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Yokoyama, R. et al, Tain, J. L., Algora, A., Agramunt, J., Domingo-Pardo, C., Morales, A. I., et al. (2023). β-delayed neutron emissions from N > 50 gallium isotopes. Phys. Rev. C, 108(6), 064307–15pp.
Abstract: beta-delayed gamma-neutron spectroscopy has been performed on the decay of A=84 to 87 gallium isotopes at the RI-beam Factory at the RIKEN Nishina Center using a high-efficiency array of 3He neutron counters (BRIKEN). beta-2n-gamma events were measured in the decays of all of the four isotopes for the first time, which is direct evidence for populating the excited states of two-neutron daughter nuclei. Detailed decay schemes with the gamma branching ratios were obtained for these isotopes, and the neutron emission probabilities (P-xn) were updated from the previous study. Hauser-Feshbach statistical model calculations were performed to understand the experimental branching ratios. We found that the P-1n and P-2n values are sensitive to the nuclear level densities of 1n daughter nuclei and showed that the statistical model reproduced the P-2n/P-1n ratio better when experimental levels plus shell-model level densities fit by the Gilbert-Cameron formula were used as the level-density input. We also showed the neutron and gamma branching ratios are sensitive to the ground-state spin of the parent nucleus. Our statistical model analysis suggested J <= 3 for the unknown ground-state spin of the odd-odd nucleus Ga-86, from the I gamma(4(+)-> 2(+))/I-gamma(2(+)-> 0(+)) ratio of Ga-84 and the P-2n/P-1n ratio. These results show the necessity of detailed understanding of the decay scheme, including data from neutron spectroscopy, in addition to gamma measurements of the multineutron emitters.
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Briz, J. A., Borge, M. J. G., Rubio, B., Agramunt, J., Algora, A., Deo, A. Y., et al. (2022). Clarifying the structure of low-lying states in Br-72. Phys. Rev. C, 105(1), 014323–17pp.
Abstract: The spins and parities of low-lying states in 72Br populated in the beta decay of 72Kr have been studied via conversion electron spectroscopy. The measurements were carried out at ISOLDE using a miniorange spectrometer with Si(Li) and HPGe detectors for electrons and gamma ray detection. Results of the conversion coefficients corresponding to transitions deexciting 12 levels in 72Br are reported. The multipolarities of the transitions are deduced and the spins and parities of the levels involved are discussed. From the multipolarities of the most intense transitions to the ground state, the spin and parity of the 72Br ground state have been definitely established as 1+. The spin of the 101.2-keV isomeric state is determined to be 3-. The level scheme is compared with mean-field and shell-model calculations and oblate deformation for the 72Br ground state is deduced. No E0 transitions have been found in 72Br. E0 transitions in the neighboring isobaric nuclei, 72Se and 72Ge, have also been studied.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2022). Total absorption gamma-ray spectroscopy of the ss decays of Y-96gs,Y-m. Phys. Rev. C, 106(1), 014306–14pp.
Abstract: The ss decays of the ground state (gs) and isomeric state (m) of Y-96 have been studied with the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8(+) isomeric state from the 0(-) ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The ss-intensity distributions of both decays have been independently determined. In the analyses the deexcitation of the 1581.6 keV level in Zr-96, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the ss-detector efficiency, influencing the ss-intensity distribution obtained. Our results for Y-96gs (0(-)) confirm the large ground state to ground state ss-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to 96.6(-2.1)(+0.3) % of the total ss intensity. Given that the decay of Y-96gs is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of Y-96m (8(+)), previously undetected ss intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption gamma-ray spectroscopy measurements of ss decays with highly fragmented deexcitation patterns. Y-96m (8(+)) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average ss and gamma energies differ significantly from the previous values in evaluated databases. The discrepancy is far above the previously quoted uncertainties. Finally, we also report on the successful implementation of an innovative total absorption gamma-ray spectroscopy analysis of the module-multiplicity gated spectra, as a first proof of principle to distinguish between decaying states with very different spin-parity values.
