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Author Mendoza, E.; Alcayne, V.; Cano-Ott, D.; Gonzalez-Romero, E.; Martinez, T.; de Rada, A.P.; Sanchez-Caballero, A.; Balibrea-Correa, J.; Domingo-Pardo, C.; Lerendegui-Marco, J.; Calvino, F.; Guerrero, C.
Title Neutron capture measurements with high efficiency detectors and the Pulse Height Weighting Technique Type Journal Article
Year 2023 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume (down) 1047 Issue Pages 167894 - 16pp
Keywords Neutron capture; Total energy detector; Pulse height weighting technique; 7-ray cascades
Abstract Neutron capture cross section measurements in time-of-flight facilities are usually performed by detecting the prompt 7-rays emitted in the capture reactions. One of the difficulties to be addressed in these measurements is that the emitted 7-rays may change with the neutron energy, and therefore also the detection efficiency. To deal with this situation, many measurements use the so called Total Energy Detection (TED) technique, usually in combination with the Pulse Height Weighting Technique (PHWT). With it, it is sought that the detection efficiency depends only on the total energy of the 7-ray cascade, which does not vary much with the neutron energy. This technique was developed in the 1960s and has been used in many neutron capture experiments to date. One of the requirements of the technique is that 7-ray detectors have a low efficiency. This has meant that the PHWT has been used with experimental setups with low detection efficiencies. However, this condition does not have to be fulfilled by the experimental system as a whole. The main goal of this work is to show that it is possible to measure with a high efficiency detection system that uses the PHWT, and how to analyze the measured data.
Address [Mendoza, E.; Alcayne, V; Cano-Ott, D.; Gonzalez-Romero, E.; Martinez, T.; Perez de Rada, A.; Sanchez-Caballero, A.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain, Email: emilio.mendoza@ciemat.es
Corporate Author Thesis
Publisher Elsevier Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:000908431800002 Approved no
Is ISI yes International Collaboration no
Call Number IFIC @ pastor @ Serial 5468
Permanent link to this record
 

 
Author Chiera, N.M.; Maugeri, E.A.; Danilov, I.; Balibrea-Correa, J.; Domingo-Pardo, C.; Koster, U.; Lerendegui-Marco, J.; Veicht, M.; Zivadinovic, I.; Schumann, D.
Title Preparation of PbSe targets for Se-79 neutron capture cross section studies Type Journal Article
Year 2022 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume (down) 1029 Issue Pages 166443 - 7pp
Keywords Lead selenide; Selenium-79; Neutron capture; PbSe target; Se separation
Abstract A methodology for the production of PbSe targets for Se-79 neutron capture cross section studies is presented. PbSe material was synthesized by direct reaction of its constituents at high temperature, and characterized by X-ray diffraction. Thin PbSe targets, produced for cross section experiments with the surrogate reaction method, were obtained by applying a physical vapor deposition technique, and their morphology and composition were analyzed by X-ray fluorescence, Scanning Electron Microscopy, and Energy dispersive X-ray spectroscopy. (PbSe)-Se-79 targets produced for cross section measurements with the Time of Flight method were characterized by gamma-ray spectroscopy. Finally, a procedure for the recovery of Se from PbSe is suggested. The purity of the retrieved Se was determined with Inductively Coupled Plasma Optical Emission Spectroscopy.
Address [Chiera, Nadine M.; Maugeri, Emilio Andrea; Danilov, Ivan; Veicht, Mario; Zivadinovic, Ivan; Schumann, Dorothea] Paul Scherrer Inst, Villigen, Switzerland, Email: nadine-mariel.chiera@psi.ch
Corporate Author Thesis
Publisher Elsevier Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:000783012200016 Approved no
Is ISI yes International Collaboration no
Call Number IFIC @ pastor @ Serial 5204
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Author Balibrea-Correa, J.; Lerendegui-Marco, J.; Babiano-Suarez, V.; Caballero, L.; Calvo, D.; Ladarescu, I.; Olleros-Rodriguez, P.; Domingo-Pardo, C.
Title Machine Learning aided 3D-position reconstruction in large LaCl3 crystals Type Journal Article
Year 2021 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume (down) 1001 Issue Pages 165249 - 17pp
Keywords Gamma-ray; Position sensitive detectors; Monolithic crystals; Compton imaging; Machine Learning; Convolutional Neural Networks; Total Energy Detector; Neutron capture cross-section
Abstract We investigate five different models to reconstruct the 3D gamma-ray hit coordinates in five large LaCl3(Ce) monolithic crystals optically coupled to pixelated silicon photomultipliers. These scintillators have a base surface of 50 x 50 mm(2) and five different thicknesses, from 10 mm to 30 mm. Four of these models are analytical prescriptions and one is based on a Convolutional Neural Network. Average resolutions close to 1-2 mm fwhm are obtained in the transverse crystal plane for crystal thicknesses between 10 mm and 20 mm using analytical models. For thicker crystals average resolutions of about 3-5 mm fwhm are obtained. Depth of interaction resolutions between 1 mm and 4 mm are achieved depending on the distance of the interaction point to the photosensor surface. We propose a Machine Learning algorithm to correct for linearity distortions and pin-cushion effects. The latter allows one to keep a large field of view of about 70%-80% of the crystal surface, regardless of crystal thickness. This work is aimed at optimizing the performance of the so-called Total Energy Detector with Compton imaging capability (i-TED) for time-of-flight neutron capture cross-section measurements.
Address [Balibrea-Correa, J.; Lerendegui-Marco, J.; Babiano-Suarez, V.; Caballero, L.; Calvo, D.; Ladarescu, I.; Olleros-Rodriguez, P.; Domingo-Pardo, C.] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia, Spain, Email: javier.balibrea@ific.uv.es
Corporate Author Thesis
Publisher Elsevier Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:000641308300007 Approved no
Is ISI yes International Collaboration no
Call Number IFIC @ pastor @ Serial 4803
Permanent link to this record
 

