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n_TOF Collaboration (Praena, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Measurement and resonance analysis of the S-33(n,alpha)Si-30 cross section at the CERN n_TOF facility in the energy region from 10 to 300 keV |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
6 |
Pages |
064603 - 10pp |
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Abstract |
The (33)(n , alpha)Si-30 cross section has been measured at the neutron time-of-flight (n_TOF) facility at CERN in the neutron energy range from 10 to 300 keV relative to the B-10(n, alpha)(7) Li cross-section standard. Both reactions were measured simultaneously with a set of micromegas detectors. The flight path of 185 m has allowed us to obtain the cross section with high-energy resolution. An accurate description of the resonances has been performed by means of the multilevel multichannel R-matrix code SAMMY. The results show a significantly higher area of the biggest resonance (13.45 keV) than the unique high-resolution (n , alpha) measurement. The new parametrization of the 13.45-keV resonance is similar to that of the unique transmission measurement. This resonance is a matter of research in neutron-capture therapy. The S-33(n, alpha)Si-30 cross section has been studied in previous works because of its role in the production of S-36 in stars, which is currently overproduced in stellar models compared to observations. |
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[Praena, J.; Porras, I] Univ Granada, Granada, Spain, Email: jpraena@ugr.es |
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Amer Physical Soc |
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2469-9985 |
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WOS:000434017300004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3597 |
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Author |
n_TOF Collaboration (Sabate-Gilarte et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
High-accuracy determination of the neutron flux in the new experimental area n_TOF-EAR2 at CERNx |
Type |
Journal Article |
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Year |
2017 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
53 |
Issue |
10 |
Pages |
210 - 13pp |
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Abstract |
A new high flux experimental area has recently become operational at the nTOF facility at CERN. This new measuring station, nTOF-EAR2, is placed at the end of a vertical beam line at a distance of approximately 20m from the spallation target. The characterization of the neutron beam, in terms of flux, spatial profile and resolution function, is of crucial importance for the feasibility study and data analysis of all measurements to be performed in the new area. In this paper, the measurement of the neutron flux, performed with different solid-state and gaseous detection systems, and using three neutronconverting reactions considered standard in different energy regions is reported. The results of the various measurements have been combined, yielding an evaluated neutron energy distribution in a wide energy range, from 2meV to 100MeV, with an accuracy ranging from 2%, at low energy, to 6% in the high-energy region. In addition, an absolute normalization of the n_TOF-EAR2 neutron flux has been obtained by means of an activation measurement performed with 197 Au foils in the beam. |
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Address |
[Sabate-Gilarte, M.; Vlachoudis, V.; Aberle, O.; Bacak, M.; Brugger, M.; Calviani, M.; Cardella, R.; Cerutti, F.; Chiaveri, E.; Ferrari, A.; Hernandez-Prieto, A.; Kadi, Y.; Losito, R.; Macina, D.; Mingrone, F.; Montesano, S.; Rubbia, C.; Weiss, C.] CERN, European Org Nucl Res, Geneva, Switzerland, Email: massimo.barbagallo@ba.infn.it |
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Springer |
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1434-6001 |
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WOS:000413766400002 |
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no |
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yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3350 |
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Author |
n_TOF Collaboration (Sarmento, R. et al); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Measurement of the (236)U(n, f) cross section from 170 meV to 2 MeV at the CERN n_TOF facility |
Type |
Journal Article |
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Year |
2011 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
84 |
Issue |
4 |
Pages |
044618 - 10pp |
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Abstract |
The neutron-induced fission cross section of (236)U was measured at the neutron Time-of-Flight (nTOF) facility at CERN relative to the standard (235)U(n, f) cross section for neutron energies ranging from above thermal to several MeV. The measurement, covering the full range simultaneously, was performed with a fast ionization chamber, taking advantage of the high resolution of the nTOF spectrometer. The n_TOF results confirm that the first resonance at 5.45 eV is largely overestimated in some nuclear data libraries. The resonance triplet around 1.2 keV was measured with high resolution and resonance parameters were determined with good accuracy. Resonances at high energy have also been observed and characterized and different values for the cross section are provided for the region between 10 keV and the fission threshold. The present work indicates various shortcomings of the current nuclear data libraries in the subthreshold region and provides the basis for an accurate re-evaluation of the (236)U(n, f) cross section, which is of great relevance for the development of emerging or innovative nuclear reactor technologies. |
