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Orrigo, S. E. A., Tain, J. L., Mont-Geli, N., Tarifeño-Saldivia, A., Fraile, L. M., Grieger, M., et al. (2022). Long-term evolution of the neutron rate at the Canfranc Underground Laboratory. Eur. Phys. J. C, 82(9), 814–11pp.
Abstract: We report results on the long-term variation of the neutron counting rate at the Canfranc Underground Laboratory, of importance for several low-background experiments installed there, including rare-event searches. The measurement campaign was performed employing the High Efficiency Neutron Spectrometry Array (HENSA) mounted in Hall A and lasted 412 live days. The present study is the first long-term measurement of the neutron rate with sensitivity over a wide range of neutron energies (from thermal up to 0.1 GeV and beyond) performed in any underground laboratory so far. Data on the environmental variables inside the experimental hall (radon concentration, air temperature, air pressure and humidity) were also acquired during all the measurement campaign. We have investigated for the first time the evolution of the neutron rate for different energies of the neutrons and its correlation with the ambient variables.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2022). Total absorption gamma-ray spectroscopy of the ss decays of Y-96gs,Y-m. Phys. Rev. C, 106(1), 014306–14pp.
Abstract: The ss decays of the ground state (gs) and isomeric state (m) of Y-96 have been studied with the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8(+) isomeric state from the 0(-) ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The ss-intensity distributions of both decays have been independently determined. In the analyses the deexcitation of the 1581.6 keV level in Zr-96, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the ss-detector efficiency, influencing the ss-intensity distribution obtained. Our results for Y-96gs (0(-)) confirm the large ground state to ground state ss-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to 96.6(-2.1)(+0.3) % of the total ss intensity. Given that the decay of Y-96gs is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of Y-96m (8(+)), previously undetected ss intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption gamma-ray spectroscopy measurements of ss decays with highly fragmented deexcitation patterns. Y-96m (8(+)) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average ss and gamma energies differ significantly from the previous values in evaluated databases. The discrepancy is far above the previously quoted uncertainties. Finally, we also report on the successful implementation of an innovative total absorption gamma-ray spectroscopy analysis of the module-multiplicity gated spectra, as a first proof of principle to distinguish between decaying states with very different spin-parity values.
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Algora, A., Ganioglu, E., Sarriguren, P., Guadilla, V., Fraile, L. M., Nacher, E., et al. (2021). Total absorption gamma-ray spectroscopy study of the beta-decay of Hg-186. Phys. Lett. B, 819, 136438–7pp.
Abstract: The Gamow-Teller strength distribution of the decay of Hg-186 into Au-186 has been determined for the first time using the total absorption gamma spectroscopy technique and has been compared with theoretical QRPA calculations using the SLy4 Skyrme force. The measured Gamow-Teller strength distribution and the half-life are described by mixing oblate and prolate configurations independently in the parent and daughter nuclei. In this theoretical framework the best description of the experimental beta strength is obtained with dominantly prolate components for both parent Hg-186 and daughter Au-186. The approach also allowed us to determine an upper limit of the oblate component in the parent state. The complexity of the analysis required the development of a new approach in the analysis of the X-ray gated total absorption spectrum.
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Orrigo, S. E. A. et al, Rubio, B., Gelletly, W., Aguilera, P., Algora, A., Morales, A. I., et al. (2021). beta decay of the very neutron-deficient Ge-60 and Ge-62 nuclei. Phys. Rev. C, 103(1), 014324–12pp.
Abstract: We report here the results of a study of the beta decay of the proton-rich Ge isotopes, Ge-60 and Ge-62, produced in an experiment at the RIKEN Nishina Center. We have improved our knowledge of the half-lives of Ge-62 [73.5(1) ms] and Ge-60 [25.0(3) ms] and its daughter nucleus, Ga-60 [69.4(2) ms]. We measured individual beta-delayed proton and gamma emissions and their related branching ratios. Decay schemes and absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. A total beta-delayed proton-emission branching ratio of 67(3)% has been obtained for Ge-60. New information has been obtained on the energy levels populated in Ga-60 and on the 1/2(-) excited state in the beta p daughter Zn-59. We extracted a ground state-to-ground state feeding of 85.3(3)% for the decay of Ge-62. Eight new y lines have been added to the deexcitation of levels populated in the Ga-62 daughter.
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Grieger, M., Hensel, T., Agramunt, J., Bemmerer, D., Degering, D., Dillmann, I., et al. (2020). Neutron flux and spectrum in the Dresden Felsenkeller underground facility studied by moderated He-3 counters. Phys. Rev. D, 101(12), 123027–15pp.
