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Chen, Z. Q. et al, & Montaner-Piza, A. (2019). Proton Shell Evolution below Sn-132: First Measurement of Low-Lying beta-Emitting Isomers in Ag-123,Ag-325. Phys. Rev. Lett., 122(21), 212502–6pp.
Abstract: The beta-delayed gamma-ray spectroscopy of neutron-rich Ag-123,Ag-325 isotopes is investigated at the Radioactive Isotope Beam Factory of RIKEN, and the long-predicted 1/2(-) beta-emitting isomers in Ag-123,Ag-325 are identified for the first time. With the new experimental results, the systematic trend of energy spacing between the lowest 9/2(+) and 1/2(-) levels is extended in Ag isotopes up to N = 78, providing a clear signal for the reduction of the Z = 40 subshell gap in Ag towards N = 82. Shell-model calculations with the state-of-the-art V-MU plus M3Y spin-orbit interaction give a satisfactory description of the low-lying states in Ag-123,Ag-325. The tensor force is found to play a crucial role in the evolution of the size of the Z = 40 subshell gap. The observed inversion of the single-particle levels around Ag-123 can be well interpreted in terms of the monopole shift of the pi 1g(9/2) orbitals mainly caused by the increasing occupation of nu 1h(11/2) orbitals.
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Guadilla, V. et al, Algora, A., Tain, J. L., Agramunt, J., Aysto, J., Jordan, D., et al. (2019). Large Impact of the Decay of Niobium Isomers on the Reactor (v)over-bar(e) Summation Calculations. Phys. Rev. Lett., 122(4), 042502–6pp.
Abstract: Even mass neutron-rich niobium isotopes are among the principal contributors to the reactor antineutrino energy spectrum. They are also among the most challenging to measure due to the refractory nature of niobium, and because they exhibit isomeric states lying very close in energy. The beta-intensity distributions of Nb-100gs,Nb-100m and Nb-102gs,Nb-02m beta decays have been determined using the total absorption.-ray spectroscopy technique. The measurements were performed at the upgraded Ion Guide Isotope Separator On-Line facility at the University of Jyvaskyla. Here, the double Penning trap system JYFLTRAP was employed to disentangle the beta decay of the isomeric states. The new data obtained in this challenging measurement have a large impact in antineutrino summation calculations. For the first time the discrepancy between the summation model and the reactor antineutrino measurements in the region of the shape distortion has been reduced.
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Gottardo, A. et al, Gadea, A., & Algora, A. (2019). New spectroscopic information on Tl-211,Tl-213: A changing structure beyond the N=126 shell closure. Phys. Rev. C, 99(5), 054326–7pp.
Abstract: The neutron-rich isotopes Tl-211,Tl-213, beyond the N = 126 shell closure, have been studied for the first time in isomer gamma-ray decay, exploiting the fragmentation of a primary uranium beam at the Fragment Separator-Rare Isotopes Investigation at GSI setup. The observed isomeric states in Tl-211,Tl-213 show a deviation from the seniority-like scheme of Tl-209. The possible interpretation of the data is discussed on the basis of energy-level systematics and shell-model calculations.
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Diel, F., Fujita, Y., Fujita, H., Cappuzzello, F., Ganioglu, E., Grewe, E. W., et al. (2019). High-resolution study of the Gamow-Teller (GT_) strength in the Zn-64(He-3, t) Ga-64 reaction. Phys. Rev. C, 99(5), 054322–10pp.
Abstract: Gamow-Teller (GT) transitions starting from the T-z = +2 nucleus Zn-64 to the T-z = +1 nucleus Ga-64 were studied in a (p, n)-type (He-3,t) charge-exchange reaction at a beam energy of 140 MeV/nucleon and scattering angles close to 0 degrees. Here, T-z is the z component of the isospin T. The experiment was conducted at the Research Center for Nuclear Physics (RCNP) in Osaka, Japan. An energy resolution of approximate to 34 keV was achieved by applying beam matching techniques to the Grand Raiden magnetic spectrometer system. With our good resolution, we could observe GT strength fragmented in many states up to an excitation energy of approximate to 11 MeV. By performing angular distribution analysis, we could identify states in Ga-64 excited by GT transitions. The reduced GT transition strengths [B(GT)values] were calculated assuming the proportionality between the cross sections and the B(GT)values. Shell-model calculations using the GXPF1J interaction reproduced the B(GT)strength distribution throughout the spectrum. States with isospin T = 3 were identified by comparing the Zn-64(He-3,t)Ga-64 spectrum with a Zn-64(d, He-2)Cu-64 spectrum. Relative excitation energies of the corresponding structures are in good agreement, supporting the robustness of isospin symmetry in the mass number A = 64 nuclei.
