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Author |
n_TOF Collaboration (Paradela, C. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron-induced fission cross section of U-234 and Np-237 measured at the CERN Neutron Time-of-Flight (n_TOF) facility |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
82 |
Issue |
3 |
Pages |
034601 - 11pp |
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Keywords |
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Abstract |
A high-resolution measurement of the neutron-induced fission cross section of U-234 and Np-237 has been performed at the CERN Neutron Time-of-Flight facility. The cross sections have been determined in a wide energy range from 1 eV to 1 GeV using the evaluated U-235 cross section as reference. In these measurements the energy determination for the U-234 resonances could be improved, whereas previous discrepancies for the Np-237 resonances were confirmed. New cross-section data are provided for high neutron energies that go beyond the limits of prior evaluations, obtaining important differences in the case of Np-237. |
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Address |
[Paradela, C.; Duran, I.; Tarrio, D.; Alvarez, H.] Univ Santiago de Compostela, Santiago De Compostela, Spain, Email: carlos.paradela@usc.es |
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Amer Physical Soc |
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English |
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ISSN |
0556-2813 |
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Expedition |
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Conference |
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Notes |
ISI:000281651400002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number  |
IFIC @ elepoucu @ |
Serial |
382 |
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Author |
Algora, A. et al; Jordan, D.; Tain, J.L.; Rubio, B.; Agramunt, J.; Perez-Cerdan, A.B.; Molina, F.; Caballero, L.; Nacher, E. |
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Title |
Reactor Decay Heat in Pu-239: Solving the gamma Discrepancy in the 4-3000-s Cooling Period |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
105 |
Issue |
20 |
Pages |
202501 - 4pp |
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Abstract |
The beta feeding probability of Tc-102,Tc- 104,Tc- 105,Tc- 106,Tc- 107, Mo-105, and Nb-101 nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the gamma component of the decay heat for Pu-239 in the 4-3000 s range. |
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Address |
[Algora, A.; Jordan, D.; Tain, J. L.; Rubio, B.; Agramunt, J.; Perez-Cerdan, A. B.; Molina, F.; Caballero, L.; Nacher, E.] Univ Valencia, IFIC, CSIC, Valencia, Spain, Email: algora@ific.uv.es |
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Amer Physical Soc |
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English |
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Abbreviated Series Title |
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Series Issue |
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Edition |
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ISSN |
0031-9007 |
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Conference |
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Notes |
ISI:000283927700004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
328 |
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Author |
n_TOF Collaboration (Mosconi, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron physics of the Re/Os clock. I. Measurement of the (n, gamma) cross sections of Os-186,Os-187,Os-188 at the CERN n_TOF facility |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
82 |
Issue |
1 |
Pages |
015802 - 10pp |
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Keywords |
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Abstract |
The precise determination of the neutron capture cross sections of Os-186 and Os-187 is important to define the s-process abundance of Os-187 at the formation of the solar system. This quantity can be used to evaluate the radiogenic component of the abundance of Os-187 due to the decay of the unstable Re-187 (t(1/2) = 41.2 Gyr) and from this to infer the time duration of the nucleosynthesis in our galaxy (Re/Os cosmochronometer). The neutron capture cross sections of Os-186, Os-187, and Os-188 have been measured at the CERN n_TOF facility from 1 eV to 1 MeV, covering the entire energy range of astrophysical interest. The measurement has been performed by time-of-flight technique using isotopically enriched samples and two C6D6 scintillation detectors for recording the prompt. rays emitted in the capture events. Maxwellian averaged capture cross sections have been determined for thermal energies between kT = 5 and 100 keV corresponding to all possible s-process scenarios. The estimated uncertainties for the values at 30 keV are 4.1, 3.3, and 4.7% for Os-186, Os-187, and Os-188, respectively. |
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Address |
[Mosconi, M.; Domingo-Pardo, C.; Kaeppeler, F.; Audouin, L.; Bisterzo, S.; Dillmann, I.; Heil, M.; Plag, R.; Voss, F.; Walter, S.; Wisshak, K.] KIT, Inst Kernphys, D-76021 Karlsruhe, Germany, Email: Marita.Mosconi@ptb.de |
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Amer Physical Soc |
Place of Publication |
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English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000279940200007 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
409 |
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Author |
n_TOF Collaboration (Fujii, K. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron physics of the Re/Os clock. III. Resonance analyses and stellar (n, gamma) cross sections of Os-186,Os-187,Os-188 |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
82 |
Issue |
1 |
Pages |
015804 - 18pp |
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Keywords |
