Abstract: The neutron flux of the nTOF facility at CERN was measured, after installation of the new spallation target, with four different systems based on three neutron-converting reactions, which represent accepted cross sections standards in different energy regions. A careful comparison and combination of the different measurements allowed us to reach an unprecedented accuracy on the energy dependence of the neutron flux in the very wide range (thermal to 1 GeV) that characterizes the nTOF neutron beam. This is a pre-requisite for the high accuracy of cross section measurements at n_TOF. An unexpected anomaly in the neutron-induced fission cross section of U-235 is observed in the energy region between 10 and 30keV, hinting at a possible overestimation of this important cross section, well above currently assigned uncertainties.

Abstract: The neutron sensitivity of the Cr6D6 detector setup used at nTOF facility for capture measurements has been studied by means of detailed GEANT4 simulations. A realistic software replica of the entire nTOF experimental hall, including the neutron beam line, sample, detector supports and the walls of the experimental area has been implemented in the simulations. The simulations have been analyzed in the same manner as experimental data, in particular by applying the Pulse Height Weighting Technique. The simulations have been validated against a measurement of the neutron background performed with a(nat)-C sample, showing an excellent agreement above 1 keV. At lower energies, an additional component in the measured C-nat yield has been discovered, which prevents the use of C-nat data for neutron background estimates at neutron energies below a few hundred eV. The origin and time structure of the neutron background have been derived from the simulations. Examples of the neutron background for two different samples are demonstrating the important role of accurate simulations of the neutron background in capture cross-section measurements.

Abstract: We report on the spatial response characterization of large LaCl3(Ce) monolithic crystals optically coupled to 8 x 8 pixel silicon photomultiplier (SiPM) sensors. A systematic study has been carried out for 511 keV gamma-rays using three different crystal thicknesses of 10 mm, 20 mm and 30 mm, all of them with planar geometry and a base size of 50 x 50 mm(2). In this work we investigate and compare two different approaches for the determination of the main gamma-ray hit location. On one hand, methods based on the fit of an analytical model for the scintillation light distribution provide the best results in terms of linearity and field of view, with spatial resolutions close to similar to 1 mm FWHM. On the other hand, position reconstruction techniques based on neural networks provide similar linearity and field-of-view, becoming the attainable spatial resolution similar to 3 mm FWHM. For the third space coordinate z or depth-of-interaction we have implemented an inverse linear calibration approach based on the cross-section of the measured scintillation-light distribution at a certain height. The detectors characterized in this work are intended for the development of so-called Total Energy Detectors with Compton imaging capability (i-TED), aimed at enhanced sensitivity and selectivity measurements of neutron capture cross sections via the time-of-flight (TOF) technique.

Abstract: Neutron-induced fission cross-sections of minor actinides have been measured using the nTOF white neutron source at CERN. Geneva, as part of a large experimental program aiming at collecting new data relevant for nuclear astrophysics and for the design of advanced reactor systems. The measurements at nTOF take advantage of the innovative features of the n_TOF facility, namely the wide energy range, high instantaneous neutron flux and good energy resolution. Final results on the fission cross-section of (233)U, (245)cm and (243)Am from thermal to 20 MeV are here reported, together with preliminary results for (241)Am. The measurement have been performed with a dedicated Fast Ionization Chamber (FIC), a fission fragment detector with a very high efficiency, relative to the very well known cross-section of (235)U, measured simultaneously with the same detector.

Abstract: An accurate measurement of the Ce-140(n,gamma) energy-dependent cross-section was performed at the n_TOF facility at CERN. This cross-section is of great importance because it represents a bottleneck for the s-process nucleosynthesis and determines to a large extent the cerium abundance in stars. The measurement was motivated by the significant difference between the cerium abundance measured in globular clusters and the value predicted by theoretical stellar models. This discrepancy can be ascribed to an overestimation of the Ce-140 capture cross-section due to a lack of accurate nuclear data. For this measurement, we used a sample of cerium oxide enriched in Ce-140 to 99.4%. The experimental apparatus consisted of four deuterated benzene liquid scintillator detectors, which allowed us to overcome the difficulties present in the previous measurements, thanks to their very low neutron sensitivity. The accurate analysis of the p-wave resonances and the calculation of their average parameters are fundamental to improve the evaluation of the Ce-140 Maxwellian-averaged cross-section.