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n_TOF Collaboration(Belloni, F. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Neutron-induced fission cross-section of U-233 in the energy range 0.5 < E-n < 20 MeV. Eur. Phys. J. A, 47(1), 2–7pp.
Abstract: The neutron-induced fission cross-section of U-233 has been measured at the CERN nTOF facility relative to the standard fission cross-section of U-235 between 0.5 and 20MeV. The experiment was performed with a fast ionization chamber for the detection of the fission fragments and to discriminate against alpha-particles from the natural radioactivity of the samples. The high instantaneous flux and the low background of the nTOF facility result in data with uncertainties of approximate to 3%, which were found in good agreement with previous experiments. The high quality of the present results allows to improve the evaluation of the U-233(n, f) cross-section and, consequently, the design of energy systems based on the Th/U cycle.
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n_TOF Collaboration(Belloni, F. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Measurement of the neutron-induced fission cross-section of Am-243 relative to U-235 from 0.5 to 20 MeV. Eur. Phys. J. A, 47(12), 160–8pp.
Abstract: The ratio of the neutron-induced fission cross-sections of Am-243 and U-235 was measured in the energy range from 0.5 to 20 MeV with uncertainties of approximate to 4%. The experiment was performed at the CERN n_TOF facility using a fast ionization chamber. With the good counting statistics that could be achieved thanks to the high instantaneous flux and the low backgrounds, the present results are useful for resolving discrepancies in previous data sets and are important for future reactors with improved fuel burn-up.
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Domingo-Pardo, C. (2016). Beta-delayed neutron emission: first measurements in the heavy mass region and future prospects. Acta Phys. Pol. B, 47(3), 729–737.
Abstract: Beta-delayed neutrons play a key role in the formation of heavy elements in explosive stellar environments. The final r-process abundance distribution, including the rare-earth peak, is tailored to a large extent by the neutrons released after the beta decay of very exotic neutron-rich nuclei encountered along the r-process path and during the freeze-out phase. Such scenarios involve a vast amount of – yet undiscovered – nuclei, and most of them are expected to be neutron emitters. In this respect, existing beta-delayed neutron emission data is rather scarce, spanning from the lightest isotopes up to the region of the fission-fragments with masses up to A similar to 150. This contribution gives an overview on the latest measurements of neutron branching ratios in the heavy mass region around N = 126, which was practically unexplored in the past. Present plans to access very exotic nuclei at the RIB-facility of RIKEN in the framework of the BRIKEN project, are presented, together with the expected impact in r-process nucleosynthesis studies.
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AGATA Collaboration(Lalovic, N. et al), Gadea, A., & Domingo-Pardo, C. (2018). Study of isomeric states in Pb-198, Pb-200, Pb-202, Pb-206 and Hg-206 populated in fragmentation reactions. J. Phys. G, 45(3), 035105–27pp.
Abstract: Isomeric states in isotopes in the vicinity of doubly-magic Pb-208 were populated following reactions of a relativistic Pb-208 primary beam impinging on a Be-9 fragmentation target. Secondary beams of Pb-198,Pb-200,Pb-202,Pb-206 and Hg-206 were isotopically separated and implanted in a passive stopper positioned in the focal plane of the GSI Fragment Separator. Delayed gamma rays were detected with the Advanced Gamma Tracking Array (AGATA). Decay schemes were reevaluated and interpreted with shell-model calculations. The momentum-dependent population of isomeric states in the two-nucleon hole nuclei Pb-206/Hg-206 was found to differ from the population of multi neutron-hole isomeric states in Pb-198,Pb-200,Pb-202.
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Jordan, D., Tain, J. L., Algora, A., Agramunt, J., Domingo-Pardo, C., Gomez-Hornillos, M. B., et al. (2013). Measurement of the neutron background at the Canfranc Underground Laboratory LSC. Astropart Phys., 42, 1–6.
Abstract: The energy distribution of the neutron background was measured for the first time at Hall A of the Canfranc Underground Laboratory. For this purpose we used a novel approach based on the combination of the information obtained with six large high-pressure He-3 proportional counters embedded in individual polyethylene blocks of different size. In this way not only the integral value but also the flux distribution as a function of neutron energy was determined in the range from 1 eV to 10 MeV. This information is of importance because different underground experiments show different neutron background energy dependence. The high sensitivity of the setup allowed to measure a neutron flux level which is about four orders of magnitude smaller that the neutron background at sea level. The integral value obtained is Phi(Hall A) = (3.44 +/- 0.35) x 10(-6) cm(-2) s(-1).
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Esposito, R. et al, & Domingo-Pardo, C. (2021). Design of the third-generation lead-based neutron spallation target for the neutron time-of-flight facility at CERN. Phys. Rev. Accel. Beams, 24(9), 093001–17pp.
Abstract: The neutron time-of-flight (n_TOF) facility at the European Laboratory for Particle Physics (CERN) is a pulsed white-spectrum neutron spallation source producing neutrons for two experimental areas: the Experimental Area 1 (EAR1), located 185 m horizontally from the target, and the Experimental Area 2 (EAR2), located 20 m above the target. The target, based on pure lead, is impacted by a high-intensity 20-GeV/c pulsed proton beam. The facility was conceived to study neutron-nucleus interactions for neutron kinetic energies between a few meV to several GeV, with applications of interest for nuclear astrophysics, nuclear technology, and medical research. After the second-generation target reached the end of its lifetime, the facility underwent a major upgrade during CERN's Long Shutdown 2 (LS2, 2019-2021), which included the installation of the new third-generation neutron target. The first- and second-generation targets were based on water-cooled massive lead blocks and were designed focusing on EAR1, since EAR2 was built later. The new target is cooled by nitrogen gas to avoid erosion-corrosion and contamination of cooling water with radioactive lead spallation products. Moreover, the new design is optimized also for the vertical flight path and EAR2. This paper presents an overview of the target design focused on both physics and thermomechanical performance, and includes a description of the nitrogen cooling circuit and radiation protection studies.
