significantly lower than earlier results for Sn-106 and heavier isotopes. The result is well reproduced by shell model predictions and therefore indicates a robust N = Z = 50 shell closure.
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Guerrero, C., Cano-Ott, D., Mendoza, E., Tain, J. L., Algora, A., Berthoumieux, E., et al. (2012). Monte Carlo simulation of the n_TOF Total Absorption Calorimeter. Nucl. Instrum. Methods Phys. Res. A, 671, 108–117.
Abstract: The n_TOF Total Absorption Calorimeter (TAC) is a 4 pi BaF2 segmented detector used at CERN for measuring neutron capture cross-sections of importance for the design of advanced nuclear reactors. This work presents the simulation code that has been developed in GEANT4 for the accurate determination of the detection efficiency of the TAC for neutron capture events. The code allows to calculate the efficiency of the TAC for every neutron capture state, as a function of energy, crystal multiplicity, and counting rate. The code includes all instrumental effects such as the single crystal detection threshold and energy resolution, finite size of the coincidence time window, and signal pile-up. The results from the simulation have been validated with experimental data for a large set of electromagnetic de-excitation patterns: beta-decay of well known calibration sources, neutron capture reactions in light nuclei with well known level schemes like Ti-nat, reference samples used in (n,gamma) measurements like Au-197 and experimental data from an actinide sample like Pu-240. The systematic uncertainty in the determination of the detection efficiency has been estimated for all the cases. As a representative example, the accuracy reached for the case of Au-197(n,gamma) ranges between 0.5% and 2%, depending on the experimental and analysis conditions. Such a value matches the high accuracy required for the nuclear cross-section data needed in advanced reactor design.
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Guess, C. J. et al, Algora, A., Estevez, E., Molina, F., & Rubio, B. (2011). The Nd-150(He-3,t) and Sm-150(t,He-3) reactions with applications to beta beta decay of Nd-150. Phys. Rev. C, 83(6), 064318–17pp.
Abstract: The Nd-150(3He,t) reaction at 140 MeV/u and Sm-150(t,He-3) reaction at 115 MeV/u were measured, populating excited states in Pm-150. The transitions studied populate intermediate states of importance for the (neutrinoless) beta beta decay of Nd-150 to Sm-150. Monopole and dipole contributions to the measured excitation-energy spectra were extracted by using multipole decomposition analyses. The experimental results were compared with theoretical calculations obtained within the framework of the quasiparticle random-phase approximation, which is one of the main methods employed for estimating the half-life of the neutrinoless beta beta decay (0 nu beta beta) of Nd-150. The present results thus provide useful information on the neutrino responses for evaluating the 0 nu beta beta and 2 nu beta beta matrix elements. The 2 nu beta beta matrix element calculated from the Gamow-Teller transitions through the lowest 1(+) state in the intermediate nucleus is maximally about half that deduced from the half-life measured in 2 nu beta beta direct counting experiments, and at least several transitions through 1+ intermediate states in Pm-150 are required to explain the 2 nu beta beta half-life. Because Gamow-Teller transitions in the Sm-150(t,3He) experiment are strongly Pauli blocked, the extraction of Gamow-Teller strengths was complicated by the excitation of the 2 (h) over bar omega, Lambda L = 0, Delta S = 1 isovector spin-flip giant monopole resonance (IVSGMR). However, the near absence of Gamow-Teller transition strength made it possible to cleanly identify this resonance, and the strength observed is consistent with the full exhaustion of the non-energy-weighted sum rule for the IVSGMR.
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Hafner, G. et al, & Algora, A. (2021). First lifetime investigations of N > 82 iodine isotopes: The quest for collectivity. Phys. Rev. C, 104(1), 014316–18pp.
Abstract: We report on spectroscopic information and lifetime measurements in the neutron-rich I-135,I-137,I-139 isotopes. This is the first lifetime data on iodine isotopes beyond N = 82. Excited states were populated in fast neutron-induced fission of U-238 at the ALTO facility of IJCLab with the LICORNE neutron source and detected using the hybrid nu-ball spectrometer. The level schemes of the I-135,I-137,I-139 isotopes are revised in terms of excited states with up to maximum spin-parity of (33/2(+)), populated for the first time in fast neutron-induced fission. We provide first results on the lifetimes of the (9/2(1)(+)) and (13/2(1)(+)) states in I-137 and I-139, and the (17/2(1)(+)) state in 137I. In addition, we give upper lifetime limits for the (11/2(1)(+)) states in I135-139, the (15/2(1)(+)) state in I-137, the (17/2(1)(+)) state in I-139, and reexamine the (29/2(1)(+)) state in I-137. The isomeric data in I-13(5) are reinvestigated, such as the previously known (15/2(1)(+)) and (23/21) isomers with T-1/2 of 1.64(14) and 4.6(7) ns, respectively, as obtained in this work. The new spectroscopic information is compared to that from spontaneous or thermal-neutron induced fission and discussed in the context of large scale shell-model (LSSM) calculations for the region beyond Sn-132, indicating the behavior of collectivity for the three valence-proton iodine chain with N = 82, 84, 86.
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Hall, O. et al, Agramunt, J., Algora, A., Domingo-Pardo, C., Morales, A. I., Rubio, B., et al. (2021). beta-delayed neutron emission of r-process nuclei at the N=82 shell closure. Phys. Lett. B, 816, 136266–7pp.
Abstract: Theoretical models of beta-delayed neutron emission are used as crucial inputs in r-process calculations. Benchmarking the predictions of these models is a challenge due to a lack of currently available experimental data. In this work the beta-delayed neutron emission probabilities of 33 nuclides in the important mass regions south and south-west of Sn-132 are presented, 16 for the first time. The measurements were performed at RIKEN using the Advanced Implantation Detector Array (AIDA) and the BRIKEN neutron detector array. The P-1n values presented constrain the predictions of theoretical models in the region, affecting the final abundance distribution of the second r-process peak at A approximate to 130.
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