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Author n_TOF Collaboration (Praena, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Measurement and resonance analysis of the S-33(n,alpha)Si-30 cross section at the CERN n_TOF facility in the energy region from 10 to 300 keV Type Journal Article
Year 2018 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 97 Issue 6 Pages 064603 - 10pp
Keywords
Abstract The (33)(n , alpha)Si-30 cross section has been measured at the neutron time-of-flight (n_TOF) facility at CERN in the neutron energy range from 10 to 300 keV relative to the B-10(n, alpha)(7) Li cross-section standard. Both reactions were measured simultaneously with a set of micromegas detectors. The flight path of 185 m has allowed us to obtain the cross section with high-energy resolution. An accurate description of the resonances has been performed by means of the multilevel multichannel R-matrix code SAMMY. The results show a significantly higher area of the biggest resonance (13.45 keV) than the unique high-resolution (n , alpha) measurement. The new parametrization of the 13.45-keV resonance is similar to that of the unique transmission measurement. This resonance is a matter of research in neutron-capture therapy. The S-33(n, alpha)Si-30 cross section has been studied in previous works because of its role in the production of S-36 in stars, which is currently overproduced in stellar models compared to observations.
Address [Praena, J.; Porras, I] Univ Granada, Granada, Spain, Email: jpraena@ugr.es
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000434017300004 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3597
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Author n_TOF Collaboration (Mendoza, E. et al); Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Measurement and analysis of the Am-241 neutron capture cross section at the n_TOF facility at CERN Type Journal Article
Year 2018 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 97 Issue 5 Pages 054616 - 21pp
Keywords
Abstract The Am-241(n, gamma) cross section has been measured at the nTOF facility at CERN with the nTOF BaF2 Total Absorption Calorimeter in the energy range between 0.2 eV and 10 keV. Our results are analyzed as resolved resonances up to 700 eV, allowing a more detailed description of the cross section than in the current evaluations, which contain resolved resonances only up to 150-160 eV. The cross section in the unresolved resonance region is perfectly consistent with the predictions based on the average resonance parameters deduced from the resolved resonances, thus obtaining a consistent description of the cross section in the full neutron energy range under study. Below 20 eV, our results are in reasonable agreement with JEFF-3.2 as well as with the most recent direct measurements of the resonance integral, and differ up to 20-30% with other experimental data. Between 20 eV and 1 keV, the disagreement with other experimental data and evaluations gradually decreases, in general, with the neutron energy. Above 1 keV, we find compatible results with previously existing values.
Address [Mendoza, E.; Cano-Ott, D.; Balibrea, J.; Becares, V; Garcia, A. R.; Gonzalez, E.; Lopez, D.; Martinez, T.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain, Email: emilio.mendoza@ciemat.es
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000433032300001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3584
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Author n_TOF Collaboration (Lerendegui-Marco, J. et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility Type Journal Article
Year 2018 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 97 Issue 2 Pages 024605 - 21pp
Keywords
Abstract The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA.
Address [Lerendegui-Marco, J.; Guerrero, C.; Quesada, J. M.; Cortes-Giraldo, M. A.; Praena, J.; Sabate-Gilarte, M.] Univ Seville, Dept Fis Atom Mol & Nucl, E-41012 Seville, Spain, Email: cguerrero4@us.es
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000424190700001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3474
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Author n_TOF Collaboration (Wright, T. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Measurement of the U-238(n,gamma) cross section up to 80 keV with the Total Absorption Calorimeter at the CERN n_TOF facility Type Journal Article
Year 2017 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 96 Issue 6 Pages 064601 - 11pp
Keywords
Abstract The radiative capture cross section of a highly pure (99.999%), 6.125(2) grams and 9.56(5) x 10(-4) atoms/barn areal density U-238 sample has been measured with the Total Absorption Calorimeter (TAC) in the 185 m flight path at the CERN neutron time-of-flight facility n_TOF. This measurement is in response to the NEA High Priority Request list, which demands an accuracy in this cross section of less than 3% below 25 keV. These data have undergone careful background subtraction, with special care being given to the background originating from neutrons scattered by the 238U sample. Pileup and dead-time effects have been corrected for. The measured cross section covers an energy range between 0.2 eV and 80 keV, with an accuracy that varies with neutron energy, being better than 4% below 25 keV and reaching at most 6% at higher energies.
Address [Wright, T.; Billowes, J.; Ryan, J. A.; Ware, T.] Univ Manchester, Manchester, Lancs, England, Email: tobias.wright@manchester.ac.uk
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000416848700005 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3392
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Author Wu, J. et al; Algora, A.; Agramunt, J.; Morales, A.I.; Orrigo, S.E.A.; Tain, J.L.; Tarifeño-Saldivia, A.; Tolosa-Delgado, A.