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Address |
[Sarmento, R; Goncalves, IF; Vaz, P; Carrapico, C; de Albornoz, AC; Marques, L; Salgado, J; Tavora, L] ITN, Sacavem, Portugal |
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Amer Physical Soc |
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English |
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0556-2813 |
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Notes |
WOS:000296521000006 |
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no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
818 |
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Author |
n_TOF Collaboration (Sosnin, N.V. et al.); Babiano-Suarez, V.; Caballero, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L. |
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Title |
Measurement of the 77Se(n,gamma) cross section up to 200 keV at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2023 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
107 |
Issue |
6 |
Pages |
065805 - 9pp |
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Abstract |
The 77Se(n,gamma) reaction is of importance for 77Se abundance during the slow neutron capture process in massive stars. We have performed a new measurement of the 77Se radiative neutron capture cross section at the Neutron Time-of-Flight facility at CERN. Resonance capture kernels were derived up to 51 keV and cross sections up to 200 keV. Maxwellian-averaged cross sections were calculated for stellar temperatures between kT = 5 keV and kT = 100 keV, with uncertainties between 4.2% and 5.7%. Our results lead to substantial decreases of 14% and 19% in 77Se abundances produced through the slow neutron capture process in selected stellar models of 15M0 and 2M0, respectively, compared to using previous recommendation of the cross section. |
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Address |
[V. Sosnin, N.; Lederer-Woods, C.; Garg, R.; Dietz, M.; Murphy, A. St. J.; Lonsdale, S.; Woods, P. J.] Univ Edinburgh, Sch Phys & Astron, Edinburgh, Scotland, Email: nsosnin@ed.ac.uk |
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Amer Physical Soc |
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2469-9985 |
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Notes |
WOS:001023903800002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5599 |
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Author |
n_TOF Collaboration (Stamatopoulos, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Investigation of the Pu-240(n, f) reaction at the n_TOF/EAR2 facility in the 9 meV-6 MeV range |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
1 |
Pages |
014616 - 23pp |
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Abstract |
Background: Nuclear waste management is considered amongst the major challenges in the field of nuclear energy. A possible means of addressing this issue is waste transmutation in advanced nuclear systems, whose operation requires a fast neutron spectrum. In this regard, the accurate knowledge of neutron-induced reaction cross sections of several (minor) actinide isotopes is essential for design optimization and improvement of safety margins of such systems. One such case is Pu-240, due to its accumulation in spent nuclear fuel of thermal reactors and its usage in fast reactor fuel. The measurement of the Pu-240(n, f) cross section was previously attempted at the CERN nTOF facility EAR1 measuring station using the time-of-flight technique. Due to the low amount of available material and the given flux at EAR1, the measurement had to last several months to achieve a sufficient statistical accuracy. This long duration led to detector deterioration due to the prolonged exposure to the high alpha activity of the fission foils, therefore the measurement could not be successfully completed. Purpose: It is aimed to determine whether it is feasible to study neutron-induced fission at nTOF/EAR2 and provide data on the Pu-240(n, f) reaction in energy regions requested for applications. Methods: The study of the Pu-240(n, f) reaction was made at a new experimental area (EAR2) with a shorter flight path which delivered on average 30 times higher flux at fast neutron energies. This enabled the measurement to be performed much faster, thus limiting the exposure of the detectors to the intrinsic activity of the fission foils. The experimental setup was based on microbulk Micromegas detectors and the time-of-flight data were analyzed with an optimized pulse-shape analysis algorithm. Special attention was dedicated to the estimation of the non-negligible counting loss corrections with the development of a new methodology, and other corrections were estimated via Monte Carlo simulations of the experimental setup. Results: This new measurement of the Pu-240(n, f) cross section yielded data from 9 meV up to 6 MeV incident neutron energy and fission resonance kernels were extracted up to 10 keV. Conclusions: Neutron-induced fission of high activity samples can be successfully studied at the n_TOF/EAR2 facility at CERN covering a wide range of neutron energies, from thermal to a few MeV. |
