Abstract: Neutron capture cross section measurements in time-of-flight facilities are usually performed by detecting the prompt 7-rays emitted in the capture reactions. One of the difficulties to be addressed in these measurements is that the emitted 7-rays may change with the neutron energy, and therefore also the detection efficiency. To deal with this situation, many measurements use the so called Total Energy Detection (TED) technique, usually in combination with the Pulse Height Weighting Technique (PHWT). With it, it is sought that the detection efficiency depends only on the total energy of the 7-ray cascade, which does not vary much with the neutron energy. This technique was developed in the 1960s and has been used in many neutron capture experiments to date. One of the requirements of the technique is that 7-ray detectors have a low efficiency. This has meant that the PHWT has been used with experimental setups with low detection efficiencies. However, this condition does not have to be fulfilled by the experimental system as a whole. The main goal of this work is to show that it is possible to measure with a high efficiency detection system that uses the PHWT, and how to analyze the measured data.

Abstract: This paper presents the design of a total absorption gamma-ray spectrometer for the determination of beta-decay intensity distributions of exotic nuclear species at the focal plane of the FAIR-NUSTAR Super Fragment Separator. The spectrometer is a key instrument in the DESPEC experiment and the proposed implementation follows extensive design studies and prototype tests. Two options were contemplated, based on Nal(TI) and LaBr3:Ce inorganic scintillation crystals respectively. Monte Carlo simulations and technical considerations determined the optimal configurations consisting of sixteen 15 x 15 x 25 cm(3) crystals for the Nal(Tl) option and one hundred and twenty-eight 5.5 x 5.5 x 11 cm(3) crystals for the LaBr3:Ce option. Minimization of dead material was crucial for maximizing the spectrometer full-energy peak efficiency. Module prototypes were build to verify constructional details and characterize their performance. The measured energy and timing resolution was found to agree rather well with estimates based on simulations of scintillation light transport and collection. The neutron sensitivity of the spectrometer, important when measuring beta-delayed neutron emitters, was investigated by means of Monte Carlo simulations.

Abstract: The n_TOF Total Absorption Calorimeter (TAC) is a 4 pi BaF2 segmented detector used at CERN for measuring neutron capture cross-sections of importance for the design of advanced nuclear reactors. This work presents the simulation code that has been developed in GEANT4 for the accurate determination of the detection efficiency of the TAC for neutron capture events. The code allows to calculate the efficiency of the TAC for every neutron capture state, as a function of energy, crystal multiplicity, and counting rate. The code includes all instrumental effects such as the single crystal detection threshold and energy resolution, finite size of the coincidence time window, and signal pile-up. The results from the simulation have been validated with experimental data for a large set of electromagnetic de-excitation patterns: beta-decay of well known calibration sources, neutron capture reactions in light nuclei with well known level schemes like Ti-nat, reference samples used in (n,gamma) measurements like Au-197 and experimental data from an actinide sample like Pu-240. The systematic uncertainty in the determination of the detection efficiency has been estimated for all the cases. As a representative example, the accuracy reached for the case of Au-197(n,gamma) ranges between 0.5% and 2%, depending on the experimental and analysis conditions. Such a value matches the high accuracy required for the nuclear cross-section data needed in advanced reactor design.