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Author n_TOF Collaboration; Gunsing, F.; Berthoumieux, E.; Borella, A.; Belgya, T.; Szentmiklosi, L.; Schillebeeckx, P.; Drohe, J.C.; Wynants, R.; Colonna, N.; Marrone, S.; Tagliente, G.; Terlizzi, R.; Domingo-Pardo, C.; Tain, J.L.; Martinez, T.; Massimi, C.; Mastinu, P.M.; Milazzo, P.M.
Title (down) Neutron Capture on (209)Bi: Determination of the Production Ratio of (210m)Bi/(210g)Bi Type Journal Article
Year 2011 Publication Journal of the Korean Physical Society Abbreviated Journal J. Korean Phys. Soc.
Volume 59 Issue 2 Pages 1670-1675
Keywords ND2010; Nuclear data; Neutron capture; Branching ratio; Statistical decay; (209)Bi; (210)Bi; (210)Po
Abstract Neutron capture on (209)Bi produces either an isomeric state (210m)Bi with a half life of 3 x 106 years, or the ground state (210g)Bi which decays with a half life of 5 days to the alpha emitter (210)Po. Therefore the neutron capture cross section ratio (209)Bi(n,gamma)(210m)Bi/(210g)Bi plays an important role in predicting the short- and long-term radio-toxicity produced by (209)Bi under neutron irradiation. This ratio is dependent on the neutron energy. We have measured this ratio for cold neutrons at the cold neutron beam facility of the Budapest Neutron Centre by observing the population of the ground-and the metastable state using high resolution gamma-ray spectroscopy. The same technique has been used at the pulsed white neutron source GELINA of the IRMM, Geel in combination with the neutron time-of-flight technique. Results for the neutron-energy dependent branching ratio will be presented. In addition we performed simulations using a statistical decay code.
Address [Gunsing, F; Berthoumieux, E; Borella, A] CEA Saclay, IRFU, SPhN, F-91911 Gif Sur Yvette, France, Email: gunsing@cea.fr
Corporate Author Thesis
Publisher Korean Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0374-4884 ISBN Medium
Area Expedition Conference
Notes WOS:000294080700051 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ elepoucu @ Serial 736
Permanent link to this record
 
 
Author n_TOF Collaboration (Cano-Ott, D. et al); Domingo-Pardo, C.; Tain, J.L.
Title (down) Neutron Capture Measuremetns on Minor Actinides at the n_TOF Facility at CERN: Past, Present and Future Type Journal Article
Year 2011 Publication Journal of the Korean Physical Society Abbreviated Journal J. Korean Phys. Soc.
Volume 59 Issue 2 Pages 1809-1812
Keywords n_TOF; Total Absorption Calorimeter; TAC; Neutron capture; Cross section; Nuclear waste; Transmutation; Generation IV; Accelerator driven system; ADS; Nuclear reactor; Nuclear energy; Nuclear data; Barium fluoride; Actinides; Plutonium; Americium; Uranium
Abstract The successful development of advanced nuclear systems for sustainable energy production and nuclear waste management depends on high quality nuclear data libraries. Recent sensitivity studies and reports [1-3] have identified the need for substantially improving the accuracy of neutron cross-section data for minor actinides. The n_TOF collaboration has initiated an ambitious experimental program for the measurement of neutron capture cross sections of minor actinides. Two experimental setups have been constructed for this purpose: a Total Absorption Calorimeter (TAC) [4] for measuring neutron capture cross-sections of low-mass and/or radioactive samples and a set of two low neutron sensitivity C(6)D(6) detectors for the less radioactive materials.
