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n_TOF Collaboration(Mastromarco, M. et al), Domingo-Pardo, C., & Tain, J. L. (2019). Cross section measurements of Gd-155,Gd-157(n,) induced by thermal and epithermal neutrons. Eur. Phys. J. A, 55(1), 9–20pp.
Abstract: Neutron capture cross section measurements on Gd-155 and Gd-157 were performed using the time-of-flight technique at the nTOF facility at CERN on isotopically enriched samples. The measurements were carried out in the nTOF experimental area EAR1, at 185 m from the neutron source, with an array of 4 C6D6 liquid scintillation detectors. At a neutron kinetic energy of 0.0253 eV, capture cross sections of 62.2(2.2) and 239.8(8.4) kilobarn have been derived for Gd-155 and Gd-157, respectively, with up to 6% deviation relative to values presently reported in nuclear data libraries, but consistent with those values within 1.6 standard deviations. A resonance shape analysis has been performed in the resolved resonance region up to 181 eV and 307 eV, respectively for Gd-155 and Gd-157, where on average, resonance parameters have been found in good agreement with evaluations. Above these energies and up to 1 keV, the observed resonance-like structure of the cross section has been analysed and characterised. From a statistical analysis of the observed neutron resonances we deduced: neutron strength function of 2.01(28)x10-4 and 2.17(41)x10-4; average total radiative width of 106.8(14) meV and 101.1(20) meV and s-wave resonance spacing 1.6(2) eV and 4.8(5) eV for n + Gd-155 and n + Gd-157 systems, respectively.
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Dillmann, I., Coquard, L., Domingo-Pardo, C., Kappeler, F., Marganiec, J., Uberseder, E., et al. (2011). Cross sections for proton-induced reactions on Pd isotopes at energies relevant for the gamma process. Phys. Rev. C, 84(1), 015802–11pp.
Abstract: Proton-activation reactions on natural and enriched palladium samples were investigated via the activation technique in the energy range of E(p) = 2.75-9 MeV, close to the upper end of the respective Gamow window of the. process. We have determined cross sections for (102)Pd(p,gamma)(103)Ag, (104)Pd(p,gamma)(105)Ag, and (105)Pd(p,n)(105)Ag, as well as partial cross sections of (104)Pd(p,n)(104)Ag(g), (105)Pd(p,gamma)(106)Ag(m), (106)Pd(p,n)(106)Ag(m), and (110)Pd(p,n)(110)Ag(m) with uncertainties between 3% and 15% for constraining theoretical Hauser-Feshbach rates and for direct use in gamma-process calculations.
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Esposito, R. et al, & Domingo-Pardo, C. (2021). Design of the third-generation lead-based neutron spallation target for the neutron time-of-flight facility at CERN. Phys. Rev. Accel. Beams, 24(9), 093001–17pp.
Abstract: The neutron time-of-flight (n_TOF) facility at the European Laboratory for Particle Physics (CERN) is a pulsed white-spectrum neutron spallation source producing neutrons for two experimental areas: the Experimental Area 1 (EAR1), located 185 m horizontally from the target, and the Experimental Area 2 (EAR2), located 20 m above the target. The target, based on pure lead, is impacted by a high-intensity 20-GeV/c pulsed proton beam. The facility was conceived to study neutron-nucleus interactions for neutron kinetic energies between a few meV to several GeV, with applications of interest for nuclear astrophysics, nuclear technology, and medical research. After the second-generation target reached the end of its lifetime, the facility underwent a major upgrade during CERN's Long Shutdown 2 (LS2, 2019-2021), which included the installation of the new third-generation neutron target. The first- and second-generation targets were based on water-cooled massive lead blocks and were designed focusing on EAR1, since EAR2 was built later. The new target is cooled by nitrogen gas to avoid erosion-corrosion and contamination of cooling water with radioactive lead spallation products. Moreover, the new design is optimized also for the vertical flight path and EAR2. This paper presents an overview of the target design focused on both physics and thermomechanical performance, and includes a description of the nitrogen cooling circuit and radiation protection studies.
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n_TOF Collaboration(Lederer-Woods, C. et al.), Domingo-Pardo, C., & Tain, J. L. (2021). Destruction of the cosmic gamma-ray emitter Al-26 in massive stars: Study of the key Al-26(n, alpha) reaction. Phys. Rev. C, 104(3), L032803–6pp.
