Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Aysto, J., Jordan, D., et al. (2019). Large Impact of the Decay of Niobium Isomers on the Reactor (v)over-bar(e) Summation Calculations. Phys. Rev. Lett., 122(4), 042502–6pp.
Abstract: Even mass neutron-rich niobium isotopes are among the principal contributors to the reactor antineutrino energy spectrum. They are also among the most challenging to measure due to the refractory nature of niobium, and because they exhibit isomeric states lying very close in energy. The beta-intensity distributions of Nb-100gs,Nb-100m and Nb-102gs,Nb-02m beta decays have been determined using the total absorption.-ray spectroscopy technique. The measurements were performed at the upgraded Ion Guide Isotope Separator On-Line facility at the University of Jyvaskyla. Here, the double Penning trap system JYFLTRAP was employed to disentangle the beta decay of the isomeric states. The new data obtained in this challenging measurement have a large impact in antineutrino summation calculations. For the first time the discrepancy between the summation model and the reactor antineutrino measurements in the region of the shape distortion has been reduced.
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Delafosse, C. et al, Gadea, A., Perez-Vidal, R. M., & Domingo-Pardo, C. (2018). Pseudospin Symmetry and Microscopic Origin of Shape Coexistence in the Ni-78 Region: A Hint from Lifetime Measurements. Phys. Rev. Lett., 121(19), 192502–7pp.
Abstract: Lifetime measurements of excited states of the light N = 52 isotones Kr-88, Se-86, and Ge-84 have been performed, using the recoil distance Doppler shift method and VAMOS and AGATA spectrometers for particle identification and gamma spectroscopy, respectively. The reduced electric quadrupole transition probabilities B(E2; 2(+)-> 0(+)) and B(E2; 4(+)-> 2(+)) were obtained for the first time for the hard-to-reach 84Ge. While the B(E2; 2(+)-> 0(+) ) values of Kr-88, Se-86 saturate the maximum quadrupole collectivity offered by the natural valence (3s, 2d, 1g(7/2), 1h(11/2)) space of an inert Ni-78 core, the value obtained for Ge-84 largely exceeds it, suggesting that shape coexistence phenomena, previously reported at N less than or similar to 49, extend beyond N = 50. The onset of collectivity at Z = 32 is understood as due to a pseudo-SU(3) organization of the proton single-particle sequence reflecting a clear manifestation of pseudospin symmetry. It is realized that the latter provides actually reliable guidance for understanding the observed proton and neutron single particle structure in the whole medium-mass region, from Ni to Sn, pointing towards the important role of the isovector-vector rho field in shell-structure evolution.
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Gottardo, A. et al, Gadea, A., & Algora, A. (2019). New spectroscopic information on Tl-211,Tl-213: A changing structure beyond the N=126 shell closure. Phys. Rev. C, 99(5), 054326–7pp.
Abstract: The neutron-rich isotopes Tl-211,Tl-213, beyond the N = 126 shell closure, have been studied for the first time in isomer gamma-ray decay, exploiting the fragmentation of a primary uranium beam at the Fragment Separator-Rare Isotopes Investigation at GSI setup. The observed isomeric states in Tl-211,Tl-213 show a deviation from the seniority-like scheme of Tl-209. The possible interpretation of the data is discussed on the basis of energy-level systematics and shell-model calculations.
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Diel, F., Fujita, Y., Fujita, H., Cappuzzello, F., Ganioglu, E., Grewe, E. W., et al. (2019). High-resolution study of the Gamow-Teller (GT_) strength in the Zn-64(He-3, t) Ga-64 reaction. Phys. Rev. C, 99(5), 054322–10pp.