Address [Cano-Ott, D; Alvarez-Velarde, F; Gonzalez-Romero, E; Guerrero, C; Martinez, T; Mendoza, E; Villamarin, D; Vicente, MC] Ctr Invest Energet Medioambientales & Technol CIE, Madrid, Spain, Email: daniel.cano@ciemat.es
Corporate Author Thesis
Publisher Korean Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0374-4884 ISBN Medium
Area Expedition Conference
Notes WOS:000294080700085 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ elepoucu @ Serial 737
Permanent link to this record
 
 
Author Mendoza, E.; Alcayne, V.; Cano-Ott, D.; Gonzalez-Romero, E.; Martinez, T.; de Rada, A.P.; Sanchez-Caballero, A.; Balibrea-Correa, J.; Domingo-Pardo, C.; Lerendegui-Marco, J.; Calvino, F.; Guerrero, C.
Title (down) Neutron capture measurements with high efficiency detectors and the Pulse Height Weighting Technique Type Journal Article
Year 2023 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume 1047 Issue Pages 167894 - 16pp
Keywords Neutron capture; Total energy detector; Pulse height weighting technique; 7-ray cascades
Abstract Neutron capture cross section measurements in time-of-flight facilities are usually performed by detecting the prompt 7-rays emitted in the capture reactions. One of the difficulties to be addressed in these measurements is that the emitted 7-rays may change with the neutron energy, and therefore also the detection efficiency. To deal with this situation, many measurements use the so called Total Energy Detection (TED) technique, usually in combination with the Pulse Height Weighting Technique (PHWT). With it, it is sought that the detection efficiency depends only on the total energy of the 7-ray cascade, which does not vary much with the neutron energy. This technique was developed in the 1960s and has been used in many neutron capture experiments to date. One of the requirements of the technique is that 7-ray detectors have a low efficiency. This has meant that the PHWT has been used with experimental setups with low detection efficiencies. However, this condition does not have to be fulfilled by the experimental system as a whole. The main goal of this work is to show that it is possible to measure with a high efficiency detection system that uses the PHWT, and how to analyze the measured data.
Address [Mendoza, E.; Alcayne, V; Cano-Ott, D.; Gonzalez-Romero, E.; Martinez, T.; Perez de Rada, A.; Sanchez-Caballero, A.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain, Email: emilio.mendoza@ciemat.es
Corporate Author Thesis
Publisher Elsevier Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:000908431800002 Approved no
Is ISI yes International Collaboration no
Call Number IFIC @ pastor @ Serial 5468
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Author n_TOF Collaboration (Lederer, C. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.
Title (down) Neutron Capture Cross Section of Unstable Ni-63: Implications for Stellar Nucleosynthesis Type Journal Article
Year 2013 Publication Physical Review Letters Abbreviated Journal Phys. Rev. Lett.
Volume 110 Issue 2 Pages 022501 - 5pp
Keywords
Abstract The Ni-63(n, gamma) cross section has been measured for the first time at the neutron time-of-flight facility n_TOF at CERN from thermal neutron energies up to 200 keV. In total, capture kernels of 12 (new) resonances were determined. Maxwellian averaged cross sections were calculated for thermal energies from kT = 5-100 keV with uncertainties around 20%. Stellar model calculations for a 25M(circle dot) star show that the new data have a significant effect on the s-process production of Cu-63, Ni-64, and Zn-64 in massive stars, allowing stronger constraints on the Cu yields from explosive nucleosynthesis in the subsequent supernova.
Address [Lederer, C.; Paradela, C.; Wallner, A.] Univ Vienna, Fac Phys, A-1090 Vienna, Austria
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0031-9007 ISBN Medium
Area Expedition Conference
Notes WOS:000313336500005 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 1305
Permanent link to this record
 
 
Author n_TOF Collaboration (Mingrone, F. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.
