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Author |
n_TOF Collaboration (Stamatopoulos, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Investigation of the Pu-240(n, f) reaction at the n_TOF/EAR2 facility in the 9 meV-6 MeV range |
Type |
Journal Article |
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Year |
2020 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
102 |
Issue |
1 |
Pages |
014616 - 23pp |
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Keywords |
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Abstract |
Background: Nuclear waste management is considered amongst the major challenges in the field of nuclear energy. A possible means of addressing this issue is waste transmutation in advanced nuclear systems, whose operation requires a fast neutron spectrum. In this regard, the accurate knowledge of neutron-induced reaction cross sections of several (minor) actinide isotopes is essential for design optimization and improvement of safety margins of such systems. One such case is Pu-240, due to its accumulation in spent nuclear fuel of thermal reactors and its usage in fast reactor fuel. The measurement of the Pu-240(n, f) cross section was previously attempted at the CERN nTOF facility EAR1 measuring station using the time-of-flight technique. Due to the low amount of available material and the given flux at EAR1, the measurement had to last several months to achieve a sufficient statistical accuracy. This long duration led to detector deterioration due to the prolonged exposure to the high alpha activity of the fission foils, therefore the measurement could not be successfully completed. Purpose: It is aimed to determine whether it is feasible to study neutron-induced fission at nTOF/EAR2 and provide data on the Pu-240(n, f) reaction in energy regions requested for applications. Methods: The study of the Pu-240(n, f) reaction was made at a new experimental area (EAR2) with a shorter flight path which delivered on average 30 times higher flux at fast neutron energies. This enabled the measurement to be performed much faster, thus limiting the exposure of the detectors to the intrinsic activity of the fission foils. The experimental setup was based on microbulk Micromegas detectors and the time-of-flight data were analyzed with an optimized pulse-shape analysis algorithm. Special attention was dedicated to the estimation of the non-negligible counting loss corrections with the development of a new methodology, and other corrections were estimated via Monte Carlo simulations of the experimental setup. Results: This new measurement of the Pu-240(n, f) cross section yielded data from 9 meV up to 6 MeV incident neutron energy and fission resonance kernels were extracted up to 10 keV. Conclusions: Neutron-induced fission of high activity samples can be successfully studied at the n_TOF/EAR2 facility at CERN covering a wide range of neutron energies, from thermal to a few MeV. |
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Address |
[Stamatopoulos, A.; Tsinganis, A.; Kokkoris, M.; Vlastou, R.; Diakaki, M.] Natl Tech Univ Athens, Athens, Greece, Email: athanasios.stamatopoulos@cern.ch |
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Amer Physical Soc |
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English |
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ISSN |
0556-2813 |
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Conference |
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Notes |
WOS:000551057500002 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4466 |
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Author |
AGATA Collaboration (Goldkuhle, A. et al); Perez-Vidal, R.M.; Domingo-Pardo, C.; Gadea, A. |
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Title |
Lifetime measurements in Ti-52,Ti-54 to study shell evolution toward N=32 |
Type |
Journal Article |
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Year |
2019 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
100 |
Issue |
5 |
Pages |
054317 - 12pp |
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Keywords |
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Abstract |
Lifetimes of the excited states in the neutron-rich Ti-52,Ti-54 nuclei, produced in a multinucleon-transfer reaction, were measured by employing the Cologne plunger device and the recoil-distance Doppler-shift method. The experiment was performed at the Grand Accelerateur National d'Ions Lourds facility by using the Advanced Gamma Tracking Array for the gamma-ray detection, coupled to the large-acceptance variable mode spectrometer for an event-by-event particle identification. A comparison between the transition probabilities obtained from the measured lifetimes of the 2(1)(+) to 8(1)(+) yrast states in Ti-52,Ti-54 and that from the shell-model calculations based on the well-established GXPF1A, GXPF1B, and KB3G fp shell interactions support the N = 32 subshell closure. The B(E2) values for Ti-52 determined in this work are in disagreement with the known data, but are consistent with the predictions of the shell-model calculations and reduce the previously observed pronounced staggering across the even-even titanium isotopes. |