Title First observation of isomeric states in 111Zr, 113Nb, and 115Mo Type Journal Article
Year 2022 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 106 Issue 6 Pages 064328 - 5pp
Keywords
Abstract Isomeric states in the neutron-rich nuclei 111Zr [T1/2 = 0.10(7) μs], 113Nb [T1/2 = 0.7(4) μs], 115Mo [T1/2 = 46(3) μs] were first identified at the Radioactive Ion Beam Factory (RIBF) of RIKEN by using in-flight fission and fragmentation of a 238U beam at an energy of 345 MeV/u. This is a brief report of the gamma transitions de -exciting from isomeric states and half-lives measurements, which provides the first spectroscopy in the nuclear region of prolate-to-oblate shape-phase transition around mass A approximate to 110.
Address [Wu, J.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA, Email: jwu2@bnl.gov
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000906391600002 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5452
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Author n_TOF Collaboration (Tagliente, G. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Zr-92(n, gamma) and (n,tot) measurements at the GELINA and n_TOF facilities Type Journal Article
Year 2022 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 105 Issue 2 Pages 025805 - 14pp
Keywords
Abstract Background: Stellar nucleosynthesis of elements heavier than iron is driven by neutron capture processes. Zr-92 is positioned at a strategic point along the slow nucleosynthesis path, given its proximity to the neutron magic number N = 50 and its position at the matching region between the weak and main slow processes. Purpose: In parallel with recent improved astronomical data, the extraction of accurate Maxwellian averaged cross sections (MACSs) derived from a more complete and accurate set of resonance parameters should allow for a better understanding of the stellar conditions at which nucleosynthesis takes place. Methods: Transmission and capture cross section measurements using enriched Zr-92 metallic samples were performed at the time-of flight facilities GELINA of JRC-Geel (BE) and nTOF of CERN (CH). The neutron beam passing through the samples was investigated in transmission measurements at GELINA using a Li-glass scintillator. The gamma rays emitted during the neutron capture reactions were detected by C6D6 detectors at both GELINA and nTOF. Results: Resonance parameters of individual resonances up to 81 keV were extracted from a combined resonance shape analysis of experimental transmissions and capture yields. For the majority of the resonances the parity was determined from an analysis of the transmission data obtained with different sample thicknesses. Average resonance parameters were calculated. Conclusions: Maxwellian averaged cross sections were extracted from resonances observed up to 81 keV. The MACS for kT = 30 keV is fully consistent with experimental data reported in the literature. The MACSs for kT less than or similar to 15 keV are in good agreement with those derived from the ENDF/B-VIII.0 library and recommended in the KADoNTS database. For kT higher than 30 keV differences are observed. A comparison with MACSs obtained with the cross sections recommended in the JEFF-3.3 and JENDL-4.0 libraries shows discrepancies even for kT less than or similar to 15 keV.
Address [Tagliente, G.; Barbagallo, M.; Colonna, N.; Mastromarco, M.; Variale, V.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy, Email: giuseppe.tagliente@ba.infn.it
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000766732800002 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5163
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Author n_TOF Collaboration (Gawlik, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Measurement of the Ge-76(n, gamma) cross section at the n_TOF facility at CERN Type Journal Article
Year 2021 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 104 Issue 4 Pages 044610 - 7pp
Keywords
Abstract The Ge-76(n, gamma) reaction has been measured at the n_TOF facility at CERN via the time-of-flight technique. Neutron capture cross sections on Ge-76 are of interest to a variety of low-background experiments, such as neutrinoless double beta decay searches, and to nuclear astrophysics. We have determined resonance capture kernels up to 52 keV neutron energy and used the new data to calculate Maxwellian-averaged neutron capture cross sections for k(B)T values of 5 to 100 keV.
Address [Gawlik-Ramiega, A.; Andrzejewski, J.; Perkowski, J.] Univ Lodz, Lodz, Poland, Email: aleksandra.gawlik@uni.lodz.pl
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000707420400002 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5003
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Author n_TOF Collaboration (Balibrea-Correa, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Measurement of the alpha ratio and (n, gamma) cross section of U-235 from 0.2 to 200 eV at n_TOF Type Journal Article
Year 2020 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 102 Issue 4 Pages 044615 - 18pp
Keywords
Abstract We measured the neutron capture-to-fission cross-section ratio (alpha ratio) and the capture cross section of U-235 between 0.2 and 200 eV at the nTOF facility at CERN. The simultaneous measurement of neutron-induced capture and fission rates was performed by means of the nTOF BaF2 Total Absorption Calorimeter (TAC), used for detection of gamma rays, in combination with a set of micromegas detectors used as fission tagging detectors. The energy dependence of the capture cross section was obtained with help of the Li-6(n, t) standard reaction determining the n_TOF neutron fluence; the well-known integral of the U-235(n, f) cross section between 7.8 and 11 eV was then used for its absolute normalization. The alpha ratio, obtained with slightly higher statistical fluctuations, was determined directly, without need for any reference cross section. To perform the analysis of this measurement we developed a new methodology to correct the experimentally observed effect that the probabilities of detecting a fission reaction in the TAC and the micromegas detectors are not independent. The results of this work have been used in a new evaluation of U-235 performed within the scope of the Collaborative International Evaluated Library Organisation (CIELO) Project, and are consistent with the ENDF/B-VIII.0 and JEFF-3.3 capture cross sections below 4 eV and above 100 eV. However, the measured capture cross section is on average 10% larger between 4 and 100 eV.