Title (down) Neutron capture cross section measurement of U-238 at the CERN n_TOF facility in the energy region from 1 eV to 700 keV Type Journal Article
Year 2017 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 95 Issue 3 Pages 034604 - 14pp
Keywords
Abstract The aim of this work is to provide a precise and accurate measurement of the U-238(n,gamma) reaction cross section in the energy region from 1 eV to 700 keV. This reaction is of fundamental importance for the design calculations of nuclear reactors, governing the behavior of the reactor core. In particular, fast reactors, which are experiencing a growing interest for their ability to burn radioactive waste, operate in the high energy region of the neutron spectrum. In this energy region most recent evaluations disagree due to inconsistencies in the existing measurements of up to 15%. In addition, the assessment of nuclear data uncertainty performed for innovative reactor systems shows that the uncertainty in the radiative capture cross section of U-238 should be further reduced to 1-3% in the energy region from 20 eV to 25 keV. To this purpose, addressed by the Nuclear Energy Agency as a priority nuclear data need, complementary experiments, one at the GELINA and two at the nTOF facility, were proposed and carried out within the 7th Framework Project ANDES of the European Commission. The results of one of these U-238(n, gamma) measurements performed at the nTOF CERN facility are presented in this work. The gamma-ray cascade following the radiative neutron capture has been detected exploiting a setup of two C6D6 liquid scintillators. Resonance parameters obtained from this work are on average in excellent agreement with the ones reported in evaluated libraries. In the unresolved resonance region, this work yields a cross section in agreement with evaluated libraries up to 80 keV, while for higher energies our results are significantly higher.
Address [Mingrone, F.; Berthoumieux, E.; Brugger, M.; Calviani, M.; Cerutti, F.; Chiaveri, E.; Chin, M.; Guerrero, C.; Hernandez-Prieto, A.; Kadi, Y.; Losito, R.; Rubbia, C.; Tsinganis, A.; Vlachoudis, V.] CERN, European Org Nucl Res, Geneva, Switzerland, Email: federica.mingrone@cern.ch
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000396022500002 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3030
Permanent link to this record
 
 
Author Guerrero, C.; Cano-Ott, D.; Mendoza, E.; Tain, J.L.; Algora, A.; Berthoumieux, E.; Colonna, N.; Domingo-Pardo, C.; Gonzalez-Romero, E.; Heil, M.; Jordan, D.; Kappeler, F.; Lampoudis, C.; Martinez, T.; Massimi, C.; Plag, R.
Title (down) Monte Carlo simulation of the n_TOF Total Absorption Calorimeter Type Journal Article
Year 2012 Publication Nuclear Instruments & Methods in Physics Research A Abbreviated Journal Nucl. Instrum. Methods Phys. Res. A
Volume 671 Issue Pages 108-117
Keywords Monte Carlo simulation; Geant4; Neutron cross-sections; Time-of-flight; Neutron capture
Abstract The n_TOF Total Absorption Calorimeter (TAC) is a 4 pi BaF2 segmented detector used at CERN for measuring neutron capture cross-sections of importance for the design of advanced nuclear reactors. This work presents the simulation code that has been developed in GEANT4 for the accurate determination of the detection efficiency of the TAC for neutron capture events. The code allows to calculate the efficiency of the TAC for every neutron capture state, as a function of energy, crystal multiplicity, and counting rate. The code includes all instrumental effects such as the single crystal detection threshold and energy resolution, finite size of the coincidence time window, and signal pile-up. The results from the simulation have been validated with experimental data for a large set of electromagnetic de-excitation patterns: beta-decay of well known calibration sources, neutron capture reactions in light nuclei with well known level schemes like Ti-nat, reference samples used in (n,gamma) measurements like Au-197 and experimental data from an actinide sample like Pu-240. The systematic uncertainty in the determination of the detection efficiency has been estimated for all the cases. As a representative example, the accuracy reached for the case of Au-197(n,gamma) ranges between 0.5% and 2%, depending on the experimental and analysis conditions. Such a value matches the high accuracy required for the nuclear cross-section data needed in advanced reactor design.
Address [Guerrero, C.; Cano-Ott, D.; Mendoza, E.; Gonzalez-Romero, E.; Martinez, T.] CIEMAT, Ctr Invest Energet Medioambientales & Tecnol, E-28040 Madrid, Spain, Email: carlos.guerrero@cern.ch
Corporate Author Thesis
Publisher Elsevier Science Bv Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0168-9002 ISBN Medium
Area Expedition Conference
Notes WOS:000301474600013 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 973
Permanent link to this record
 
 
Author Martinez, T. et al; Agramunt, J.; Algora, A.; Domingo-Pardo, C.; Jordan, M.D.; Rubio, B.; Tain, J.L.
