Abstract: We investigate the performance of large area radiation detectors, with high energy-and spatial-resolution, intended for the development of a Total Energy Detector with gamma-ray imaging capability, so-called i-TED. This new development aims for an enhancement in detection sensitivity in time-of-flight neutron capture measurements, versus the commonly used C6D6 liquid scintillation total-energy detectors. In this work, we study in detail the impact of the readout photosensor on the energy response of large area (50 x 50 mm(2)) monolithic LaCl3(Ce) crystals, in particular when replacing a conventional mono-cathode photomultiplier tube by an 8 x 8 pixelated silicon photomultiplier. Using the largest commercially available monolithic SiPM array (25 cm(2)), with a pixel size of 6 x 6 mm(2), we have measured an average energy resolution of 3.92% FWHM at 662 keV for crystal thick-nesses of 10, 20 and 30 mm. The results are confronted with detailed Monte Carlo (MC) calculations, where optical processes and properties have been included for the reliable tracking of the scintillation photons. After the experimental validation of the MC model, we use our MC code to explore the impact of a smaller photosensor segmentation on the energy resolution. Our optical MC simulations predict only a marginal deterioration of the spectroscopic performance for pixels of 3 x 3 mm(2).

Abstract: The decay of excited states of the nucleus Sn-135, with three neutrons outside the doubly-magic Sn-132 core, was studied in an experiment performed at the Radioactive Isotope Beam Factory at RIKEN. Several gamma rays emitted from excited Sn-135 ions were observed following one-neutron and one-neutron-one-proton removal from Sn-136 and Sb-137 beams, respectively, on a beryllium target at relativistic energies. Based on the analogy to 133Sn populated via one-neutron removal from Sn-134, an excitation energy of 695(15) keV is assigned to the 3/2(-) state with strongest single-particle character in 135Sn. This result provides the first direct information about the evolution of the neutron shell structure beyond N = 82 and thus allows for a crucial test of shellmodel calculations in this region. The experimental findings are in full agreement with calculations performed employing microscopic effective two-body interactions derived from CD-Bonn and N3LO nucleon-nucleon potentials, which do not predict a pronounced subshell gap at neutron number N=90. The occurrence of such a gap in Sn-140, i.e., when the 1f(7/2) orbital is completely filled, had been proposed in the past, in analogy to the magicity of Ca-48, featuring a completely filled 0f(7/2) orbital one harmonic oscillator shell below.

Abstract: The beta feeding probability of Tc-102,Tc- 104,Tc- 105,Tc- 106,Tc- 107, Mo-105, and Nb-101 nuclei, which are important contributors to the decay heat in nuclear reactors, has been measured using the total absorption technique. We have coupled for the first time a total absorption spectrometer to a Penning trap in order to obtain sources of very high isobaric purity. Our results solve a significant part of a long-standing discrepancy in the gamma component of the decay heat for Pu-239 in the 4-3000 s range.

Abstract: Background: The mercury isotopes around N = 104 are a well-known example of nuclei exhibiting shape coex-istence. Mixing of configurations can be studied by measuring the monopole strength rho^2(E0), however, currently the experimental information is scarce and lacks precision, especially for the I^pi -> I^pi (I not = 0) transitions. Purpose: The goals of this study were to increase the precision of the known branching ratios and internal conversion coefficients, to increase the amount of available information regarding excited states in 182,184,186Hg, and to interpret the results in the framework of shape coexistence using different models. Method: The low-energy structures in 182,184,186Hg were populated in the & beta; decay of 182,184,186Tl, produced at ISOLDE, CERN and purified by laser ionization and mass separation. The & gamma;-ray and internal conversion electron events were detected by five germanium clover detectors and a segmented silicon detector, respectively, and correlated in time to build decay schemes.Results: In total, 193, 178, and 156 transitions, including 144, 140, and 108 observed for the first time in a & beta;-decay experiment, were assigned to 182,184,186Hg, respectively. Internal conversion coefficients were determined for 23 transitions, out of which 12 had an E0 component. Extracted branching ratios allowed the sign of the interference term in 182Hg as well as & rho;2(E 0; 0+2 & RARR; 0+1 ) and B(E2; 0+2 & RARR; 2+1 ) in 184Hg to be determined. By means of electron-electron coincidences, the 0+3 state was identified in 184Hg. The experimental results were qualitatively reproduced by five theoretical approaches, the interacting boson model with configuration mixing with two different parametrizations, the general Bohr Hamiltonian, the beyond mean-field model, and the symmetry-conserving configuration-mixing model. However, a quantitative description is lacking. Conclusions: The presence of shape coexistence in neutron-deficient mercury isotopes was confirmed and evidence for the phenomenon existing at higher energies was found. The new experimental results provide important spectroscopic input for future Coulomb excitation studies.

Abstract: The decays of the beta-delayed neutron emitters( 137)I and Rb-95 have been studied with the total absorption gamma-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyvaskyla allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption gamma-ray spectrometer, a segmented detector composed of 18 NaI(T1) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt gamma rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of beta intensity to states above the neutron separation energy that deexcite by gamma rays, comparable to the neutron emission probability. The competition between gamma deexcitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the beta-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers.