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Author |
n_TOF Collaboration (Torres-Sanchez, P. et al); Babiano-Suarez, V.; Caballero, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L. |
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Title |
Measurement of the 14N(n, p) 14C cross section at the CERN n_TOF facility from subthermal energy to 800 keV |
Type |
Journal Article |
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Year |
2023 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume  |
107 |
Issue |
6 |
Pages |
064617 - 15pp |
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Abstract |
Background: The 14N(n, p) 14C reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where 14N acts as a neutron poison in the s process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region, and resonance region. Purpose: We aim to measure the 14N(n, p) 14C cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and provide calculations of Maxwellian averaged cross sections (MACS). Method: We apply the time-of-flight technique at Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. 10B(n, & alpha;) 7Li and 235U(n, f ) reactions are used as references. Two detection systems are run simultaneously, one on beam and another off beam. Resonances are described with the R-matrix code SAMMY. Results: The cross section was measured from subthermal energy to 800 keV, resolving the first two resonances (at 492.7 and 644 keV). A thermal cross section was obtained (1.809 & PLUSMN; 0.045 b) that is lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations. A 1/v energy dependence of the cross section was confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed determination of the 14N(n, p) cross section over a wide energy range for the first time. We have obtained cross sections with high accuracy (2.5%) from subthermal energy to 800 keV and used these data to calculate the MACS for kT = 5 to kT = 100 keV. |
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Address |
[Torres-Sanchez, Pablo; Praena, Javier; Porras, Ignacio; Ogallar, Francisco] Univ Granada, Granada, Spain, Email: pablotorres@ugr.es |
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Amer Physical Soc |
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2469-9985 |
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Notes |
WOS:001063209900001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5701 |
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Author |
n_TOF Collaboration (Michalopoulou, V. et al); Babiano-Suarez, V.; Caballero, L.; Domingo-Pardo, C.; Ladarescu, I.; Tain, J.L. |
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Title |
Measurement of the neutron-induced fission cross section of Th-230 at the CERN n_TOF facility |
Type |
Journal Article |
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Year |
2023 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
108 |
Issue |
1 |
Pages |
014616 - 15pp |
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Abstract |
The neutron-induced fission cross section of Th-230 has been measured at the neutron time-of-flight facility n_TOF located at CERN. The experiment was performed at the experimental area EAR-1 with a neutron flight path of 185 m, using Micromegas detectors for the detection of the fission fragments. The Th-230(n, f ) cross section was determined relative to the U-235(n, f ) one, covering the energy range from the fission threshold up to 400 MeV. The results from the present work are compared with existing cross-section datasets and the observed discrepancies are discussed and analyzed. Finally, using the code EMPIRE 3.2.3 a theoretical study, based on the statistical model, was performed leading to a satisfactory reproduction of the experimental results with the proper tuning of the respective parameters, while for incident neutron energy beyond 200 MeV the fission of( 230)Th was described by Monte Carlo simulations. |
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Address |
[Michalopoulou, V; Stamatopoulos, A.; Diakaki, M.; Vlastou, R.; Kokkoris, M.; Tassan-Got, L.] Natl Tech Univ Athens, Dept Phys, Zografou Campus, Athens, Greece, Email: veatriki.michalopoulou@cern.ch |
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Amer Physical Soc |
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ISSN |
2469-9985 |
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Conference |
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Notes |
WOS:001063908000001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5700 |
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Author |
Yokoyama, R. et al; Tain, J.L.; Algora, A.; Agramunt, J.; Domingo-Pardo, C.; Morales, A.I.; Rubio, B.; Tolosa-Delgado, A. |
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Title |
β-delayed neutron emissions from N > 50 gallium isotopes |
Type |
Journal Article |
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Year |
2023 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
108 |
Issue |
6 |
Pages |
064307 - 15pp |
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Keywords |
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Abstract |
