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Valencia, E. et al, Tain, J. L., Algora, A., Agramunt, J., Estevez, E., Jordan, M. D., et al. (2017). Total absorption gamma-ray spectroscopy of the beta-delayed neutron emitters Br-87, Br-88, and Rb-94. Phys. Rev. C, 95(2), 024320–18pp.
Abstract: We investigate the decay of Br-87,Br-88 and Rb-94 using total absorption gamma-ray spectroscopy. These important fission products are beta-delayed neutron emitters. Our data show considerable beta gamma intensity, so far unobserved in high-resolution gamma-ray spectroscopy, from states at high excitation energy. We also find significant differences with the beta intensity that can be deduced from existing measurements of the beta spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for U-235 fission at cooling times in the range 1-100 s. We also use summation calculations to evaluate the impact of present data on reactor antineutrino spectra. We find a significant effect at antineutrino energies in the range of 5 to 9 MeV. In addition, we observe an unexpected strong probability for. emission from neutron unbound states populated in the daughter nucleus. The. branching is compared to Hauser-Feshbach calculations, which allow one to explain the large value for bromine isotopes as due to nuclear structure. However the branching for Rb-94, although much smaller, hints of the need to increase the radiative width gamma by one order of magnitude. This increase in gamma would lead to a similar increase in the calculated (n, gamma) cross section for this very neutron-rich nucleus with a potential impact on r process abundance calculations.
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Guadilla, V., Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of niobium isomers. Phys. Rev. C, 100(2), 024311–15pp.
Abstract: The beta-intensity distributions of the decays of Nb-100gs,Nb-100m and Nb-102gs,Nb-102m have been determined using the total absorption gamma-ray spectroscopy technique. The JYFLTRAP double Penning trap system was employed in a campaign of challenging measurements performed with the decay total absorption gamma-ray spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. Different strategies were applied to disentangle the isomeric states involved, lying very close in energy. The low-spin component of each niobium case was populated through the decay of the zirconium parent, which was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained beta-intensity distributions for these zirconium decays. The beta-strength distributions evaluated with these results were compared with calculations in a quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of Zr-100,Zr-102. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The beta-intensities of the decay of Nb-102m, for which there were no previous data, were obtained. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported, and here we detail the significant impact on decay heat calculations.
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Tain, J. L., Agramunt, J., Algora, A., Aprahamian, A., Cano-Ott, D., Fraile, L. M., et al. (2015). The sensitivity of LaBr3:Ce scintillation detectors to low energy neutrons: Measurement and Monte Carlo simulation. Nucl. Instrum. Methods Phys. Res. A, 774, 17–24.
Abstract: The neutron sensitivity of a cylindrical circle minus 1.5 in x 1.5 in LaBr3:Ce scintillation detector was measured using quasi-monoenergetic neutron beams in the energy range from 40 keV to 2.5 MeV. In this energy range the detector is sensitive to gamma-rays generated in neutron inelastic and capture processes. The experimental energy response was compared with Monte Carlo simulations performed with the Geant4 simulation toolkit using the so-called High Precision Neutron Models. These models rely on relevant information stored in evaluated nuclear data libraries. The performance of the Geant4 Neutron Data Library as well as several standard nuclear data libraries was investigated. In the latter case this was made possible by the use of a conversion tool that allowed the direct use of the data from other libraries in Geant4. Overall it was found that there was good agreement with experiment for some of the neutron data bases like ENDF/B-VII.0 or JENDL-3.3 but not with the others such as ENDF/B-VI.8 or JEFF-3.1.
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Rasco, B. C., Brewer, N. T., Yokoyama, R., Grzywacz, R., Rykaczewski, K. P., Tolosa-Delgado, A., et al. (2018). The ORNL analysis technique for extracting beta-delayed multi-neutron branching ratios with BRIKEN. Nucl. Instrum. Methods Phys. Res. A, 911, 79–86.