Title (down) MONSTER: a TOF Spectrometer for beta-delayed Neutron Spectroscopy Type Journal Article
Year 2014 Publication Nuclear Data Sheets Abbreviated Journal Nucl. Data Sheets
Volume 120 Issue Pages 78-80
Keywords
Abstract beta-delayed neutron (DN) data, including emission probabilities, P-n, and energy spectrum, play an important role in our understanding of nuclear structure, nuclear astrophysics and nuclear technologies. A MOdular Neutron time-of-flight SpectromeTER (MONSTER) is being built for the measurement of the neutron energy spectra and branching ratios. The TOF spectrometer will consist of one hundred liquid scintillator cells covering a significant solid angle. The MONSTER design has been optimized by using Monte Carlo (MC) techniques. The response function of the MONSTER cell has been characterized with mono-energetic neutron beams and compared to dedicated MC simulations.
Address [Martinez, T.; Cano-Ott, D.; Castilla, J.; Garcia, A. R.; Marin, J.; Martinez, G.; Mendoza, E.; Santos, C.; Tera, F. J.; Villamarin, D.] CIEMAT, Ctr Invest Energet, Medio Ambient Tecnol, E-28040 Madrid, Spain, Email: trino.martinez@ciemat.es
Corporate Author Thesis
Publisher Academic Press Inc Elsevier Science Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0090-3752 ISBN Medium
Area Expedition Conference
Notes WOS:000339860100021 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 1872
Permanent link to this record
 
 
Author Kiss, G.G. et al; Tarifeño-Saldivia, A.; Tain, J.L.; Agramunt, J.; Algora, A.; Domingo-Pardo, C.; Morales, A.I.; Nacher, E.; Rubio, B.; Tolosa, A.
Title (down) Measuring the beta-decay Properties of Neutron-rich Exotic Pm, Sm, Eu, and Gd Isotopes to Constrain the Nucleosynthesis Yields in the Rare-earth Region Type Journal Article
Year 2022 Publication Astrophysical Journal Abbreviated Journal Astrophys. J.
Volume 936 Issue 2 Pages 107 - 18pp
Keywords
Abstract The beta-delayed neutron-emission probabilities of 28 exotic neutron-rich isotopes of Pm, Sm, Eu, and Gd were measured for the first time at RIKEN Nishina Center using the Advanced Implantation Detector Array (AIDA) and the BRIKEN neutron detector array. The existing beta-decay half-life (T (1/2)) database was significantly increased toward more neutron-rich isotopes, and uncertainties for previously measured values were decreased. The new data not only constrain the theoretical predictions of half-lives and beta-delayed neutron-emission probabilities, but also allow for probing the mechanisms of formation of the high-mass wing of the rare-earth peak located at A approximate to 160 in the r-process abundance distribution through astrophysical reaction network calculations. An uncertainty quantification of the calculated abundance patterns with the new data shows a reduction of the uncertainty in the rare-earth peak region. The newly introduced variance-based sensitivity analysis method offers valuable insight into the influence of important nuclear physics inputs on the calculated abundance patterns. The analysis has identified the half-lives of Sm-168 and of several gadolinium isotopes as some of the key variables among the current experimental data to understand the remaining abundance uncertainty at A = 167-172.
Address [Kiss, G. G.; Vitez-Sveiczer, A.; Algora, A.; Szegedi, T. N.] Inst Nucl Res ATOMKI, Bem Ter 18-c, H-4026 Debrecen, Hungary, Email: ggkiss@atomki.hu;
Corporate Author Thesis
Publisher IOP Publishing Ltd Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 0004-637x ISBN Medium
Area Expedition Conference
Notes WOS:000850804600001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 5353
Permanent link to this record
 
 
Author n_TOF Collaboration (Wright, T. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A.