 
Author Balibrea-Correa, J.; Lerendegui-Marco, J.; Calvo, D.; Caballero, L.; Babiano, V.; Ladarescu, I.; Redondo, M.L.; Tain, J.L.; Tolosa, A.; Domingo-Pardo, C.; Calvino, F.; Casanovas, A.; Tarifeño-Saldivia, A.; Alcayne, V.; Cano-Ott, D.; Martinez, T.; Guerrero, C.; Barbagallo, M.; Macina, D.; Bacak, M.
Title A first prototype of C6D6 total-energy detector with SiPM readout for neutron capture time-of-flight experiments Type Journal Article
Year 2021 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume (down) 985 Issue Pages 164709 - 8pp
Keywords Silicon photomultiplier; Radiation detectors; Time-of-flight; Radiative capture; Total energy detector; Pulse-height weighting technique
Abstract Low efficiency total-energy detectors (TEDs) are one of the main tools for neutron capture cross section measurements utilizing the time-of-flight (TOF) technique. State-of-the-art TEDs are based on a C6D6 liquid-scintillation cell optically coupled to a fast photomultiplier tube. The large photomultiplier tube represents yet a significant contribution to the so-called neutron sensitivity background, which is one of the most conspicuous sources of uncertainty in this type of experiments. Here we report on the development of a first prototype of a TED based on a silicon-photomultiplier (SiPM) readout, thus resulting in a lightweight and much more compact detector. Apart from the envisaged improvement in neutron sensitivity, the new system uses low voltage (+28 V) and low current supply (-50 mA), which is more practical than the-kV supply required by conventional photomultipliers. One important difficulty hindering the earlier implementation of SiPM readout for this type of detector was the large capacitance for the output signal when all pixels of a SiPM array are summed together. The latter leads to long pulse rise and decay times, which are not suitable for time-of-flight experiments. In this work we demonstrate the feasibility of a Schottky-diode multiplexing readout approach, that allows one to preserve the excellent timing properties of SiPMs, hereby paving the way for their implementation in future neutron TOF experiments.
Address [Balibrea-Correa, J.; Lerendegui-Marco, J.; Calvo, D.; Caballero, L.; Babiano, V; Ladarescu, I; Redondo, M. Lopez; Tain, J. L.; Tolosa, A.; Domingo-Pardo, C.] Univ Valencia, Inst Fis Corpuscular, CSIC, Valencia, Spain, Email: dacaldia@ific.uv.es;
Corporate Author Thesis
Publisher Elsevier Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:000592358200019 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 4638
Permanent link to this record
 

 
Author Magan, D.L.P.; Caballero, L.; Domingo-Pardo, C.; Agramunt-Ros, J.; Albiol, F.; Casanovas, A.; Gonzalez, A.; Guerrero, C.; Lerendegui-Marco, J.; Tarifeño-Saldivia, A.
Title First tests of the applicability of gamma-ray imaging for background discrimination in time-of-flight neutron capture measurements Type Journal Article
Year 2016 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume (down) 823 Issue Pages 107-119
Keywords Neutron capture cross-sections; gamma-ray imaging; Total energy detectors; Pulse-height weighting technique; Time-of-flight method
Abstract In this work we explore for the first time the applicability of using gamma-ray imaging in neutron capture measurements to identify and suppress spatially localized background. For this aim, a pinhole gamma camera is assembled, tested and characterized in terms of energy and spatial performance. It consists of a monolithic CeBr3 scintillating crystal coupled to a position-sensitive photomultiplier and readout through an integrated circuit AMIC2GR. The pinhole collimator is a massive carven block of lead. A series of dedicated measurements with calibrated sources and with a neutron beam incident on a Au-197 sample have been carried out at n_TOF, achieving an enhancement of a factor of two in the signal-to-background ratio when selecting only those events coming from the direction of the sample.
Address [Perez Magan, D. L.; Caballero, L.; Domingo-Pardo, C.; Agramunt-Ros, J.; Albiol, F.; Tarifeno-Saldivia, A.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain, Email: domingo@ific.uv.es
Corporate Author Thesis
Publisher Elsevier Science Bv Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:000374661600015 Approved no
Is ISI yes International Collaboration no
Call Number IFIC @ pastor @ Serial 2665
Permanent link to this record
 