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Abstract |
Neutron resonance analyses have been performed for the capture cross sections of Os-186, Os-187, and Os-188 measured at the n_TOF facility at CERN. Resonance parameters have been extracted up to 5, 3, and 8 keV, respectively, using the SAMMY code for a full R-matrix fit of the capture yields. From these results average resonance parameters were derived by a statistical analysis to provide a comprehensive experimental basis for modeling of the stellar neutron capture rates of these isotopes in terms of the Hauser-Feshbach statistical model. Consistent calculations for the capture and inelastic reaction channels are crucial for the evaluation of stellar enhancement factors to correct the Maxwellian averaged cross sections obtained from experimental data for the effect of thermally populated excited states. These factors have been calculated for the full temperature range of current scenarios of s-process nucleosynthesis using the combined information of the experimental data in the region of resolved resonances and in the continuum. The consequences of this analysis for the s-process component of the Os-187 abundance and the related impact on the evaluation of the time duration of galactic nucleosynthesis via the Re/Os cosmochronometer are discussed. |
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Address |
[Fujii, K.; Abbondanno, U.; Belloni, F.; Milazzo, P. M.; Moreau, C.] Ist Nazl Fis Nucl, I-34149 Trieste, Italy, Email: Kaori.Fujii@ts.infn.it |
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Corporate Author |
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Publisher |
Amer Physical Soc |
Place of Publication |
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English |
Summary Language |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000279940200009 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
410 |
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Author |
Rodriguez, D. et al; Algora, A.; Rubio, B.; Tain, J.L. |
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Title |
MATS and LaSpec: High-precision experiments using ion traps and lasers at FAIR |
Type |
Journal Article |
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Year |
2010 |
Publication |
European Physical Journal-Special Topics |
Abbreviated Journal |
Eur. Phys. J.-Spec. Top. |
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Volume |
183 |
Issue |
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Pages |
1-123 |
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Keywords |
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Abstract |
Nuclear ground state properties including mass, charge radii, spins and moments can be determined by applying atomic physics techniques such as Penning-trap based mass spectrometry and laser spectroscopy. The MATS and LaSpec setups at the low-energy beamline at FAIR will allow us to extend the knowledge of these properties further into the region far from stability. The mass and its inherent connection with the nuclear binding energy is a fundamental property of a nuclide, a unique “fingerprint”. Thus, precise mass values are important for a variety of applications, ranging from nuclear-structure studies like the investigation of shell closures and the onset of deformation, tests of nuclear mass models and mass formulas, to tests of the weak interaction and of the Standard Model. The required relative accuracy ranges from 10(-5) to below 10(-8) for radionuclides, which most often have half-lives well below 1 s. Substantial progress in Penning trap mass spectrometry has made this method a prime choice for precision measurements on rare isotopes. The technique has the potential to provide high accuracy and sensitivity even for very short-lived nuclides. Furthermore, ion traps can be used for precision decay studies and offer advantages over existing methods. With MATS (Precision Measurements of very short-lived nuclei using an Advanced Trapping System for highly-charged ions) at FAIR we aim to apply several techniques to very short-lived radionuclides: High-accuracy mass measurements, in-trap conversion electron and alpha spectroscopy, and trap-assisted spectroscopy. The experimental setup of MATS is a unique combination of an electron beam ion trap for charge breeding, ion traps for beam preparation, and a high-precision Penning trap system for mass measurements and decay studies. For the mass measurements, MATS offers both a high accuracy and a high sensitivity. A relative mass uncertainty of 10(-9) can be reached by employing highly-charged ions and a non-destructive Fourier-Transform Ion-Cyclotron-Resonance (FT-ICR) detection technique on single stored ions. This accuracy limit is important for fundamental interaction tests, but also allows for the study of the fine structure of the nuclear mass surface with unprecedented accuracy, whenever required. The use of the FT-ICR technique provides true single ion sensitivity. This is essential to access isotopes that are produced with minimum rates which are very often the most interesting ones. Instead of pushing for highest accuracy, the high charge state of the ions can also be used to reduce the storage time of the ions, hence making measurements on even shorter-lived isotopes possible. Decay studies in ion traps will become possible with MATS. Novel spectroscopic tools for in-trap high-resolution conversion-electron and charged-particle spectroscopy from carrier-free sources will be developed, aiming e. g. at the measurements of quadrupole moments and E0 strengths. With the possibility of both high-accuracy mass measurements of the shortest-lived isotopes and decay studies, the high sensitivity and accuracy potential of MATS is ideally suited for the study of very exotic nuclides that will only be produced at the FAIR facility. Laser spectroscopy of radioactive isotopes and isomers is an efficient and model-independent approach for the determination of nuclear ground and isomeric state