|
|
Watanabe, H. et al, & Montaner-Piza, A. (2019). New isomers in (125)Pd(79)( )and Pd-127(81): Competing proton and neutron excitations in neutron-rich palladium nuclides towards the N=82 shell closure. Phys. Lett. B, 792, 263–268.
Abstract: The neutron-rich isotopes of palladium have attracted considerable interest in terms of the evolution of the N = 82 neutron shell closure and its influence on the r-process nucleosynthesis. In this Letter, we present the first spectroscopic information on the excited states in Pd-125(79) and Pd-127(81) studied using the EURICA gamma-ray spectrometer, following production via in-flight fission of a high-intensity U-238 beam at the RIBF facility. New isomeric states with half-lives of 144(4) ns and 39(6) μs have been assigned spins and parities of (23/2(+)) and (19/2(+)) in Pd-125 and Pd-127, respectively. The observed level properties are compared to a shell-model calculation, suggesting the competition between proton excitations and neutron excitations in the proton-hole and neutron-hole systems in the vicinity of the doubly magic nucleus Sn-132.
|
|
|
|
Chen, Z. Q. et al, & Montaner-Piza, A. (2019). Proton Shell Evolution below Sn-132: First Measurement of Low-Lying beta-Emitting Isomers in Ag-123,Ag-325. Phys. Rev. Lett., 122(21), 212502–6pp.
Abstract: The beta-delayed gamma-ray spectroscopy of neutron-rich Ag-123,Ag-325 isotopes is investigated at the Radioactive Isotope Beam Factory of RIKEN, and the long-predicted 1/2(-) beta-emitting isomers in Ag-123,Ag-325 are identified for the first time. With the new experimental results, the systematic trend of energy spacing between the lowest 9/2(+) and 1/2(-) levels is extended in Ag isotopes up to N = 78, providing a clear signal for the reduction of the Z = 40 subshell gap in Ag towards N = 82. Shell-model calculations with the state-of-the-art V-MU plus M3Y spin-orbit interaction give a satisfactory description of the low-lying states in Ag-123,Ag-325. The tensor force is found to play a crucial role in the evolution of the size of the Z = 40 subshell gap. The observed inversion of the single-particle levels around Ag-123 can be well interpreted in terms of the monopole shift of the pi 1g(9/2) orbitals mainly caused by the increasing occupation of nu 1h(11/2) orbitals.
|
|
|
|
Guadilla, V., Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of niobium isomers. Phys. Rev. C, 100(2), 024311–15pp.
Abstract: The beta-intensity distributions of the decays of Nb-100gs,Nb-100m and Nb-102gs,Nb-102m have been determined using the total absorption gamma-ray spectroscopy technique. The JYFLTRAP double Penning trap system was employed in a campaign of challenging measurements performed with the decay total absorption gamma-ray spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. Different strategies were applied to disentangle the isomeric states involved, lying very close in energy. The low-spin component of each niobium case was populated through the decay of the zirconium parent, which was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained beta-intensity distributions for these zirconium decays. The beta-strength distributions evaluated with these results were compared with calculations in a quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of Zr-100,Zr-102. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The beta-intensities of the decay of Nb-102m, for which there were no previous data, were obtained. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported, and here we detail the significant impact on decay heat calculations.
|
|
|
|
Guadilla, V. et al, Tain, J. L., Algora, A., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters I-137 and Rb-95. Phys. Rev. C, 100(4), 044305–17pp.
Abstract: The decays of the beta-delayed neutron emitters( 137)I and Rb-95 have been studied with the total absorption gamma-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyvaskyla allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption gamma-ray spectrometer, a segmented detector composed of 18 NaI(T1) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt gamma rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of beta intensity to states above the neutron separation energy that deexcite by gamma rays, comparable to the neutron emission probability. The competition between gamma deexcitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the beta-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers.
|
|
|
|
Jungclaus, A. et al, & Montaner-Piza, A. (2020). Evolution of proton single-particle states in neutron-rich Sb isotopes beyond N=82. Phys. Rev. C, 102(3), 034324–11pp.
Abstract: The beta decay of the semimagic Sn isotopes Sn-136,Sn-137,Sn-138 has been studied at the Radioactive Isotope Beam Factory at the RIKEN Nishina Center. The first experimental information on excited states was obtained for Sb-137 while, in the case of Sb-136, the established excitation scheme could be extended by ten previously unidentified levels. In the decay of the most-neutron-rich isotope Sn-138, two gamma rays were observed for the first time. The new experimental results, in combination with state-of-the-art shell-model calculations, provide the first information with respect to the evolution of the Og(7/2) and 1d(5/2) proton single-particle states with increasing neutron number beyond N = 84.
|
|
