Abstract: The beta feeding probability of Tc-102,Tc- 104,Tc- 105,Tc- 106,Tc- 107, Mo-105, and Nb-101 nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the gamma component of the decay heat for Pu-239 in the 4-3000 s range.

Abstract: We measured 135 cross sections of residual nuclei produced in fragmentation reactions of C-12, N-14, and O-13-16,O-20,O-22 projectiles impinging on a carbon target at kinetic energies of near 400A MeV, most of them for the first time, with the R B-3/LAND setup at the GSI facility in Darmstadt (Germany). The use of this state-of-the-art experimental setup in combination with the inverse kinematics technique gave the full identification in atomic and mass numbers of fragmentation residues with a high precision. The cross sections of these residues were determined with uncertainties below 20% for most of the cases. These data are compared to other previous measurements with stable isotopes and are also used to benchmark different model calculations.

Abstract: Background: The mercury isotopes around N = 104 are a well-known example of nuclei exhibiting shape coex-istence. Mixing of configurations can be studied by measuring the monopole strength rho^2(E0), however, currently the experimental information is scarce and lacks precision, especially for the I^pi -> I^pi (I not = 0) transitions. Purpose: The goals of this study were to increase the precision of the known branching ratios and internal conversion coefficients, to increase the amount of available information regarding excited states in 182,184,186Hg, and to interpret the results in the framework of shape coexistence using different models. Method: The low-energy structures in 182,184,186Hg were populated in the & beta; decay of 182,184,186Tl, produced at ISOLDE, CERN and purified by laser ionization and mass separation. The & gamma;-ray and internal conversion electron events were detected by five germanium clover detectors and a segmented silicon detector, respectively, and correlated in time to build decay schemes.Results: In total, 193, 178, and 156 transitions, including 144, 140, and 108 observed for the first time in a & beta;-decay experiment, were assigned to 182,184,186Hg, respectively. Internal conversion coefficients were determined for 23 transitions, out of which 12 had an E0 component. Extracted branching ratios allowed the sign of the interference term in 182Hg as well as & rho;2(E 0; 0+2 & RARR; 0+1 ) and B(E2; 0+2 & RARR; 2+1 ) in 184Hg to be determined. By means of electron-electron coincidences, the 0+3 state was identified in 184Hg. The experimental results were qualitatively reproduced by five theoretical approaches, the interacting boson model with configuration mixing with two different parametrizations, the general Bohr Hamiltonian, the beyond mean-field model, and the symmetry-conserving configuration-mixing model. However, a quantitative description is lacking. Conclusions: The presence of shape coexistence in neutron-deficient mercury isotopes was confirmed and evidence for the phenomenon existing at higher energies was found. The new experimental results provide important spectroscopic input for future Coulomb excitation studies.

Abstract: Treatment planning systems at proton-therapy centres entirely use X-ray computed tomography (CT) as primary imaging technique to infer the proton treatment doses to tumour and healthy tissues. However, proton stopping powers in the body, as derived from X-ray images, suffer from important proton-range uncertainties. In order to reduce this uncertainty in range, one could use proton-CT images instead. The main goal of this work is to test the capabilities of a newly-developed proton-CT scanner, based on the use of a set of tracking detectors and a high energy resolution scintillator for the residual energy of the protons. Different custom-made phantoms were positioned at the field of view of the scanner and were irradiated with protons at the CCB proton-therapy center in Krakow. We measured with the phantoms at different angles and produced sinograms that were used to obtain reconstructed images by Filtered Back-Projection. The obtained images were used to determine the capabilities of our scanner in terms of spatial resolution and proton Relative Stopping Power (RSP) mapping and validate its use as proton-CT scanner. The results show that the scanner can produce medium-high quality images, with spatial resolution better than 2 mm in radiography, below 3 mm in tomography and resolving power in the RSP comparable to other state-of-the-art pCT scanners.

Abstract: The magnetic dipole moments (mu) of Tl-209(g)(N =128) and Tl-207(m)(N = 126) have been measured for the first time using the in -source laser resonance -ionization spectroscopy technique with the Laser Ion Source and Trap (LIST) at ISOLDE (CERN). The application of the LIST suppresses the usually overwhelming background of the isobaric francium isotopes and allows access to heavy thallium isotopes with >207. The self -consistent theory of finite Fermi systems based on the energy density functional by Fayans et al. well describes the N dependence of μfor 1/2(+) thallium ground states, as well as μfor the 11/2(-) isomeric states in europium, gold and thallium isotopes. The inclusion of particle-vibration coupling leads to a better agreement between the theory and experiment for mu(Tl-g , I-pi = 1/2(+)). It is shown that beyond mean-field contributions tocannot be neglected at least for thallium isotopes with I-pi = 1/2(+).