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Fougeres, C. et al, & Domingo-Pardo, C. (2023). Search for Na-22 in novae supported by a novel method for measuring femtosecond nuclear lifetimes. Nat. Commun., 14(1), 4536–7pp.
Abstract: Classical novae are thermonuclear explosions in stellar binary systems, and important sources of Al-26 and Na-22. While ? rays from the decay of the former radioisotope have been observed throughout the Galaxy, Na-22 remains untraceable. Its half-life (2.6 yr) would allow the observation of its 1.275 MeV ?-ray line from a cosmic source. However, the prediction of such an observation requires good knowledge of its nucleosynthesis. The Na-22(p, ?)Mg-23 reaction remains the only source of large uncertainty about the amount of Na-22 ejected. Its rate is dominated by a single resonance on the short-lived state at 7785.0(7) keV in Mg-23. Here, we propose a combined analysis of particle-particle correlations and velocity-difference profiles to measure femtosecond nuclear lifetimes. The application of this method to the study of the Mg-23 states, places strong limits on the amount of Na-22 produced in novae and constrains its detectability with future space-borne observatories. The authors report a particle-particle correlation and velocity-difference profile method to measure nuclear lifetime. The results obtained for excited states of 23Mg are used to constrain the production of 22Na in the astrophysical novae explosions.
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Caballero, L., Albiol, F., Corbi Bellot, A., Domingo-Pardo, C., Leganes Nieto, J. L., Agramunt Ros, J., et al. (2018). Gamma-ray imaging system for real-time measurements in nuclear waste characterisation. J. Instrum., 13, P03016–23pp.
Abstract: Acompact, portable and large field-of-viewgamma camera that is able to identify, locate and quantify gamma-ray emitting radioisotopes in real-time has been developed. The device delivers spectroscopic and imaging capabilities that enable its use it in a variety of nuclear waste characterisation scenarios, such as radioactivity monitoring in nuclear power plants and more specifically for the decommissioning of nuclear facilities. The technical development of this apparatus and some examples of its application in field measurements are reported in this article. The performance of the presented gamma-camera is also benchmarked against other conventional techniques.
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Olleros, P., Caballero, L., Domingo-Pardo, C., Babiano, V., Ladarescu, I., Calvo, D., et al. (2018). On the performance of large monolithic LaCl3(Ce) crystals coupled to pixelated silicon photosensors. J. Instrum., 13, P03014–17pp.
Abstract: We investigate the performance of large area radiation detectors, with high energy-and spatial-resolution, intended for the development of a Total Energy Detector with gamma-ray imaging capability, so-called i-TED. This new development aims for an enhancement in detection sensitivity in time-of-flight neutron capture measurements, versus the commonly used C6D6 liquid scintillation total-energy detectors. In this work, we study in detail the impact of the readout photosensor on the energy response of large area (50 x 50 mm(2)) monolithic LaCl3(Ce) crystals, in particular when replacing a conventional mono-cathode photomultiplier tube by an 8 x 8 pixelated silicon photomultiplier. Using the largest commercially available monolithic SiPM array (25 cm(2)), with a pixel size of 6 x 6 mm(2), we have measured an average energy resolution of 3.92% FWHM at 662 keV for crystal thick-nesses of 10, 20 and 30 mm. The results are confronted with detailed Monte Carlo (MC) calculations, where optical processes and properties have been included for the reliable tracking of the scintillation photons. After the experimental validation of the MC model, we use our MC code to explore the impact of a smaller photosensor segmentation on the energy resolution. Our optical MC simulations predict only a marginal deterioration of the spectroscopic performance for pixels of 3 x 3 mm(2).
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BRIKEN Collaboration(Tarifeño-Saldivia, A. et al), Tain, J. L., Domingo-Pardo, C., Agramunt, J., Algora, A., Morales, A. I., et al. (2017). Conceptual design of a hybrid neutron-gamma detector for study of beta-delayed neutrons at the RIB facility of RIKEN. J. Instrum., 12, P04006–22pp.
Abstract: BRIKEN is a complex detection system to be installed at the RIB-facility of the RIKEN Nishina Center. It is aimed at the detection of heavy-ion implants, β-particles, γ-rays and β-delayed neutrons. The whole detection setup involves the Advanced Implantation Detection Array (AIDA), two HPGe Clover detectors and a large set of 166 counters of 3He embedded in a high-density polyethylene matrix. This article reports on a novel methodology developed for the conceptual design and optimisation of the 3He-tubes array, aiming at the best possible performance in terms of neutron detection. The algorithm is based on a geometric representation of two selected parameters of merit, namely, average neutron detection efficiency and efficiency flatness, as a function of a reduced number of geometric variables. The response of the detection system itself, for each configuration, is obtained from a systematic MC-simulation implemented realistically in Geant4. This approach has been found to be particularly useful. On the one hand, due to the different types and large number of 3He-tubes involved and, on the other hand, due to the additional constraints introduced by the ancillary detectors for charged particles and gamma-rays. Empowered by the robustness of the algorithm, we have been able to design a versatile detection system, which can be easily re-arranged into a compact mode in order to maximize the neutron detection performance, at the cost of the gamma-ray sensitivity. In summary, we have designed a system which shows, for neutron energies up to 1(5) MeV, a rather flat and high average efficiency of 68.6%(64%) and 75.7%(71%) for the hybrid and compact modes, respectively. The performance of the BRIKEN system has been also quantified realistically by means of MC-simulations made with different neutron energy distributions.
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