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Address |
[Goldkuhle, A.; Fransen, C.; Blazhev, A.; Beckers, M.; Birkenbach, B.; Braunroth, T.; Dewald, A.; Eberth, J.; Hess, H.; Jolie, J.; Litzinger, J.; Mueller-Gatermann, C.; Reiter, P.; Vogt, A.; Warr, N.; Zell, K. O.] Univ Cologne, Inst Kernphys, D-50937 Cologne, Germany, Email: agoldkuhle@ikp.uni-koeln.de |
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Amer Physical Soc |
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English |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Conference |
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Notes |
WOS:000496925500001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4201 |
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Author |
Fujita, H. et al; Algora, A.; Estevez-Aguado, E.; Molina, F.; Rubio, B. |
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Title |
Experimental study of Gamow-Teller transitions via the high-energy-resolution O-18(He-3, t)F-18 reaction: Identification of the low-energy “super” -Gamow-Teller state |
Type |
Journal Article |
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Year |
2019 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
100 |
Issue |
3 |
Pages |
034618 - 13pp |
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Keywords |
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Abstract |
Using the high-resolution O-18(He-3, t)F-18 reaction at 0 degrees and at 140 MeV/nucleon, Gamow-Teller (GT) transitions were studied. A high energy resolution of 31 keV was achieved by applying dispersion matching techniques. The main part of the observed GT transition strength is concentrated in the transition to the F-18 ground state (g.s.). The absolute values of the reduced GT transition strengths, B(GT), were derived up to E-x = 12 MeV assuming proportionality between the B(GT) values and the reaction cross sections at 0 degrees. The B(GT) value obtained from the beta decay of F-18 (g.s.) -> O-18 (g.s.) was used to determine the proportionality constant. A total B(GT) of 4.06(5) was found and 76(1)% of the strength is concentrated to the ground state of F-18. The obtained B(GT) values were compared with those from the O-18(p, n) F-18 reaction and the mirror symmetric beta(+) decay of Ne-18 -> F-18. The candidates for 1(+) states with isospin T = 1 were identified by comparison with the O-18(p, p') data. The results of shell-model and quasiparticle-random-phase approximation calculations suggest constructive contributions of various configurations to the F-18 ground state, suggesting that this state is the low-energy super GT state. |
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Address |
[Fujita, H.; Fujita, Y.; Adachi, T.; Hatanaka, K.; Hirota, K.; Ishikawa, D.; Matsubara, H.; Okamura, H.; Ong, H. J.; Susoy, G.; Suzuki, T.; Tamii, A.; Zenihiro, J.] Osaka Univ, Res Ctr Nucl Phys, Ibaraki, Osaka 5670047, Japan, Email: hfujita@rcnp.osaka-u.ac.jp |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Conference |
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Notes |
WOS:000488259800004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4165 |
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Author |
Yokoyama, R. et al; Tain, J.L.; Algora, A.; Agramunt, J.; Domingo-Pardo, C.; Morales, A.I.; Rubio, B.; Tolosa-Delgado, A. |
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Title |
Strong one-neutron emission from two-neutron unbound states in beta decays of the r-process nuclei Ga-86,Ga-87 |
Type |
Journal Article |
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Year |
2019 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
100 |
Issue |
3 |
Pages |
031302 - 6pp |
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Keywords |
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Abstract |
