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Algora, A. et al, Valencia, E., Tain, J. L., Jordan, M. D., Agramunt, J., Rubio, B., et al. (2014). Total Absorption Study of Beta Decays Relevant for Nuclear Applications and Nuclear Structure. Nucl. Data Sheets, 120, 12–15.
Abstract: An overview is given of our activities related to the study of the beta decay of neutron rich nuclei relevant for nuclear applications. Recent results of the study of the beta decay of Br-87,Br-88 using a new segmented total absorption spectrometer are presented. The measurements were performed at the IGISOL facility using trap-assisted total absorption spectroscopy.
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Rubio, B. et al, Orrigo, S. E. A., Montaner-Piza, A., Agramunt, J., Algora, A., & Molina, F. (2014). Beta Decay Study of the T-z =-2 Zn-56 Nucleus and the Determination of the Half-Lives of a Few fp-shell Nuclei. Nucl. Data Sheets, 120, 37–40.
Abstract: This paper concerns the experimental study of the beta decay properties of few proton-rich fp-shell nuclei. The nuclei were produced at GANIL in fragmentation reactions, separated with the LISE spectrometer and stopped in an implantation detector surrounded by Ge detectors. The beta-delayed gammas, beta-delayed protons and the exotic beta-delayed gamma-proton emission have been studied. Preliminary results are presented. The decay of the T-z = -2 nucleus Zn-56 has been studied in detail. Information from the beta-delayed protons and beta-delayed gammas has been used to deduce the decay scheme. The exotic beta-delayed gamma-proton decay has been observed for the first time in the fp-shell. The interpretation of the data was made possible thanks to the detailed knowledge of the mirror Charge Exchange (CE) process and the gamma de-excitation of the states in Co-56, the mirror nucleus of Cu-56.
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Goigoux, T. et al, Algora, A., Guadilla, V., Montaner-Piza, A., Morales, A. I., Orrigo, S. E. A., et al. (2016). Two-Proton Radioactivity of Kr-67. Phys. Rev. Lett., 117(16), 162501–6pp.
Abstract: In an experiment with the BigRIPS separator at the RIKEN Nishina Center, we observed two-proton (2p) emission from Kr-67. At the same time, no evidence for 2p emission of Ge-59 and Se-63, two other potential candidates for this exotic radioactivity, could be observed. This observation is in line with Q value predictions which pointed to Kr-67 as being the best new candidate among the three for two-proton radioactivity. Kr-67 is only the fourth 2p ground-state emitter to be observed with a half-life of the order of a few milliseconds. The decay energy was determined to be 1690(17) keV, the 2p emission branching ratio is 37(14)%, and the half-life of Kr-67 is 7.4(30) ms.
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Lorusso, G. et al, & Montaner-Piza, A. (2015). beta-Decay Half-Lives of 110 Neutron-Rich Nuclei across the N=82 Shell Gap: Implications for the Mechanism and Universality of the Astrophysical r Process. Phys. Rev. Lett., 114(19), 192501–7pp.
Abstract: The beta-decay half-lives of 110 neutron-rich isotopes of the elements from 37 Rb to 50 Sn were measured at the Radioactive Isotope Beam Factory. The 40 new half-lives follow robust systematics and highlight the persistence of shell effects. The new data have direct implications for r-process calculations and reinforce the notion that the second (A approximate to 130) and the rare-earth-element (A approximate to 160) abundance peaks may result from the freeze-out of an (n, gamma) reversible arrow (gamma, n) equilibrium. In such an equilibrium, the new half-lives are important factors determining the abundance of rare-earth elements, and allow for a more reliable discussion of the r process universality. It is anticipated that universality may not extend to the elements Sn, Sb, I, and Cs, making the detection of these elements in metal-poor stars of the utmost importance to determine the exact conditions of individual r-process events.
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Watanabe, H. et al, & Montaner-Piza, A. (2014). Monopole-Driven Shell Evolution below the Doubly Magic Nucleus Sn-132 Explored with the Long-Lived Isomer in Pd-126. Phys. Rev. Lett., 113(4), 042502–6pp.
Abstract: A new isomer with a half-life of 23.0(8) ms has been identified at 2406 keV in Pd-126 and is proposed to have a spin and parity of 10(+) with a maximally aligned configuration comprising two neutron holes in the 1h(11/2) orbit. In addition to an internal-decay branch through a hindered electric octupole transition, beta decay from the long-lived isomer was observed to populate excited states at high spins in Ag-126. The smaller energy difference between the 10(+) and 7(-) isomers in Pd-126 than in the heavier N = 80 isotones can be interpreted as being ascribed to the monopole shift of the 1h(11/2) neutron orbit. The effects of the monopole interaction on the evolution of single-neutron energies below Sn-132 are discussed in terms of the central and tensor forces.
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Simpson, G. S. et al, & Montaner-Piza, A. (2014). Yrast 6(+) Seniority Isomers of Sn-136,Sn-138. Phys. Rev. Lett., 113(13), 132502–6pp.