 
Author Guerrero, C.; Tessler, M.; Paul, M.; Lerendegui-Marco, J.; Heinitz, S.; Maugeri, E.A.; Domingo-Pardo, C.; Dressler, R.; Halfon, S.; Kivel, N.; Koster, U.; Palchan-Hazan, T.; Quesada, J.M.; Schumann, D.; Weissman, L.
Title The s-process in the Nd-Pm-Sm region: Neutron activation of Pm-147 Type Journal Article
Year 2019 Publication Physics Letters B Abbreviated Journal Phys. Lett. B
Volume (down) 797 Issue Pages 134809 - 6pp
Keywords Nucleosynthesis; Neutron capture; Nuclear reactions; s-process; MACS; Neutron activation
Abstract The Nd-Pm-Sm branching is of interest for the study of the s-process, related to the production of heavy elements in stars. As Sm-148 and Sm-150 are s-only isotopes, the understanding of the branching allows constraining the s-process neutron density. In this context the key physics input needed is the cross section of the three unstable nuclides in the region: Nd-147 (10.98 d half-life), Pm-147 (2.62 yr) and Pm-148 (5.37 d). This paper reports on the activation measurement of Pm-147, the longest-lived of the three nuclides. The cross section measurement has been carried out by activation at the SARAF LiLiT facility using a 56(2) μg target. Compared to the single previous measurement of Pm-147, the measurement presented herein benefits from a target 2000 times more massive. The resulting Maxwellian Averaged Cross Section (MACS) to the ground and metastable states in Pm-148 are 469(50) mb and 357(27) mb. These values are 41% higher (to the ground state) and 15% lower (to the metastable state) than the values reported so far, leading however to a total cross section of 826(107) mb consistent within uncertainties with the previous result and hence leaving unchanged the previous calculation of the s-process neutron density.
Address [Guerrero, C.; Lerendegui-Marco, J.; Quesada, J. M.] Univ Seville, Seville, Spain, Email: cguerrero4@us.es
Corporate Author Thesis
Publisher Elsevier Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0370-2693 ISBN Medium
Area Expedition Conference
Notes WOS:000488071200026 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 4161
Permanent link to this record
 

 
Author n_TOF Collaboration (Alcayne, V. et al); Balibrea-Correa, J.; Domingo-Pardo, C.; Lerendegui-Marco, J.; Babiano-Suarez, V.; Ladarescu, I.
Title A Segmented Total Energy Detector (sTED) optimized for (n,γ) cross-section measurements at n_TOF EAR2 Type Journal Article
Year 2024 Publication Radiation Physics and Chemistry Abbreviated Journal Radiat. Phys. Chem.
Volume (down) 217 Issue Pages 11pp
Keywords Neutron capture; PHWT; Scintillation detectors; Monte Carlo simulation
Abstract The neutron time-of-flight facility nTOF at CERN is a spallation source dedicated to measurements of neutroninduced reaction cross-sections of interest in nuclear technologies, astrophysics, and other applications. Since 2014, Experimental ARea 2 (EAR2) is operational and delivers a neutron fluence of similar to 4 center dot 10(7) neutrons per nominal proton pulse, which is similar to 50 times higher than the one of Experimental ARea 1 (EAR1) of similar to 8 center dot 10(5) neutrons per pulse. The high neutron flux at EAR2 results in high counting rates in the detectors that challenged the previously existing capture detection systems. For this reason, a Segmented Total Energy Detector (sTED) has been developed to overcome the limitations in the detector's response, by reducing the active volume per module and by using a photo-multiplier (PMT) optimized for high counting rates. This paper presents the main characteristics of the sTED, including energy and time resolution, response to gamma-rays, and provides as well details of the use of the Pulse Height Weighting Technique (PHWT) with this detector. The sTED has been validated to perform neutron-capture cross-section measurements in EAR2 in the neutron energy range from thermal up to at least 400 keV. The detector has already been successfully used in several measurements at nTOF EAR2.
Address [Alcayne, V.; Cano-Ott, D.; Garcia, J.; Gonzalez-Romero, E.; Martinez, T.; de Rada, A. Perez; Plaza, J.; Sanchez-Caballero, A.; Mendoza, E.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain, Email: victor.alcayne@ciemat.es
Corporate Author Thesis
Publisher Pergamon-Elsevier Science Ltd Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0969-806x ISBN Medium
Area Expedition Conference
Notes WOS:001185584800001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5999
Permanent link to this record
 