Title (down) Measurement of the U-238(n,gamma) cross section up to 80 keV with the Total Absorption Calorimeter at the CERN n_TOF facility Type Journal Article
Year 2017 Publication Physical Review C Abbreviated Journal Phys. Rev. C
Volume 96 Issue 6 Pages 064601 - 11pp
Keywords
Abstract The radiative capture cross section of a highly pure (99.999%), 6.125(2) grams and 9.56(5) x 10(-4) atoms/barn areal density U-238 sample has been measured with the Total Absorption Calorimeter (TAC) in the 185 m flight path at the CERN neutron time-of-flight facility n_TOF. This measurement is in response to the NEA High Priority Request list, which demands an accuracy in this cross section of less than 3% below 25 keV. These data have undergone careful background subtraction, with special care being given to the background originating from neutrons scattered by the 238U sample. Pileup and dead-time effects have been corrected for. The measured cross section covers an energy range between 0.2 eV and 80 keV, with an accuracy that varies with neutron energy, being better than 4% below 25 keV and reaching at most 6% at higher energies.
Address [Wright, T.; Billowes, J.; Ryan, J. A.; Ware, T.] Univ Manchester, Manchester, Lancs, England, Email: tobias.wright@manchester.ac.uk
Corporate Author Thesis
Publisher Amer Physical Soc Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 2469-9985 ISBN Medium
Area Expedition Conference
Notes WOS:000416848700005 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 3392
Permanent link to this record
 
 
Author n_TOF Collaboration (Amaducci, S. et al); Domingo-Pardo, C.; Tain, J.L.
Title (down) Measurement of the U-235(n, f) cross section relative to the Li-6(n, t) and B-10(n,alpha) standards from thermal to 170 keV neutron energy range at n_TOF Type Journal Article
Year 2019 Publication European Physical Journal A Abbreviated Journal Eur. Phys. J. A
Volume 55 Issue 7 Pages 120 - 19pp
Keywords
Abstract .The U-235(n, f ) cross section was measured at n_TOF relative to Li-6(n, t) and B-10(n,alpha) , with high resolution ( L=183.49(2) m) and in a wide energy range (25meV-170keV) with 1.5% systematic uncertainty, making use of a stack of six samples and six silicon detectors placed in the neutron beam. This allowed us to make a direct comparison of the yields of the U-235(n, f ) and of the two reference reactions under the same experimental conditions, and taking into account the forward/backward emission asymmetry. A hint of an anomaly in the 10-30keV neutron energy range had been previously observed in other experiments, indicating a cross section systematically lower by several percent relative to major evaluations. The present results indicate that the cross section in the 9-18keV neutron energy range is indeed overestimated by almost 5% in the recently released evaluated data files ENDF/B-VIII.0 and JEFF3.3, as a consequence of a 7% overestimate in a single GMA node in the IAEA reference file. Furthermore, these new high-resolution data confirm the existence of resonance-like structures in the keV neutron energy region. The results here reported may lead to a reduction of the uncertainty in the 1-100keV neutron energy region. Finally, from the present data, a value of 249.7 +/- 1.4( stat )+/- 0.94( syst ) b<bold>eV has been extracted for the cross section integral between </bold>7.8 and 11eV, confirming the value of 247.5 +/- 3 b<bold>eV recently established as a standard</bold>.
Address [Amaducci, S.; Cosentino, L.; Finocchiaro, P.; Musumarra, A.] INFN, Lab Nazl Sud, Catania, Italy, Email: finocchiaro@lns.infn.it
Corporate Author Thesis
Publisher Springer Place of Publication Editor
Language English Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1434-6001 ISBN Medium
Area Expedition Conference
Notes WOS:000477050900001 Approved no
Is ISI yes International Collaboration yes
Call Number IFIC @ pastor @ Serial 4083
Permanent link to this record