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Algora, A. et al, Jordan, D., Tain, J. L., Rubio, B., Agramunt, J., Perez-Cerdan, A. B., et al. (2010). Reactor Decay Heat in Pu-239: Solving the gamma Discrepancy in the 4-3000-s Cooling Period. Phys. Rev. Lett., 105(20), 202501–4pp.
Abstract: The beta feeding probability of Tc-102,Tc- 104,Tc- 105,Tc- 106,Tc- 107, Mo-105, and Nb-101 nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the gamma component of the decay heat for Pu-239 in the 4-3000 s range.
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Guess, C. J. et al, Algora, A., Estevez, E., Molina, F., & Rubio, B. (2011). The Nd-150(He-3,t) and Sm-150(t,He-3) reactions with applications to beta beta decay of Nd-150. Phys. Rev. C, 83(6), 064318–17pp.
Abstract: The Nd-150(3He,t) reaction at 140 MeV/u and Sm-150(t,He-3) reaction at 115 MeV/u were measured, populating excited states in Pm-150. The transitions studied populate intermediate states of importance for the (neutrinoless) beta beta decay of Nd-150 to Sm-150. Monopole and dipole contributions to the measured excitation-energy spectra were extracted by using multipole decomposition analyses. The experimental results were compared with theoretical calculations obtained within the framework of the quasiparticle random-phase approximation, which is one of the main methods employed for estimating the half-life of the neutrinoless beta beta decay (0 nu beta beta) of Nd-150. The present results thus provide useful information on the neutrino responses for evaluating the 0 nu beta beta and 2 nu beta beta matrix elements. The 2 nu beta beta matrix element calculated from the Gamow-Teller transitions through the lowest 1(+) state in the intermediate nucleus is maximally about half that deduced from the half-life measured in 2 nu beta beta direct counting experiments, and at least several transitions through 1+ intermediate states in Pm-150 are required to explain the 2 nu beta beta half-life. Because Gamow-Teller transitions in the Sm-150(t,3He) experiment are strongly Pauli blocked, the extraction of Gamow-Teller strengths was complicated by the excitation of the 2 (h) over bar omega, Lambda L = 0, Delta S = 1 isovector spin-flip giant monopole resonance (IVSGMR). However, the near absence of Gamow-Teller transition strength made it possible to cleanly identify this resonance, and the strength observed is consistent with the full exhaustion of the non-energy-weighted sum rule for the IVSGMR.
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Morales, A. I. et al, Agramunt, J., Algora, A., Gadea, A., Molina, F., & Rubio, B. (2011). Synthesis of N=127 isotones through (p,n) charge-exchange reactions induced by relativistic (208)Pb projectiles. Phys. Rev. C, 84(1), 011601–5pp.
Abstract: The production cross sections of four N = 127 isotones ((207)Hg, (206)Au, (205)Pt, and (204)Ir) have been measured using (p,n) charge-exchange reactions, induced in collisions of a (208)Pb primary beam at 1 A GeV with a Be target. These data allow one to investigate the use of a reaction mechanism to extend the limits of the chart of nuclides toward the important r-process nuclei in the region of the third peak of elemental abundance distribution.
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Algora, A. et al, Jordan, D., Tain, J. L., Rubio, B., Agramunt, J., Perez-Cerdan, A. B., et al. (2011). Improvements on Decay Heat Summation Calculations by Means of Total Absorption Gamma-ray Spectroscopy Measurements. J. Korean Phys. Soc., 59(2), 1479–1482.
Abstract: The decay heat of fission products plays an important role in predictions of the heat released by nuclear fuel in reactors. In this contribution we present results of the analysis of the measurement of the beta decay of some refractory isotopes that were considered possible important contributors to the decay heat in reactors. The measurements presented here were performed at the IGISOL facility of the University of Jyvaskyla, Finland. In our measurements we have combined for the first time a Penning trap (JYFLTRAP), which was used as a high resolution isobaric separator, with a total absorption spectrometer. The results of the measurements as well as their consequences for decay heat summation calculations are discussed.
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Perez-Cerdan, A. B., Rubio, B., Gelletly, W., Algora, A., Agramunt, J., Burkard, K., et al. (2011). beta decay of (78)Sr. Phys. Rev. C, 84(5), 054311–15pp.
