n_TOF Collaboration(Tarrío, D. et al), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2023). Neutron-induced fission cross sections of Th-232 and U-233 up to 1 GeV using parallel plate avalanche counters at the CERN n_TOF facility. Phys. Rev. C, 107(4), 044616–21pp.
Abstract: The neutron-induced fission cross sections of Th-232 and U-233 were measured relative to U-235 in a wide neutron energy range up to 1 GeV (and from fission threshold in the case of Th-232, and from 0.7 eV in case of U-233), using the white-spectrum neutron source at the CERN Neutron Time-of-Flight (nTOF) facility. Parallel plate avalanche counters (PPACs) were used, installed at the Experimental Area 1 (EAR1), which is located at 185 m from the neutron spallation target. The anisotropic emission of fission fragments were taken into account in the detection efficiency by using, in the case of U-233, previous results available in EXFOR, whereas in the case of Th-232 these data were obtained from our measurement, using PPACs and targets tilted 45 degrees with respect to the neutron beam direction. Finally, the obtained results are compared with past measurements and major evaluated nuclear data libraries. Calculations using the high-energy reaction models INCL++ and ABLA07 were performed and some of their parameters were modified to reproduce the experimental results. At high energies, where no other neutron data exist, our results are compared with experimental data on proton-induced fission. Moreover, the dependence of the fission cross section at 1 GeV with the fissility parameter of the target nucleus is studied by combining those ( p, f) data with our (n, f) data on Th-232 and U-233 and on other isotopes studied earlier at nTOF using the same experimental setup.
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Clement, E. et al, Domingo-Pardo, C., & Gadea, A. (2023). Spectroscopic quadrupole moments in 124Xe. Phys. Rev. C, 107(1), 014324–8pp.
Abstract: Background: The Xe isotopic chain with four valence protons above the Z = 50 shell closure is an ideal laboratory for the study of the evolution of nuclear deformation. At the N = 82 shell closure, 136Xe presents all characteristics of a doubly closed shell nucleus with a spherical shape. In the very neutron-deficient isotopes close to N = 50, the alpha-decay chain of Xe was investigated to probe the radioactive decay properties near the drip-line and the magicity of 100Sn. Additionally, the Xe isotopes present higher order symmetries in the nuclear deformation such as the octupole degree of freedom near N = 60 and N = 90 or O(6) symmetry in stable isotopes.Purpose: The relevance of the O(6) symmetry has been investigated by measuring the spectroscopic quadrupole moment of the first excited states in 124Xe. In the O(6) symmetry limit, the spectroscopic quadrupole moment of collective states is expected to be null.Method: A stable 124Xe beam with energies of 4.03A MeV and 4.11A MeV was used to bombard a natW target at the GANIL facility. Excited states were populated via the safe Coulomb excitation reaction. The collision of the heavy ions with a large Z at low energy make this reaction sensitive to the diagonal E2 matrix element of the excited states. The recoils were detected in the VAMOS++ magnetic spectrometer and the gamma rays in the AGATA tracking array. The least squares fitting code GOSIA was used for the analysis to extract both E2 and M1 transitional and E2 diagonal matrix elements.Results: The rotational ground state band was populated up to the 8+1 state as well as the 2+2 and 4+2 states. Using high precision spectroscopic data to constrain the GOSIA fit, the spectroscopic quadrupole moments of the 2+1 , 4+1 , and 6+1 states were determined for the first time. Conclusions: The spectroscopic quadrupole moments were found to be negative, large, and constant in the ground state band underlining the prolate axially deformed ground state band of 124Xe. The present experimental data confirm that the is broken in 124Xe.
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AGATA Collaboration(Liu, X. et al), Gadea, A., Jurado, M., Domingo-Pardo, C., Huyuk, T., & Perez-Vidal, R. M. (2022). Evidence for spherical-oblate shape coexistence in Tc-87. Phys. Rev. C, 106(3), 034304–6pp.
Abstract: Excited states in the neutron-deficient nucleus Tc-87 have been studied via the fusion-evaporation reaction 54Fe(36Ar, 2n1p) Tc-87 at 115 MeV beam energy. The AGATA gamma-ray spectrometer coupled to the DIAMANT, NEDA, and Neutron Wall detector arrays for light-particle detection was used to measure the prompt coincidence of gamma rays and light particles. Six transitions from the deexcitation of excited states belonging to a new band in Tc-87 were identified by comparing gamma-ray intensities in the spectra gated under different reaction channel selection conditions. The constructed level structure was compared with the shell model and total Routhian surface calculations. The results indicate that the new band structure in 87Tc is built on a spherical configuration, which is different from that assigned to the previously identified oblate yrast rotational band.
