Abstract: The structure of Po-208 populated through the EC/beta(+) decay of At-208 is investigated using gamma-ray spectroscopy at the ISOLDE Decay Station. The presented level scheme contains 27 new excited states and 43 new transitions, as well as a further 50 previously observed. rays which have been (re)assigned a position. The level scheme is compared to shell model calculations. Through this analysis approximately half of the beta-decay strength of At-208 is found to proceed via allowed decay and half via first-forbidden decay. The first-forbidden transitions predominantly populate core excited states at high excitation energies, which is qualitatively understood using shell model considerations. This mass region provides an excellent testing ground for the competition between allowed and first-forbidden beta-decay calculations, important for the detailed understanding of the nucleosynthesis of heavy elements.

Abstract: Background: The evolution of shell structure around doubly magic exotic nuclei is of great interest in nuclear physics and astrophysics. In the 'southwest' region of Ni-78, the development of deformation might trigger a major shift in our understanding of explosive nucleosynthesis. To this end, new spectroscopic information on key close-lying nuclei is very valuable. Purpose: We intend to measure the isomeric and beta decay of Co-75, with one-proton and two-neutron holes relative to Ni-78, to access new nuclear structure information in Co-75 and its beta-decay daughters Ni-75 and Ni-74. Methods: The nucleus Co-75 is produced in relativistic in-flight fission reactions of U-238 at the Radioactive Ion Beam Factory in the RIKEN Nishina Center. Its isomeric and f decay are studied exploiting the BigRIPS and EURICA setups. Results: We obtain partial beta-decay spectra for Ni-75 and Ni-74, and report a new isomeric transition in Co-75. The energy [E-gamma = 1914(2) keV] and half-life [t(1/2) = 13(6) μs] of the delayed gamma ray lend support for the existence of aJ(pi) = (1/2(-)) isomeric state at 1914(2) keV. A comparison with PFSDG-U shell-model calculations provides a good account for the observed states in Ni-75, but the first calculated 1/2(-) level in Co-75, a prolate K = 1/2 state, is predicted about 1 MeV below the observed (1/2(-)) level. Conclusions: The spherical-like structure of the lowest-lying excited states in Ni-75 is proved. In the case of Co-75, the results suggest that the dominance of the spherical configurations over the deformed ones might be stronger than expected below Ni-78. Further experimental efforts to discern the nature of the J(pi) = (1/2(-)) isomer are necessary.

Abstract: Background: Shape coexistence in the Z approximate to 82 region has been established in mercury, lead, and polonium isotopes. For even-even mercury isotopes with 100 <= N <= 106 multiple fingerprints of this phenomenon are observed, which seems to be no longer present for N >= 110. According to a number of theoretical calculations, shape coexistence is predicted in the Hg-188 isotope. Purpose: The aim of this work was to measure lifetimes of excited states in Hg-188 to infer their collective properties, such as the deformation. Extending the investigation to higher-spin states, which are expected to be less affected by band-mixing effects, can provide additional information on the coexisting structures. Methods: The Hg-188 nucleus was populated using two different fusion-evaporation reactions with two targets, Gd-158 and Gd-160, and a beam of S-34 provided by the Tandem-ALPI accelerator complex at the Laboratori Nazionali di Legnaro. The channels of interest were selected using the information from the Neutron Wall array, while the gamma rays were detected using the GALILEO gamma-ray spectrometer. Lifetimes of excited states were determined using the recoil-distance Doppler-shift method, employing the dedicated GALILEO plunger device. Results: Lifetimes of the states up to spin 16 (h) over bar were measured and the corresponding reduced transition probabilities were calculated. Assuming two-band mixing and adopting, as done commonly, the rotational model, the mixing strengths and the deformation parameters of the unperturbed structures were obtained from the experimental results. In order to shed light on the nature of the observed configurations in the Hg-188 nucleus, the extracted transition strengths were compared with those resulting from state-of-the-art beyond-mean-field calculations using the symmetry-conserving configuration-mixing approach, limited to axial shapes, and the five-dimensional collective Hamiltonian, including the triaxial degree of freedom. Conclusions: The first lifetime measurement for states with spin >= 6 suggested the presence of an almost spherical structure above the 12(1)(+) isomer and allowed elucidating the structure of the intruder band. The comparison of the extracted B(E2) strengths with the two-band mixing model allowed the determination of the ground-state band deformation. Both beyond-mean-field calculations predict coexistence of a weakly deformed band with a strongly prolate-deformed one, characterized by elongation parameters similar to those obtained experimentally, but the calculated relative position of the bands and their mixing strongly differ.

Abstract: The structure of the doubly magic Sn-132(50)82 has been investigated at the ISOLDE facility at CERN, populated both by the beta(-) decay of In-132 and beta(-)-delayed neutron emission of In-133. The level scheme of Sn-13(2) is greatly expanded with the addition of 68 gamma transitions and 17 levels observed for the first time in the beta decay. The information on the excited structure is completed by new gamma transitions and states populated in the beta-n decay of In-133. Improved delayed neutron emission probabilities are obtained both for In-132 and In-133. Level lifetimes are measured via the advanced time-delayed beta gamma gamma(t) fast-timing method. An interpretation of the level structure is given based on the experimental findings and the particle-hole configurations arising from core excitations both from the N = 82 and Z = 50 shells, leading to positive- and negative-parity particle-hole multiplets. The experimental information provides new data to challenge the theoretical description of Sn-132.

Abstract: Decay spectroscopy of the long-lived states in Tl-186 has been performed at the ISOLDE Decay Station at ISOLDE, CERN. The a decay from the low-spin (2(-)) state in Tl-186 was observed for the first time and a half-life of 3.4(-0.)(4)(+0.5) s was determined. Based on the alpha-decay energy, the relative positions of the long-lived states were fixed, with the (2(-)) state as the ground state, the 7((+)) state at 77(56) keV, and the 10((-)) state at 451(56) keV. The level scheme of the internal decay of the Tl-186(10((-))) state [T-1/2 = 3.40(9) s], which was known to decay solely through emission of 374-keV gamma-ray transition, was extended and a lower limit for the beta-decay branching b(beta) > 5.9(3)% was determined. The extracted retardation factors for the gamma decay of the 10((-) )state were compared to the available data in neighboring odd-odd thallium isotopes indicating the importance of the pi d(3/2) shell in the isomeric decay and significant structure differences between Tl-184 and Tl-186.