XENON Collaboration(Aprile, E. et al), & Orrigo, S. E. A. (2017). Removing krypton from xenon by cryogenic distillation to the ppq level. Eur. Phys. J. C, 77(5), 275–12pp.
Abstract: The XENON1T experiment aims for the direct detection of dark matter in a detector filled with 3.3 tons of liquid xenon. In order to achieve the desired sensitivity, the background induced by radioactive decays inside the detector has to be sufficiently low. One major contributor is the beta-emitter Kr-85 which is present in the xenon. For XENON1T a concentration of natural krypton in xenon Kr-nat/Xe < 200 ppq (parts per quadrillion, 1 ppq = 10(-15) mol/mol) is required. In this work, the design, construction and test of a novel cryogenic distillation column using the common McCabe-Thiele approach is described. The system demonstrated a krypton reduction factor of 6.4 . 10(5) with thermodynamic stability at process speeds above 3 kg/h. The resulting concentration of natKr/Xe < 26 ppq is the lowest ever achieved, almost one order of magnitude below the requirements for XENON1T and even sufficient for future dark matter experiments using liquid xenon, such as XENONnT and DARWIN.
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XENON Collaboration(Aprile, E. et al), & Orrigo, S. E. A. (2017). Results from a calibration of XENON100 using a source of dissolved radon-220. Phys. Rev. D, 95(7), 072008–10pp.
Abstract: A Rn-220 source is deployed on the XENON100 dark matter detector in order to address the challenges in calibration of tonne-scale liquid noble element detectors. We show that the Pb-212 beta emission can be used for low-energy electronic recoil calibration in searches for dark matter. The isotope spreads throughout the entire active region of the detector, and its activity naturally decays below background level within a week after the source is closed. We find no increase in the activity of the troublesome Rn-222 background after calibration. Alpha emitters are also distributed throughout the detector and facilitate calibration of its response to Rn-222. Using the delayed coincidence of Rn-220-Po-216, we map for the first time the convective motion of particles in the XENON100 detector. Additionally, we make a competitive measurement of the half-life of Po-212, t(1/2) = (293.9 +/- (1.0)(stat) +/- (0.6)(sys)) ns.
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XENON Collaboration(Aprile, E. et al), & Orrigo, S. E. A. (2015). Search for Event Rate Modulation in XENON100 Electronic Recoil Data. Phys. Rev. Lett., 115(9), 091302–6pp.
Abstract: We have searched for periodic variations of the electronic recoil event rate in the (2-6) keVenergy range recorded between February 2011 and March 2012 with the XENON100 detector, adding up to 224.6 live days in total. Following a detailed study to establish the stability of the detector and its background contributions during this run, we performed an unbinned profile likelihood analysis to identify any periodicity up to 500 days. We find a global significance of less than 1 sigma for all periods, suggesting no statistically significant modulation in the data. While the local significance for an annual modulation is 2.8 sigma, the analysis of a multiple-scatter control sample and the phase of the modulation disfavor a dark matter interpretation. The DAMA/LIBRA annual modulation interpreted as a dark matter signature with axial-vector coupling of weakly interacting massive particles to electrons is excluded at 4.8 sigma.
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XENON Collaboration(Aprile, E. et al), & Orrigo, S. E. A. (2017). Search for two-neutrino double electron capture of Xe-124 with XENON100. Phys. Rev. C, 95(2), 024605–6pp.
Abstract: Two-neutrino double electron capture is a rare nuclear decay where two electrons are simultaneously captured from the atomic shell. For Xe-124 this process has not yet been observed and its detection would provide a new reference for nuclear matrix element calculations. We have conducted a search for two-neutrino double electron capture from the K shell of 124Xe using 7636 kg d of data from the XENON100 dark matter detector. Using a Bayesian analysis we observed no significant excess above background, leading to a lower 90% credibility limit on the half-life T-1/2 > 6.5 x 10(20) yr. We have also evaluated the sensitivity of the XENON1T experiment, which is currently being commissioned, and found a sensitivity of T-1/2 > 6.1 x 10(22) yr after an exposure of 2 t yr.
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Morales, A. I. et al, Algora, A., Rubio, B., Orrigo, S. E. A., Agramunt, J., Gelletly, W., et al. (2017). Simultaneous investigation of the T=1(J(pi)=0(+)) and T=0(J(pi)=9(+)) beta decays in Br-70. Phys. Rev. C, 95(6), 064327–11pp.
Abstract: The beta decay of the odd-odd nucleus Br-70 has been investigated with the BigRIPS and EURICA setups at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center. The T = 0(J(pi) = 9(+)) and T = 1(J(pi) = 0(+)) isomers have both been produced in in-flight fragmentation of Kr-78 with ratios of 41.6(8)% and 58.4(8)%, respectively. A half-life of t(1/2) = 2157(-49)(+53) ms has been measured for the J pi = 9(+) isomer from gamma-ray time decay analysis. Based on this result, we provide a new value of the half-life for the J pi = 0(+) ground state of Br-70, t(1/2) = 78.42 +/- 0.51 ms, which is slightly more precise, and in excellent agreement, with the best measurement reported hitherto in the literature. For this decay, we provide the first estimate of the total branching fraction decaying through the 2(1)(+) state in the daughter nucleus Se-70, R(2(1)(+)) = 1.3 +/- 1.1%. We also report four new low-intensity gamma-ray transitions at 661, 1103, 1561, and 1749 keV following the beta decay of the J pi = 9(+) isomer. Based on their coincidence relationships, we tentatively propose two new excited states at 3945 and 4752 keV in 70Se with most probable spins and parities of J(pi) = (6(+)) and (8(+)), respectively. The observed structure is interpreted with the help of shell-model calculations, which predict a complex interplay between oblate and prolate configurations at low excitation energies.
