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Fujita, Y. et al, Algora, A., Estevez-Aguado, E., Molina, F., & Rubio, B. (2014). Observation of Low- and High-Energy Gamow-Teller Phonon Excitations in Nuclei. Phys. Rev. Lett., 112(11), 112502–5pp.
Abstract: Gamow-Teller (GT) transitions in atomic nuclei are sensitive to both nuclear shell structure and effective residual interactions. The nuclear GT excitations were studied for the mass number A = 42, 46, 50, and 54 “f-shell” nuclei in (He-3, t) charge-exchange reactions. In the Ca-42 -> Sc-42 reaction, most of the GT strength is concentrated in the lowest excited state at 0.6 MeV, suggesting the existence of a low-energy GT phonon excitation. As A increases, a high-energy GT phonon excitation develops in the 6-11 MeV region. In the Fe-54 -> Co-54 reaction, the high-energy GT phonon excitation mainly carries the GT strength. The existence of these two GT phonon excitations are attributed to the 2 fermionic degrees of freedom in nuclei.
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Fujita, Y. et al, Algora, A., Estevez-Aguado, E., Molina, F., & Rubio, B. (2013). High-resolution study of T-z =+2 ->+1 Gamow-Teller transitions in the Ca-44(3He,t)Sc-44 reaction. Phys. Rev. C, 88(1), 014308–18pp.
Abstract: In order to study the Gamow-Teller (GT) transitions from the T-z = +2 nucleus Ca-44 to the T-z = +1 nucleus Sc-44, where T-z is the z component of isospin T, we performed the (p, n)-type (He-3, t) charge-exchange (CE) reaction at 140 MeV/nucleon and the scattering angles 0 degrees and 2.5 degrees. An energy resolution of 28 keV, that was realized by applying matching techniques to the magnetic spectrometer system, allowed the study of fragmented states. The GT transition strengths, B(GT), were derived up to the excitation energy (E-x) of 13.7 MeV assuming the proportionality between cross sections and B(GT) values. The total sum of B(GT) values in discrete states was 3.7, which was 31% of the sum-rule-limit value of 12. Shell model calculations using the GXPF1J interaction could reproduce the gross features of the experimental B(GT) distribution, but not the fragmentation of the strength. By introducing the concepts of isospin, properties of isospin analogous transitions and states were investigated. (i) Assuming isospin symmetry, the T-z = +2 -> +1 and T-z = -2 -> -1 mirror GT transitions should have the same properties, where the latter can be studied in the beta decay of Cr-44 to V-44. First, we confirmed that the beta-decay half-life T-1/2 of Cr-44 can be reproduced using the B(GT) distribution from the Ca-44(He-3, t) measurement. Then, the 0 degrees, (3He, t) spectrum was modified to deduce the “beta-decay spectrum” and it was compared with the delayed-proton spectrum from the Cr-44 beta decay. The two spectra were mostly in agreement for the GT excitations, but suppression of the proton decay was found for the T = 2 isobaric analog state (IAS). (ii) Starting from the T = 2 ground state of 44Ca, the (3He, t) can excite GT states (state populated by GT transitions) with T = 1, 2, and 3. On the other hand, the Ca-44(p, p') reaction can excite spin-M1 states (states populated by spin-M1 transitions) with T = 2 and 3 that are analogous to the T = 2 and 3 GT states, respectively. By comparing the spectra from these two reactions, a T value of 2 is suggested for several GT states in the E-x = 11.5-13.7 MeV region. (iii) It has been suggested that the T = 2, J(pi) = 0(+) double isobaric analog state (DIAS) at 9.338 MeV in the T-z = 0 nucleus Ti-44 forms an isospin-mixed doublet with a subsidiary 0(+) state at 9.298 MeV. Since no corresponding state was found in the T-z = +1 nucleus Sc-44, we suggest T = 0 for the subsidiary state.
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Fujita, Y. et al, Algora, A., Estevez-Aguado, E., Molina, F., & Rubio, B. (2015). High-resolution study of Gamow-Teller excitations in the Ca-42(He-3,t)Sc-42 reaction and the observation of a “low-energy super-Gamow-Teller state”. Phys. Rev. C, 91(6), 064316–15pp.
Abstract: To study the Gamow-Teller (GT) transitions from the T-z = +1 nucleus Ca-42 to the T-z = 0 nucleus Sc-42, where T-z is the z component of isospin T, we performed a (p, n)-type (He-3, t) charge-exchange reaction at 140 MeV/nucleon and scattering angles around 0 degrees. With an energy resolution of 29 keV, states excited by GT transitions (GT states) could be studied accurately. The reduced GT transition strengths B(GT) were derived up to the excitation energy of 13 MeV, assuming the proportionality between the cross sections at 0 degrees and B(GT) values. The main part of the observed GT transition strength is concentrated in the lowest 0.611-MeV, J(pi) = 1(+) GT state. All the other states at higher energies are weakly excited. Shell-model calculations could reproduce the gross feature of the experimental B(GT) distribution, and random-phase-approximation calculations including an attractive isoscalar interaction showed that the 0.611-MeV state has a collective nature. It was found that this state has all of the properties of a “low-energy super-Gamow-Teller state.” It is expected that low-lying J(pi) = 1(+) GT states have T = 0 in the T-z = 0 nucleus Sc-42. However, T = 1 states are situated in a higher energy region. Assuming an isospin-analogous structure in A = 42 isobars, analogous T = 1, 1(+) states are also expected in Ca-42. Comparing the Ca-42(He-3, t)Sc-42 and Ca-42(p, p') spectra measured at 0 degrees, candidates for T = 1 GT states could be found in the 10-12-MeV region of Sc-42. They were all weakly excited. The mass dependence of the GT strength distributions in Sc isotopes is also discussed.
