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Guerrero, C., Cano-Ott, D., Mendoza, E., Tain, J. L., Algora, A., Berthoumieux, E., et al. (2012). Monte Carlo simulation of the n_TOF Total Absorption Calorimeter. Nucl. Instrum. Methods Phys. Res. A, 671, 108–117.
Abstract: The n_TOF Total Absorption Calorimeter (TAC) is a 4 pi BaF2 segmented detector used at CERN for measuring neutron capture cross-sections of importance for the design of advanced nuclear reactors. This work presents the simulation code that has been developed in GEANT4 for the accurate determination of the detection efficiency of the TAC for neutron capture events. The code allows to calculate the efficiency of the TAC for every neutron capture state, as a function of energy, crystal multiplicity, and counting rate. The code includes all instrumental effects such as the single crystal detection threshold and energy resolution, finite size of the coincidence time window, and signal pile-up. The results from the simulation have been validated with experimental data for a large set of electromagnetic de-excitation patterns: beta-decay of well known calibration sources, neutron capture reactions in light nuclei with well known level schemes like Ti-nat, reference samples used in (n,gamma) measurements like Au-197 and experimental data from an actinide sample like Pu-240. The systematic uncertainty in the determination of the detection efficiency has been estimated for all the cases. As a representative example, the accuracy reached for the case of Au-197(n,gamma) ranges between 0.5% and 2%, depending on the experimental and analysis conditions. Such a value matches the high accuracy required for the nuclear cross-section data needed in advanced reactor design.
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n_TOF Collaboration(Guerrero, C. et al), Domingo-Pardo, C., & Tain, J. L. (2012). Measurement and resonance analysis of the Np-237 neutron capture cross section. Phys. Rev. C, 85(4), 044616–15pp.
Abstract: The neutron capture cross section of Np-237 was measured between 0.7 and 500 eV at the CERN n_TOF facility using the 4 pi BaF2 Total Absorption Calorimeter. The experimental capture yield was extracted minimizing all the systematic uncertainties and was analyzed together with the most reliable transmission data available using the SAMMY code. The result is a complete set of individual as well as average resonance parameters [D-0 = 0.56(2) eV, <Gamma(gamma)> = 40.9(18) meV, 10(4)S(0) = 0.98(6), R' = 9.8(6) fm]. The capture cross section obtained in this work is in overall agreement with the evaluations and the data of Weston and Todd [Nucl. Sci. Eng. 79, 184 (1981)], thus showing sizable differences with respect to previous data from Scherbakov et al. [J. Nucl. Sci. Technol. 42, 135 (2005)] and large discrepancies with data Kobayashi et al. [J. Nucl. Sci. Technol. 39, 111 (2002)]. The results indicate that a new evaluation combining the present capture data with reliable transmission data would allow reaching an accuracy better than 4%, in line with the uncertainty requirements of the nuclear data community for the design and operation of current and future nuclear devices.
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n_TOF Collaboration(Guerrero, C. et al), Giubrone, G., & Tain, J. L. (2012). Simultaneous measurement of neutron-induced capture and fission reactions at CERN. Eur. Phys. J. A, 48(3), 29–9pp.
Abstract: The measurement of the capture cross-section of fissile elements, of utmost importance for the design of innovative nuclear reactors and the management of nuclear waste, faces particular difficulties related to the.-ray background generated in the competing fission reactions. At the CERN neutron time-of-flight facility nTOF we have combined the Total Absorption Calorimeter (TAC) capture detector with a set of three U-235 loaded MicroMegas (MGAS) fission detectors for measuring simultaneously two reactions: capture and fission. The results presented here include the determination of the three detection efficiencies involved in the process: epsilon(TAC)(n, f), epsilon(TAC)(n, gamma) and epsilon(MGAS)(n, f). In the test measurement we have succeeded in measuring simultaneously with a high total efficiency the U-235 capture and fission cross-sections, disentangling accurately the two types of reactions. The work presented here proves that accurate capture cross-section measurements of fissile isotopes are feasible at nTOF.
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Garcia, A. R., Martinez, T., Cano-Ott, D., Castilla, J., Guerrero, C., Marin, J., et al. (2012). MONSTER: a time of flight spectrometer for beta-delayed neutron emission measurements. J. Instrum., 7, C05012–12pp.
Abstract: The knowledge of the beta-decay properties of nuclei contributes decisively to our understanding of nuclear phenomena: the beta-delayed neutron emission of neutron rich nuclei plays an important role in the nucleosynthesis r-process and constitutes a probe for nuclear structure of very neutron rich nuclei providing information about the high energy part of the full beta strength (S-beta) function. In addition, beta-delayed neutrons are essential for the control and safety of nuclear reactors. In order to determine the neutron energy spectra and emission probabilities from neutron precursors a MOdular Neutron time-of-flight SpectromeTER (MONSTER) has been proposed for the DESPEC experiment at the future FAIR facility. The design of MONSTER and status of its construction are reported in this work.
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n_TOF Collaboration(Guerrero, C. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Study of Photon Strength Function of Actinides: the Case of (235)U, (238)Np and (241)Pu. J. Korean Phys. Soc., 59(2), 1510–1513.
Abstract: The decay from excited levels in medium and heavy nuclei can be described in a statistical approach by means of Photon Strength Functions and Level Density distributions. The study of electromagnetic cascades following neutron capture based on the use of high efficiency detectors has been shown to be well suited for probing the properties of the Photon Strength Function of heavy (high level density) and/or radioactive (high background) nuclei. In this work we have investigated for the first time the validity of the recommended PSF of actinides, in particular (235)U, (238)Np and (241)Pu. Our study includes the search for resonance structures in the PSF below S(n) and draws conclusions regarding their existence and their characteristics in terms of energy, width and electromagnetic nature.
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