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Vitez-Sveiczer, A. et al, Algora, A., Morales, A. I., Rubio, B., Agramunt, J., Guadilla, V., et al. (2022). The beta-decay of Kr-70 into Br-70: Restoration of the pseudo-SU(4) symmetry. Phys. Lett. B, 830, 137123–8pp.
Abstract: The beta-decay of the even-even nucleus Kr-70 with Z=N+2, has been investigated at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center using the BigRIPS fragment separator, the ZeroDegree Spectrometer, the WAS3ABI implantation station and the EURICA HPGe cluster array. Fifteen gamma-rays associated with the beta-decay of( 70)Kr into Br-70 have been identified for the first time, defining ten populated states below E-exc=3300 keV. The half-life of Kr-70 was derived with increased precision and found to be t(1/2)=45.19 +/- 0.14 ms. The beta-delayed proton emission probability has also been determined as epsilon(p)=0.545(23)%. An increase in the beta-strength to the yrast 1(+) state in comparison with the heaviest Z=N+2 system studied so far (Ge-62 decay) is observed that may indicate increased np correlations in the T=0 channel. The beta-decay strength deduced from the results is interpreted in terms of the proton-neutron quasiparticle random-phase approximation (pnQRPA) and also with a schematic model that includes isoscalar and isovector pairing in addition to quadrupole deformation. The application of this last model indicates an approximate realization of pseudo-SU(4) symmetry in this system.
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Mistry, A. K. et al, Tain, J. L., Agramunt, J., Algora, A., Guadilla, V., Morales, A. I., et al. (2022). The DESPEC setup for GSI and FAIR. Nucl. Instrum. Methods Phys. Res. A, 1033, 166662–18pp.
Abstract: The DEcay SPECtroscopy (DESPEC) setup for nuclear structure investigations was developed and commissioned at GSI, Germany in preparation for a full campaign of experiments at the FRS and Super-FRS. In this paper, we report on the first employment of the setup in the hybrid configuration with the AIDA implanter coupled to the FATIMA LaBr3(Ce) fast-timing array, and high-purity germanium detectors. Initial results are shown from the first experiments carried out with the setup. An overview of the setup and function is discussed, including technical advancements along the path.
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Kiss, G. G. et al, Tarifeño-Saldivia, A., Tain, J. L., Agramunt, J., Algora, A., Domingo-Pardo, C., et al. (2022). Measuring the beta-decay Properties of Neutron-rich Exotic Pm, Sm, Eu, and Gd Isotopes to Constrain the Nucleosynthesis Yields in the Rare-earth Region. Astrophys. J., 936(2), 107–18pp.
Abstract: The beta-delayed neutron-emission probabilities of 28 exotic neutron-rich isotopes of Pm, Sm, Eu, and Gd were measured for the first time at RIKEN Nishina Center using the Advanced Implantation Detector Array (AIDA) and the BRIKEN neutron detector array. The existing beta-decay half-life (T (1/2)) database was significantly increased toward more neutron-rich isotopes, and uncertainties for previously measured values were decreased. The new data not only constrain the theoretical predictions of half-lives and beta-delayed neutron-emission probabilities, but also allow for probing the mechanisms of formation of the high-mass wing of the rare-earth peak located at A approximate to 160 in the r-process abundance distribution through astrophysical reaction network calculations. An uncertainty quantification of the calculated abundance patterns with the new data shows a reduction of the uncertainty in the rare-earth peak region. The newly introduced variance-based sensitivity analysis method offers valuable insight into the influence of important nuclear physics inputs on the calculated abundance patterns. The analysis has identified the half-lives of Sm-168 and of several gadolinium isotopes as some of the key variables among the current experimental data to understand the remaining abundance uncertainty at A = 167-172.
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Orrigo, S. E. A., Tain, J. L., Mont-Geli, N., Tarifeño-Saldivia, A., Fraile, L. M., Grieger, M., et al. (2022). Long-term evolution of the neutron rate at the Canfranc Underground Laboratory. Eur. Phys. J. C, 82(9), 814–11pp.