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Ganioglu, E. et al, Algora, A., Estevez-Aguado, E., Molina, F., & Rubio, B. (2013). High-resolution study of Gamow-Teller transitions in the Ti-47(He-3, t)V-47 reaction. Phys. Rev. C, 87(1), 014321–12pp.
Abstract: Given the importance of Gamow-Teller (GT) transitions in nuclear structure and astrophysical nuclear processes, we have studied T-z = +3/2 -> +1/2, GT transitions starting from the Ti-47 nucleus in the (He-3, t) charge-exchange reaction at 0 degrees and at an intermediate incident energy of 140 MeV/nucleon. The experiments were carried out at the Research Center for Nuclear Physics (RCNP), Osaka, using the high-resolution facility with a high-dispersion beam line and the Grand-Raiden spectrometer. With an energy resolution of 20 keV, individual GT transitions were observed and GT strength was derived for each state populated up to an excitation energy (E-x) of 12.5 MeV. The GT strength was widely distributed from low excitation energy up to 12.5 MeV, where we had to stop the analysis because of the high level density. The distribution of the GT strengths was compared with the results of shell model calculations using the GXPF1 interaction. The calculations could reproduce the experimental GT distributions well. The GT transitions from the ground state of Ti-47 and the M1 transitions from the isobaric analog state in V-47 to the same low-lying states in V-47 are analogous. It was found that the ratios of GT transition strengths to the ground state, the 0.088-MeV state, and the 0.146-MeV state are similar to the ratios of the strengths of the analogous M1 transitions from the isobaric analog state (IAS) to these states. The measured distribution of the GT strengths was also compared with those starting from the T-z = +3/2 nucleus K-41 to the T-z = +1/2 nucleus Ca-41.
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Ganioglu, E. et al, Rubio, B., Algora, A., Estevez-Aguado, E., & Molina, F. (2016). High-resolution study of Gamow-Teller transitions in the Ti-48(He-3,t)V-48 reaction. Phys. Rev. C, 93(6), 064326–10pp.
Abstract: In this work we have studied T-z = +2 -> +1, Gamow-Teller (GT) transitions in the Ti-48(He-3, t)V-48 chargeexchange reaction at 140 MeV/nucleon and 0 degrees at the Research Center for Nuclear Physics, Osaka. From the high-resolution facility, consisting of a high-dispersion beamline and the Grand Raiden spectrometer, the spectrum had an energy resolution of 21 keV, among the best achieved. Individual GT transitions were observed and GT strength was derived for each state populated up to an excitation energy of 12 MeV. The total sum of the B(GT) strength observed in discrete states was 4.0, which is 33% of the sum-rule-limit value of 12. The results were compared with the results of shell-model calculations carried out with the GXPF1J interaction. The measured B(GT) distribution was also compared with that obtained in the (He-3, t) charge-exchange reaction on Ti-47. On the assumption of isospin symmetry the beta spectrum of the T-z = -2 nucleus Fe-48 was deduced from the observed spectrum in the Ti-48(He-3, t)V-48 reaction and this predicted spectrum was compared with the measured one.
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Garcia, A. R., Martinez, T., Cano-Ott, D., Castilla, J., Guerrero, C., Marin, J., et al. (2012). MONSTER: a time of flight spectrometer for beta-delayed neutron emission measurements. J. Instrum., 7, C05012–12pp.
Abstract: The knowledge of the beta-decay properties of nuclei contributes decisively to our understanding of nuclear phenomena: the beta-delayed neutron emission of neutron rich nuclei plays an important role in the nucleosynthesis r-process and constitutes a probe for nuclear structure of very neutron rich nuclei providing information about the high energy part of the full beta strength (S-beta) function. In addition, beta-delayed neutrons are essential for the control and safety of nuclear reactors. In order to determine the neutron energy spectra and emission probabilities from neutron precursors a MOdular Neutron time-of-flight SpectromeTER (MONSTER) has been proposed for the DESPEC experiment at the future FAIR facility. The design of MONSTER and status of its construction are reported in this work.
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Garcia, A. R., Mendoza, E., Cano-Ott, D., Nolte, R., Martinez, T., Algora, A., et al. (2017). New physics model in GEANT4 for the simulation of neutron interactions with organic scintillation detectors. Nucl. Instrum. Methods Phys. Res. A, 868, 73–81.