Abstract: Many choices are available in order to evaluate large radioactive decay networks. There are many parameters that influence the calculated beta-decay delayed single and multi-neutron emission branching fractions. We describe assumptions about the decay model, background, and other parameters and their influence on beta-decay delayed multi-neutron emission analysis. An analysis technique, the ORNL BRIKEN analysis procedure, for determining beta-delayed multi-neutron branching ratios in beta-neutron precursors produced by means of heavy-ion fragmentation is presented. The technique is based on estimating the initial activities of zero, one, and two neutrons occurring in coincidence with an ion-implant and beta trigger. The technique allows one to extract beta-delayed multi-neutron decay branching ratios measured with the He-3 BRIKEN neutron counter. As an example, two analyses of the beta-neutron emitter Cu-77 based on different a priori assumptions are presented along with comparisons to literature values.
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Mistry, A. K. et al, Tain, J. L., Agramunt, J., Algora, A., Guadilla, V., Morales, A. I., et al. (2022). The DESPEC setup for GSI and FAIR. Nucl. Instrum. Methods Phys. Res. A, 1033, 166662–18pp.
Abstract: The DEcay SPECtroscopy (DESPEC) setup for nuclear structure investigations was developed and commissioned at GSI, Germany in preparation for a full campaign of experiments at the FRS and Super-FRS. In this paper, we report on the first employment of the setup in the hybrid configuration with the AIDA implanter coupled to the FATIMA LaBr3(Ce) fast-timing array, and high-purity germanium detectors. Initial results are shown from the first experiments carried out with the setup. An overview of the setup and function is discussed, including technical advancements along the path.
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Vitez-Sveiczer, A. et al, Algora, A., Morales, A. I., Rubio, B., Agramunt, J., Guadilla, V., et al. (2022). The beta-decay of Kr-70 into Br-70: Restoration of the pseudo-SU(4) symmetry. Phys. Lett. B, 830, 137123–8pp.
Abstract: The beta-decay of the even-even nucleus Kr-70 with Z=N+2, has been investigated at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center using the BigRIPS fragment separator, the ZeroDegree Spectrometer, the WAS3ABI implantation station and the EURICA HPGe cluster array. Fifteen gamma-rays associated with the beta-decay of( 70)Kr into Br-70 have been identified for the first time, defining ten populated states below E-exc=3300 keV. The half-life of Kr-70 was derived with increased precision and found to be t(1/2)=45.19 +/- 0.14 ms. The beta-delayed proton emission probability has also been determined as epsilon(p)=0.545(23)%. An increase in the beta-strength to the yrast 1(+) state in comparison with the heaviest Z=N+2 system studied so far (Ge-62 decay) is observed that may indicate increased np correlations in the T=0 channel. The beta-decay strength deduced from the results is interpreted in terms of the proton-neutron quasiparticle random-phase approximation (pnQRPA) and also with a schematic model that includes isoscalar and isovector pairing in addition to quadrupole deformation. The application of this last model indicates an approximate realization of pseudo-SU(4) symmetry in this system.
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Luo, X. L. et al, Agramunt, J., Egea, F. J., Gadea, A., & Huyuk, T. (2014). Test of digital neutron-gamma discrimination with four different photomultiplier tubes for the NEutron Detector Array (NEDA). Nucl. Instrum. Methods Phys. Res. A, 767, 83–91.
Abstract: A comparative study of the neutron-gamma discrimination performance of a liquid scintillator detector BC501A coupled to four different 5 in photomultiplier tubes (ET9390kb, R11833-100, XP4512 and R4144) was carried out Both the Charge Comparison method and the Integrated Rise-Time method were implemented digitally to discriminate between neutrons and gamma rays emitted by a Cf-252 source. In both methods, the neutron-gamma discrimination capabilities of the four photomultiplier tubes were quantitatively compared by evaluating their figure-of-merit values at different energy regions between 50 keVee and 1000 keVee. Additionally, the results were further verified qualitatively using time-of-flight to distinguish gamma rays and neutrons. The results consistently show that photomultiplier tubes R11833-100 and ET9390kb generally perform best regarding neutron-gamma discrimination with only slight differences in figure-of-merit values. This superiority can be explained by their relatively higher photoelectron yield, which indicates that a scintillator detector coupled to a photomultiplier tube with higher photoelectron yield tends to result in better neutron-gamma discrimination performance. The results of this work will provide reference for the choice of photomultiplier tubes for future neutron detector arrays like NEDA.
