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Author |
n_TOF Collaboration (Lerendegui-Marco, J. et al.); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title  |
Radiative neutron capture on Pu-242 in the resonance region at the CERN n_TOF-EAR1 facility |
Type |
Journal Article |
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Year |
2018 |
Publication |
Physical Review C |
Abbreviated Journal |
Phys. Rev. C |
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Volume |
97 |
Issue |
2 |
Pages |
024605 - 21pp |
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Abstract |
The spent fuel of current nuclear reactors contains fissile plutonium isotopes that can be combined with uranium to make mixed oxide (MOX) fuel. In this way the Pu from spent fuel is used in a new reactor cycle, contributing to the long-term sustainability of nuclear energy. However, an extensive use of MOX fuels, in particular in fast reactors, requires more accurate capture and fission cross sections for some Pu isotopes. In the case of Pu-242 there are sizable discrepancies among the existing capture cross-section measurements included in the evaluations (all from the 1970s) resulting in an uncertainty as high as 35% in the fast energy region. Moreover, postirradiation experiments evaluated with JEFF-3.1 indicate an overestimation of 14% in the capture cross section in the fast neutron energy region. In this context, the Nuclear Energy Agency (NEA) requested an accuracy of 8% in this cross section in the energy region between 500 meV and 500 keV. This paper presents a new time-of-flight capture measurement on Pu-242 carried out at nTOF-EAR1 (CERN), focusing on the analysis and statistical properties of the resonance region, below 4 keV. The Pu-242(n, gamma) reaction on a sample containing 95(4) mg enriched to 99.959% was measured with an array of four C6D6 detectors and applying the total energy detection technique. The high neutron energy resolution of nTOF-EAR1 and the good statistics accumulated have allowed us to extend the resonance analysis up to 4 keV, obtaining new individual and average resonance parameters from a capture cross section featuring a systematic uncertainty of 5%, fulfilling the request of the NEA. |
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Address |
[Lerendegui-Marco, J.; Guerrero, C.; Quesada, J. M.; Cortes-Giraldo, M. A.; Praena, J.; Sabate-Gilarte, M.] Univ Seville, Dept Fis Atom Mol & Nucl, E-41012 Seville, Spain, Email: cguerrero4@us.es |
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Amer Physical Soc |
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English |
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ISSN |
2469-9985 |
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Notes |
WOS:000424190700001 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3474 |
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Author |
n_TOF Collaboration (Gawlik, A. et al); Domingo-Pardo, C.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Radiative Neutron Capture Cross-Section Measurement of Ge Isotopes at n_TOF CERN Facility and Its Importance for Stellar Nucleosynthesis |
Type |
Journal Article |
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Year |
2021 |
Publication |
Acta Physica Polonica A |
Abbreviated Journal |
Acta Phys. Pol. A |
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Volume |
139 |
Issue |
4 |
Pages |
383-388 |
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Keywords |
n_TOF; neutron time-of-flight; neutron capture cross-section; MACS |
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Abstract |
This manuscript summarizes the results of radiative neutron capture cross-section measurements on two stable germanium isotopes, Ge-70 and Ge-73. Experiments were performed at the n_TOF facility at CERN via the time-of-flight technique, over a wide neutron energy range, for all stable germanium isotopes (70,72,73,74, and 76). Results for Ge-70 [Phys. Rev. C 100, 045804 (2019)] and Ge-73 [Phys. Lett. B 790, 458 (2019)] are already published. In the field of nuclear structure, such measurements allow to study excited levels close to the neutron binding energy and to obtain information on nuclear properties. In stellar nucleosynthesis research, neutron induced reactions on germanium are of importance for nucleosynthesis in the weak component of the slow neutron capture processes. |
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Address |
[Gawlik, A.; Andrzejewski, J.; Perkowski, J.] Univ Lodz, Lodz, Poland, Email: aleksandra.gawlik@uni.lodz.pl |
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Polish Acad Sciences Inst Physics |
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English |
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ISSN |
0587-4246 |
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Notes |
WOS:000653413700004 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
4840 |
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Author |
n_TOF Collaboration (Praena, J. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L.; Tarifeño-Saldivia, A. |
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Title |
Preparation and characterization of S-33 samples for S-33(n,alpha)Si-30 cross-section measurements at the n_TOF facility at CERN |
Type |
Journal Article |
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Year |
2018 |
Publication |
Nuclear Instruments & Methods in Physics Research A |
Abbreviated Journal |
Nucl. Instrum. Methods Phys. Res. A |
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Volume |
890 |
Issue |
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Pages |
142-147 |
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Keywords |
Neutron induced alpha emission; Thermal evaporation; Rutherford backscattering |
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Abstract |
Thin S-33 samples for the study of the S-33(n,alpha)Si-30 cross-section at the n_TOF facility at CERN were made by thermal evaporation of S-33 powder onto a dedicated substrate made of kapton covered with thin layers of copper, chromium and titanium. This method has provided for the first time bare sulfur samples a few centimeters in diameter. The samples have shown an excellent adherence with no mass loss after few years and no sublimation in vacuum at room temperature. The determination of the mass thickness of S-33 has been performed by means of Rutherford backscattering spectrometry. The samples have been successfully tested under neutron irradiation. |