Abstract: We report results on the long-term variation of the neutron counting rate at the Canfranc Underground Laboratory, of importance for several low-background experiments installed there, including rare-event searches. The measurement campaign was performed employing the High Efficiency Neutron Spectrometry Array (HENSA) mounted in Hall A and lasted 412 live days. The present study is the first long-term measurement of the neutron rate with sensitivity over a wide range of neutron energies (from thermal up to 0.1 GeV and beyond) performed in any underground laboratory so far. Data on the environmental variables inside the experimental hall (radon concentration, air temperature, air pressure and humidity) were also acquired during all the measurement campaign. We have investigated for the first time the evolution of the neutron rate for different energies of the neutrons and its correlation with the ambient variables.
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Wu, J. et al, Algora, A., Agramunt, J., Morales, A. I., Orrigo, S. E. A., Tain, J. L., et al. (2022). First observation of isomeric states in 111Zr, 113Nb, and 115Mo. Phys. Rev. C, 106(6), 064328–5pp.
Abstract: Isomeric states in the neutron-rich nuclei 111Zr [T1/2 = 0.10(7) μs], 113Nb [T1/2 = 0.7(4) μs], 115Mo [T1/2 = 46(3) μs] were first identified at the Radioactive Ion Beam Factory (RIBF) of RIKEN by using in-flight fission and fragmentation of a 238U beam at an energy of 345 MeV/u. This is a brief report of the gamma transitions de -exciting from isomeric states and half-lives measurements, which provides the first spectroscopy in the nuclear region of prolate-to-oblate shape-phase transition around mass A approximate to 110.
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Phong, V. H. et al, Agramunt, J., Algora, A., Domingo-Pardo, C., Morales, A. I., Rubio, B., et al. (2022). Beta-Delayed One and Two Neutron Emission Probabilities South-East of Sn-132 and the Odd-Even Systematics in r-Process Nuclide Abundances. Phys. Rev. Lett., 129(18), 172701–7pp.
Abstract: The beta-delayed one- and two-neutron emission probabilities (P-1n and P-2n) of 20 neutron-rich nuclei with N >= 82 have been measured at the RIBF facility of the RIKEN Nishina Center. P-1n of Ag-130;131, Cd-133;134, In-135;136, and (138;13)9Sn were determined for the first time, and stringent upper limits were placed on P-2n for nearly all cases. beta-delayed two-neutron emission (beta 2n) was unambiguously identified in Cd-133 and In-135;136, and their P-2n were measured. Weak beta 2n was also detected from Sn-137;138. Our results highlight the effect of the N = 82 and Z = 50 shell closures on beta-delayed neutron emission probability and provide stringent benchmarks for newly developed macroscopic-microscopic and self-consistent global models with the inclusion of a statistical treatment of neutron and. emission. The impact of our measurements on r-process nucleosynthesis was studied in a neutron star merger scenario. Our P-1n and P-2n have a direct impact on the
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Orrigo, S. E. A. et al, Rubio, B., Gelletly, W., Aguilera, P., Algora, A., Morales, A. I., et al. (2021). beta decay of the very neutron-deficient Ge-60 and Ge-62 nuclei. Phys. Rev. C, 103(1), 014324–12pp.
Abstract: We report here the results of a study of the beta decay of the proton-rich Ge isotopes, Ge-60 and Ge-62, produced in an experiment at the RIKEN Nishina Center. We have improved our knowledge of the half-lives of Ge-62 [73.5(1) ms] and Ge-60 [25.0(3) ms] and its daughter nucleus, Ga-60 [69.4(2) ms]. We measured individual beta-delayed proton and gamma emissions and their related branching ratios. Decay schemes and absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. A total beta-delayed proton-emission branching ratio of 67(3)% has been obtained for Ge-60. New information has been obtained on the energy levels populated in Ga-60 and on the 1/2(-) excited state in the beta p daughter Zn-59. We extracted a ground state-to-ground state feeding of 85.3(3)% for the decay of Ge-62. Eight new y lines have been added to the deexcitation of levels populated in the Ga-62 daughter.
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