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Gjestvang, D. et al, & Algora, A. (2023). Examination of how properties of a fissioning system impact isomeric yield ratios of the fragments. Phys. Rev. C, 108(6), 064602–12pp.
Abstract: The population of isomeric states in the prompt decay of fission fragments-so-called isomeric yield ratios (IYRs)-is known to be sensitive to the angular momentum J that the fragment emerged with, and may therefore contain valuable information on the mechanism behind the fission process. In this work, we investigate how changes in the fissioning system impact the measured IYRs of fission fragments to learn more about what parameters affect angular momentum generation. To enable this, a new technique for measuring IYRs is first demonstrated. It is based on the time of arrival of discrete gamma rays, and has the advantage that it enables the study of the IYR as a function of properties of the partner nucleus. This technique is used to extract the IYR of 134Te, strongly populated in actinide fission, from the three different fissioning systems: 232Th(n, f), 238U(n, f), at two different neutron energies, as well as 252Cf(sf). The impacts of changing the fissioning system, the compound nuclear excitation energy, the minimum J of the binary partner, and the number of neutrons emitted on the IYR of 134Te are determined. The decay code TALYS is used in combination with the fission simulation code FREYA to calculate the primary fragment angular momentum from the IYR. We find that the IYR of 134Te has a slope of 0.004 +/- 0.002 with increase in compound nucleus (CN) mass. When investigating the impact on the IYR of increased CN excitation energy, we find no change with an energy increase similar to the difference between thermal and fast fission. By varying the mass of the partner fragment emerging with 134Te, it is revealed that the IYR of 134Te is independent of the total amount of prompt neutrons emitted from the fragment pair. This indicates that neutrons carry minimal angular momentum away from the fission fragments. Comparisons with the FREYA+TALYS simulations reveal that the average angular momentum in 134Te following 238U(n, f) is 6.0 h over bar . This is not consistent with the value deduced from recent CGMF calculations. Finally, the IYR sensitivity to the angular momentum of the primary fragment is discussed. These results are not only important to help understanding the underlying mechanism in nuclear fission, but can also be used to constrain and benchmark fission models, and are relevant to the gamma -ray heating problem of reactors.
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Yokoyama, R. et al, Tain, J. L., Algora, A., Agramunt, J., Domingo-Pardo, C., Morales, A. I., et al. (2023). β-delayed neutron emissions from N > 50 gallium isotopes. Phys. Rev. C, 108(6), 064307–15pp.
Abstract: beta-delayed gamma-neutron spectroscopy has been performed on the decay of A=84 to 87 gallium isotopes at the RI-beam Factory at the RIKEN Nishina Center using a high-efficiency array of 3He neutron counters (BRIKEN). beta-2n-gamma events were measured in the decays of all of the four isotopes for the first time, which is direct evidence for populating the excited states of two-neutron daughter nuclei. Detailed decay schemes with the gamma branching ratios were obtained for these isotopes, and the neutron emission probabilities (P-xn) were updated from the previous study. Hauser-Feshbach statistical model calculations were performed to understand the experimental branching ratios. We found that the P-1n and P-2n values are sensitive to the nuclear level densities of 1n daughter nuclei and showed that the statistical model reproduced the P-2n/P-1n ratio better when experimental levels plus shell-model level densities fit by the Gilbert-Cameron formula were used as the level-density input. We also showed the neutron and gamma branching ratios are sensitive to the ground-state spin of the parent nucleus. Our statistical model analysis suggested J <= 3 for the unknown ground-state spin of the odd-odd nucleus Ga-86, from the I gamma(4(+)-> 2(+))/I-gamma(2(+)-> 0(+)) ratio of Ga-84 and the P-2n/P-1n ratio. These results show the necessity of detailed understanding of the decay scheme, including data from neutron spectroscopy, in addition to gamma measurements of the multineutron emitters.
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Davesne, D., Holt, J. W., Navarro, J., & Pastore, A. (2023). Landau sum rules with noncentral quasiparticle interactions. Phys. Rev. C, 108(3), 034003–7pp.
Abstract: We derive explicit expressions for the Landau sum rules for the case of the most general spin-dependent quasiparticle interaction including all possible tensor interactions. For pure neutron matter, we investigate the convergence of the sum rules at different orders of approximation. Employing modern nuclear Hamiltonians based on chiral effective field theory, we find that the inclusion of noncentral interactions improves the convergence of the sum rules only for low densities (n <= 0.1 fm-3). Around nuclear matter saturation density, we find that even ostensibly perturbative nuclear interactions violate the sum rules considerably. By artificially weakening the strength of the nuclear Hamiltonian, the convergence can be improved.