Abstract: The gamma rays and conversion electrons emitted in the beta decay of (78)Sr to levels in (78)Rb have been studied using Ge detectors and a mini-orange spectrometer. A reliable level scheme based on the results of these experiments has been established. The properties of the levels in (78)Rb have been compared with calculations based on deformed Hartree-Fock with Skyrme interactions and pairing correlations in the BCS approximation. This has allowed an interpretation of the nature of the observed sets of levels in the odd-odd nucleus (78)Rb.
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Al-Dahan, N. et al, Algora, A., Molina, F., & Rubio, B. (2012). Multiple beta(-) decaying states in Re-194: Shape evolution in neutron-rich osmium isotopes. Phys. Rev. C, 85(3), 034301–9pp.
Abstract: beta decays from heavy, neutron-rich nuclei with A similar to 190 have been investigated following their production via the relativistic projectile fragmentation of an E/A = 1 GeV Pb-208 primary beam on a similar to 2.5 g/cm(2) Be-9 target. The reaction products were separated and identified using the GSI FRagment Separator (FRS) and stopped in the RISING active stopper. gamma decays were observed and correlated with these secondary ions on an event-by-event basis such that gamma-ray transitions following from both internal (isomeric) and beta decays were recorded. A number of discrete, beta-delayed gamma-ray transitions associated with beta decays from Re-194 to excited states in Os-194 have been observed, including previously reported decays from the yrast I-pi = (6(+)) state. Three previously unreported gamma-ray transitions with energies 194, 349, and 554 keV are also identified; these transitions are associated with decays from higher spin states in Os-194. The results of these investigations are compared with theoretical predictions from Nilsson multi-quasiparticle (MQP) calculations. Based on lifetime measurements and the observed feeding pattern to states in Os-194, it is concluded that there are three beta(-)-decaying states in Re-194.
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Ganioglu, E. et al, Algora, A., Estevez-Aguado, E., Molina, F., & Rubio, B. (2013). High-resolution study of Gamow-Teller transitions in the Ti-47(He-3, t)V-47 reaction. Phys. Rev. C, 87(1), 014321–12pp.
Abstract: Given the importance of Gamow-Teller (GT) transitions in nuclear structure and astrophysical nuclear processes, we have studied T-z = +3/2 -> +1/2, GT transitions starting from the Ti-47 nucleus in the (He-3, t) charge-exchange reaction at 0 degrees and at an intermediate incident energy of 140 MeV/nucleon. The experiments were carried out at the Research Center for Nuclear Physics (RCNP), Osaka, using the high-resolution facility with a high-dispersion beam line and the Grand-Raiden spectrometer. With an energy resolution of 20 keV, individual GT transitions were observed and GT strength was derived for each state populated up to an excitation energy (E-x) of 12.5 MeV. The GT strength was widely distributed from low excitation energy up to 12.5 MeV, where we had to stop the analysis because of the high level density. The distribution of the GT strengths was compared with the results of shell model calculations using the GXPF1 interaction. The calculations could reproduce the experimental GT distributions well. The GT transitions from the ground state of Ti-47 and the M1 transitions from the isobaric analog state in V-47 to the same low-lying states in V-47 are analogous. It was found that the ratios of GT transition strengths to the ground state, the 0.088-MeV state, and the 0.146-MeV state are similar to the ratios of the strengths of the analogous M1 transitions from the isobaric analog state (IAS) to these states. The measured distribution of the GT strengths was also compared with those starting from the T-z = +3/2 nucleus K-41 to the T-z = +1/2 nucleus Ca-41.
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Jordan, D. et al, Algora, A., Tain, J. L., Rubio, B., Agramunt, J., Perez-Cerdan, A. B., et al. (2013). Total absorption study of the beta decay of Tc-102,Tc-104,Tc-105. Phys. Rev. C, 87(4), 044318–14pp.