Address [Balibrea-Correa, J.; Mendoza, E.; Cano-Ott, D.] Ctr Invest Energet Medioambientales & Tecnol, CIEMAT, Madrid, Spain, Email: emilio.mendoza@ciemat.es
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0556-2813 ISBN Medium
Area Expedition Conference
Notes WOS:000579839000003 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 4575
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Author n_TOF Collaboration (Stamatopoulos, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A.
Title Investigation of the Pu-240(n, f) reaction at the n_TOF/EAR2 facility in the 9 meV-6 MeV range Type Journal Article
Year 2020 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 102 Issue 1 Pages 014616 - 23pp
Keywords
Abstract Background: Nuclear waste management is considered amongst the major challenges in the field of nuclear energy. A possible means of addressing this issue is waste transmutation in advanced nuclear systems, whose operation requires a fast neutron spectrum. In this regard, the accurate knowledge of neutron-induced reaction cross sections of several (minor) actinide isotopes is essential for design optimization and improvement of safety margins of such systems. One such case is Pu-240, due to its accumulation in spent nuclear fuel of thermal reactors and its usage in fast reactor fuel. The measurement of the Pu-240(n, f) cross section was previously attempted at the CERN nTOF facility EAR1 measuring station using the time-of-flight technique. Due to the low amount of available material and the given flux at EAR1, the measurement had to last several months to achieve a sufficient statistical accuracy. This long duration led to detector deterioration due to the prolonged exposure to the high alpha activity of the fission foils, therefore the measurement could not be successfully completed. Purpose: It is aimed to determine whether it is feasible to study neutron-induced fission at nTOF/EAR2 and provide data on the Pu-240(n, f) reaction in energy regions requested for applications. Methods: The study of the Pu-240(n, f) reaction was made at a new experimental area (EAR2) with a shorter flight path which delivered on average 30 times higher flux at fast neutron energies. This enabled the measurement to be performed much faster, thus limiting the exposure of the detectors to the intrinsic activity of the fission foils. The experimental setup was based on microbulk Micromegas detectors and the time-of-flight data were analyzed with an optimized pulse-shape analysis algorithm. Special attention was dedicated to the estimation of the non-negligible counting loss corrections with the development of a new methodology, and other corrections were estimated via Monte Carlo simulations of the experimental setup. Results: This new measurement of the Pu-240(n, f) cross section yielded data from 9 meV up to 6 MeV incident neutron energy and fission resonance kernels were extracted up to 10 keV. Conclusions: Neutron-induced fission of high activity samples can be successfully studied at the n_TOF/EAR2 facility at CERN covering a wide range of neutron energies, from thermal to a few MeV.
Address [Stamatopoulos, A.; Tsinganis, A.; Kokkoris, M.; Vlastou, R.; Diakaki, M.] Natl Tech Univ Athens, Athens, Greece, Email: athanasios.stamatopoulos@cern.ch
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0556-2813 ISBN Medium
Area Expedition Conference
Notes WOS:000551057500002 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 4466
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Author Phong, V.H. et al; Agramunt, J.; Algora, A.; Domingo-Pardo, C.; Morales, A.I.; Tain, J.L.; Tarifeño-Saldivia, A.; Tolosa-Delgado, A.
Title Observation of a μs isomer in In-134(49)85: Proton-neutron coupling “southeast” of Sn-132(50)82 Type Journal Article
Year 2019 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 100 Issue 1 Pages 011302 - 6pp
Keywords
Abstract We report on the observation of a microsecond isomeric state in the single-proton-hole, three-neutron-particle nucleus In-134. The nuclei of interest were produced by in-flight fission of a U-238 beam at the Radioactive Isotope Beam Factory at RIKEN. The isomer depopulates through a gamma ray of energy 56.7(1) keV and with a half-life of T-1/2 = 3.5(4) μs. Based on the comparison with shell-model calculations, we interpret the isomer as the I-pi = 5(-) member of the pi 0g(9/2)(-1) circle times nu 1f(7/2)(3) multiplet, decaying to the I-pi = 7(-) ground state with a reduced-transition probability of B(E2; 5(-) -> 7(-)) = 0.53(6) W.u. Observation of this isomer, and lack of evidence in the current work for a I-pi = 5(-) isomer decay in In-132, provides a benchmark of the proton-neutron interaction in the region of the nuclear chart “southeast” of Sn-132, where experimental information on excited states is sparse.
Address [Phong, V. H.; Lorusso, G.; Liu, J.; Matsui, K.; Nishimura, S.; Ahn, D. S.; Baba, H.; Go, S.; Isobe, T.; Kiss, G.; Kubono, S.; Sakurai, H.; Shimizu, Y.; Sumikama, T.; Suzuki, H.; Takeda, H.] RIKEN, RIKEN Nishina Ctr, 2-1 Hirosawa, Wako, Saitama 3510198, Japan, Email: giuseppe.lorusso@npl.co.uk
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000477895400001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 4080
Permanent link to this record