beta-delayed one-neutron and two-neutron branching ratios (P-1n and P-2n) have been measured in the decay of A = 84 to 87 Ga isotopes at the Radioactive-Isotope Beam Factory (RIBF) at the RIKEN Nishina Center using a high-efficiency array of He-3 neutron counters (BRIKEN). Two-neutron emission was observed in the decay of Ga-84,Ga-85,Ga-87 for the first time and the branching ratios were measured to be P-2n = 1.6(2)%, 1.3(2)%, and 10.2(28)(stat)(5)(sys)%, respectively. One-neutron branching ratio of Ga-87 (P-1n = 81(9)(stat)(8)(sys)%) and half-life of 29(4) ms were measured for the first time. The branching ratios of Ga-86 were also measured to be P-1n = 74(2)(stat)(8)(sys)% and 16.2(9)(stat)(6)(sys)% with better precision than a previous study. The observation that P-1n > P-2n for both Ga-86,Ga-87 was unexpected and is interpreted as a signature of dominating one-neutron emission from the two-neutron unbound excited states in Ge-86,Ge-87. In order to interpret the experimental results, shell-model and Hauser-Feshbach statistical model calculations of delayed particle and gamma-ray emission probabilities were performed. This model framework reproduces the experimental results. The shell model alone predicts P-2n significantly larger than P-1n for the Ga-87 decay, and it is necessary to invoke a statistical description to successfully explain the observation that P-1n > P-2n. Our new results demonstrate the relevance and importance of a statistical description of neutron emission for the prediction of the decay properties of multineutron emitters and that it must be included in the r-process modeling. |
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Address |
[Yokoyama, R.; Grzywacz, R.; Rasco, B. C.; Brewer, N.; Heideman, J.; King, T. T.; Madurga, M.; Singh, M.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA, Email: ryokoyam@utk.edu |
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Publisher |
Amer Physical Soc |
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English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Conference |
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Notes |
WOS:000486641000001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4145 |
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Author |
AGATA Collaboration (Kaya, L. et al); Gadea, A. |
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Title |
Isomer spectroscopy in Ba-133 and high-spin structure of Ba-134 |
Type |
Journal Article |
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Year |
2019 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
100 |
Issue |
2 |
Pages |
024323 - 18pp |
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Keywords |
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Abstract |
The transitional nuclei Ba-134 and Ba-133 are investigated after multinucleon transfer employing the high-resolution Advanced GAmma Tracking Array coupled to the magnetic spectrometer PRISMA at the Laboratori Nazionali di Legnaro, Italy, and after fusion-evaporation reaction at the FN tandem accelerator of the University of Cologne, Germany. The J(pi) = 19/2(+) state at 1942 keV in Ba-133 is identified as an isomer with a half-life of 66.6(20) ns corresponding to a B(E1) value of 7.7(4) x 10(-6) e(2) fm(2) for the J(pi) = 19/2(+) to J(pi) = 19/2(-) transition. The level scheme of Ba-134 above the J(pi) = 10(+) isomer is extended to approximately 6 MeV. A pronounced backbending is observed at h omega = 0.38 MeV along the positive-parity yrast band. The results are compared to the high-spin systematics of the Z = 56 isotopes. Large-scale shell-model calculations employing the GCN50:82, SN100PN, SNV, PQM130, Realistic SM, and EPQQM interactions reproduce the experimental findings and elucidate the structure of the high-spin states. The shell-model calculations employing the GCN50:82 and PQM130 interactions reproduce alignment properties and provide detailed insight into the microscopic origin of this phenomenon in transitional Ba-134. |
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Address |
[Kaya, L.; Vogt, A.; Reiter, P.; Arnswald, K.; Birkenbach, B.; Blazhev, A.; Droste, M.; Eberth, J.; Esmaylzadeh, A.; Fransen, C.; Hess, H.; Hirsch, R.; Jolie, J.; Karayonchev, V; Kornwebel, L.; Lewandowski, L.; Mueller-Gatermann, C.; Regis, J-M; Saed-Samii, N.; Schomacker, K.; Seidlitz, M.; Siebeck, B.; Wolf, K.; Zell, K. O.] Univ Cologne, Inst Kernphys, D-50937 Cologne, Germany, Email: levent.kaya@ikp.uni-koeln.de |
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Publisher |
Amer Physical Soc |
Place of Publication |
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Language |
English |
Summary Language |
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Original Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
2469-9985 |
ISBN |
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Conference |
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Notes |
WOS:000480688200004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4106 |
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