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n_TOF Collaboration(Mendoza, E. et al), Giubrone, G., & Tain, J. L. (2011). Improved Neutron Capture Cross Section Measurements with the n_TOF Total Absorption Calorimeter. J. Korean Phys. Soc., 59(2), 1813–1816.
Abstract: The n_TOF collaboration operates a Total Absorption Calorimeter (TAC) [1] for measuring neutron capture cross-sections of low-mass and/or radioactive samples. The results obtained with the TAC have led to a substantial improvement of the capture cross sections of (237)Np and (240)Pu [2]. The experience acquired during the first measurements has allowed us to optimize the performance of the TAC and to improve the capture signal to background ratio, thus opening the way to more complex and demanding measurements on rare radioactive materials. The new design has been reached by a series of detailed Monte Carlo simulations of complete experiments and dedicated test measurements. The new capture setup will be presented and the main achievements highlighted.
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n_TOF Collaboration(Tarrio, D. et al), Domingo-Pardo, C., Plag, R., Plompen, A., & Tain, J. L. (2011). High-energy Neutron-induced Fission Cross Sections of Natural Lead and Bismuth-209. J. Korean Phys. Soc., 59(2), 1904–1907.
Abstract: The CERN Neutron Time-Of-Flight (n_TOF) facility is well suited to measure small neutron-induced fission cross sections, as those of subactinides. The cross section ratios of (nat)Pb and (209)Bi relative to (235)U and (238)U were measured using PPAC detectors. The fragment coincidence method allows to unambiguously identify the fission events. The present experiment provides the first results for neutron-induced fission up to 1 GeV for (nat)Pb and (209)Bi. A good agreement with previous experimental data below 200 MeV is shown. The comparison with proton-induced fission indicates that the limiting regime where neutron-induced and proton-induced fission reach equal cross section is close to 1 GeV.
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n_TOF Collaboration(Paradela, C. et al), Domingo-Pardo, C., Plag, R., Plompen, A., & Tain, J. L. (2011). (237)Np(n,f) Cross Section: New Data and Present Status. J. Korean Phys. Soc., 59(2), 1908–1911.
Abstract: In this document, we present the final result obtained at the nTOF experiment; for the neutron-induced fission cross section of the (237)Np, from the fission threshold up to 1 GeV. The method applied to get tins result is briefly discussed. nTOF data are compared to the last experimental measurements using other TOF facilities or the surrogate method, reported experiments performed with monoenergetic sources and the FISCAL systematic, including a discussion about the existing discrepancies.
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n_TOF Collaboration(Calviani, M. et al), Domingo-Pardo, C., & Tain, J. L. (2011). Fission Cross-section Measurements of (233)U, (245)Cm and (241,243)Am at CERN n_TOF Facility. J. Korean Phys. Soc., 59(2), 1912–1915.
Abstract: Neutron-induced fission cross-sections of minor actinides have been measured using the nTOF white neutron source at CERN. Geneva, as part of a large experimental program aiming at collecting new data relevant for nuclear astrophysics and for the design of advanced reactor systems. The measurements at nTOF take advantage of the innovative features of the n_TOF facility, namely the wide energy range, high instantaneous neutron flux and good energy resolution. Final results on the fission cross-section of (233)U, (245)cm and (243)Am from thermal to 20 MeV are here reported, together with preliminary results for (241)Am. The measurement have been performed with a dedicated Fast Ionization Chamber (FIC), a fission fragment detector with a very high efficiency, relative to the very well known cross-section of (235)U, measured simultaneously with the same detector.
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n_TOF Collaboration(Giubrone, G. et al), & Tain, J. L. (2011). The Role of Fe and Ni for S-process Nucleosynthesis and Innovative Nuclear Technologies. J. Korean Phys. Soc., 59(2), 2106–2109.
Abstract: The accurate measurement of neutron capture cross sections of all Fe and Ni isotopes is important for disentangling the contribution of the s-process and the r-process to the stellar nucleosynthesis of elements in the mass range 60 < A < 120. At the same time, Fe and Ni are important components of structural materials and improved neutron cross section data is relevant in the design of new nuclear systems. With the aim of obtaining improved capture data on all stable iron and nickel isotopes, a program of measurements has been launched at the CERN Neutron Time of Flight Facility n_TOF.
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n_TOF Collaboration(Domingo-Pardo, C. et al), Babiano-Suarez, V., Balibrea-Correa, J., Caballero, L., Ladarescu, I., Lerendegui-Marco, J., et al. (2023). Advances and new ideas for neutron-capture astrophysics experiments at CERN n_TOF. Eur. Phys. J. A, 59(1), 8–11pp.
