| Records |
| Author |
Ancilotto, F.; Barranco, M.; Navarro, J.; Pi, M. |
| Title |
A Density Functional Approach to Para-hydrogen at Zero Temperature |
Type |
Journal Article |
| Year |
2016 |
Publication |
Journal of Low Temperature Physics |
Abbreviated Journal |
J. Low Temp. Phys. |
Volume  |
185 |
Issue |
1-2 |
Pages |
26-38 |
| Keywords |
Solid and liquid bulk para-hydrogen; Small para-hydrogen clusters; Density functional theory |
| Abstract |
We have developed a density functional (DF) built so as to reproduce either the metastable liquid or the solid equation of state of bulk para-hydrogen, as derived from quantum Monte Carlo zero temperature calculations. As an application, we have used it to study the structure and energetics of small para-hydrogen clusters made of up to molecules. We compare our results for liquid clusters with diffusion Monte Carlo (DMC) calculations and find a fair agreement between them. In particular, the transition found within DMC between hollow-core structures for small N values and center-filled structures at higher N values is reproduced. The present DF approach yields results for (pH) clusters indicating that for small N values a liquid-like character of the clusters prevails, while solid-like clusters are instead energetically favored for . |
| Address |
[Ancilotto, Francesco] Dipartimento Fis & Astron Galileo Galilei, Padua, Italy, Email: manuel@ecm.ub.edu |
| Corporate Author |
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Thesis |
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| Publisher |
Springer/Plenum Publishers |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
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| ISSN |
0022-2291 |
ISBN |
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Medium |
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| Area |
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Expedition |
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Conference |
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| Notes |
WOS:000382142000003 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ pastor @ |
Serial |
2814 |
| Permanent link to this record |
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| Author |
Fernandez, A.; Hufschmidt, D.; Colaux, J.L.; Valiente-Dobon, J.J.; Godinho, V.; Jimenez de Haro, M.C.; Feria, D.; Gadea, A.; Lucas, S. |
| Title |
Low gas consumption fabrication of He-3 solid targets for nuclear reactions |
Type |
Journal Article |
| Year |
2020 |
Publication |
Materials & Design |
Abbreviated Journal |
Mater. Des. |
| Volume |
186 |
Issue |
|
Pages |
108337 - 10pp |
| Keywords |
He-3 solid targets; Quasistatic magnetron sputtering; Low gas consumption; Nuclear reactions; Inverse kinematics; Target stability |
| Abstract |
Nanoporous solids that stabilize trapped gas nanobubbles open new possibilities to fabricate solid targets for nuclear reactions. A methodology is described based on the magnetron sputtering (MS) technique operated under quasistatic flux conditions to produce such nanocomposites films with He-3 contents of up to 16 at.% in an amorphous-silicon matrix. In addition to the characteristic low pressure (3-6 Pa) needed for the gas discharge, the method ensures almost complete reduction of the process gas flow during film fabrication. The method could produce similar materials to those obtained under classical dynamic flux conditions for MS. The drastic reduction (>99.5%) of the gas consumption is fundamental for the fabrication of targets with scarce and expensive gases. Si:He-3 and W:He-3 targets are presented together with their microstructural (scanning and transmission electron microscopy, SEM and TEM respectively) and compositional (Ion Beam Analysis, IBA) characterization. The He-3 content achieved was over 1 x 10(18) at/cm(2) for film thicknesses between 1.5 and 3 μm for both Si and W matrices. First experiments to probe the stability of the targets for nuclear reaction studies in inverse kinematics configurations are presented. |
| Address |
[Fernandez, Asuncion; Hufschmidt, Dirk; Godinho, Vanda; Jimenez de Haro, Maria C.; Feria, David] Univ Seville, CSIC, Inst Ciencia Mat Sevilla, Avda Amer Vespucio 49, Seville 41092, Spain, Email: asuncion@icmse.csic.es |
| Corporate Author |
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Thesis |
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| Publisher |
Elsevier Sci Ltd |
Place of Publication |
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Editor |
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| Language |
English |
Summary Language |
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Original Title |
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| Series Editor |
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Series Title |
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Abbreviated Series Title |
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| Series Volume |
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Series Issue |
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Edition |
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| ISSN |
0264-1275 |
ISBN |
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Medium |
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| Area |
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Expedition |
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Conference |
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| Notes |
WOS:000505221700053 |
Approved |
no |
| Is ISI |
yes |
International Collaboration |
yes |
| Call Number |
IFIC @ pastor @ |
Serial |
4239 |
| Permanent link to this record |
