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n_TOF Collaboration(Calviani, M. et al), Giubrone, G., & Tain, J. L. (2012). Neutron-induced fission cross section of Cm-245: New results from data taken at the time-of-flight facility n_TOF. Phys. Rev. C, 85(3), 034616–10pp.
Abstract: The neutron-induced fission cross section of Cm-245 was measured at n_TOF in a wide energy range and with high resolution. The energy dependence, measured in a single measurement from 30 meV to 1 MeV neutron energy, has been determined with 5% accuracy relative to the U-235(n,f) cross section. In order to reduce the uncertainty on the absolute value, the data have been normalized at thermal energy to recent measurements performed at ILL and BR1. In the energy range of overlap, the results are in fair agreement with some previous measurements and confirm, on average, the evaluated cross section in the ENDF/B-VII.0 database, although sizable differences are observed for some important resonances below 20 eV. A similar behavior is observed relative to JENDL/AC-2008, a reactor-oriented database for actinides. The new results contribute to the overall improvement of the databases needed for the design of advanced reactor systems and may lead to refinements of fission models for the actinides.
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n_TOF Collaboration(Belloni, F. et al), Domingo-Pardo, C., & Tain, J. L. (2012). Neutron-induced fission cross section measurement of U-233, Am-241 and Am-243 in the energy range 0.5 MeV <= E-n <= 20 MeV at n_TOF at CERN. Phys. Scr., T150, 014005–4pp.
Abstract: Neutron-induced fission cross section measurements of U-233, Am-243 and Am-241 relative to U-235 have been carried out at the neutron time-of-flight facility n_TOF at CERN. A fast ionization chamber has been employed. All samples were located in the same detector; therefore the studied elements and the reference U-235 target are subject to the same neutron beam.
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n_TOF Collaboration(Massimi, C. et al.), Domingo-Pardo, C., Giubrone, G., & Tain, J. L. (2017). Neutron spectroscopy of Mg-26 states: Constraining the stellar neutron source Ne-22(alpha, n)Mg-25. Phys. Lett. B, 768, 1–6.
Abstract: This work reports on accurate, high-resolution measurements of the Mg-25(n, gamma)Mg-26 and Mg-25(n, tot) cross sections in the neutron energy range from thermal to about 300 keV, leading to a significantly improved Mg-25(n, gamma)Mg-26 parametrization. The relevant resonances for n+Mg-25 were characterized from a combined R-matrix analysis of the experimental data. This resulted in an unambiguous spin/parity assignment of the corresponding excited states in Mg-26. With this information experimental upper limits of the reaction rates for Ne-22(alpha, n)Mg-25 and Ne-22(alpha, gamma)Mg-26 were established, potentially leading to a significantly higher (alpha, n)/(alpha, gamma) ratio than previously evaluated. The impact of these results has been studied for stellar models in the mass range 2 to 25 M-circle dot. (C) 2017 The Author(s). Published by Elsevier B.V.
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n_TOF Collaboration(Fujii, K. et al), Domingo-Pardo, C., & Tain, J. L. (2010). Neutron physics of the Re/Os clock. III. Resonance analyses and stellar (n, gamma) cross sections of Os-186,Os-187,Os-188. Phys. Rev. C, 82(1), 015804–18pp.
Abstract: Neutron resonance analyses have been performed for the capture cross sections of Os-186, Os-187, and Os-188 measured at the n_TOF facility at CERN. Resonance parameters have been extracted up to 5, 3, and 8 keV, respectively, using the SAMMY code for a full R-matrix fit of the capture yields. From these results average resonance parameters were derived by a statistical analysis to provide a comprehensive experimental basis for modeling of the stellar neutron capture rates of these isotopes in terms of the Hauser-Feshbach statistical model. Consistent calculations for the capture and inelastic reaction channels are crucial for the evaluation of stellar enhancement factors to correct the Maxwellian averaged cross sections obtained from experimental data for the effect of thermally populated excited states. These factors have been calculated for the full temperature range of current scenarios of s-process nucleosynthesis using the combined information of the experimental data in the region of resolved resonances and in the continuum. The consequences of this analysis for the s-process component of the Os-187 abundance and the related impact on the evaluation of the time duration of galactic nucleosynthesis via the Re/Os cosmochronometer are discussed.
