Abstract: The U-238 to U-235 fission cross section ratio has been determined at nTOF up to approximate to 1 GeV, with two different detection systems, in different geometrical configurations. A total of four datasets has been collected and compared. They are all consistent to each other within the relative systematic uncertainty of 3-4%. The data collected at nTOF have been suitably combined to yield a unique fission cross section ratio as a function of neutron energy. The result confirms current evaluations up to 200 MeV. Good agreement is also observed with theoretical calculations based on the INCL++ /Gemini++ combination up to the highest measured energy. The n_TOF results may help solve a long-standing discrepancy between the two most important experimental datasets available so far above 20 MeV, while extending the neutron energy range for the first time up to approximate to 1 GeV.

Abstract: The Ni-58(n,gamma) cross section has been measured at the neutron time of flight facility n_TOF at CERN, in the energy range from 27 meV up to 400 keV. In total, 51 resonances have been analyzed up to 122 keV. Maxwellian averaged cross sections (MACS) have been calculated for stellar temperatures of kT = 5-100 keV with uncertainties of less than 6%, showing fair agreement with recent experimental and evaluated data up to kT = 50 keV. The MACS extracted in the present work at 30 keV is 34.2 +/- 0.6(stat) +/- 1.8(sys) mb, in agreement with latest results and evaluations, but 12% lower relative to the recent KADoNIS compilation of astrophysical cross sections. When included in models of the s-process nucleosynthesis in massive stars, this change results in a 60% increase of the abundance of Ni-58, with a negligible propagation on heavier isotopes. The reason is that, using both the old or the new MACS, Ni-58 is efficiently depleted by neutron captures.

Abstract: The Ni-63(n, gamma) cross section has been measured for the first time at the neutron time-of-flight facility n_TOF at CERN from thermal neutron energies up to 200 keV. In total, capture kernels of 12 (new) resonances were determined. Maxwellian averaged cross sections were calculated for thermal energies from kT = 5-100 keV with uncertainties around 20%. Stellar model calculations for a 25M(circle dot) star show that the new data have a significant effect on the s-process production of Cu-63, Ni-64, and Zn-64 in massive stars, allowing stronger constraints on the Cu yields from explosive nucleosynthesis in the subsequent supernova.

Abstract: The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first 2(+) state and the increase in the transition strength B(E2; 2(1)(+) -> 0(1)(+) ) going from Zr-98 to Zr-100 has been the first example of “quantum phase transition” in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the gamma gamma-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in Zr98-104 carried out to extract reduced transition probabilities. The new lifetime values in gamma gamma-coincidence and gamma-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree-Fock- Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

Abstract: The neutron capture cross sections of (186)Os and (187)Os are of key importance for defining the 8-process abundance of (187)Os at the formation of the solar system. This quantity can be used to determine the radiogenic abundance component of (187)Os from the decay of (187)Re (t(1/2) = 41.2 Gyr) and to infer the time-duration of the nucleosynthesis in our galaxy (Re/Os cosmochronometer). The neutron capture cross sections of (186)Os, (187)Os, and (188)Os have been measured at the CERN nTOF facility from 1 eV to 1 MeV, covering the entire energy range of astrophysical interest. From these data Maxwellian averaged capture cross sections have been calculated with uncertainties between 3.3 and 4.7%. Additional information was obtained by measuring the inelastic scattering cross section of (187)Os at the Karlsruhe 3.7 MV Van de Graaff accelerator and by neutron resonance analyses of the nTOF capture data to establish a comprehensive experimental basis for the Hauser-Feshbach statistical model. Consistent I-IF calculations for the capture and inelastic reaction channels were performed to determine the stellar enhancement factors, which are required to correct the Maxwellian averaged cross sections for the effect of thermally populated excited states. The consequences of this analysis for the s-process component of the (187)Os abundance and the related impact on the evaluation of the time-duration of Galactic nucleosynthesis via the Re/Os cosmo-chronometer are discussed.