Abstract: The measurement of the capture cross-section of fissile elements, of utmost importance for the design of innovative nuclear reactors and the management of nuclear waste, faces particular difficulties related to the.-ray background generated in the competing fission reactions. At the CERN neutron time-of-flight facility nTOF we have combined the Total Absorption Calorimeter (TAC) capture detector with a set of three U-235 loaded MicroMegas (MGAS) fission detectors for measuring simultaneously two reactions: capture and fission. The results presented here include the determination of the three detection efficiencies involved in the process: epsilon(TAC)(n, f), epsilon(TAC)(n, gamma) and epsilon(MGAS)(n, f). In the test measurement we have succeeded in measuring simultaneously with a high total efficiency the U-235 capture and fission cross-sections, disentangling accurately the two types of reactions. The work presented here proves that accurate capture cross-section measurements of fissile isotopes are feasible at nTOF.

Abstract: A beta-gamma spectroscopy of the J(pi) = 1(+), 426 keV isomeric state of Al-24 ( Al-24m) has been carried out by using a Al-24 secondary beam with high purity and high isomeric ratio. From the absolute gamma-ray and beta-particle intensities observed in the decay of the isomeric state, the branching ratio R-B of the isomeric gamma-decay from Al-24m to the J(pi) = 4(+), ground state of Al-24 have been derived. The obtained R-B value of 69.6(7)% is much smaller than the previously accepted value of 82.5(30)%. The precise half-life for the isomer decay, T-1/2(m) = 130.9(13) ms, has been also determined in this experiment. Accordingly, the M3 gamma-decay strength B(M3) of the Al-24m decay becomes smaller and the total beta-decay branching ratio becomes larger. In particular, the beta-decay branching ratio to the ground state of Mg-24 becomes 24.3(9)%, which is 2.4 times larger than the previous value of 10.1(28)%. By combining the branching ratio and the half-life, the Gamow-Teller (GT) transition strength B(GT) of 0.0194(7) is deduced for the GT transition from Al-24m to the J(pi) = 0(+), ground state of Mg-24. This value is in good agreement with the values derived from charge-exchange reactions.

Abstract: The response function of the magnetic spectrometer PRISMA is studied via a Monte Carlo simulation that employs a ray tracing code to determine the trajectories of individual rays through the electromagnetic fields. The calculated response is tested on angular and energy distributions provided by theoretical calculations for the Ca-48 + Ni-64 multinucleon transfer reaction and applied to the corresponding experimental data.

Abstract: The energy centroids and integrated strengths of Gamow-Teller transitions in the beta(+) and electron-capture decay are analyzed for nuclei whose proton number Z and neutron number N are restricted to 44 <= Z <= 50 and 50 <= N <= 58. The analysis is based on data measured both with high-resolution gamma-ray spectrometry and total gamma-ray absorption techniques. The dependence of the considered quantities on the relative neutron excess are established after taking into account the effects due to the Coulomb interaction and mean-field level occupancies. An extrapolation of this dependence to the lightest known tin isotopes is used to estimate the decay characteristics of Sn-100 and Sn-101. The values extrapolated for the half-lives of Sn-100 and Sn-101 agree with experimental data. Using the extrapolated values together with shell model predictions, the Q values for the electron-capture decay of Sn-100 is evaluated. The quenching factor for beta(+) and the electron-capture decay of the nuclei under consideration here is established to be 0.56(2) with a possible weak dependence on N – Z.