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n_TOF Collaboration(Mosconi, M. et al), Domingo-Pardo, C., & Tain, J. L. (2010). Neutron physics of the Re/Os clock. I. Measurement of the (n, gamma) cross sections of Os-186,Os-187,Os-188 at the CERN n_TOF facility. Phys. Rev. C, 82(1), 015802–10pp.
Abstract: The precise determination of the neutron capture cross sections of Os-186 and Os-187 is important to define the s-process abundance of Os-187 at the formation of the solar system. This quantity can be used to evaluate the radiogenic component of the abundance of Os-187 due to the decay of the unstable Re-187 (t(1/2) = 41.2 Gyr) and from this to infer the time duration of the nucleosynthesis in our galaxy (Re/Os cosmochronometer). The neutron capture cross sections of Os-186, Os-187, and Os-188 have been measured at the CERN n_TOF facility from 1 eV to 1 MeV, covering the entire energy range of astrophysical interest. The measurement has been performed by time-of-flight technique using isotopically enriched samples and two C6D6 scintillation detectors for recording the prompt. rays emitted in the capture events. Maxwellian averaged capture cross sections have been determined for thermal energies between kT = 5 and 100 keV corresponding to all possible s-process scenarios. The estimated uncertainties for the values at 30 keV are 4.1, 3.3, and 4.7% for Os-186, Os-187, and Os-188, respectively.
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Grieger, M., Hensel, T., Agramunt, J., Bemmerer, D., Degering, D., Dillmann, I., et al. (2020). Neutron flux and spectrum in the Dresden Felsenkeller underground facility studied by moderated He-3 counters. Phys. Rev. D, 101(12), 123027–15pp.
Abstract: Ambient neutrons may cause significant background for underground experiments. Therefore, it is necessary to investigate their flux and energy spectrum in order to devise a proper shielding. Here, two sets of altogether ten moderated He-3 neutron counters are used for a detailed study of the ambient neutron background in tunnel IV of the Felsenkeller facility, underground below 45 m of rock in Dresden/Germany. One of the moderators is lined with lead and thus sensitive to neutrons of energies higher than 10 MeV. For each He-3 counter moderator assembly, the energy-dependent neutron sensitivity was calculated with the FLUKA code. The count rates of the ten detectors were then fitted with the MAXED and GRAVEL packages. As a result, both the neutron energy spectrum from 10(-9) to 300 MeV and the flux integrated over the same energy range were determined experimentally. The data show that at a given depth, both the flux and the spectrum vary significantly depending on local conditions. Energy-integrated fluxes of (0.61 +/- 0.05), (1.96 +/- 0.15), and (4.6 +/- 0.4) x 10(-4) cm(-2) s(-1), respectively, are measured for three sites within Felsenkeller tunnel IV which have similar muon flux but different shielding wall configurations. The integrated neutron flux data and the obtained spectra for the three sites are matched reasonably well by FLUKA Monte Carlo calculations that are based on the known muon flux and composition of the measurement room walls.
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n_TOF Collaboration(Lederer, C. et al), Giubrone, G., Domingo-Pardo, C., & Tain, J. L. (2014). Neutron Capture Reactions on Fe and Ni Isotopes for the Astrophysical s-process. Nucl. Data Sheets, 120, 201–204.
Abstract: Neutron capture cross sections in the keV neutron energy region are the key nuclear physics input to study the astrophysical slow neutron capture process. In the past years, a series of neutron capture cross section measurements has been performed at the neutron time-of-flight facility n_TOF at CERN focussing on the Fe/Ni mass region. Recent results and future developments in the neutron time-of-flight technique are discussed.
