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Author  |
n_TOF Collaboration (Amaducci, S. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Measurement of the U-235(n, f) cross section relative to the Li-6(n, t) and B-10(n,alpha) standards from thermal to 170 keV neutron energy range at n_TOF |
Type |
Journal Article |
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Year |
2019 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
55 |
Issue |
7 |
Pages |
120 - 19pp |
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Keywords |
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Abstract |
.The U-235(n, f ) cross section was measured at n_TOF relative to Li-6(n, t) and B-10(n,alpha) , with high resolution ( L=183.49(2) m) and in a wide energy range (25meV-170keV) with 1.5% systematic uncertainty, making use of a stack of six samples and six silicon detectors placed in the neutron beam. This allowed us to make a direct comparison of the yields of the U-235(n, f ) and of the two reference reactions under the same experimental conditions, and taking into account the forward/backward emission asymmetry. A hint of an anomaly in the 10-30keV neutron energy range had been previously observed in other experiments, indicating a cross section systematically lower by several percent relative to major evaluations. The present results indicate that the cross section in the 9-18keV neutron energy range is indeed overestimated by almost 5% in the recently released evaluated data files ENDF/B-VIII.0 and JEFF3.3, as a consequence of a 7% overestimate in a single GMA node in the IAEA reference file. Furthermore, these new high-resolution data confirm the existence of resonance-like structures in the keV neutron energy region. The results here reported may lead to a reduction of the uncertainty in the 1-100keV neutron energy region. Finally, from the present data, a value of 249.7 +/- 1.4( stat )+/- 0.94( syst ) b<bold>eV has been extracted for the cross section integral between </bold>7.8 and 11eV, confirming the value of 247.5 +/- 3 b<bold>eV recently established as a standard</bold>. |
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Address |
[Amaducci, S.; Cosentino, L.; Finocchiaro, P.; Musumarra, A.] INFN, Lab Nazl Sud, Catania, Italy, Email: finocchiaro@lns.infn.it |
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Springer |
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English |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Expedition |
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Conference |
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Notes |
WOS:000477050900001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4083 |
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Author |
n_TOF Collaboration (Bacak, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
A compact fission detector for fission-tagging neutron capture experiments with radioactive fissile isotopes |
Type |
Journal Article |
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Year |
2020 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
969 |
Issue |
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Pages |
163981 - 10pp |
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Keywords |
Fission detector; U-233; n_TOF; Time-of-flight |
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Abstract |
In the measurement of neutron capture cross-sections of fissile isotopes, the fission channel is a source of background which can be removed efficiently using the so-called fission-tagging or fission-veto technique. For this purpose a new compact and fast fission chamber has been developed. The design criteria and technical description of the chamber are given within the context of a measurement of the U-233(n, gamma) cross-section at the nTOF facility at CERN, where it was coupled to the nTOF Total Absorption Calorimeter. For this measurement the fission detector was optimized for time resolution, minimization of material in the neutron beam and for alpha-fission discrimination. The performance of the fission chamber and its application as a fission tagging detector are discussed. |
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Address |
[Bacak, M.; Gunsing, F.; Vlachoudis, V.; Aberle, O.; Calviani, M.; Cardella, R.; Cerutti, F.; Chiaveri, E.; Ferrari, A.; Gilardoni, S.; Kadi, Y.; Macina, D.; Masi, A.; Mingrone, F.; Rubbia, C.; Sabate-Gilarte, M.; Zugec, P.] CERN, European Org Nucl Res, Geneva, Switzerland, Email: michael.bacak@cern.ch |
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Elsevier |
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English |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0168-9002 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000536792400015 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4413 |
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Author |
n_TOF Collaboration (Balibrea-Correa, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement of the alpha ratio and (n, gamma) cross section of U-235 from 0.2 to 200 eV at n_TOF |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
4 |
Pages |
044615 - 18pp |
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Keywords |
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Abstract |
We measured the neutron capture-to-fission cross-section ratio (alpha ratio) and the capture cross section of U-235 between 0.2 and 200 eV at the nTOF facility at CERN. The simultaneous measurement of neutron-induced capture and fission rates was performed by means of the nTOF BaF2 Total Absorption Calorimeter (TAC), used for detection of gamma rays, in combination with a set of micromegas detectors used as fission tagging detectors. The energy dependence of the capture cross section was obtained with help of the Li-6(n, t) standard reaction determining the n_TOF neutron fluence; the well-known integral of the U-235(n, f) cross section between 7.8 and 11 eV was then used for its absolute normalization. The alpha ratio, obtained with slightly higher statistical fluctuations, was determined directly, without need for any reference cross section. To perform the analysis of this measurement we developed a new methodology to correct the experimentally observed effect that the probabilities of detecting a fission reaction in the TAC and the micromegas detectors are not independent. The results of this work have been used in a new evaluation of U-235 performed within the scope of the Collaborative International Evaluated Library Organisation (CIELO) Project, and are consistent with the ENDF/B-VIII.0 and JEFF-3.3 capture cross sections below 4 eV and above 100 eV. However, the measured capture cross section is on average 10% larger between 4 and 100 eV. |
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Address |