 
Author Balibrea-Correa, J.; Lerendegui-Marco, J.; Ladarescu, I.; Guerrero, C.; Rodriguez-Gonzalez, T.; Jimenez-Ramos, M.C.; Fernandez-Martinez, B.; Domingo-Pardo, C.
Title Hybrid in-beam PET- and Compton prompt-gamma imaging aimed at enhanced proton-range verification Type Journal Article
Year 2022 Publication European Physical Journal Plus Abbreviated Journal Eur. Phys. J. Plus
Volume (down) 137 Issue 11 Pages 1258 - 18pp
Keywords
Abstract We report on a hybrid in-beam PET and prompt-gamma Compton imaging system aimed at quasi real-time ion-range verification in proton-therapy treatments. Proof-of-concept experiments were carried out at the radiobiology beam line of the CNA cyclotron facility using a set of two synchronous Compton imagers and different target materials. The time structure of the 18 MeV proton beam was shaped with a series of beam-on and beam-off intervals, thereby mimicking a pulsed proton beam on a long time scale. During beam-on intervals, Compton imagingwas performed utilizing the high energy. -rays promptly emitted from the nuclear reactions occurring in the targets. In the course of the beam-off intervals in situ positron-emission tomography was accomplished with the same imagers using the beta+ decay of activated nuclei. The targets used were stacks of different materials covering also various proton ranges and energies. A systematic study on the performance of these two complementary imaging techniques is reported and the experimental results interpreted on the basis ofMonte Carlo calculations. The results demonstrate the possibility to combine both imaging techniques in a concomitant way, where high-efficiency prompt-gamma imaging is complemented with the high spatial accuracy of PET. Empowered by these results we suggest that a pulsed beam with a suitable duty cycle, in conjunction with in situ Compton- and PET-imaging may help to attain complementary information and quasi real-time range monitoring with high accuracy.
Address [Balibrea-Correa, J.; Lerendegui-Marco, J.; Ladarescu, I; Domingo-Pardo, C.] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia, Spain, Email: javier.balibrea@ific.uv.es
Corporate Author Thesis
Publisher Springer Heidelberg Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2190-5444 ISBN Medium
Area Expedition Conference
Notes WOS:000886327900002 Approved no
Is ISI yes International Collaboration no
Call Number IFIC @ pastor @ Serial 5420
Permanent link to this record
 

 
Author n_TOF Collaboration (Lerendegui-Marco, J. et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility Type Journal Article
Year 2018 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume (down) 97 Issue 2 Pages 024605 - 21pp
Keywords
Abstract The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA.
Address [Lerendegui-Marco, J.; Guerrero, C.; Quesada, J. M.; Cortes-Giraldo, M. A.; Praena, J.; Sabate-Gilarte, M.] Univ Seville, Dept Fis Atom Mol & Nucl, E-41012 Seville, Spain, Email: cguerrero4@us.es
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000424190700001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3474
Permanent link to this record
 

 
Author n_TOF Collaboration (Domingo-Pardo, C. et al); Babiano-Suarez, V.; Balibrea-Correa, J.; Caballero, L.; Ladarescu, I.; Lerendegui-Marco, J.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Advances and new ideas for neutron-capture astrophysics experiments at CERN n_TOF Type Journal Article
Year 2023 Publication European Physical Journal A Abbreviated Journal Eur. Phys. J. A
Volume (down) 59 Issue 1 Pages 8 - 11pp
Keywords
Abstract This article presents a few selected developments and future ideas related to the measurement of (n, gamma ) data of astrophysical interest at CERN n_TOF. The MC-aided analysis methodology for the use of low-efficiency radiation detectors in time-of-flight neutron-capture measurements is discussed, with particular emphasis on the systematic accuracy. Several recent instrumental advances are also presented, such as the development of total-energy detectors with gamma- ray imaging capability for background suppression, and the development of an array of small-volume organic scintilla tors aimed at exploiting the high instantaneous neutron-flux of EAR2. Finally, astrophysics prospects related to the intermediate i neutron-capture process of nucleosynthesis are discussed in the context of the new NEAR activation area.
Address [Domingo-Pardo, C.; Babiano-Suarez, V.; Balibrea-Correa, J.; Caballero, L.; Ladarescu, I.; Lerendegui-Marco, J.; Tain, J. L.; Tarifeno-Saldivia, A.] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia, Spain, Email: domingo@ific.uv.es
Corporate Author Thesis
Publisher Springer Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1434-6001 ISBN Medium
Area Expedition Conference
Notes WOS:000926364900001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5479
Permanent link to this record