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Address |
[Praena, J.; Porras, I.] Univ Granada, Granada, Spain, Email: jpraena@ugr.es |
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Publisher |
Elsevier Science Bv |
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English |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0168-9002 |
ISBN |
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Notes |
WOS:000427814900020 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
3537 |
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Author |
n_TOF Collaboration (Guerrero, C. et al); Domingo-Pardo, C.; Giubrone, G.; Tain, J.L. |
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Title |
Performance of the neutron time-of-flight facility n_TOF at CERN |
Type |
Journal Article |
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Year |
2013 |
Publication |
European Physical Journal A |
Abbreviated Journal |
Eur. Phys. J. A |
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Volume |
49 |
Issue |
2 |
Pages |
27 - 15pp |
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Abstract |
The neutron time-of-flight facility n_TOF features a white neutron source produced by spallation through 20 GeV/c protons impinging on a lead target. The facility, aiming primarily at the measurement of neutron-induced reaction cross sections, was operating at CERN between 2001 and 2004, and then underwent a major upgrade in 2008. This paper presents in detail all the characteristics of the new neutron beam in the currently available configurations, which correspond to two different collimation systems and two choices of neutron moderator. The characteristics discussed include the intensity and energy dependence of the neutron flux, the spatial profile of the beam, the in-beam background components and the energy resolution/broadening. The discussion of these features is based on dedicated measurements and Monte Carlo simulations, and includes estimations of the systematic uncertainties of the mentioned quantities. |
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Address |
[Guerrero, C.; Tsinganis, A.; Berthoumieux, E.; Weiss, C.; Chiaveri, E.; Calviani, M.; Vlachoudis, V.; Andriamonje, S.; Boccone, V.; Brugger, M.; Cerutti, F.; Chin, M.; Ferrari, A.; Hernandez-Prieto, A.; Kadi, Y.; Losito, R.; Roman, F.; Rubbia, C.; Versaci, R.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland, Email: carlos.guerrero@cern.ch |
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Publisher |
Springer |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
1434-6001 |
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Notes |
WOS:000315601600011 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ pastor @ |
Serial |
1358 |
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Author |
n_TOF Collaboration (Chiaveri, E. et al); Giubrone, G.; Tain, J.L. |
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Title |
Past, Present and Future of the n_TOF Facility at CERN |
Type |
Journal Article |
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Year |
2011 |
Publication |
Journal of the Korean Physical Society |
Abbreviated Journal |
J. Korean Phys. Soc. |
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Volume |
59 |
Issue |
2 |
Pages |
1620-1623 |
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Keywords |
ND2010; Nuclear data; ENDF; n_TOF; Spallation |
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Abstract |
The nTOF spallation neutron facility is operating at CERN since 2001. Neutrons are produced with a very wide energy range, from thermal up to 1 GeV and with a very high instantaneous flux (10(5)n/cm(2)/pulse at 200 m from target) thanks to the high intensity (7 x 10(12) protons/pulse) and low repetition rate of the Proton Synchrotron (PS) which is delivering protons to a lead spallation target. The experimental area is located at 200 m from the target, resulting in a very good energy resolution and beam quality thanks to the adoption of an optimal collimation system. At the end of 2008 the nTOF facility has resumed operation after a halt of 3 years due to technical issues. This contribution will outline the main physics results obtained by the facility since its inception in 1999, and show the importance of the measured nuclear data in the field of Nuclear Astrophysics and Nuclear Technology. Then it will present the future perspectives of the facility, aiming mainly in the direction of measuring highly radioactive samples, for which the facility has unique capabilities, with a lower background. |
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Address |
[Chiaveri, E; Andriamonje, S; Calviani, M; Vlachoudis, V; Brugger, M; Cennini, P; Cerutti, F; Chin, M; Ferrari, A; Kadi, Y; Lebbos, E; Losito, R; Rubbia, C] CERN, Geneva, Switzerland, Email: Enrico.Chiaveri@cern.ch |
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Corporate Author |
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Publisher |
Korean Physical Soc |
Place of Publication |
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Editor |
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Language |
English |
Summary Language |
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Original Title |
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Series Editor |
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Series Title |
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Abbreviated Series Title |
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Series Volume |
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Series Issue |
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Edition |
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ISSN |
0374-4884 |
ISBN |
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Conference |
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Notes |
WOS:000294080700040 |
Approved |
no |
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Is ISI |
yes |
International Collaboration |
yes |
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Call Number |
IFIC @ elepoucu @ |
Serial |
734 |
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