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IDS Collaboration(Heideman, J. et al), Algora, A., & Morales, A. I. (2023). Evidence of nonstatistical neutron emission following beta decay near doubly magic Sn-132. Phys. Rev. C, 108(2), 024311–9pp.
Abstract: Models of the beta-delayed neutron emission (beta n) assume that neutrons are emitted statistically via an intermediate compound nucleus post beta decay. Evidence to the contrary was found in an In-134 beta-decay experiment carried out at ISOLDE CERN. Neutron emission probabilities from the unbound states in Sn-134 to known low-lying, single-particle states in Sn-133 were measured. The neutron energies were determined using the time-of-flight technique, and the subsequent decay of excited states in Sn-133 was studied using gamma-ray detectors. Individual beta n probabilities were determined by correlating the relative intensities and energies of neutrons and gamma rays. The experimental data disagree with the predictions of representative statistical models which are based upon the compound nucleus postulate. Our results suggest that violation of the compound nucleus assumption may occur in beta-delayed neutron emission. This impacts the neutron-emission probabilities and other properties of nuclei participating in the r-process. A model of neutron emission, which links the observed neutron emission probabilities to nuclear shell effects, is proposed.
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n_TOF Collaboration(Michalopoulou, V. et al), Babiano-Suarez, V., Caballero, L., Domingo-Pardo, C., Ladarescu, I., & Tain, J. L. (2023). Measurement of the neutron-induced fission cross section of Th-230 at the CERN n_TOF facility. Phys. Rev. C, 108(1), 014616–15pp.
Abstract: The neutron-induced fission cross section of Th-230 has been measured at the neutron time-of-flight facility n_TOF located at CERN. The experiment was performed at the experimental area EAR-1 with a neutron flight path of 185 m, using Micromegas detectors for the detection of the fission fragments. The Th-230(n, f ) cross section was determined relative to the U-235(n, f ) one, covering the energy range from the fission threshold up to 400 MeV. The results from the present work are compared with existing cross-section datasets and the observed discrepancies are discussed and analyzed. Finally, using the code EMPIRE 3.2.3 a theoretical study, based on the statistical model, was performed leading to a satisfactory reproduction of the experimental results with the proper tuning of the respective parameters, while for incident neutron energy beyond 200 MeV the fission of( 230)Th was described by Monte Carlo simulations.
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IDS Collaboration(Stryjczyk, M. et al.), & Nacher, E. (2023). Simultaneous gamma-ray and electron spectroscopy of 182,184,186Hg isotopes. Phys. Rev. C, 108(1), 014308–20pp.
Abstract: Background: The mercury isotopes around N = 104 are a well-known example of nuclei exhibiting shape coex-istence. Mixing of configurations can be studied by measuring the monopole strength rho^2(E0), however, currently the experimental information is scarce and lacks precision, especially for the I^pi -> I^pi (I not = 0) transitions. Purpose: The goals of this study were to increase the precision of the known branching ratios and internal conversion coefficients, to increase the amount of available information regarding excited states in 182,184,186Hg, and to interpret the results in the framework of shape coexistence using different models. Method: The low-energy structures in 182,184,186Hg were populated in the & beta; decay of 182,184,186Tl, produced at ISOLDE, CERN and purified by laser ionization and mass separation. The & gamma;-ray and internal conversion electron events were detected by five germanium clover detectors and a segmented silicon detector, respectively, and correlated in time to build decay schemes.Results: In total, 193, 178, and 156 transitions, including 144, 140, and 108 observed for the first time in a & beta;-decay experiment, were assigned to 182,184,186Hg, respectively. Internal conversion coefficients were determined for 23 transitions, out of which 12 had an E0 component. Extracted branching ratios allowed the sign of the interference term in 182Hg as well as & rho;2(E 0; 0+2 & RARR; 0+1 ) and B(E2; 0+2 & RARR; 2+1 ) in 184Hg to be determined. By means of electron-electron coincidences, the 0+3 state was identified in 184Hg. The experimental results were qualitatively reproduced by five theoretical approaches, the interacting boson model with configuration mixing with two different parametrizations, the general Bohr Hamiltonian, the beyond mean-field model, and the symmetry-conserving configuration-mixing model. However, a quantitative description is lacking. Conclusions: The presence of shape coexistence in neutron-deficient mercury isotopes was confirmed and evidence for the phenomenon existing at higher energies was found. The new experimental results provide important spectroscopic input for future Coulomb excitation studies.
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