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AGATA Collaboration(Kaya, L. et al), & Gadea, A. (2018). High-spin structure in the transitional nucleus Xe-131: Competitive neutron and proton alignment in the vicinity of the N=82 shell closure. Phys. Rev. C, 98(1), 014309–19pp.
Abstract: The transitional nucleus Xe-131 is investigated after multinucleon transfer in the Xe-136 + Pb-208 and Xe-136 +U-238 reactions employing the high-resolution Advanced gamma-Tracking Array (AGATA) coupled to the magnetic spectrometer PRISMA at the Laboratori Nazionali di Legnaro, Italy, and as an elusive reaction product in the fusion-evaporation reaction Sn-124(B-11) ,p3n)Xe-131 employing the High-efficiency Observatory for gamma-Ray Unique Spectroscopy (HORUS) gamma-ray array coupled to a double-sided silicon strip detector at the University of Cologne, Germany. The level scheme of Xe-131 is extended to 5 MeV. A pronounced backbending is observed at (h) over bar omega approximate to 0.4 MeV along the negative-parity one-quasiparticle vh(11/12)(alpha = -1/2) band. The results are compared to the high-spin systematics of the Z = 54 isotopes and the N = 77 isotones. Large-scale shell-model calculations employing the PQM130, SN100PN, GCN50:82, SN100-KTH, and a realistic effective interaction reproduce the experimental findings and provide guidance to elucidate the structure of the high-spin states. Further calculations in Xe129-132 provide insight into the changing nuclear structure along the Xe chain towards the N = 82 shell closure. Proton occupancy in the pi 0h(11/2) orbital is found to be decisive for the description of the observed backbending phenomenon.
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Valiente-Dobon, J. J., Poves, A., Gadea, A., & Fernandez-Dominguez, B. (2018). Broken mirror symmetry in S-36 and Ca-36. Phys. Rev. C, 98(1), 011302–5pp.
Abstract: Shape coexistence is a ubiquitous phenomenon in the neutron-rich nuclei belonging to (or sitting at the shores of) the N = 20 island of inversion (IoI). Exact isospin symmetry predicts the same behavior for their mirrors and the existence of a proton-rich IoI around Z = 20, centered in the (surely unbound) nucleus Ca-32. In this article we show that in Ca-36 and S-36, Coulomb effects break dramatically the mirror symmetry in the excitation energies due to the different structures of the intruder and normal states. The mirror energy difference (MED) of their 2(+) states is known to be very large at – 246 keV. We reproduce this value and predict the first excited state in Ca-36 to be a 0(+) at 2.7 MeV, 250 keV below the first 2(+). In its mirror S-36 the 0(+) lies at 55keV above the 2(+) measured at 3.291 MeV. Our calculations predict a huge MED of -720 keV, that we dub the “colossal” mirror energy difference. A possible reaction mechanism to access the O-2(+) in Ca-36 will be discussed. In addition, we theoretically address the MEDs of the A = 34, T = 3 and A = 32, T = 4 mirrors.
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n_TOF Collaboration(Praena, J. et al), Domingo-Pardo, C., Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2018). Measurement and resonance analysis of the S-33(n,alpha)Si-30 cross section at the CERN n_TOF facility in the energy region from 10 to 300 keV. Phys. Rev. C, 97(6), 064603–10pp.
Abstract: The (33)(n , alpha)Si-30 cross section has been measured at the neutron time-of-flight (n_TOF) facility at CERN in the neutron energy range from 10 to 300 keV relative to the B-10(n, alpha)(7) Li cross-section standard. Both reactions were measured simultaneously with a set of micromegas detectors. The flight path of 185 m has allowed us to obtain the cross section with high-energy resolution. An accurate description of the resonances has been performed by means of the multilevel multichannel R-matrix code SAMMY. The results show a significantly higher area of the biggest resonance (13.45 keV) than the unique high-resolution (n , alpha) measurement. The new parametrization of the 13.45-keV resonance is similar to that of the unique transmission measurement. This resonance is a matter of research in neutron-capture therapy. The S-33(n, alpha)Si-30 cross section has been studied in previous works because of its role in the production of S-36 in stars, which is currently overproduced in stellar models compared to observations.
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n_TOF Collaboration(Mendoza, E. et al), Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2018). Measurement and analysis of the Am-241 neutron capture cross section at the n_TOF facility at CERN. Phys. Rev. C, 97(5), 054616–21pp.
Abstract: The Am-241(n, gamma) cross section has been measured at the nTOF facility at CERN with the nTOF BaF2 Total Absorption Calorimeter in the energy range between 0.2 eV and 10 keV. Our results are analyzed as resolved resonances up to 700 eV, allowing a more detailed description of the cross section than in the current evaluations, which contain resolved resonances only up to 150-160 eV. The cross section in the unresolved resonance region is perfectly consistent with the predictions based on the average resonance parameters deduced from the resolved resonances, thus obtaining a consistent description of the cross section in the full neutron energy range under study. Below 20 eV, our results are in reasonable agreement with JEFF-3.2 as well as with the most recent direct measurements of the resonance integral, and differ up to 20-30% with other experimental data. Between 20 eV and 1 keV, the disagreement with other experimental data and evaluations gradually decreases, in general, with the neutron energy. Above 1 keV, we find compatible results with previously existing values.
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n_TOF Collaboration(Lerendegui-Marco, J. et al.), Domingo-Pardo, C., Tain, J. L., & Tarifeño-Saldivia, A. (2018). Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility. Phys. Rev. C, 97(2), 024605–21pp.
Abstract: The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA.