Abstract: Ambient neutrons may cause significant background for underground experiments. Therefore, it is necessary to investigate their flux and energy spectrum in order to devise a proper shielding. Here, two sets of altogether ten moderated He-3 neutron counters are used for a detailed study of the ambient neutron background in tunnel IV of the Felsenkeller facility, underground below 45 m of rock in Dresden/Germany. One of the moderators is lined with lead and thus sensitive to neutrons of energies higher than 10 MeV. For each He-3 counter moderator assembly, the energy-dependent neutron sensitivity was calculated with the FLUKA code. The count rates of the ten detectors were then fitted with the MAXED and GRAVEL packages. As a result, both the neutron energy spectrum from 10(-9) to 300 MeV and the flux integrated over the same energy range were determined experimentally. The data show that at a given depth, both the flux and the spectrum vary significantly depending on local conditions. Energy-integrated fluxes of (0.61 +/- 0.05), (1.96 +/- 0.15), and (4.6 +/- 0.4) x 10(-4) cm(-2) s(-1), respectively, are measured for three sites within Felsenkeller tunnel IV which have similar muon flux but different shielding wall configurations. The integrated neutron flux data and the obtained spectra for the three sites are matched reasonably well by FLUKA Monte Carlo calculations that are based on the known muon flux and composition of the measurement room walls.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Jordan, D., Monserrate, M., et al. (2020). Determination of beta-decay ground state feeding of nuclei of importance for reactor applications. Phys. Rev. C, 102(6), 064304–12pp.
Abstract: In beta-decay studies the determination of the decay probability to the ground state (g.s.) of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed gamma-ray emission. In this work we revisit the 4 pi gamma – beta method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the beta-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large g.s. branches. The method is relevant for nuclear structure studies as well. Pertinent formulas are revised and extended to the special case of beta-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain g.s. feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method.
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Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters I-137 and Rb-95. Phys. Rev. C, 100(4), 044305–17pp.
Abstract: The decays of the beta-delayed neutron emitters( 137)I and Rb-95 have been studied with the total absorption gamma-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyvaskyla allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption gamma-ray spectrometer, a segmented detector composed of 18 NaI(T1) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt gamma rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of beta intensity to states above the neutron separation energy that deexcite by gamma rays, comparable to the neutron emission probability. The competition between gamma deexcitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the beta-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers.
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Guadilla, V., Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of niobium isomers. Phys. Rev. C, 100(2), 024311–15pp.
Abstract: The beta-intensity distributions of the decays of Nb-100gs,Nb-100m and Nb-102gs,Nb-102m have been determined using the total absorption gamma-ray spectroscopy technique. The JYFLTRAP double Penning trap system was employed in a campaign of challenging measurements performed with the decay total absorption gamma-ray spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. Different strategies were applied to disentangle the isomeric states involved, lying very close in energy. The low-spin component of each niobium case was populated through the decay of the zirconium parent, which was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained beta-intensity distributions for these zirconium decays. The beta-strength distributions evaluated with these results were compared with calculations in a quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of Zr-100,Zr-102. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The beta-intensities of the decay of Nb-102m, for which there were no previous data, were obtained. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported, and here we detail the significant impact on decay heat calculations.
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Yokoyama, R., Singh, M., Grzywacz, R., Keeler, A., King, T. T., Agramunt, J., et al. (2019). Segmented YSO scintillation detectors as a new beta-implant detection tool for decay spectroscopy in fragmentation facilities. Nucl. Instrum. Methods Phys. Res. A, 937, 93–97.
Abstract: A newly developed segmented YSO scintillator detector was implemented for the first time at the RI-beam Factory at RIKEN Nishina Center as an implantation-decay counter. The results from the experiment demonstrate that the detector is a viable alternative to conventional silicon-strip detectors with its good timing resolution and high detection efficiency for beta particles. A Position-Sensitive Photo-Multiplier Tube (PSPMT) is coupled with a 48 x 48 segmented YSO crystal. To demonstrate its capabilities, a known short-lived isomer in Ni-76 and the beta decay of Co-74 were measured by implanting those ions into the YSO detector. The half-lives and gamma-rays observed in this work are consistent with the known values. The beta-ray detection efficiency is more than 80 % for the decay of Co-74.
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BRIKEN Collaboration(Tolosa-Delgado, A. et al), Agramunt, J., Tain, J. L., Algora, A., Domingo-Pardo, C., Morales, A. I., et al. (2019). Commissioning of the BRIKEN detector for the measurement of very exotic beta-delayed neutron emitters. Nucl. Instrum. Methods Phys. Res. A, 925, 133–147.
Abstract: A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.
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