beta-delayed gamma-neutron spectroscopy has been performed on the decay of A=84 to 87 gallium isotopes at the RI-beam Factory at the RIKEN Nishina Center using a high-efficiency array of 3He neutron counters (BRIKEN). beta-2n-gamma events were measured in the decays of all of the four isotopes for the first time, which is direct evidence for populating the excited states of two-neutron daughter nuclei. Detailed decay schemes with the gamma branching ratios were obtained for these isotopes, and the neutron emission probabilities (P-xn) were updated from the previous study. Hauser-Feshbach statistical model calculations were performed to understand the experimental branching ratios. We found that the P-1n and P-2n values are sensitive to the nuclear level densities of 1n daughter nuclei and showed that the statistical model reproduced the P-2n/P-1n ratio better when experimental levels plus shell-model level densities fit by the Gilbert-Cameron formula were used as the level-density input. We also showed the neutron and gamma branching ratios are sensitive to the ground-state spin of the parent nucleus. Our statistical model analysis suggested J <= 3 for the unknown ground-state spin of the odd-odd nucleus Ga-86, from the I gamma(4(+)-> 2(+))/I-gamma(2(+)-> 0(+)) ratio of Ga-84 and the P-2n/P-1n ratio. These results show the necessity of detailed understanding of the decay scheme, including data from neutron spectroscopy, in addition to gamma measurements of the multineutron emitters. |
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Address |
[Yokoyama, R.; Grzywacz, R.; Rasco, B. C.; Brewer, N.; Heideman, J.; King, T. T.; Madurga, M.; Singh, M.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA, Email: yokoyama@cns.s.u-tokyo.ac.jp |
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Amer Physical Soc |
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ISSN |
2469-9985 |
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Notes |
WOS:001159167500001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
5939 |
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Author |
Fallot, M.; Cormon, S.; Estienne, M.; Algora, A.; Bui, V.M.; Cucoanes, A.; Elnimr, M.; Giot, L.; Jordan, D.; Martino, J.; Onillon, A.; Porta, A.; Pronost, G.; Remoto, A.; Tain, J.L.; Yermia, F.; Zakari-Issoufou, A.A. |
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Title |
New Antineutrino Energy Spectra Predictions from the Summation of Beta Decay Branches of the Fission Products |
Type |
Journal Article |
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Year |
2012 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
109 |
Issue |
20 |
Pages |
202504 - 5pp |
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Keywords |
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Abstract |
In this Letter, we study the impact of the inclusion of the recently measured beta decay properties of the Tc-102;104;105;106;107, Mo-105, and Nb-101 nuclei in an updated calculation of the antineutrino energy spectra of the four fissible isotopes U-235,U-238 and Pu-239,Pu-241. These actinides are the main contributors to the fission processes in pressurized water reactors. The beta feeding probabilities of the above-mentioned Tc, Mo, and Nb isotopes have been found to play a major role in the gamma component of the decay heat of Pu-239, solving a large part of the gamma discrepancy in the 4-3000 s range. They have been measured by using the total absorption technique, insensitive to the pandemonium effect. The calculations are performed by using the information available nowadays in the nuclear databases, summing all the contributions of the beta decay branches of the fission products. Our results provide a new prediction of the antineutrino energy spectra of U-235, Pu-239,Pu-241, and, in particular, U-238 for which no measurement has been published yet. We conclude that new total absorption technique measurements are mandatory to improve the reliability of the predicted spectra. |
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Address |
[Fallot, M.; Cormon, S.; Estienne, M.; Bui, V. M.; Cucoanes, A.; Elnimr, M.; Giot, L.; Martino, J.; Onillon, A.; Porta, A.; Pronost, G.; Remoto, A.; Yermia, F.; Zakari-Issoufou, A. -A.] Univ Nantes, Ecole Mines Nantes, CNRS, IN2P3,SUBATECH, F-44307 Nantes, France |
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Amer Physical Soc |
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English |
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Series Volume |
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Series Issue |
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ISSN |
0031-9007 |
ISBN |
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Conference |
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Notes |
WOS:000310991700009 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1250 |
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Author |
n_TOF Collaboration (Lederer, C. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
Neutron Capture Cross Section of Unstable Ni-63: Implications for Stellar Nucleosynthesis |
Type |
Journal Article |
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Year |
2013 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
110 |
Issue |
2 |
Pages |
022501 - 5pp |
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Keywords |
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Abstract |
The Ni-63(n, gamma) cross section has been measured for the first time at the neutron time-of-flight facility n_TOF at CERN from thermal neutron energies up to 200 keV. In total, capture kernels of 12 (new) resonances were determined. Maxwellian averaged cross sections were calculated for thermal energies from kT = 5-100 keV with uncertainties around 20%. Stellar model calculations for a 25M(circle dot) star show that the new data have a significant effect on the s-process production of Cu-63, Ni-64, and Zn-64 in massive stars, allowing stronger constraints on the Cu yields from explosive nucleosynthesis in the subsequent supernova. |
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Address |
[Lederer, C.; Paradela, C.; Wallner, A.] Univ Vienna, Fac Phys, A-1090 Vienna, Austria |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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ISSN |
0031-9007 |
ISBN |
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Conference |
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Notes |
WOS:000313336500005 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1305 |
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Author |