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n_TOF Collaboration(Tagliente, G. et al), Domingo-Pardo, C., Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2022). Zr-92(n, gamma) and (n,tot) measurements at the GELINA and n_TOF facilities. Phys. Rev. C, 105(2), 025805–14pp.
Abstract: Background: Stellar nucleosynthesis of elements heavier than iron is driven by neutron capture processes. Zr-92 is positioned at a strategic point along the slow nucleosynthesis path, given its proximity to the neutron magic number N = 50 and its position at the matching region between the weak and main slow processes. Purpose: In parallel with recent improved astronomical data, the extraction of accurate Maxwellian averaged cross sections (MACSs) derived from a more complete and accurate set of resonance parameters should allow for a better understanding of the stellar conditions at which nucleosynthesis takes place. Methods: Transmission and capture cross section measurements using enriched Zr-92 metallic samples were performed at the time-of flight facilities GELINA of JRC-Geel (BE) and nTOF of CERN (CH). The neutron beam passing through the samples was investigated in transmission measurements at GELINA using a Li-glass scintillator. The gamma rays emitted during the neutron capture reactions were detected by C6D6 detectors at both GELINA and nTOF. Results: Resonance parameters of individual resonances up to 81 keV were extracted from a combined resonance shape analysis of experimental transmissions and capture yields. For the majority of the resonances the parity was determined from an analysis of the transmission data obtained with different sample thicknesses. Average resonance parameters were calculated. Conclusions: Maxwellian averaged cross sections were extracted from resonances observed up to 81 keV. The MACS for kT = 30 keV is fully consistent with experimental data reported in the literature. The MACSs for kT less than or similar to 15 keV are in good agreement with those derived from the ENDF/B-VIII.0 library and recommended in the KADoNTS database. For kT higher than 30 keV differences are observed. A comparison with MACSs obtained with the cross sections recommended in the JEFF-3.3 and JENDL-4.0 libraries shows discrepancies even for kT less than or similar to 15 keV.
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n_TOF Collaboration(Moreno-Soto, J. et al), Babiano-Suarez, V., Caballero-Ontanaya, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2022). Constraints on the dipole photon strength for the odd uranium isotopes. Phys. Rev. C, 105(2), 024618–14pp.
Abstract: Background: The photon strength functions (PSFs) and nuclear level density (NLD) are key ingredients for calculation of the photon interaction with nuclei, in particular the reaction cross sections. These cross sections are important especially in nuclear astrophysics and in the development of advanced nuclear technologies. Purpose: The role of the scissors mode in the M1 PSF of (well-deformed) actinides was investigated by several experimental techniques. The analyses of different experiments result in significant differences, especially on the strength of the mode. The shape of the low-energy tail of the giant electric dipole resonance is uncertain as well. In particular, some works proposed a presence of the E1 pygmy resonance just above 7 MeV. Because of these inconsistencies additional information on PSFs in this region is of great interest. Methods: The gamma-ray spectra from neutron-capture reactions on the U-234, U-236, and U-238 nuclei have been measured with the total absorption calorimeter of the n_TOF facility at CERN. The background-corrected sum-energy and multi-step-cascade spectra were extracted for several isolated s-wave resonances up to about 140 eV. Results: The experimental spectra were compared to statistical model predictions coming from a large selection of models of photon strength functions and nuclear level density. No combination of PSF and NLD models from literature is able to globally describe our spectra. After extensive search we were able to find model combinations with modified generalized Lorentzian (MGLO) E1 PSF, which match the experimental spectra as well as the total radiative widths. Conclusions: The constant temperature energy dependence is favored for a NLD. The tail of giant electric dipole resonance is well described by the MGLO model of the E1 PSF with no hint of pygmy resonance. The M1 PSF must contain a very strong, relatively wide, and likely double-resonance scissors mode. The mode is responsible for about a half of the total radiative width of neutron resonances and significantly affects the radiative cross section.
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n_TOF Collaboration(Lederer-Woods, C. et al.), Domingo-Pardo, C., & Tain, J. L. (2021). Destruction of the cosmic gamma-ray emitter Al-26 in massive stars: Study of the key Al-26(n, alpha) reaction. Phys. Rev. C, 104(3), L032803–6pp.
Abstract: Neutron destruction reactions of the cosmic gamma-ray emitter Al-26 are of importance to determine the amount of Al-26 ejected into our galaxy by supernova explosions and for Al-26 production in asymptotic giant branch stars. We performed a new measurement of the Al-26(n, alpha) reaction up to 160-keV neutron energy at the neutron time-of-flight facilities n_TOF at CERN and GELINA at EC-JRC. We provide strengths for ten resonances, six of them for the first time. We use our data to calculate astrophysical reactivities for stellar temperatures up to 0.7 GK. Our results resolve a discrepancy between the two previous direct measurements of this reaction, and indicate higher stellar destruction rates than the most recently recommended reactivity.