Abstract: The beta-feeding probabilities for three important contributors to the decay heat in nuclear reactors, namely Tc-102,Tc-104,Tc-105, have been measured using the total absorption spectroscopy technique. For the measurements, sources of very high isobaric purity have been obtained using a Penning trap (JYFLTRAP). A detailed description of the data analysis is given and the results are compared with high-resolution measurements and theoretical calculations. DOI: 10.1103/PhysRevC.87.044318
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Fujita, Y. et al, Algora, A., Estevez-Aguado, E., Molina, F., & Rubio, B. (2013). High-resolution study of T-z =+2 ->+1 Gamow-Teller transitions in the Ca-44(3He,t)Sc-44 reaction. Phys. Rev. C, 88(1), 014308–18pp.
Abstract: In order to study the Gamow-Teller (GT) transitions from the T-z = +2 nucleus Ca-44 to the T-z = +1 nucleus Sc-44, where T-z is the z component of isospin T, we performed the (p, n)-type (He-3, t) charge-exchange (CE) reaction at 140 MeV/nucleon and the scattering angles 0 degrees and 2.5 degrees. An energy resolution of 28 keV, that was realized by applying matching techniques to the magnetic spectrometer system, allowed the study of fragmented states. The GT transition strengths, B(GT), were derived up to the excitation energy (E-x) of 13.7 MeV assuming the proportionality between cross sections and B(GT) values. The total sum of B(GT) values in discrete states was 3.7, which was 31% of the sum-rule-limit value of 12. Shell model calculations using the GXPF1J interaction could reproduce the gross features of the experimental B(GT) distribution, but not the fragmentation of the strength. By introducing the concepts of isospin, properties of isospin analogous transitions and states were investigated. (i) Assuming isospin symmetry, the T-z = +2 -> +1 and T-z = -2 -> -1 mirror GT transitions should have the same properties, where the latter can be studied in the beta decay of Cr-44 to V-44. First, we confirmed that the beta-decay half-life T-1/2 of Cr-44 can be reproduced using the B(GT) distribution from the Ca-44(He-3, t) measurement. Then, the 0 degrees, (3He, t) spectrum was modified to deduce the “beta-decay spectrum” and it was compared with the delayed-proton spectrum from the Cr-44 beta decay. The two spectra were mostly in agreement for the GT excitations, but suppression of the proton decay was found for the T = 2 isobaric analog state (IAS). (ii) Starting from the T = 2 ground state of 44Ca, the (3He, t) can excite GT states (state populated by GT transitions) with T = 1, 2, and 3. On the other hand, the Ca-44(p, p') reaction can excite spin-M1 states (states populated by spin-M1 transitions) with T = 2 and 3 that are analogous to the T = 2 and 3 GT states, respectively. By comparing the spectra from these two reactions, a T value of 2 is suggested for several GT states in the E-x = 11.5-13.7 MeV region. (iii) It has been suggested that the T = 2, J(pi) = 0(+) double isobaric analog state (DIAS) at 9.338 MeV in the T-z = 0 nucleus Ti-44 forms an isospin-mixed doublet with a subsidiary 0(+) state at 9.298 MeV. Since no corresponding state was found in the T-z = +1 nucleus Sc-44, we suggest T = 0 for the subsidiary state.
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Denis Bacelar, A. M. et al, Algora, A., Molina, F., & Rubio, B. (2013). The population of metastable states as a probe of relativistic-energy fragmentation reactions. Phys. Lett. B, 723(4-5), 302–306.
Abstract: Isomeric ratios have been measured for high-spin states in Po-198,200,206,208(84), At-208,209,210,211(85), Rn-210,211,212,213,214(86), Fr-208,211,212,213,214(87), Ra-210,211,212,214,215(88), and Ac-215(89) following the projectile fragmentation of a 1 AGeV U-238 beam by a Be-9 target at GSI Helmholtzzentrum fur Schwerionenforschung. The fragments were separated in the fragment separator (FRS) and identified by means of energy loss and time-of-flight techniques. They were brought to rest at the centre of the RISING gamma-ray detector array and intensities of gamma rays emitted in the decay of isomeric states with half-lives between 100 ns and 40 μs and spin values up to 55/2 (h) over bar were used to obtain the corresponding isomeric ratios. The data are compared to theoretical isomeric ratios calculated in the framework of the abrasion-ablation model. Large experimental enhancements are obtained for high-spin isomers in comparison to expected values.
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