properties. Hyperfine structures and isotope shifts in electronic transitions exhibit readily accessible information on the nuclear spin, magnetic dipole and electric quadrupole moments as well as root-mean-square charge radii. The dependencies of the hyperfine splitting and isotope shift on the nuclear moments and mean square nuclear charge radii are well known and the theoretical framework for the extraction of nuclear parameters is well established. These extracted parameters provide fundamental information on the structure of nuclei at the limits of stability. Vital information on both bulk and valence nuclear properties are derived and an exceptional sensitivity to changes in nuclear deformation is achieved. Laser spectroscopy provides the only mechanism for such studies in exotic systems and uniquely facilitates these studies in a model-independent manner. The accuracy of laser-spectroscopic-determined nuclear properties is very high. Requirements concerning production rates are moderate; collinear spectroscopy has been performed with production rates as few as 100 ions per second and laser-desorption resonance ionization mass spectroscopy (combined with beta-delayed neutron detection) has been achieved with rates of only a few atoms per second. This Technical Design Report describes a new Penning trap mass spectrometry setup as well as a number of complementary experimental devices for laser spectroscopy, which will provide a complete system with respect to the physics and isotopes that can be studied. Since MATS and LaSpec require high-quality low-energy beams, the two collaborations have a common beamline to stop the radioactive beam of in-flight produced isotopes and prepare them in a suitable way for transfer to the MATS and LaSpec setups, respectively. |
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Address |
[Rodriguez, D.; Lallena, A. M.] Univ Granada, Dept Fis Atom Mol & Nucl, E-18071 Granada, Spain, Email: danielrodriguez@ugr.es |
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Corporate Author |
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Thesis |
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Publisher |
Springer Heidelberg |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1951-6355 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000280061400001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
412 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Tagliente, G. et al.); Domingo-Pardo, C.; Tain, J.L. |
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Title |
The Zr-92(n,gamma) reaction and its implications for stellar nucleosynthesis |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
81 |
Issue |
5 |
Pages |
055801 - 9pp |
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Keywords |
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Abstract |
Because the relatively small neutron capture cross sections of the zirconium isotopes are difficult to measure, the results of previous measurements are often not adequate for a number of problems in astrophysics and nuclear technology. Therefore, the Zr-92(n,gamma) cross section has been remeasured at the CERN n_TOF facility, providing a set of improved parameters for 44 resonances in the neutron energy range up to 40 keV. With this information the cross-section uncertainties in the keV region could be reduced to 5% as required for s-process nucleosynthesis studies and technological applications. |
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Address |
[Tagliente, G.; Colonna, N.; Marrone, S.; Terlizzi, R.] Ist Nazl Fis Nucl, I-70126 Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000278144800074 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
444 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Massimi, C. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Au-197(n,gamma) cross section in the resonance region |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
81 |
Issue |
4 |
Pages |
044616 - 22pp |
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Keywords |
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Abstract |
The (n,gamma) cross section of Au-197 has been measured at nTOF in the resolved resonance region, up to 5 keV, with the aim of improving the accuracy in an energy range where it is not yet considered standard. The measurements were performed with two different experimental setup and detection techniques, the total energy method based on C6D6 detectors, and the total absorption calorimetry based on a 4 pi BaF2 array. By comparing the data collected with the two techniques, two accurate sets of neutron-capture yields have been obtained, which could be the basis for a new evaluation leading to an extended cross-section standard. Overall good agreement is found between the n_TOF results and evaluated cross sections, with some significant exceptions for small resonances. A few resonances not included in the existing databases have also been observed. |
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Address |
[Domingo-Pardo, C.] GSI Helmholtzzentrum Schwerionenforsch GmbH, Darmstadt, Germany, Email: c.domingopardo@gsi.de |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000277209500051 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
463 |
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| Permanent link to this record |
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Author |
Algora, A. et al; Jordan, D.; Tain, J.L.; Rubio, B.; Agramunt, J.; Perez-Cerdan, A.B.; Molina, F.; Caballero, L.; Nacher, E. |
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Title |
Improvements on Decay Heat Summation Calculations by Means of Total Absorption Gamma-ray Spectroscopy Measurements |
Type |
Journal Article |
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Year |
2011 |
Publication |
Journal of the Korean Physical Society |
Abbreviated Journal |
J. Korean Phys. Soc. |
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Volume |
59 |
Issue |
2 |
Pages |
1479-1482 |