Abstract: Neutron destruction reactions of the cosmic gamma-ray emitter Al-26 are of importance to determine the amount of Al-26 ejected into our galaxy by supernova explosions and for Al-26 production in asymptotic giant branch stars. We performed a new measurement of the Al-26(n, alpha) reaction up to 160-keV neutron energy at the neutron time-of-flight facilities n_TOF at CERN and GELINA at EC-JRC. We provide strengths for ten resonances, six of them for the first time. We use our data to calculate astrophysical reactivities for stellar temperatures up to 0.7 GK. Our results resolve a discrepancy between the two previous direct measurements of this reaction, and indicate higher stellar destruction rates than the most recently recommended reactivity.
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n_TOF Collaboration(Lederer-Woods, C. et al.), Domingo-Pardo, C., & Tain, J. L. (2021). Destruction of the cosmic gamma-ray emitter Al-26 in massive stars: Study of the key Al-26(n, p) reaction. Phys. Rev. C, 104(2), L022803–7pp.
Abstract: The Al-26(n, p) Mg-26 reaction is the key reaction impacting on the abundances of the cosmic gamma-ray emitter Al-26 produced in massive stars and impacts on the potential pollution of the early solar system with Al-26 by asymptotic giant branch stars. We performed a measurement of the Al-26(n, p) Mg-26 cross section at the high-flux beam line EAR-2 at the n_TOF facility (CERN). We report resonance strengths for eleven resonances, nine being measured for the first time, while there is only one previous measurement for the other two. Our resonance strengths are significantly lower than the only previous values available. Our cross-section data range to 150 keV neutron energy, which is sufficient for a reliable determination of astrophysical reactivities up to 0.5 GK stellar temperature.
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Langer, C. et al, & Domingo-Pardo, C. (2014). Determining the rp-Process Flow through Ni-56: Resonances in Cu-57(p,gamma)Zn-58 Identified with GRETINA. Phys. Rev. Lett., 113(3), 032502–5pp.
Abstract: An approach is presented to experimentally constrain previously unreachable (p,gamma) reaction rates on nuclei far from stability in the astrophysical rp process. Energies of all critical resonances in the Cu-57(p,gamma)Zn-58 reaction are deduced by populating states in Zn-58 with a (d, n) reaction in inverse kinematics at 75 MeV/u, and detecting.-ray-recoil coincidences with the state-of-the-art gamma-ray tracking array GRETINA and the S800 spectrograph at the National Superconducting Cyclotron Laboratory. The results reduce the uncertainty in the Cu-57(p,gamma) reaction rate by several orders of magnitude. The effective lifetime of Ni-56, an important waiting point in the rp process in x-ray bursts, can now be determined entirely from experimentally constrained reaction rates.
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Biswas, S. et al, Perez-Vidal, R. M., & Domingo-Pardo, C. (2019). Effects of one valence proton on seniority and angular momentum of neutrons in neutron-rich(51)( 122-)(131)Sb isotopes. Phys. Rev. C, 99(6), 064302–21pp.
Abstract: Background: Levels fulfilling the seniority scheme and relevant isomers are commonly observed features in semimagic nuclei; for example, in Sn isotopes (Z = 50). Seniority isomers in Sn, with dominantly pure neutron configurations, directly probe the underlying neutron-neutron (vv) interaction. Furthermore, an addition of a valence proton particle or hole, through neutron-proton (v pi) interaction, affects the neutron seniority as well as the angular momentum. Purpose: Benchmark the reproducibility of the experimental observables, like the excitation energies (E-x) and the reduced electric-quadrupole transition probabilities [B(E2)], with the results obtained from shell-model interactions for neutron-rich Sn and Sb isotopes with N < 82. Study the sensitivity of the aforementioned experimental observables to the model interaction components. Furthermore, explore from a microscopic point of view the structural similarity between the isomers in Sn and Sb, and thus the importance of the valence proton. Methods: The neutron-rich Sb122-131 isotopes were produced as fission fragments in the reaction Be-9(U-238, f) with 6.2 MeV/u beam energy. A unique setup, consisting of AGATA, VAMOS++, and EXOGAM detectors, was used which enabled the prompt-delayed gamma-ray spectroscopy of fission fragments in the time range of 100 ns to 200 μs. Results: New isomers and prompt and delayed transitions were established in the even-A Sb122-131 isotopes. In the odd-A Sb122-131 isotopes, new prompt and delayed gamma-ray transitions were identified, in addition to the confirmation of the previously known isomers. The half-lives of the isomeric states and the B(E2) transition probabilities of the observed transitions depopulating these isomers were extracted. Conclusions: The experimental data was compared with the theoretical results obtained in the framework of large-scale shell-model (LSSM) calculations in a restricted model space. Modifications of several components of the shell-model interaction were introduced to obtain a consistent agreement with the excitation energies and the B(E2) transition probabilities in neutron-rich Sn and Sb isotopes. The isomeric configurations in Sn and Sb were found to be relatively pure. Furthermore, the calculations revealed that the presence of a single valence proton, mainly in the g(7/2) orbital in Sb isotopes, leads to significant mixing (due to the v pi interaction) of (i) the neutron seniorities (upsilon(v)) and (ii) the neutron angular momentum (I-v). The above features have a weak impact on the excitation energies, but have an important impact on the B(E2) transition probabilities. In addition, a constancy of the relative excitation energies irrespective of neutron seniority and neutron number in Sn and Sb was observed.