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AGATA Collaboration(Hadynska-Klek, K. et al), & Gadea, A. (2018). Quadrupole collectivity in Ca-42 from low-energy Coulomb excitation with AGATA. Phys. Rev. C, 97(2), 024326–20pp.
Abstract: ACoulomb-excitation experiment to study electromagnetic properties of Ca-42 was performed using a 170-MeV calcium beam from the TANDEM XPU facility at INFN Laboratori Nazionali di Legnaro. gamma rays from excited states in Ca-42 were measured with the AGATA spectrometer. The magnitudes and relative signs of ten E2 matrix elements coupling six low-lying states in Ca-42, including the diagonal E2 matrix elements of 2(1)(+) and 2(2)(+) states, were determined using the least-squares code GOSIA. The obtained set of reduced E2 matrix elements was analyzed using the quadrupole sum rule method and yielded overall quadrupole deformation for 0(1),(+)(2) and 2(1,2)(+) states, as well as triaxiality for 0(1,2)(+) states, establishing the coexistence of a weakly deformed ground-state band and highly deformed slightly triaxial sideband in Ca-42. The experimental results were compared with the state-of-the-art large-scale shell-model and beyond-mean-field calculations, which reproduce well the general picture of shape coexistence in Ca-42.
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IDS Collaboration(Lica, R. et al), & Morales, A. I. (2018). Evolution of deformation in neutron-rich Ba isotopes up to A=150. Phys. Rev. C, 97(2), 024305–12pp.
Abstract: The occurrence of octupolar shapes in the Ba isotopic chain was recently established experimentally up to N = 90. To further extend the systematics, the evolution of shapes in the most neutron-rich members of the Z = 56 isotopic chain accessible at present, Ba-148,Ba-150, has been studied via beta decay at the ISOLDE Decay Station. This paper reports on the first measurement of the positive-and negative-parity low-spin excited states of 150Ba and presents an extension of the beta-decay scheme of Cs-148. Employing the fast timing technique, half-lives for the 2(1)(+) level in both nuclei have been determined, resulting in T-1/2 = 1.51(1) ns for Ba-148 and T-1/2 = 3.4(2) ns for Ba-150. The systematics of low-spin states, together with the experimental determination of the B(E2 : 2(+) -> 0(+)) transition probabilities, indicate an increasing collectivity in Ba148-150, towards prolate deformed shapes. The experimental data are compared to symmetry conserving configuration mixing (SCCM) calculations, confirming an evolution of increasingly quadrupole deformed shapes with a definite octupolar character.
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n_TOF Collaboration(Wright, T. et al), Domingo-Pardo, C., Giubrone, G., Tain, J. L., & Tarifeño-Saldivia, A. (2017). Measurement of the U-238(n,gamma) cross section up to 80 keV with the Total Absorption Calorimeter at the CERN n_TOF facility. Phys. Rev. C, 96(6), 064601–11pp.
Abstract: The radiative capture cross section of a highly pure (99.999%), 6.125(2) grams and 9.56(5) x 10(-4) atoms/barn areal density U-238 sample has been measured with the Total Absorption Calorimeter (TAC) in the 185 m flight path at the CERN neutron time-of-flight facility n_TOF. This measurement is in response to the NEA High Priority Request list, which demands an accuracy in this cross section of less than 3% below 25 keV. These data have undergone careful background subtraction, with special care being given to the background originating from neutrons scattered by the 238U sample. Pileup and dead-time effects have been corrected for. The measured cross section covers an energy range between 0.2 eV and 80 keV, with an accuracy that varies with neutron energy, being better than 4% below 25 keV and reaching at most 6% at higher energies.
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AGATA Collaboration(Vogt, A. et al), & Gadea, A. (2017). High-spin structures in Xe-132 and Xe-133 and evidence for isomers along the N=79 isotones. Phys. Rev. C, 96(2), 024321–14pp.
Abstract: The transitional nuclei Xe-132 and Xe-133 are investigated after multinucleon-transfer (MNT) and fusionevaporation reactions. Both nuclei are populated (i) in Xe-136 + 2(08P)b MNT reactions employing the highresolution Advanced GAmma Tracking Array (AGATA) coupled to the magnetic spectrometer PRISMA, (ii) in the Xe-136 + Pt-198 MNT reaction employing the GAMMASPHERE spectrometer in combination with the gas-detector array CHICO, and (iii) as an evaporation residue after a Te-130(alpha, xn) Xe134-xn fusion-evaporation reaction employing the HORUS gamma-ray array at the University of Cologne. The high-spin level schemes are considerably extended above the J(pi) = (7(-)) and (10+) isomers in Xe-132 and above the 11/2(-) isomer in Xe-133. The results are compared to the high-spin systematics of the Z = 54 as well as the N = 78 and N = 79 chains. Furthermore, evidence is found for a long-lived (T-1/2 >> μs) isomer in Xe-133 which closes a gap along the N = isotones. Shell-model calculations employing the SN100PN and PQM130 effective interactions reproduce the experimental findings and provide guidance to the interpretation of the observed high-spin features.
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Aydin, S. et al, Gadea, A., & Huyuk, T. (2017). High-spin states and lifetimes in S-33 and shell-model interpretation in the sd-fp space. Phys. Rev. C, 96(2), 024315–10pp.
Abstract: The structure of the S-33 nucleus was investigated in the Mg-24(N-14, alpha p) fusion-evaporation reaction using a 40-MeV N-14 beam. The level scheme was extended up to an excitation energy of 11.7 MeV and spin 19/2+. Lifetimes of the intermediate-and high-spin states have been investigated by the Doppler shift attenuation method. Data were compared with different shell-model calculations where effective interactions involving two main shells, the sd and the fp, are used.
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