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Vitez-Sveiczer, A. et al, Algora, A., Morales, A. I., Rubio, B., Agramunt, J., Guadilla, V., et al. (2022). The beta-decay of Kr-70 into Br-70: Restoration of the pseudo-SU(4) symmetry. Phys. Lett. B, 830, 137123–8pp.
Abstract: The beta-decay of the even-even nucleus Kr-70 with Z=N+2, has been investigated at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center using the BigRIPS fragment separator, the ZeroDegree Spectrometer, the WAS3ABI implantation station and the EURICA HPGe cluster array. Fifteen gamma-rays associated with the beta-decay of( 70)Kr into Br-70 have been identified for the first time, defining ten populated states below E-exc=3300 keV. The half-life of Kr-70 was derived with increased precision and found to be t(1/2)=45.19 +/- 0.14 ms. The beta-delayed proton emission probability has also been determined as epsilon(p)=0.545(23)%. An increase in the beta-strength to the yrast 1(+) state in comparison with the heaviest Z=N+2 system studied so far (Ge-62 decay) is observed that may indicate increased np correlations in the T=0 channel. The beta-decay strength deduced from the results is interpreted in terms of the proton-neutron quasiparticle random-phase approximation (pnQRPA) and also with a schematic model that includes isoscalar and isovector pairing in addition to quadrupole deformation. The application of this last model indicates an approximate realization of pseudo-SU(4) symmetry in this system.
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Mistry, A. K. et al, Tain, J. L., Agramunt, J., Algora, A., Guadilla, V., Morales, A. I., et al. (2022). The DESPEC setup for GSI and FAIR. Nucl. Instrum. Methods Phys. Res. A, 1033, 166662–18pp.
Abstract: The DEcay SPECtroscopy (DESPEC) setup for nuclear structure investigations was developed and commissioned at GSI, Germany in preparation for a full campaign of experiments at the FRS and Super-FRS. In this paper, we report on the first employment of the setup in the hybrid configuration with the AIDA implanter coupled to the FATIMA LaBr3(Ce) fast-timing array, and high-purity germanium detectors. Initial results are shown from the first experiments carried out with the setup. An overview of the setup and function is discussed, including technical advancements along the path.
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XENON100 Collaboration(Aprile, E. et al), & Orrigo, S. E. A. (2013). The neutron background of the XENON100 dark matter search experiment. J. Phys. G, 40(11), 115201–17pp.
Abstract: TheXENON100 experiment, installed underground at the LaboratoriNazionali del Gran Sasso, aims to directly detect dark matter in the form of weakly interacting massive particles (WIMPs) via their elastic scattering off xenon nuclei. This paper presents a study on the nuclear recoil background of the experiment, taking into account neutron backgrounds from (alpha, n) reactions and spontaneous fission due to natural radioactivity in the detector and shield materials, as well as muon-induced neutrons. Based on MonteCarlo simulations and using measured radioactive contaminations of all detector components, we predict the nuclear recoil backgrounds for the WIMP search results published by theXENON100 experiment in 2011 and 2012, 0.11(-0.04)(+0.08) events and 0.17(-0.07)(+0.12) events, respectively, and conclude that they do not limit the sensitivity of the experiment.
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Fujita, Y., Rubio, B., Molina, F., Adachi, T., Fujita, H., Blank, B., et al. (2016). The Tz = ±1 → 0 and ±2 →±1 Mirror Gamow–Teller transitions in pf-shell nuclei. Acta Phys. Pol. B, 47(3), 867–881.
Abstract: Gamow-Teller (GT) transitions are the most common weak-interaction processes in the Universe. They play important roles in various processes of nucleosynthesis, for example, in the rapid proton-capture process (rp-process). In the pf-shell region, the rp-process runs through neutron-deficient nuclei with T-z = -2, -1, and 0 mainly by means of GT and Fermi transitions, where T-z is the z component of isospin T defined by T-z = (N = Z)/2. Under the assumption of isospin symmetry, mirror nuclei with reversed Z and N numbers, and thus with opposite signs of T-z, have the same structure. Therefore, symmetry is also expected for the GT transitions starting from and ending up in mirror nuclei. We have been studying the T-z = -2 -> -1 and -1 -> 0 GT transitions in beta decays, while those from stable T-z = +2 and +1 nuclei by means of hadronic (He-3; t) charge-exchange (CE) reactions. The results from these studies are compared in order to examine the mirror-symmetry structure in nuclei. In addition, these results are combined for the better understanding of GT transitions in the pf-shell region.
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Guadilla, V., Algora, A., Tain, J. L., Agramunt, J., Jordan, D., Monserrate, M., et al. (2019). Total absorption gamma-ray spectroscopy of niobium isomers. Phys. Rev. C, 100(2), 024311–15pp.
Abstract: The beta-intensity distributions of the decays of Nb-100gs,Nb-100m and Nb-102gs,Nb-102m have been determined using the total absorption gamma-ray spectroscopy technique. The JYFLTRAP double Penning trap system was employed in a campaign of challenging measurements performed with the decay total absorption gamma-ray spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyvaskyla. Different strategies were applied to disentangle the isomeric states involved, lying very close in energy. The low-spin component of each niobium case was populated through the decay of the zirconium parent, which was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained beta-intensity distributions for these zirconium decays. The beta-strength distributions evaluated with these results were compared with calculations in a quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of Zr-100,Zr-102. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The beta-intensities of the decay of Nb-102m, for which there were no previous data, were obtained. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported, and here we detail the significant impact on decay heat calculations.
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