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AGATA Collaboration(Liu, X. et al), Gadea, A., Jurado, M., Domingo-Pardo, C., Huyuk, T., & Perez-Vidal, R. M. (2021). Evidence for enhanced neutron-proton correlations from the level structure of the N = Z+1 nucleus Tc-87(43)44. Phys. Rev. C, 104(2), L021302–5pp.
Abstract: The low-lying excited states in the neutron-deficient N = Z + 1 nucleus (87)(43)Tcc(44) have been studied via the fusion-evaporation reaction Fe-54(Ar-36, 2n1p)Tc-87 at the Grand Accelerateur National d'Ions Lourds (GANIL), France. The AGATA spectrometer was used in conjunction with the auxiliary NEDA, Neutron Wall, and DIAMANT detector arrays to measure coincident prompt gamma rays, neutrons, and charged particles emitted in the reaction. A level scheme of Tc-87 from the (9/2(g.s.)(+)) state to the (33/2(1)(+)) state was established based on six mutually coincident gamma-ray transitions. The constructed level structure exhibits a rotational behavior with a sharp backbending at (h) over bar omega approximate to 0.50 MeV. A decrease in alignment frequency and increase in alignment sharpness in the odd-mass isotonic chains around N = 44 is proposed as an effect of the enhanced isoscalar neutron-proton interactions in odd-mass nuclei when approaching the N = Z line.
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AGATA Collaboration(Liu, X. et al), Gadea, A., Jurado, M., Domingo-Pardo, C., Huyuk, T., & Perez-Vidal, R. M. (2022). Evidence for spherical-oblate shape coexistence in Tc-87. Phys. Rev. C, 106(3), 034304–6pp.
Abstract: Excited states in the neutron-deficient nucleus Tc-87 have been studied via the fusion-evaporation reaction 54Fe(36Ar, 2n1p) Tc-87 at 115 MeV beam energy. The AGATA gamma-ray spectrometer coupled to the DIAMANT, NEDA, and Neutron Wall detector arrays for light-particle detection was used to measure the prompt coincidence of gamma rays and light particles. Six transitions from the deexcitation of excited states belonging to a new band in Tc-87 were identified by comparing gamma-ray intensities in the spectra gated under different reaction channel selection conditions. The constructed level structure was compared with the shell model and total Routhian surface calculations. The results indicate that the new band structure in 87Tc is built on a spherical configuration, which is different from that assigned to the previously identified oblate yrast rotational band.
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Perez-Vidal, R. M. et al, Gadea, A., Jurado, M., Domingo-Pardo, C., & Huyuk, T. (2022). Evidence of Partial Seniority Conservation in the pi g9/2 Shell for the N=50 Isotones. Phys. Rev. Lett., 129(11), 112501–7pp.
Abstract: The reduced transition probabilities for the 4+1 -2+1 and 2+1 -0+1 transitions in 92Mo and 94Ru and for the 4+1 -2+1 and 6+1 -4+1 transitions in 90Zr have been determined in this experiment making use of a multinucleon transfer reaction. These results have been interpreted on the basis of realistic shell-model calculations in the f5=2, p3=2, p1=2, and g9=2 proton valence space. Only the combination of extensive lifetime information and large scale shell-model calculations allowed the extent of the seniority conservation in the N = 50 g9=2 orbital to be understood. The conclusion is that seniority is largely conserved in the first 71g9=2 orbital.
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