Tain, J.L. et al; Valencia, E.; Algora, A.; Agramunt, J.; Rubio, B.; Estevez, E.; Jordan, M.D. |
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Title |
Enhanced gamma-Ray Emission from Neutron Unbound States Populated in beta Decay |
Type |
Journal Article |
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Year |
2015 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
115 |
Issue |
6 |
Pages |
062502 - 5pp |
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Keywords |
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Abstract |
Total absorption spectroscopy is used to investigate the beta-decay intensity to states above the neutron separation energy followed by gamma-ray emission in Br-87,Br-88 and Rb-94. Accurate results are obtained thanks to a careful control of systematic errors. An unexpectedly large. intensity is observed in all three cases extending well beyond the excitation energy region where neutron penetration is hindered by low neutron energy. The gamma branching as a function of excitation energy is compared to Hauser-Feshbach model calculations. For Br-87 and Br-88 the gamma branching reaches 57% and 20%, respectively, and could be explained as a nuclear structure effect. Some of the states populated in the daughter can only decay through the emission of a large orbital angular momentum neutron with a strongly reduced barrier penetrability. In the case of neutron-rich Rb-94 the observed 4.5% branching is much larger than the calculations performed with standard nuclear statistical model parameters, even after proper correction for fluctuation effects on individual transition widths. The difference can be reconciled by introducing an enhancement of 1 order of magnitude in the photon strength to neutron strength ratio. An increase in the photon strength function of such magnitude for very neutron-rich nuclei, if it proves to be correct, leads to a similar increase in the (n, gamma) cross section that would have an impact on r process abundance calculations. |
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Address |
[Tain, J. L.; Valencia, E.; Algora, A.; Agramunt, J.; Rubio, B.; Estevez, E.; Jordan, M. D.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46071 Valencia, Spain, Email: tain@ific.uv.es |
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Publisher |
Amer Physical Soc |
Place of Publication |
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English |
Summary Language |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0031-9007 |
ISBN |
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Area |
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Expedition |
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Conference |
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Notes |
WOS:000359059100002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2319 |
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Author |
IGISOL Collaboration (Zakari-Issoufou, A.A. et al); Algora, A.; Tain, J.L.; Valencia, E.; Agramunt, J.; Estevez, E.; Gelletly, W.; Jordan, M.D.; Molina, F.; Perez-Cerdan, A.B.; Rubio, B. |
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Title |
Total Absorption Spectroscopy Study of Rb-92 Decay: A Major Contributor to Reactor Antineutrino Spectrum Shape |
Type |
Journal Article |
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Year |
2015 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
115 |
Issue |
10 |
Pages |
102503 - 6pp |
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Keywords |
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Abstract |
The antineutrino spectra measured in recent experiments at reactors are inconsistent with calculations based on the conversion of integral beta spectra recorded at the ILL reactor. Rb-92 makes the dominant contribution to the reactor antineutrino spectrum in the 5-8 MeV range but its decay properties are in question. We have studied Rb-92 decay with total absorption spectroscopy. Previously unobserved beta feeding was seen in the 4.5-5.5 region and the GS to GS feeding was found to be 87.5(25)%. The impact on the reactor antineutrino spectra calculated with the summation method is shown and discussed. |
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Address |
[Zakari-Issoufou, A. -A.; Fallot, M.; Porta, A.; Bui, V. M.; Cormon, S.; Estienne, M.; Briz, J. A.; Cucoanes, A.; Shiba, T.] Univ Nantes, Ecole Mines Nantes, SUBATECH, CNRS,IN2P3, F-44307 Nantes, France, Email: porta@subatech.in2p3.fr |
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Amer Physical Soc |
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English |
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ISSN |
0031-9007 |
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Conference |
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Notes |
WOS:000360603500002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2375 |
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Author |
Caballero-Folch, R. et al; Domingo-Pardo, C.; Agramunt, J.; Algora, A.; Rubio, B.; Tain, J.L. |
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Title |
First Measurement of Several beta-Delayed Neutron Emitting Isotopes Beyond N=126 |
Type |
Journal Article |
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Year |
2016 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
117 |
Issue |
1 |
Pages |
012501 - 6pp |
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Keywords |
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Abstract |
The beta-delayed neutron emission probabilities of neutron rich Hg and Tl nuclei have been measured together with beta-decay half-lives for 20 isotopes of Au, Hg, Tl, Pb, and Bi in the mass region N greater than or similar to 126. These are the heaviest species where neutron emission has been observed so far. These measurements provide key information to evaluate the performance of nuclear microscopic and phenomenological models in reproducing the high-energy part of the beta-decay strength distribution. This provides important constraints on global theoretical models currently used in r-process nucleosynthesis. |