[Balibrea-Correa, J.; Mendoza, E.; Cano-Ott, D.] Ctr Invest Energet Medioambientales & Tecnol, CIEMAT, Madrid, Spain, Email: emilio.mendoza@ciemat.es |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Language |
English |
Summary Language |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0556-2813 |
ISBN |
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Conference |
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Notes |
WOS:000579839000003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4575 |
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Author |
n_TOF Collaboration (Barbagallo, M. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
High-accuracy determination of the neutron flux at n_TOF |
Type |
Journal Article |
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Year |
2013 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
49 |
Issue |
12 |
Pages |
156 - 11pp |
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Keywords |
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Abstract |
The neutron flux of the nTOF facility at CERN was measured, after installation of the new spallation target, with four different systems based on three neutron-converting reactions, which represent accepted cross sections standards in different energy regions. A careful comparison and combination of the different measurements allowed us to reach an unprecedented accuracy on the energy dependence of the neutron flux in the very wide range (thermal to 1 GeV) that characterizes the nTOF neutron beam. This is a pre-requisite for the high accuracy of cross section measurements at n_TOF. An unexpected anomaly in the neutron-induced fission cross section of U-235 is observed in the energy region between 10 and 30keV, hinting at a possible overestimation of this important cross section, well above currently assigned uncertainties. |
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Address |
[Barbagallo, M.; Colonna, N.; Mastromarco, M.; Meaze, M.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, I-70125 Bari, Italy, Email: massimo.barbagallo@ba.infn.it |
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Corporate Author |
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Publisher |
Springer |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000328351000001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1663 |
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Author |
n_TOF Collaboration (Barbagallo, M. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Experimental setup and procedure for the measurement of the Be-7(n,p)Li-7 reaction at n_TOF |
Type |
Journal Article |
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Year |
2018 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
887 |
Issue |
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Pages |
27-33 |
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Keywords |
Cosmological Lithium problem; Big bang nucleosynthesis; Be-7(n,p)Li-7 reaction; n_TOF spallation neutron source |
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Abstract |
Following the completion of the second neutron beam line and the related experimental area (EAR2) at the n_TOF spallation neutron source at CERN, several experiments were planned and performed. The high instantaneous neutron flux available in EAR2 allows to investigate neutron induced reactions with charged particles in the exit channel even employing targets made out of small amounts of short-lived radioactive isotopes. After the successful measurement of the Be-7(n,alpha)alpha cross section, the Be-7(n,p)Li-7 reaction was studied in order to provide still missing cross section data of relevance for Big Bang Nucleosynthesis (BBN), in an attempt to find a solution to the cosmological Lithium abundance problem. This paper describes the experimental setup employed in such a measurement and its characterization. |
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Address |
[Barbagallo, M.; Mastromarco, M.; Damone, L. A.; Mazzone, A.; Colonna, N.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: finocchiaro@lns.infn.ir |
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Corporate Author |
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Publisher |
Elsevier Science Bv |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0168-9002 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000427814400005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3528 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Barbagallo, M. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Be-7(n,alpha)He-4 Reaction and the Cosmological Lithium Problem: Measurement of the Cross Section in a Wide Energy Range at n_TOF at CERN |
Type |
Journal Article |
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Year |
2016 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
117 |
Issue |
15 |
Pages |
152701 - 7pp |
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Keywords |
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Abstract |
The energy-dependent cross section of the (7)Bed(n,alpha)He-4 reaction, of interest for the so-called cosmological lithium problem in big bang nucleosynthesis, has been measured for the first time from 10 meV to 10 keV neutron energy. The challenges posed by the short half-life of Be-7 and by the low reaction cross section have been overcome at nTOF thanks to an unprecedented combination of the extremely high luminosity and good resolution of the neutron beam in the new experimental area (EAR2) of the nTOF facility at CERN, the availability of a sufficient amount of chemically pure Be-7, and a specifically designed experimental setup. Coincidences between the two alpha particles have been recorded in two Si-Be-7-Si arrays placed directly in the neutron beam. The present results are consistent, at thermal neutron energy, with the only previous measurement performed in the 1960s at a nuclear reactor. The energy dependence reported here clearly indicates the inadequacy of the cross section estimates currently used in BBN calculations. Although new measurements at higher neutron energy may still be needed, the n_TOF results hint at a minor role of this reaction in BBN, leaving the long-standing cosmological lithium problem unsolved. |
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Address |
[Barbagallo, M.; Colonna, N.; Damone, L.; Mastromarco, M.; Mazzone, A.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: nicola.colonna@ba.infn.it |
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Corporate Author |
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Thesis |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0031-9007 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000384479300003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2822 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Belloni, F. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Measurement of the neutron-induced fission cross-section of Am-241 at the time-of-flight facility n_TOF |