Abstract: This article presents a few selected developments and future ideas related to the measurement of (n, gamma ) data of astrophysical interest at CERN n_TOF. The MC-aided analysis methodology for the use of low-efficiency radiation detectors in time-of-flight neutron-capture measurements is discussed, with particular emphasis on the systematic accuracy. Several recent instrumental advances are also presented, such as the development of total-energy detectors with gamma- ray imaging capability for background suppression, and the development of an array of small-volume organic scintilla tors aimed at exploiting the high instantaneous neutron-flux of EAR2. Finally, astrophysics prospects related to the intermediate i neutron-capture process of nucleosynthesis are discussed in the context of the new NEAR activation area.
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Nichols, A. L., Dimitriou, P., Algora, A., Fallot, M., Giot, L., Kondev, F. G., et al. (2023). Improving fission-product decay data for reactor applications: part I-decay heat. Eur. Phys. J. A, 59(4), 78–78pp.
Abstract: Effort has been expended to assess the relative merits of undertaking further decay-data measurements of the main fission-product contributors to the decay heat of neutron-irradiated fissionable fuel and related actinides by means of Total Absorption Gamma-ray Spectroscopy (TAGS – sometimes abbreviated to TAS) and Discrete Gamma-ray Spectroscopy (DGS). This review has been carried out following similar work performed under the auspices of OECD/WPEC-Subgroup 25 (2005-2007) and the International Atomic Energy Agency (2009, 2014), and various highly relevant TAGS measurements completed as a consequence of such assessments. We present our recommendations for new decay-data evaluations, along with possible requirements for total absorption and discrete high-resolution gamma-ray spectroscopy studies that cover approximately 120 fission products and various isomeric states.
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Tagliente, G. et al, Babiano-Suarez, V., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2024). High-resolution cross section measurements for neutron interactions on 89Y with incident neutron energies up to 95 keV. Eur. Phys. J. A, 60(1), 21–18pp.
Abstract: The cross section of the Y-89(n,gamma) reaction has important implications in nuclear astrophysics and for advanced nuclear technology. Given its neutron magic number N = 50 and a consequent small neutron capture crosssection,89Y represents one of the key nuclides for the stellars-process. It acts as a bottleneck in the neutron capture chain between the Fe seed and the heavier elements. Moreover, it is located at the overlapping region, where both the weak and mains-process components take place.Y-89, the only stable yttrium isotope, is also used in innovative nuclear reactors. Neutron capture and transmission measurements were per-formed at the time-of-flight facilities n_TOF at CERN and GELINA at JRC-Geel. Resonance parameters of individual resonances were extracted from a resonance analysis of the experimental transmission and capture yields, up to a neutron incident energy of 95 keV. Even though a comparison with results reported in the literature shows differences in resonance parameters, the present data are consistent with the Maxwellian averaged cross section suggested by the astro-physical database KADoNiS.
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n_TOF Collaboration(Wright, T. et al), Domingo-Pardo, C., & Tain, J. L. (2024). Measurement of the prompt fission γ-rays from slow neutron-induced fission of 235U with STEFF. Eur. Phys. J. A, 60(3), 70–11pp.
Abstract: The amount of energy carried by gamma-rays during the fission process is an important consideration when developing new reactor designs. Many studies of gamma-ray energy and multiplicity, from a multitude of fissioning systems, were measured during the 1970s. However the data from such experiments largely underestimates the heating effect caused by gamma-rays in the structure of a reactor. It is therefore essential to obtain more accurate measurements of the energy carried during gamma-ray emission. As such, the OECD Nuclear Energy Agency has put out a high priority request [1] for measurements of the mean gamma-ray energy and multiplicity to an accuracy better than 7.5 percent from several fissioning systems; including U-235(n(thermal)). Measurements of the rays from these fissioning nuclei were performed with the SpecTrometer for Exotic Fission Fagments (STEFF).
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n_TOF Collaboration(Tagliente, G. et al.), Domingo-Pardo, C., & Tain, J. L. (2010). The Zr-92(n,gamma) reaction and its implications for stellar nucleosynthesis. Phys. Rev. C, 81(5), 055801–9pp.
Abstract: Because the relatively small neutron capture cross sections of the zirconium isotopes are difficult to measure, the results of previous measurements are often not adequate for a number of problems in astrophysics and nuclear technology. Therefore, the Zr-92(n,gamma) cross section has been remeasured at the CERN n_TOF facility, providing a set of improved parameters for 44 resonances in the neutron energy range up to 40 keV. With this information the cross-section uncertainties in the keV region could be reduced to 5% as required for s-process nucleosynthesis studies and technological applications.
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