Abstract: Gamow-Teller (GT) transitions starting from the T-z = +2 nucleus Zn-64 to the T-z = +1 nucleus Ga-64 were studied in a (p, n)-type (He-3,t) charge-exchange reaction at a beam energy of 140 MeV/nucleon and scattering angles close to 0 degrees. Here, T-z is the z component of the isospin T. The experiment was conducted at the Research Center for Nuclear Physics (RCNP) in Osaka, Japan. An energy resolution of approximate to 34 keV was achieved by applying beam matching techniques to the Grand Raiden magnetic spectrometer system. With our good resolution, we could observe GT strength fragmented in many states up to an excitation energy of approximate to 11 MeV. By performing angular distribution analysis, we could identify states in Ga-64 excited by GT transitions. The reduced GT transition strengths [B(GT)values] were calculated assuming the proportionality between the cross sections and the B(GT)values. Shell-model calculations using the GXPF1J interaction reproduced the B(GT)strength distribution throughout the spectrum. States with isospin T = 3 were identified by comparing the Zn-64(He-3,t)Ga-64 spectrum with a Zn-64(d, He-2)Cu-64 spectrum. Relative excitation energies of the corresponding structures are in good agreement, supporting the robustness of isospin symmetry in the mass number A = 64 nuclei.
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Dombos, A. C., Spyrou, A., Naqvi, F., Quinn, S. J., Liddick, S. N., Algora, A., et al. (2019). beta-decay half-lives of neutron-rich nuclides in the A=100-110 mass region. Phys. Rev. C, 99(1), 015802–8pp.
Abstract: beta-decay half-lives of neutron-rich nuclides in the A = 100-110 mass region have been measured using an implantation station installed inside of the Summing NaI(T1) (SuN) detector at the National Superconducting Cyclotron Laboratory. Accurate half-lives for these nuclides are important for nuclear astrophysics, nuclear structure, and nuclear technology. The half-lives from the present work are compared with previous measurements, showing overall good agreement.
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AGATA Collaboration(Kaya, L. et al), & Gadea, A. (2019). Identification of high-spin proton configurations in Ba-136 and Ba-137. Phys. Rev. C, 99(1), 014301–19pp.
Abstract: The high-spin structures of Ba-136 and Ba-137 are investigated after multinucleon-transfer (MNT) and fusion-evaporation reactions. Ba-136 is populated in a Xe-136 + U-238 MNT reaction employing the high-resolution Advanced GAmma Tracking Array (AGATA) coupled to the magnetic spectrometer PRISMA at the Laboratori Nazionali di Legnaro, Italy, and in two Be-9 + Te-130 fusion-evaporation reactions using the High-efficiency Observatory for gamma-Ray Unique Spectroscopy (HORUS) at the FN tandem accelerator of the University of Cologne, Germany. Furthermore, both isotopes are populated in an elusive reaction channel in the B-11 + Te-130 fusion-evaporation reaction utilizing the HORUS gamma-ray array. The level scheme above the J(pi) = 10(+) isomer in Ba-136 is revised and extended up to an excitation energy of approximately 5.5 MeV. From the results of angular-correlation measurements, the E-x = 3707- and E-x = 4920-keV states are identified as the bandheads of positive- and negative-parity cascades. While the high-spin regimes of both Te-132 and Xe-134 are characterized by high-energy 12(+) -> 10(+) transitions, the Ba-136 E2 ground-state band is interrupted by negative-parity states only a few hundred keV above the J(pi) = 10(+) isomer. Furthermore, spins are established for several hitherto unassigned high-spin states in Ba-137. The new results close a gap along the high-spin structure of N < 82 Ba isotopes. Experimental results are compared to large-scale shell-model calculations employing the GCN50:82, Realistic SM, PQM130, and SN100PN interactions. The calculations suggest that the bandheads of the positive-parity bands in both isotopes are predominantly of proton character.
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Kaya, L. et al, & Gadea, A. (2018). Millisecond 23/2(+) isomers in the N=79 isotones Xe-133 and Ba-135. Phys. Rev. C, 98(5), 054312–16pp.