Type |
Journal Article |
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Year |
2013 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
49 |
Issue |
1 |
Pages |
2 - 6pp |
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Keywords |
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Abstract |
The neutron-induced fission cross-section of Am-241 has been measured relative to the standard fission cross-section of U-235 between 0.5 and 20 MeV. The experiment was performed at the CERN nTOF facility. Fission fragments were detected by a fast ionization chamber by discriminating against the alpha-particles from the high radioactivity of the samples. The high instantaneous neutron flux and the low background of the nTOF facility enabled us to obtain uncertainties of approximate to 5%. With the present results it was possible to resolve discrepancies between previous data sets and to confirm current evaluations, thus providing important information for design studies of future reactors with improved fuel burn-up. |
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Address |
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Corporate Author |
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Thesis |
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Publisher |
Springer |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000315048100002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1399 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Belloni, F. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron-induced fission cross section measurement of U-233, Am-241 and Am-243 in the energy range 0.5 MeV <= E-n <= 20 MeV at n_TOF at CERN |
Type |
Journal Article |
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Year |
2012 |
Publication |
Physica Scripta |
Abbreviated Journal |
Phys. Scr. |
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Volume |
T150 |
Issue |
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Pages |
014005 - 4pp |
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Keywords |
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Abstract |
Neutron-induced fission cross section measurements of U-233, Am-243 and Am-241 relative to U-235 have been carried out at the neutron time-of-flight facility n_TOF at CERN. A fast ionization chamber has been employed. All samples were located in the same detector; therefore the studied elements and the reference U-235 target are subject to the same neutron beam. |
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Address |
[Belloni, F.; Milazzo, P. M.; Abbondanno, U.; Fujii, K.; Moreau, C.] Ist Nazl Fis Nucl, Trieste, Italy, Email: francesca.belloni@cea.fr |
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Corporate Author |
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Thesis |
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Publisher |
Iop Publishing Ltd |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0031-8949 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000309605500006 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1184 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Belloni, F. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron-induced fission cross-section of U-233 in the energy range 0.5 < E-n < 20 MeV |
Type |
Journal Article |
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Year |
2011 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
47 |
Issue |
1 |
Pages |
2 - 7pp |
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Keywords |
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Abstract |
The neutron-induced fission cross-section of U-233 has been measured at the CERN nTOF facility relative to the standard fission cross-section of U-235 between 0.5 and 20MeV. The experiment was performed with a fast ionization chamber for the detection of the fission fragments and to discriminate against alpha-particles from the natural radioactivity of the samples. The high instantaneous flux and the low background of the nTOF facility result in data with uncertainties of approximate to 3%, which were found in good agreement with previous experiments. The high quality of the present results allows to improve the evaluation of the U-233(n, f) cross-section and, consequently, the design of energy systems based on the Th/U cycle. |
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Address |
[Belloni, F.; Milazzo, P. M.; Abbondanno, U.; Fujii, K.; Moreau, C.] Ist Nazl Fis Nucl INFN, Trieste, Italy, Email: paolo.milazzo@ts.infn.it |
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Corporate Author |
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Thesis |
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Publisher |
Springer |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
ISI:000288550800006 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
539 |
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| Permanent link to this record |
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Author |
n_TOF Collaboration (Belloni, F. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Measurement of the neutron-induced fission cross-section of Am-243 relative to U-235 from 0.5 to 20 MeV |
Type |
Journal Article |
| |
Year |
2011 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
47 |
Issue |
12 |
Pages |
160 - 8pp |
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Keywords |
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Abstract |
The ratio of the neutron-induced fission cross-sections of Am-243 and U-235 was measured in the energy range from 0.5 to 20 MeV with uncertainties of approximate to 4%. The experiment was performed at the CERN n_TOF facility using a fast ionization chamber. With the good counting statistics that could be achieved thanks to the high instantaneous flux and the low backgrounds, the present results are useful for resolving discrepancies in previous data sets and are important for future reactors with improved fuel burn-up. |
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Address |
[Belloni, F.; Calviani, M.; Mastinu, P.; Milazzo, P. M.; Abbondanno, U.; Fujii, K.; Gramegna, F.; Moreau, C.] Ist Nazl Fis Nucl INFN, Lab Nazl Legnaro, Trieste, Italy, Email: paolo.milazzo@ts.infn.it |
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Corporate Author |
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Thesis |
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Publisher |
Springer |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
ISBN |
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Medium |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000300285100005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
904 |
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