Abstract: The transitional nucleus Xe-131 is investigated after multinucleon transfer in the Xe-136 + Pb-208 and Xe-136 +U-238 reactions employing the high-resolution Advanced gamma-Tracking Array (AGATA) coupled to the magnetic spectrometer PRISMA at the Laboratori Nazionali di Legnaro, Italy, and as an elusive reaction product in the fusion-evaporation reaction Sn-124(B-11) ,p3n)Xe-131 employing the High-efficiency Observatory for gamma-Ray Unique Spectroscopy (HORUS) gamma-ray array coupled to a double-sided silicon strip detector at the University of Cologne, Germany. The level scheme of Xe-131 is extended to 5 MeV. A pronounced backbending is observed at (h) over bar omega approximate to 0.4 MeV along the negative-parity one-quasiparticle vh(11/12)(alpha = -1/2) band. The results are compared to the high-spin systematics of the Z = 54 isotopes and the N = 77 isotones. Large-scale shell-model calculations employing the PQM130, SN100PN, GCN50:82, SN100-KTH, and a realistic effective interaction reproduce the experimental findings and provide guidance to elucidate the structure of the high-spin states. Further calculations in Xe129-132 provide insight into the changing nuclear structure along the Xe chain towards the N = 82 shell closure. Proton occupancy in the pi 0h(11/2) orbital is found to be decisive for the description of the observed backbending phenomenon.

Abstract: The (33)(n , alpha)Si-30 cross section has been measured at the neutron time-of-flight (n_TOF) facility at CERN in the neutron energy range from 10 to 300 keV relative to the B-10(n, alpha)(7) Li cross-section standard. Both reactions were measured simultaneously with a set of micromegas detectors. The flight path of 185 m has allowed us to obtain the cross section with high-energy resolution. An accurate description of the resonances has been performed by means of the multilevel multichannel R-matrix code SAMMY. The results show a significantly higher area of the biggest resonance (13.45 keV) than the unique high-resolution (n , alpha) measurement. The new parametrization of the 13.45-keV resonance is similar to that of the unique transmission measurement. This resonance is a matter of research in neutron-capture therapy. The S-33(n, alpha)Si-30 cross section has been studied in previous works because of its role in the production of S-36 in stars, which is currently overproduced in stellar models compared to observations.

Abstract: The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA.

Abstract: The population of isomeric states in the prompt decay of fission fragments-so-called isomeric yield ratios (IYRs)-is known to be sensitive to the angular momentum J that the fragment emerged with, and may therefore contain valuable information on the mechanism behind the fission process. In this work, we investigate how changes in the fissioning system impact the measured IYRs of fission fragments to learn more about what parameters affect angular momentum generation. To enable this, a new technique for measuring IYRs is first demonstrated. It is based on the time of arrival of discrete gamma rays, and has the advantage that it enables the study of the IYR as a function of properties of the partner nucleus. This technique is used to extract the IYR of 134Te, strongly populated in actinide fission, from the three different fissioning systems: 232Th(n, f), 238U(n, f), at two different neutron energies, as well as 252Cf(sf). The impacts of changing the fissioning system, the compound nuclear excitation energy, the minimum J of the binary partner, and the number of neutrons emitted on the IYR of 134Te are determined. The decay code TALYS is used in combination with the fission simulation code FREYA to calculate the primary fragment angular momentum from the IYR. We find that the IYR of 134Te has a slope of 0.004 +/- 0.002 with increase in compound nucleus (CN) mass. When investigating the impact on the IYR of increased CN excitation energy, we find no change with an energy increase similar to the difference between thermal and fast fission. By varying the mass of the partner fragment emerging with 134Te, it is revealed that the IYR of 134Te is independent of the total amount of prompt neutrons emitted from the fragment pair. This indicates that neutrons carry minimal angular momentum away from the fission fragments. Comparisons with the FREYA+TALYS simulations reveal that the average angular momentum in 134Te following 238U(n, f) is 6.0 h over bar . This is not consistent with the value deduced from recent CGMF calculations. Finally, the IYR sensitivity to the angular momentum of the primary fragment is discussed. These results are not only important to help understanding the underlying mechanism in nuclear fission, but can also be used to constrain and benchmark fission models, and are relevant to the gamma -ray heating problem of reactors.

Abstract: We derive explicit expressions for the Landau sum rules for the case of the most general spin-dependent quasiparticle interaction including all possible tensor interactions. For pure neutron matter, we investigate the convergence of the sum rules at different orders of approximation. Employing modern nuclear Hamiltonians based on chiral effective field theory, we find that the inclusion of noncentral interactions improves the convergence of the sum rules only for low densities (n <= 0.1 fm-3). Around nuclear matter saturation density, we find that even ostensibly perturbative nuclear interactions violate the sum rules considerably. By artificially weakening the strength of the nuclear Hamiltonian, the convergence can be improved.