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Molina, F. et al, Rubio, B., Agramunt, J., Algora, A., Domingo-Pardo, C., Gadea, A., et al. (2015). T-z =-1 -> 0 beta decays of Ni-54, Fe-50, Cr-46, and Ti-42 and comparison with mirror (He-3,t) measurements. Phys. Rev. C, 91(1), 014301–19pp.
Abstract: We have studied the beta decay of the T-z = -1, f(7/2) shell nuclei Ni-54, Fe-50, Cr-46, and Ti-42 produced in fragmentation reactions. The proton separation energies in the daughter T-z = 0 nuclei are relatively large (approximate to 4-5 MeV) so studies of the. rays are essential. The experiments were performed at GSI as part of the Stopped-beam campaign with the RISING setup consisting of 15 Euroball Cluster Ge detectors. From the newly obtained high precision beta-decay half-lives, excitation energies, and beta branching ratios, we were able to extract Fermi and Gamow-Teller transition strengths in these beta decays. With these improved results it was possible to compare in detail the Gamow-Teller (GT) transition strengths observed in beta decay including a sensitivity limit with the strengths of the T-z = +1 to T-z = 0 transitions derived from high resolution (He-3,t) reactions on the mirror target nuclei at RCNP, Osaka. The accumulated B(GT) strength obtained from both experiments looks very similar although the charge exchange reaction provides information on a broader energy range. Using the “merged analysis” one can obtain a full picture of the B(GT) over the full Q(beta) range. Looking at the individual transitions some differences are observed, especially for the weak transitions. Their possible origins are discussed.
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Morales, A. I. et al, Agramunt, J., Algora, A., Gadea, A., Molina, F., & Rubio, B. (2011). Synthesis of N=127 isotones through (p,n) charge-exchange reactions induced by relativistic (208)Pb projectiles. Phys. Rev. C, 84(1), 011601–5pp.
Abstract: The production cross sections of four N = 127 isotones ((207)Hg, (206)Au, (205)Pt, and (204)Ir) have been measured using (p,n) charge-exchange reactions, induced in collisions of a (208)Pb primary beam at 1 A GeV with a Be target. These data allow one to investigate the use of a reaction mechanism to extend the limits of the chart of nuclides toward the important r-process nuclei in the region of the third peak of elemental abundance distribution.
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Deo, A. Y., Podolyak, Z., Walker, P. M., Algora, A., Rubio, B., Agramunt, J., et al. (2010). Structures of Po-201 and Rn-205 from EC/beta(+)-decay studies. Phys. Rev. C, 81(2), 024322–8pp.
Abstract: Several low-lying excited states in Rn-205(86)119 and Po-201(84)117 were identified for the first time following EC/beta(+) decay of Fr-205 and At-201, respectively, using gamma-ray and conversion electron spectroscopy at the CERN isotope separator on-line (ISOLDE) facility. The EC/beta(+) branch from Fr-205 was measured to be 1.5(2)%. The excited states of the daughter nuclei are understood in terms of the odd nucleon coupling to the neighboring even-even core. The neutron single-particle energies of the p(3/2) orbital relative to the f(5/2) ground state in Rn-205, and the f(5/2) orbital relative to the p(3/2) ground state in Po-201, were determined to be 31.4(2) and 5.7(3) keV, respectively. We tentatively identify a 13/2(+) isomeric level at 657.1(5) keV in Rn-205. The systematic behavior of the 13/2(+) and 3/2(-) levels is also discussed.
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