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n_TOF Collaboration(Lederer-Woods, C. et al.), Domingo-Pardo, C., & Tain, J. L. (2021). Destruction of the cosmic gamma-ray emitter Al-26 in massive stars: Study of the key Al-26(n, p) reaction. Phys. Rev. C, 104(2), L022803–7pp.
Abstract: The Al-26(n, p) Mg-26 reaction is the key reaction impacting on the abundances of the cosmic gamma-ray emitter Al-26 produced in massive stars and impacts on the potential pollution of the early solar system with Al-26 by asymptotic giant branch stars. We performed a measurement of the Al-26(n, p) Mg-26 cross section at the high-flux beam line EAR-2 at the n_TOF facility (CERN). We report resonance strengths for eleven resonances, nine being measured for the first time, while there is only one previous measurement for the other two. Our resonance strengths are significantly lower than the only previous values available. Our cross-section data range to 150 keV neutron energy, which is sufficient for a reliable determination of astrophysical reactivities up to 0.5 GK stellar temperature.
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AGATA Collaboration(Liu, X. et al), Gadea, A., Jurado, M., Domingo-Pardo, C., Huyuk, T., & Perez-Vidal, R. M. (2021). Evidence for enhanced neutron-proton correlations from the level structure of the N = Z+1 nucleus Tc-87(43)44. Phys. Rev. C, 104(2), L021302–5pp.
Abstract: The low-lying excited states in the neutron-deficient N = Z + 1 nucleus (87)(43)Tcc(44) have been studied via the fusion-evaporation reaction Fe-54(Ar-36, 2n1p)Tc-87 at the Grand Accelerateur National d'Ions Lourds (GANIL), France. The AGATA spectrometer was used in conjunction with the auxiliary NEDA, Neutron Wall, and DIAMANT detector arrays to measure coincident prompt gamma rays, neutrons, and charged particles emitted in the reaction. A level scheme of Tc-87 from the (9/2(g.s.)(+)) state to the (33/2(1)(+)) state was established based on six mutually coincident gamma-ray transitions. The constructed level structure exhibits a rotational behavior with a sharp backbending at (h) over bar omega approximate to 0.50 MeV. A decrease in alignment frequency and increase in alignment sharpness in the odd-mass isotonic chains around N = 44 is proposed as an effect of the enhanced isoscalar neutron-proton interactions in odd-mass nuclei when approaching the N = Z line.
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Fernandez, A. et al, Gadea, A., Perez-Vidal, R. M., Jurado, M., & Domingo-Pardo, C. (2021). Reinterpretation of excited states in Po-212: Shell-model multiplets rather than alpha-cluster states. Phys. Rev. C, 104(5), 054316–19pp.
Abstract: A gamma-ray spectroscopic study of Po-212 was performed at the Grand Accelerateur National d'Ions Lourds, using the inverse kinematics alpha-transfer reaction C-12(Pb-208, Po-212) Be-8 and the AGATA spectrometer. A careful analysis based on gamma gamma coincidence relations allowed us to establish 14 new excited states in the energy range between 1.9 and 3.3 MeV. None of these states, however, can be considered as candidates for the levels with spins and parities of 1(-) and 2(-) and excitation energies below 2.1 MeV, which have been predicted by recent alpha-cluster model calculations. A systematic comparison of the experimentally established excitation scheme of Po-212 with shell-model calculations was performed. This comparison suggests that the six states with excitation energies (spins and parities) of 1744 (4(-)), 1751 (8(-)), 1787 (6(-)), 1946 (4(-)), 1986 (8(-)), and 2016 (6(-)) keV, which previously were interpreted as alpha-cluster states, may in fact be of positive parity and belong to low-lying shell-model multiplets. This reinterpretation of the structure of Po-212 is supported by experimental information with respect to the linear polarization of gamma rays, which suggests a magnetic character of the 432-keV gamma ray decaying from the state at an excitation energy of 1787 keV to the 6(1)(+) yrast state, and exclusive reaction cross sections.
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n_TOF Collaboration(Gawlik, A. et al), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2021). Measurement of the Ge-76(n, gamma) cross section at the n_TOF facility at CERN. Phys. Rev. C, 104(4), 044610–7pp.
Abstract: The Ge-76(n, gamma) reaction has been measured at the n_TOF facility at CERN via the time-of-flight technique. Neutron capture cross sections on Ge-76 are of interest to a variety of low-background experiments, such as neutrinoless double beta decay searches, and to nuclear astrophysics. We have determined resonance capture kernels up to 52 keV neutron energy and used the new data to calculate Maxwellian-averaged neutron capture cross sections for k(B)T values of 5 to 100 keV.
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