Abstract: Detailed information on isomeric states in A approximate to 135 nuclei is exploited to shell-model calculations in the region northwest of doubly magic nucleus Sn-132. The N = 79 isotones Xe-133 and Ba-135 are studied after multinucleon transfer in the Xe-136 + Pb-208 reaction employing the high-resolution Advanced GAmma Array (AGATA) coupled to the magnetic spectrometer PRISMA at the Laboratori Nazionali di Legnaro, Italy and in a pulsed-beam experiment at the FN tandem accelerator of the University of Cologne Germany utilizing a Be-9 + Te-130 fusion-evaporation reaction at a beam energy of 40 MeV. Isomeric states are identified via delayed gamma-ray spectroscopy. Hitherto tentative excitation energy spin and parity assignments of the 2017-keV J(pi) = 23/2(+) isomer in Xe-133 are confirmed and a half-life of T-1/2 = 8.64(13) ms is measured. The 2388-keV state in Ba-135. is identified as a J(pi) = 23/2(+) isomer with a half-life of 1.06(4) ms. The new results show a smooth onset of isomeric J(pi) = 23/2(+) states along the N = 79 isotones and close a gap in the high-spin systematics towards the recently investigated J(pi) = 23/2(+) isomer in Nd-139. The resulting systematics of M2 reduced transition probabilities is discussed within the of the nuclear shell model. Latest large-scale shell-model calculations employing the SN100PN, GCN50:82, SN100-KTH and a realistic effective interaction reproduce the experimental findings generally well and give insight into the structure of the isomers.
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n_TOF Collaboration(Praena, J. et al), Domingo-Pardo, C., Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2018). Measurement and resonance analysis of the S-33(n,alpha)Si-30 cross section at the CERN n_TOF facility in the energy region from 10 to 300 keV. Phys. Rev. C, 97(6), 064603–10pp.
Abstract: The (33)(n , alpha)Si-30 cross section has been measured at the neutron time-of-flight (n_TOF) facility at CERN in the neutron energy range from 10 to 300 keV relative to the B-10(n, alpha)(7) Li cross-section standard. Both reactions were measured simultaneously with a set of micromegas detectors. The flight path of 185 m has allowed us to obtain the cross section with high-energy resolution. An accurate description of the resonances has been performed by means of the multilevel multichannel R-matrix code SAMMY. The results show a significantly higher area of the biggest resonance (13.45 keV) than the unique high-resolution (n , alpha) measurement. The new parametrization of the 13.45-keV resonance is similar to that of the unique transmission measurement. This resonance is a matter of research in neutron-capture therapy. The S-33(n, alpha)Si-30 cross section has been studied in previous works because of its role in the production of S-36 in stars, which is currently overproduced in stellar models compared to observations.
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n_TOF Collaboration(Mendoza, E. et al), Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2018). Measurement and analysis of the Am-241 neutron capture cross section at the n_TOF facility at CERN. Phys. Rev. C, 97(5), 054616–21pp.
Abstract: The Am-241(n, gamma) cross section has been measured at the nTOF facility at CERN with the nTOF BaF2 Total Absorption Calorimeter in the energy range between 0.2 eV and 10 keV. Our results are analyzed as resolved resonances up to 700 eV, allowing a more detailed description of the cross section than in the current evaluations, which contain resolved resonances only up to 150-160 eV. The cross section in the unresolved resonance region is perfectly consistent with the predictions based on the average resonance parameters deduced from the resolved resonances, thus obtaining a consistent description of the cross section in the full neutron energy range under study. Below 20 eV, our results are in reasonable agreement with JEFF-3.2 as well as with the most recent direct measurements of the resonance integral, and differ up to 20-30% with other experimental data. Between 20 eV and 1 keV, the disagreement with other experimental data and evaluations gradually decreases, in general, with the neutron energy. Above 1 keV, we find compatible results with previously existing values.
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n_TOF Collaboration(Lerendegui-Marco, J. et al.), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2018). Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility. Phys. Rev. C, 97(2), 024605–21pp.
Abstract: The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA.
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