Abstract: Delayed gamma-ray cascades, originating from the decay of (6(+)) isomeric states, in the very neutron-rich, semimagic isotopes Sn-136,Sn-138 have been observed following the projectile fission of a U-238 beam at RIBF, RIKEN. The wave functions of these isomeric states are proposed to be predominantly a fully aligned pair of f(7/2) neutrons. Shell-model calculations, performed using a realistic effective interaction, reproduce well the energies of the excited states of these nuclei and the measured transition rates, with the exception of the B(E2; 6(+) -> 4(+)) rate of Sn-136, which deviates from a simple seniority scheme. Empirically reducing the nu f(7/2)(2) orbit matrix elements produces a 4(1)(+) state with almost equal seniority 2 and 4 components, correctly reproducing the experimental B(E2; 6(+) -> 4(+)) rate of Sn-136. These data provide a key benchmark for shell-model interactions far from stability.
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Taprogge, J. et al, Gadea, A., & Montaner-Piza, A. (2014). 1p(3/2) Proton-Hole State in Sn-132 and the Shell Structure Along N=82. Phys. Rev. Lett., 112(13), 132501–6pp.
Abstract: A low-lying state in In-131(82), the one-proton hole nucleus with respect to double magic Sn-132, was observed by its gamma decay to the I-pi 1/2(-) beta-emitting isomer. We identify the new state at an excitation energy of E-x = 1353 keV, which was populated both in the beta decay of Cd-131(83) and after beta-delayed neutron emission from Cd-132(84), as the previously unknown pi p(3/2) single-hole state with respect to the Sn-132 core. Exploiting this crucial new experimental information, shell-model calculations were performed to study the structure of experimentally inaccessible N = 82 isotones below Sn-132. The results evidence a surprising absence of proton subshell closures along the chain of N = 82 isotones. The consequences of this finding for the evolution of the N = 82 shell gap along the r-process path are discussed.
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Watanabe, H. et al, & Montaner-Piza, A. (2013). Isomers in Pd-128 and Pd-126: Evidence for a Robust Shell Closure at the Neutron Magic Number 82 in Exotic Palladium Isotopes. Phys. Rev. Lett., 111(15), 152501–5pp.
Abstract: The level structures of the very neutron-rich nuclei Pd-128 and Pd-126 have been investigated for the first time. In the r-process waiting-point nucleus Pd-128, a new isomer with a half-life of 5.8(8) μs is proposed to have a spin and parity of 8(+) and is associated with a maximally aligned configuration arising from the g(9/2) proton subshell with seniority v = 2. For Pd-126, two new isomers have been identified with half-lives of 0.33(4) and 0.44(3) μs. The yrast 2(+) energy is much higher in Pd-128 than in Pd-126, while the level sequence below the 8(+) isomer in Pd-128 is similar to that in the N = 82 isotone Cd-130. The electric quadrupole transition that depopulates the 8(+) isomer in Pd-128 is more hindered than the corresponding transition in Cd-130, as expected in the seniority scheme for a semimagic, spherical nucleus. These experimental findings indicate that the shell closure at the neutron number N = 82 is fairly robust in the neutron-rich Pd isotopes.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2022). Total absorption gamma-ray spectroscopy of the ss decays of Y-96gs,Y-m. Phys. Rev. C, 106(1), 014306–14pp.
Abstract: The ss decays of the ground state (gs) and isomeric state (m) of Y-96 have been studied with the total absorption gamma-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8(+) isomeric state from the 0(-) ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The ss-intensity distributions of both decays have been independently determined. In the analyses the deexcitation of the 1581.6 keV level in Zr-96, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the ss-detector efficiency, influencing the ss-intensity distribution obtained. Our results for Y-96gs (0(-)) confirm the large ground state to ground state ss-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to 96.6(-2.1)(+0.3) % of the total ss intensity. Given that the decay of Y-96gs is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of Y-96m (8(+)), previously undetected ss intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption gamma-ray spectroscopy measurements of ss decays with highly fragmented deexcitation patterns. Y-96m (8(+)) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average ss and gamma energies differ significantly from the previous values in evaluated databases. The discrepancy is far above the previously quoted uncertainties. Finally, we also report on the successful implementation of an innovative total absorption gamma-ray spectroscopy analysis of the module-multiplicity gated spectra, as a first proof of principle to distinguish between decaying states with very different spin-parity values.
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Orrigo, S. E. A. et al, Rubio, B., Gelletly, W., Aguilera, P., Algora, A., Morales, A. I., et al. (2021). beta decay of the very neutron-deficient Ge-60 and Ge-62 nuclei. Phys. Rev. C, 103(1), 014324–12pp.
Abstract: We report here the results of a study of the beta decay of the proton-rich Ge isotopes, Ge-60 and Ge-62, produced in an experiment at the RIKEN Nishina Center. We have improved our knowledge of the half-lives of Ge-62 [73.5(1) ms] and Ge-60 [25.0(3) ms] and its daughter nucleus, Ga-60 [69.4(2) ms]. We measured individual beta-delayed proton and gamma emissions and their related branching ratios. Decay schemes and absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. A total beta-delayed proton-emission branching ratio of 67(3)% has been obtained for Ge-60. New information has been obtained on the energy levels populated in Ga-60 and on the 1/2(-) excited state in the beta p daughter Zn-59. We extracted a ground state-to-ground state feeding of 85.3(3)% for the decay of Ge-62. Eight new y lines have been added to the deexcitation of levels populated in the Ga-62 daughter.
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