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Keywords |
Decay heat; Total absorption; Trap-assisted spectroscopy |
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Abstract |
The decay heat of fission products plays an important role in predictions of the heat released by nuclear fuel in reactors. In this contribution we present results of the analysis of the measurement of the beta decay of some refractory isotopes that were considered possible important contributors to the decay heat in reactors. The measurements presented here were performed at the IGISOL facility of the University of Jyvaskyla, Finland. In our measurements we have combined for the first time a Penning trap (JYFLTRAP), which was used as a high resolution isobaric separator, with a total absorption spectrometer. The results of the measurements as well as their consequences for decay heat summation calculations are discussed. |
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Address |
[Algora, A; Jordan, D; Tain, JL; Rubio, B; Agramunt, J; Caballero, L; Nacher, E; Perez-Cerdan, AB; Molina, F] Univ Valencia, CSIC, IFIC, Valencia, Spain, Email: algora@ific.uv.es |
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Corporate Author |
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Thesis |
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Publisher |
Korean Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0374-4884 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000294080700005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
729 |
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| Permanent link to this record |
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Author |
Tain, J.L. et al; Algora, A.; Estevez, E.; Rubio, B.; Valencia, E.; Jordan, D. |
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Title |
Beta Decay Studies of Neutron Rich Nuclei Using Total Absorption Gamma-ray Spectroscopy and Delayed Neutron Measurements |
Type |
Journal Article |
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Year |
2011 |
Publication |
Journal of the Korean Physical Society |
Abbreviated Journal |
J. Korean Phys. Soc. |
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Volume |
59 |
Issue |
2 |
Pages |
1499-1502 |
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Keywords |
Beta decay; Delayed neutron emission; Total absorption gamma-ray spectroscopy; Neutron detectors; Nuclear technology; Nuclear astrophysics |
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Abstract |
A complete characterisation of the beta-decay of neutron-rich nuclei can be obtained from the measurement of beta-delayed gamma rays and, whenever the process is energetically possible, beta-delayed neutrons. The accurate determination of the beta-intensity distribution and the beta-delayed neutron emission probability is of great relevance in the fields of reactor technology and nuclear astrophysics. A programme for combined measurements using the total absorption gamma-ray spectroscopy technique and both neutron counters and neutron time-of-flight spectrometers is presented. |
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Address |
[Tain, JL; Algora, A; Estevez, E; Rubio, B; Valencia, E; Jordan, D] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia 46071, Spain, Email: tain@ific.uv.es |
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Corporate Author |
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Thesis |
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Publisher |
Korean Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0374-4884 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000294080700010 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
730 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Guerrero, C. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Study of Photon Strength Function of Actinides: the Case of (235)U, (238)Np and (241)Pu |
Type |
Journal Article |
| |
Year |
2011 |
Publication |
Journal of the Korean Physical Society |
Abbreviated Journal |
J. Korean Phys. Soc. |
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Volume |
59 |
Issue |
2 |
Pages |
1510-1513 |
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Keywords |
Photon/Gamma strength functions; Pygmy; Scissor mode; n_TOF; Total absorption calorimeter; TAC; Neutron capture |
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Abstract |
The decay from excited levels in medium and heavy nuclei can be described in a statistical approach by means of Photon Strength Functions and Level Density distributions. The study of electromagnetic cascades following neutron capture based on the use of high efficiency detectors has been shown to be well suited for probing the properties of the Photon Strength Function of heavy (high level density) and/or radioactive (high background) nuclei. In this work we have investigated for the first time the validity of the recommended PSF of actinides, in particular (235)U, (238)Np and (241)Pu. Our study includes the search for resonance structures in the PSF below S(n) and draws conclusions regarding their existence and their characteristics in terms of energy, width and electromagnetic nature. |
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Address |
[Guerrero, C; Alvarez-Velarde, F; Ano-Ott, DC; Martinez, T; Mendoza, E; Villamarin, D] Ctr Invest Energet Medioambientales & Technol CIE, Madrid, Spain, Email: carlos.guerrero@ciemat.es |
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Korean Physical Soc |
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English |
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0374-4884 |
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WOS:000294080700013 |
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no |
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yes |
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yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
731 |
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