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n_TOF Collaboration(Guerrero, C. et al), Domingo-Pardo, C., & Tain, J. L. (2020). Neutron Capture on the s-Process Branching Point Tm-171 via Time-of-Flight and Activation. Phys. Rev. Lett., 125(14), 142701–8pp.
Abstract: The neutron capture cross sections of several unstable nuclides acting as branching points in the s process are crucial for stellar nucleosynthesis studies. The unstable Tm-171 (t(1/2) = 1.92 yr) is part of the branching around mass A similar to 170 but its neutron capture cross section as a function of the neutron energy is not known to date. In this work, following the production for the first time of more than 5 mg of Tm-171 at the high-flux reactor Institut Laue-Langevin in France, a sample was produced at the Paul Scherrer Institute in Switzerland. Two complementary experiments were carried out at the neutron time-of-flight facility (nTOF) at CERN in Switzerland and at the SARAF liquid lithium target facility at Soreq Nuclear Research Center in Israel by time of flight and activation, respectively. The result of the time -of-flight experiment consists of the first ever set of resonance parameters and the corresponding average resonance parameters, allowing us to make an estimation of the Maxwellian-averaged cross sections (MACS) by extrapolation. The activation measurement provides a direct and more precise measurement of the MACS at 30 keV: 384 (40) mb, with which the estimation from the nTOF data agree at the limit of 1 standard deviation. This value is 2.6 times lower than the JEFF-3.3 and ENDF/B-VIII evaluations, 25% lower than that of the Bao et al. compilation, and 1.6 times larger than the value recommended in the KAlloNiS (v1) database, based on the only previous experiment. Our result affects the nucleosynthesis at the A similar to 170 branching, namely, the Yb-171 abundance increases in the material lost by asymptotic giant branch stars, providing a better match to the available pre-solar SiC grain measurements compared to the calculations based on the current JEFF-3.3 model-based evaluation.
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n_TOF Collaboration(Tagliente, G. et al.), Domingo-Pardo, C., & Tain, J. L. (2011). Neutron capture on (94)Zr: Resonance parameters and Maxwellian-averaged cross sections. Phys. Rev. C, 84(1), 015801–9pp.
Abstract: The neutron capture cross sections of the Zr isotopes play an important role in nucleosynthesis studies. The s-process reaction flow between the Fe seed and the heavier isotopes passes through the neutron magic nucleus (90)Zr and through (91,92,93,94)Zr, but only part of the flow extends to (96)Zr because of the branching point at (95)Zr. Apart from their effect on the s-process flow, the comparably small isotopic (n, gamma) cross sections make Zr also an interesting structural material for nuclear reactors. The (94)Zr (n, gamma) cross section has been measured with high resolution at the spallation neutron source n_TOF at CERN and resonance parameters are reported up to 60 keV neutron energy.
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n_TOF Collaboration, Gunsing, F., Berthoumieux, E., Borella, A., Belgya, T., Szentmiklosi, L., et al. (2011). Neutron Capture on (209)Bi: Determination of the Production Ratio of (210m)Bi/(210g)Bi. J. Korean Phys. Soc., 59(2), 1670–1675.
Abstract: Neutron capture on (209)Bi produces either an isomeric state (210m)Bi with a half life of 3 x 106 years, or the ground state (210g)Bi which decays with a half life of 5 days to the alpha emitter (210)Po. Therefore the neutron capture cross section ratio (209)Bi(n,gamma)(210m)Bi/(210g)Bi plays an important role in predicting the short- and long-term radio-toxicity produced by (209)Bi under neutron irradiation. This ratio is dependent on the neutron energy. We have measured this ratio for cold neutrons at the cold neutron beam facility of the Budapest Neutron Centre by observing the population of the ground-and the metastable state using high resolution gamma-ray spectroscopy. The same technique has been used at the pulsed white neutron source GELINA of the IRMM, Geel in combination with the neutron time-of-flight technique. Results for the neutron-energy dependent branching ratio will be presented. In addition we performed simulations using a statistical decay code.
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