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Address |
[Caballero-Folch, R.; Algora, A.; Calvino, F.; Cortes, G.; Gomez-Hornillos, M. B.; Riego, A.] Univ Politecn Cataluna, INTE DFEN, E-08028 Barcelona, Spain, Email: domingo@ific.uv.es |
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Publisher |
Amer Physical Soc |
Place of Publication |
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English |
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Abbreviated Series Title |
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Series Issue |
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ISSN |
0031-9007 |
ISBN |
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Area |
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Conference |
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Notes |
WOS:000378879000008 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2742 |
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Author |
n_TOF Collaboration (Barbagallo, M. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Be-7(n,alpha)He-4 Reaction and the Cosmological Lithium Problem: Measurement of the Cross Section in a Wide Energy Range at n_TOF at CERN |
Type |
Journal Article |
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Year |
2016 |
Publication |
Physical Review Letters |
Abbreviated Journal |
Phys. Rev. Lett. |
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Volume |
117 |
Issue |
15 |
Pages |
152701 - 7pp |
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Keywords |
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Abstract |
The energy-dependent cross section of the (7)Bed(n,alpha)He-4 reaction, of interest for the so-called cosmological lithium problem in big bang nucleosynthesis, has been measured for the first time from 10 meV to 10 keV neutron energy. The challenges posed by the short half-life of Be-7 and by the low reaction cross section have been overcome at nTOF thanks to an unprecedented combination of the extremely high luminosity and good resolution of the neutron beam in the new experimental area (EAR2) of the nTOF facility at CERN, the availability of a sufficient amount of chemically pure Be-7, and a specifically designed experimental setup. Coincidences between the two alpha particles have been recorded in two Si-Be-7-Si arrays placed directly in the neutron beam. The present results are consistent, at thermal neutron energy, with the only previous measurement performed in the 1960s at a nuclear reactor. The energy dependence reported here clearly indicates the inadequacy of the cross section estimates currently used in BBN calculations. Although new measurements at higher neutron energy may still be needed, the n_TOF results hint at a minor role of this reaction in BBN, leaving the long-standing cosmological lithium problem unsolved. |
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Address |
[Barbagallo, M.; Colonna, N.; Damone, L.; Mastromarco, M.; Mazzone, A.; Tagliente, G.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: nicola.colonna@ba.infn.it |
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Publisher |
Amer Physical Soc |
Place of Publication |
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English |
Summary Language |
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ISSN |
0031-9007 |
ISBN |
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Conference |
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Notes |
WOS:000384479300003 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
2822 |
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| Permanent link to this record |
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Author |
Algora, A. et al; Valencia, E.; Tain, J.L.; Jordan, M.D.; Agramunt, J.; Rubio, B.; Estevez, E.; Molina, F.; Montaner-Piza, A.; Guadilla, V. |
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Title |
Total Absorption Study of Beta Decays Relevant for Nuclear Applications and Nuclear Structure |
Type |
Journal Article |
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Year |
2014 |
Publication |
Nuclear Data Sheets |
Abbreviated Journal |
Nucl. Data Sheets |
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Volume |
120 |
Issue |
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Pages |
12-15 |
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Keywords |
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Abstract |
An overview is given of our activities related to the study of the beta decay of neutron rich nuclei relevant for nuclear applications. Recent results of the study of the beta decay of Br-87,Br-88 using a new segmented total absorption spectrometer are presented. The measurements were performed at the IGISOL facility using trap-assisted total absorption spectroscopy. |
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[Algora, A.; Valencia, E.; Tain, J. L.; Jordan, M. D.; Agramunt, J.; Rubio, B.; Estevez, E.; Molina, F.; Montaner, A.; Guadilla, V.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain, Email: algora@ific.uv.es |
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Academic Press Inc Elsevier Science |
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English |
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0090-3752 |
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WOS:000339860100004 |
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no |
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yes |
International Collaboration |
yes |
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IFIC @ pastor @ |
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1869 |
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