Abstract: The accurate determination of the response function of organic scintillation neutron detectors complements their experimental characterization. Monte Carlo simulations with GEANT4 can reduce the effort and cost implied, especially for complex detection systems for which the characterization is more challenging. Previous studies have reported on the inaccuracy of GEANT4 in the calculation of the neutron response of organic scintillation detectors above 6 MeV, due to an incomplete description of the neutron-induced alpha production reactions on carbon. We have improved GEANT4 in this direction by incorporating models and data from NRESP, an excellent Monte Carlo simulation tool developed at the Physikalisch-Technische Bundesanstalt (PTB), Germany, for the specific purpose of calculating the neutron response function of organic scintillation detectors. The results have been verified against simulations with NRESP and validated against Time-Of-Flight measurements with an NE213 detector at PTB. This work has potential applications beyond organic scintillation detectors, to other types of detectors where reactions induced by fast neutrons on carbon require an accurate description.
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Gerst, R. B. et al, & Algora, A. (2020). Prompt and delayed gamma spectroscopy of neutron-rich Kr-94 and observation of a new isomer. Phys. Rev. C, 102(6), 064323–8pp.
Abstract: Prompt and delayed gamma-ray spectroscopy of the neutron-rich Kr-94 was performed, as part of the fission campaign at the ALTO facility of the IPN Orsay, using the fast-neutron-induced fission reaction U-238(n, f) in combination with the nu-Ball array, a novel hybrid gamma spectrometer for energy and lifetime measurements. Several new yrast and nonyrast transitions were observed for the first time, extending the previously known level scheme. Additionally, we report on the observation of a new short-lived isomer at 3444 keV with a half-life of 32(3) ns. The analysis of the Nilsson orbitals obtained from Gogny cranked Hartree-Fock-Bogoliubov calculations suggests a (9(-)) spin and an oblate deformation for this isomer corresponding to a two-quasineutron state, indicating an isomeric structure very similar to that of the neighboring isotones Sr-96 and Se-92.
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Gjestvang, D. et al, & Algora, A. (2023). Examination of how properties of a fissioning system impact isomeric yield ratios of the fragments. Phys. Rev. C, 108(6), 064602–12pp.
Abstract: The population of isomeric states in the prompt decay of fission fragments-so-called isomeric yield ratios (IYRs)-is known to be sensitive to the angular momentum J that the fragment emerged with, and may therefore contain valuable information on the mechanism behind the fission process. In this work, we investigate how changes in the fissioning system impact the measured IYRs of fission fragments to learn more about what parameters affect angular momentum generation. To enable this, a new technique for measuring IYRs is first demonstrated. It is based on the time of arrival of discrete gamma rays, and has the advantage that it enables the study of the IYR as a function of properties of the partner nucleus. This technique is used to extract the IYR of 134Te, strongly populated in actinide fission, from the three different fissioning systems: 232Th(n, f), 238U(n, f), at two different neutron energies, as well as 252Cf(sf). The impacts of changing the fissioning system, the compound nuclear excitation energy, the minimum J of the binary partner, and the number of neutrons emitted on the IYR of 134Te are determined. The decay code TALYS is used in combination with the fission simulation code FREYA to calculate the primary fragment angular momentum from the IYR. We find that the IYR of 134Te has a slope of 0.004 +/- 0.002 with increase in compound nucleus (CN) mass. When investigating the impact on the IYR of increased CN excitation energy, we find no change with an energy increase similar to the difference between thermal and fast fission. By varying the mass of the partner fragment emerging with 134Te, it is revealed that the IYR of 134Te is independent of the total amount of prompt neutrons emitted from the fragment pair. This indicates that neutrons carry minimal angular momentum away from the fission fragments. Comparisons with the FREYA+TALYS simulations reveal that the average angular momentum in 134Te following 238U(n, f) is 6.0 h over bar . This is not consistent with the value deduced from recent CGMF calculations. Finally, the IYR sensitivity to the angular momentum of the primary fragment is discussed. These results are not only important to help understanding the underlying mechanism in nuclear fission, but can also be used to constrain and benchmark fission models, and are relevant to the gamma -ray heating problem of reactors.
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Goigoux, T. et al, Algora, A., Guadilla, V., Montaner-Piza, A., Morales, A. I., Orrigo, S. E. A., et al. (2016). Two-Proton Radioactivity of Kr-67. Phys. Rev. Lett., 117(16), 162501–6pp.
Abstract: In an experiment with the BigRIPS separator at the RIKEN Nishina Center, we observed two-proton (2p) emission from Kr-67. At the same time, no evidence for 2p emission of Ge-59 and Se-63, two other potential candidates for this exotic radioactivity, could be observed. This observation is in line with Q value predictions which pointed to Kr-67 as being the best new candidate among the three for two-proton radioactivity. Kr-67 is only the fourth 2p ground-state emitter to be observed with a half-life of the order of a few milliseconds. The decay energy was determined to be 1690(17) keV, the 2p emission branching ratio is 37(14)%, and the half-life of Kr-67 is 7.4(30) ms.
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