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Address |
[Stamatopoulos, A.; Tsinganis, A.; Kokkoris, M.; Vlastou, R.; Diakaki, M.] Natl Tech Univ Athens, Athens, Greece, Email: athanasios.stamatopoulos@cern.ch |
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Amer Physical Soc |
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0556-2813 |
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Notes |
WOS:000551057500002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4466 |
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Author |
n_TOF Collaboration (Tagliente, G. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Zr-92(n, gamma) and (n,tot) measurements at the GELINA and n_TOF facilities |
Type |
Journal Article |
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Year |
2022 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
105 |
Issue |
2 |
Pages |
025805 - 14pp |
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Keywords |
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Abstract |
Background: Stellar nucleosynthesis of elements heavier than iron is driven by neutron capture processes. Zr-92 is positioned at a strategic point along the slow nucleosynthesis path, given its proximity to the neutron magic number N = 50 and its position at the matching region between the weak and main slow processes. Purpose: In parallel with recent improved astronomical data, the extraction of accurate Maxwellian averaged cross sections (MACSs) derived from a more complete and accurate set of resonance parameters should allow for a better understanding of the stellar conditions at which nucleosynthesis takes place. Methods: Transmission and capture cross section measurements using enriched Zr-92 metallic samples were performed at the time-of flight facilities GELINA of JRC-Geel (BE) and nTOF of CERN (CH). The neutron beam passing through the samples was investigated in transmission measurements at GELINA using a Li-glass scintillator. The gamma rays emitted during the neutron capture reactions were detected by C6D6 detectors at both GELINA and nTOF. Results: Resonance parameters of individual resonances up to 81 keV were extracted from a combined resonance shape analysis of experimental transmissions and capture yields. For the majority of the resonances the parity was determined from an analysis of the transmission data obtained with different sample thicknesses. Average resonance parameters were calculated. Conclusions: Maxwellian averaged cross sections were extracted from resonances observed up to 81 keV. The MACS for kT = 30 keV is fully consistent with experimental data reported in the literature. The MACSs for kT less than or similar to 15 keV are in good agreement with those derived from the ENDF/B-VIII.0 library and recommended in the KADoNTS database. For kT higher than 30 keV differences are observed. A comparison with MACSs obtained with the cross sections recommended in the JEFF-3.3 and JENDL-4.0 libraries shows discrepancies even for kT less than or similar to 15 keV. |
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Address |
[Tagliente, G.; Barbagallo, M.; Colonna, N.; Mastromarco, M.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
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Amer Physical Soc |
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2469-9985 |
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Notes |
WOS:000766732800002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5163 |
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Author |
n_TOF Collaboration (Tagliente, G. et al.); Domingo-Pardo, C.; Tain, J.L. |
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Title |
The Zr-92(n,gamma) reaction and its implications for stellar nucleosynthesis |
Type |
Journal Article |
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Year |
2010 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
81 |
Issue |
5 |
Pages |
055801 - 9pp |
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Keywords |
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Abstract |
Because the relatively small neutron capture cross sections of the zirconium isotopes are difficult to measure, the results of previous measurements are often not adequate for a number of problems in astrophysics and nuclear technology. Therefore, the Zr-92(n,gamma) cross section has been remeasured at the CERN n_TOF facility, providing a set of improved parameters for 44 resonances in the neutron energy range up to 40 keV. With this information the cross-section uncertainties in the keV region could be reduced to 5% as required for s-process nucleosynthesis studies and technological applications. |
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Address |
[Tagliente, G.; Colonna, N.; Marrone, S.; Terlizzi, R.] Ist Nazl Fis Nucl, I-70126 Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
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Amer Physical Soc |
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0556-2813 |
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Notes |
ISI:000278144800074 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
444 |
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Author |
n_TOF Collaboration (Tagliente, G. et al.); Domingo-Pardo, C.; Tain, J.L. |
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Title |
The Zr-93(n, gamma) reaction up to 8 keV neutron energy |
Type |
Journal Article |
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Year |
2013 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
87 |
Issue |
1 |
Pages |
014622 - 7pp |
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Keywords |
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Abstract |
The (n, gamma) reaction of the radioactive isotope Zr-93 has been measured at the n_TOF high-resolution time-of-flight facility at CERN. Resonance parameters have been extracted in the neutron energy range up to 8 keV, yielding capture widths smaller (14%) than reported in an earlier experiment. These results are important for detailed nucleosynthesis calculations and for refined studies of waste transmutation concepts. DOI: 10.1103/PhysRevC.87.014622 |
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Address |
[Tagliente, G.; Colonna, N.; Marrone, S.; Terlizzi, R.] Ist Nazl Fis Nucl, I-70126 Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
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Amer Physical Soc |
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English |
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0556-2813 |
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Notes |
WOS:000314335800003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1322 |
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Author |
n_TOF Collaboration (Tagliente, G. et al.); Domingo-Pardo, C.; Tain, J.L. |
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Title |
Neutron capture on (94)Zr: Resonance parameters and Maxwellian-averaged cross sections |
Type |
Journal Article |
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Year |
2011 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
84 |
Issue |
1 |
Pages |
015801 - 9pp |
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Abstract |
The neutron capture cross sections of the Zr isotopes play an important role in nucleosynthesis studies. The s-process reaction flow between the Fe seed and the heavier isotopes passes through the neutron magic nucleus (90)Zr and through (91,92,93,94)Zr, but only part of the flow extends to (96)Zr because of the branching point at (95)Zr. Apart from their effect on the s-process flow, the comparably small isotopic (n, gamma) cross sections make Zr also an interesting structural material for nuclear reactors. The (94)Zr (n, gamma) cross section has been measured with high resolution at the spallation neutron source n_TOF at CERN and resonance parameters are reported up to 60 keV neutron energy. |
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Address |
[Tagliente, G; Colonna, N; Marrone, S; Terlizzi, R] Ist Nazl Fis Nucl, I-70126 Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
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Amer Physical Soc |
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English |
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0556-2813 |
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Notes |
WOS:000292767200010 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
687 |
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Author |
n_TOF Collaboration (Tagliente, G. et al.); Domingo-Pardo, C.; Tain, J.L. |
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Title |
(96)Zr(n,gamma) measurement at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2011 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
84 |
Issue |
5 |
Pages |
055802 - 8pp |
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Keywords |
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Abstract |
The (n,gamma) cross section of (96)Zr has been investigated at the CERN n_TOF spallation neutron source. High-resolution time-of-flight measurements using an enriched ZrO(2) sample allowed us to analyze 15 resonances below 40 keV with improved accuracy. On average, the capture widths were found to be 25% smaller than reported in earlier experiments. If complemented with the contribution by direct radiative capture, the derived Maxwellian averaged cross sections are consistent with activation data at kT = 25 keV. The present results confirm the astrophysical implications for the s-process branching at (95)Zr. |
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Address |
[Tagliente, G; Colonna, N; Marrone, S; Terlizzi, R] Ist Nazl Fis Nucl, I-70126 Bari, Italy, Email: giuseppe.tagliente@ba.infn.it |
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Amer Physical Soc |
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English |
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0556-2813 |
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Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
WOS:000297121100005 |
Approved |
no |
|
| |
Is ISI |
yes |
International Collaboration |
yes |
|
| |
Call Number |
IFIC @ elepoucu @ |
Serial |
812 |
|
| Permanent link to this record |
